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Takahatake, Yoko; Watanabe, So; Watanabe, Masayuki; Sano, Yuichi; Takeuchi, Masayuki
Progress in Nuclear Science and Technology (Internet), 7, p.195 - 198, 2025/05
Extraction chromatgraphy technology for trivalent minor actinide (MA(III) ; Am(III) and Cm(III)) recovery from the solution generated by an extraction process in reprocessing of spent nuclear fuel has been developed. A fine particle is generated in the solution. The fine particle must be removed before MA recovery operation, because that leads clogging of the extraction chlomatography column. In order to prevent clogging the column, filtration system utilizing porous silica beads packed column has been designed. In this study, a fine particle trapping system was developed and particle removal performance of the system was experimentally evaluated using alumina particles as simulated fine particle. Column experiments revealed that the fine particle with the particle size from 0.12 to 15 
m is cause of clogging of the filtration column. Since simulated fine particles were trapped on filtration experiments, a filtration system using the porous silica beads column is practical,
Meigo, Shinichiro; Iwamoto, Hiroki; Sugihara, Kenta*; Hirano, Yukinori*; Tsutsumi, Kazuyoshi*; Saito, Shigeru; Maekawa, Fujio
JAEA-Technology 2024-026, 123 Pages, 2025/03
JAEA-Technology-2024-026.pdf:14.22MB
Based on the design of the ADS Target Test Facility (TEF-T) at the J-PARC Transmutation Experimental Facility, a conceptual study was conducted on the J-PARC proton beam irradiation facility. This research was carried out based on the recommendations of the Nuclear Transmutation Technology Evaluation Task Force of the MEXT. The recommendations state that it is desirable to consider facility specifications that can make the most of the benefits of using the existing J-PARC proton accelerator while also solving the engineering issues of the ADS. We considered facilities that could respond to a variety of needs while reducing the facilities that were not needed in the TEF-T design. In order to clarify these diverse needs, we investigated the usage status of representative accelerator facilities around the world. As a result, it became clear that the main purposes of these facilities were (1) Material irradiation, (2) Soft error testing of semiconductor devices using spallation neutrons, (3) Production of RI for medical use, and (4) Proton beam use, and we investigated the facilities necessary for these purposes. In considering the facility concept, we assumed a user community in 2022 and reflected user opinions in the facility design. This report summarizes the results of the conceptual study of the proton irradiation facility, various needs and responses to them, the roadmap for facility construction, and future issues.
Che, G.*; Fei, Y.*; Tang, X.*; Zhao, Z.*; Hattori, Takanori; Abe, Jun*; Wang, X.*; Ju, J.*; Dong, X.*; Wang, Y.*; et al.
Physical Chemistry Chemical Physics, 27(2), p.1112 - 1118, 2025/01
Times Cited Count：2 Percentile：47.21(Chemistry, Physical)Pressure-induced polymerization (PIP) of aromatic molecules has emerged as an effective method for synthesizing various carbon-based materials. In this work, PIP of 1,4-difluorobenzene (1,4-DFB) was investigated. 
high-pressure investigations of 1,4-DFB reveal a phase transition at approximately 12.0 GPa and an irreversible chemical reaction at 18.7 GPa. Structural analysis of the product and the kinetics of the reaction uncovered the formation of pseudohexagonal stacked fluoro-diamond nanothreads with linear growth. Compared to the crystal structures of benzene under high pressure, 1,4-DFB exhibits higher compression along the [001] axis. The anisotropic compression is attributed to the stronger H
interaction along the [01
] axis and the potential compression-inhibiting H
F interactions along the [100] and [010] axes, and it facilitates a possible reaction pathway along the [01] axis. This work emphasizes the crucial role of functionalization in modulating molecular stacking and influencing the reaction pathway.
Nishihara, Kenji
Enerugi, Shigen, 45(6), p.359 - 363, 2024/11
no abstracts in English
from 3-GeV protons and 
Hg with the 
Bi(n,xn) reactionsSugihara, Kenta*; Meigo, Shinichiro; Iwamoto, Hiroki; Maekawa, Fujio
JAEA-Conf 2024-002, p.162 - 167, 2024/11
A neutron energy spectrum is important for shielding design at an Accelerator-Driven System facility (1.5-GeV p + Lead Bismuth Eutectic). A similar spectrum can