Numerical reproduction of the seasonal variation in dissolved uranium in Lake Biwa

Saito, Tatsuo; Yamazawa, Hiromi*; Mochizuki, Akihito

Journal of Environmental Radioactivity, 255, p.107035_1 - 107035_14, 2022/12

https://doi.org/10.1016/j.jenvrad.2022.107035

The seasonal variation of dissolved U (DU) in Lake Biwa was reproduced by the following model and parameter research. The introduced models are the water-DU mass balance, and the ion exchange between UO and H on the lakeshore soil. The optimized parameters were the CEC of the lakeshore, TU as the sum of DU and AU (soil adsorbed U), kads and kdes as the first order reaction rate coefficients during rapid soil adsorption and desorption of U, respectively. Tabulated by the chemical equilibria constituting DU and analyzed the contribution of each chemical species, it is shown that the seasonal variation of DU is caused by the seasonal variation of pH. A correction to the ion-exchange equilibrium to shift to first order rate reaction only when the daily AU ratio increased above kads or decreased below kdes, improved the reproducibility of DU measurements and reproduced the delay of the DU peak from the pH peak.

Beam physics design of a 30-MW beam transport to the target for an accelerator-driven subcritical system

Yee-Rendon, B.; Meigo, Shinichiro; Kondo, Yasuhiro; Tamura, Jun; Nakano, Keita; Maekawa, Fujio; Iwamoto, Hiroki; Sugawara, Takanori; Nishihara, Kenji

Journal of Instrumentation (Internet), 17(10), p.P10005_1 - P10005_21, 2022/10

https://doi.org/10.1088/1748-0221/17/10/P10005

To reduce the hazard of minor actinides in nuclear waste, JAEA proposed an accelerator-driven subcritical system (JAEA-ADS). The JAEA-ADS drives a subcritical reactor 800-MWth by 30-MW proton linac delivering the beam to the spallation neutron target inside the reactor. The beam transport to the target (BTT) is required for high-beam power stability and low peak density to ensure the integrity of the beam window. Additionally, the design should have compatible with the reactor design for the maintenance and replacement of the fuel and the beam window. A robust-compact BTT design was developed through massive multiparticle simulations. The beam optics was optimized to guarantee beam window feasibility requirements by providing a low peak density of less than 0.3 A/mm. Beam stability was evaluated and improved by simultaneously applying the linac's input beam and element errors. The input beam errors to the reactor were based on the beam degradation obtained by implementing fast fault compensation in the linac. Those results show that the BTT fulfills the requirements for JAEA-ADS.

Measurement of nuclide production cross sections for proton-induced reactions on Ni and Zr at 0.4, 1.3, 2.2, and 3.0 GeV

Takeshita, Hayato*; Meigo, Shinichiro; Matsuda, Hiroki*; Iwamoto, Hiroki; Nakano, Keita; Watanabe, Yukinobu*; Maekawa, Fujio

Nuclear Instruments and Methods in Physics Research B, 527, p.17 - 27, 2022/09

https://doi.org/10.1016/j.nimb.2022.07.002

To improve accuracy of nuclear design of accelerator driven nuclear transmutation systems and so on, nuclide production cross sections on Ni and Zr were measured for GeV energy protons. The measured results were compared with PHITS calculations, JENDL/HE-2007 and so on.

Beam dynamics studies for fast beam trip recovery of the Japan Atomic Energy Agency accelerator-driven subcritical system

Yee-Rendon, B.; Kondo, Yasuhiro; Tamura, Jun; Nakano, Keita; Maekawa, Fujio; Meigo, Shinichiro

Physical Review Accelerators and Beams (Internet), 25(8), p.080101_1 - 080101_17, 2022/08

https://doi.org/10.1103/PhysRevAccelBeams.25.080101

High reliability and availability are primary goals for the operation of particle accelerators, especially for accelerator-driven subcritical systems (ADS). ADSs employ high-power beams for the transmutation of minor actinide; as a result, the amount and the radiotoxicity of the nuclear waste are considerably reduced. To this end, the Japan Atomic Energy Agency is designing a 30-MW continuous wave (cw) super-conducting proton linear accelerator (linac) that supplies neutrons to an 800-MW subcritical reactor by a spallation process. The major challenge for an ADS linac is the strict control of the beam trip duration and its frequency to avoid thermal stress in the subcritical reactor structures. The maximum allowed beam trips for failures longer than a few seconds are estimated to be far below the rate achieved in current accelerators. Thus, we implemented a combination of hot standby and local compensation that enables a fast beam recovery. This work comprehensively investigated the tolerance of our linac lattice for the local compensations for failures in superconducting cavities and magnets. This scheme includes simultaneous compensation of multiple cavities in independent and same cryomodules that significantly enhance the reliability of the linac. The returned schemes present acceptable beam performance to guarantee the integrity of the linac and the beam transport to the target; moreover, they satisfy the beam stability in the beam window. In addition, the readjusted elements are subjected to moderate stress to ensure a sustainable operation. This manuscript reports the beam dynamics results toward fulfilling the high reliability demanded by an ADS linac.

Development of mock-up test loop (IMMORTAL) for LBE spallation target

Obayashi, Hironari; Yamaki, Kenichi*; Yoshimoto, Hidemitsu*; Kita, Satoshi*; Wan, T.*; Sasa, Toshinobu

JAEA-Technology 2021-035, 66 Pages, 2022/03

JAEA-Technology-2021-035.pdf:4.26MB

Construction of Transmutation Experimental Facility (TEF) is under planning in Japan Proton Accelerator Research Complex (J-PARC) program to promote R&Ds on realization of transmutation technology by an accelerator driven system (ADS). As a facility of TEF, ADS Target Test Facility (TEF-T) will provide a spallation target to study target technology and perform post irradiation examination (PIE) of candidate materials of ADS. In ADS, lead-bismuth eutectic (LBE) alloy is used as a spallation target material and a core coolant. As is well known, LBE has corrosive to structural materials hence each component of the target system should provide compatibility with LBE. In addition, instrumentations for LBE are restricted by the target operation condition such as high temperature and irradiation environment. The devices for LBE have been developed individually to achieve the LBE target system. "Integrated Multi-functional MOckup for TEF-T Real-scale TArget Loop, IMMORTAL" was fabricated as a mock-up test loop of the target for the purpose of the integration testing of individually developed devices. This report describes an overview of IMMORTAL and the design of the installed devices.

Nuclide production cross section of Lu target irradiated with 0.4-, 1.3-, 2.2-, and 3.0-GeV protons

Takeshita, Hayato; Meigo, Shinichiro; Matsuda, Hiroki; Iwamoto, Hiroki; Nakano, Keita; Watanabe, Yukinobu*; Maekawa, Fujio

JAEA-Conf 2021-001, p.207 - 212, 2022/03

https://doi.org/10.11484/jaea-conf-2021-001

Prediction of nuclide production of spallation products by high-energy proton injection plays a fundamental and important role in shielding design of high-intensity proton accelerator facilities such as accelerator driven nuclear transmutation system (ADS). Since the prediction accuracy of the nuclear reaction models used in the production quantity prediction simulation is insufficient, it is necessary to improve the nuclear reaction models. We have measured nuclide production cross sections for various target materials with the aim of acquiring experimental data and improving nuclear reaction models. In this study, 1.3-, 2.2- and 3.0-GeV proton beams were irradiated to Lu target, and nuclide production cross-section data were acquired by the activation method. The measured data were compared with several nuclear reaction models used in Monte Carlo particle transport calculation codes to grasp the current prediction accuracy and to study how the nuclear reaction model could be improved.

Development of environmental mitigation technology with novel water purification agents (Contract research); FY2020 Nuclear Energy Science & Technology and Human Resource Development Project

Collaborative Laboratories for Advanced Decommissioning Science; Shinshu University*

JAEA-Review 2021-051, 81 Pages, 2022/01

JAEA-Review-2021-051.pdf:4.03MB

The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2020. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2020, this report summarizes the research results of the "Development of environmental mitigation technology with novel water purification agents" conducted in FY2020. The present study aims to develop a reusable adsorbent for strontium ions through joint research between Japan and the United Kingdom, and to reduce the amount of used adsorbent generated through the decontamination process. The basic strategy of this research is to produce adsorbents and examine their Sr adsorption performance at Shinshu University. The structural analyses of the adsorbents are conducted by the Institute for Molecular Science (IMS) and the UK teams. The adsorption data and structural information are theoretically analyzed at Tohoku University with data science, leading to a new synthetic guid

Re-examinations of MA fuel composition for accelerator-driven system and its heat removal

Sugawara, Takanori; Moriguchi, Daisuke*; Ban, Yasutoshi; Tsubata, Yasuhiro; Takano, Masahide; Nishihara, Kenji

JAEA-Research 2021-008, 63 Pages, 2021/10

JAEA-Research-2021-008.pdf:4.43MB

This study aims to perform the neutronics calculations for accelerator-driven system (ADS) with a new fuel composition based on the SELECT process developed by Japan Atomic Energy Agency because the previous studies had used the ideal MA (minor actinide) fuel composition without uranium and rare earth elements. Through the neutronics calculations, it is shown that two calculation cases, with/without neptunium, satisfy the design criteria. Although the new fuel composition includes uranium and rare earth elements, the ADS core with the new fuel composition is feasible and consistent with the partitioning and transmutation (P&T) cycle. Based on the new fuel composition, the heat removal during fuel powder storage and fuel assembly assembling is evaluated. For the fuel powder storage, it is found that a cylindrical tube container with a length of 500 [mm] and a diameter of 11 - 21 [mm] should be stored under water. For the fuel assembly assembling, CFD analysis indicates that the cladding tube temperature would satisfy the criterion if the inlet velocity of air is larger than 0.5 [m/s]. Through these studies, the new fuel composition which is consistent with the P&T cycle is obtained and the heat removal with the latest conditions is investigated. It is also shown that the new fuel composition can be practically handled with respect to heat generation, which is one of the most difficult points in handling MA fuel.

Durability of secondary electron emission for high-intensity beam on SiC wire

Meigo, Shinichiro; Nakano, Keita; Okubo, Nariaki; Yuyama, Takahiro*; Ishii, Yasuyuki*

Proceedings of 18th Annual Meeting of Particle Accelerator Society of Japan (Internet), p.296 - 301, 2021/10

no abstracts in English

Design of the MEBT for the JAEA-ADS Project

Yee-Rendon, B.; Kondo, Yasuhiro; Maekawa, Fujio; Meigo, Shinichiro; Tamura, Jun

Proceedings of 12th International Particle Accelerator Conference (IPAC 21) (Internet), p.790 - 792, 2021/08

https://doi.org/10.18429/JACoW-IPAC2021-MOPAB246

The Medium Energy Beam Transport (MEBT) will transport a CW proton beam with a current of 20 mA and energy of 2.5 MeV from the exit of the normal conducting Radiofrequency Quadrupole (RFQ) to the superconducting Half-Wave resonator (HWR) section. The MEBT must provide a good matching between the RFQ and HWR, effective control of the emittance growth and the halo formation, enough space for all the beam diagnostics devices, among others. This work reports the first lattice design and the beam dynamics studies for the MEBT of the JAEA-ADS.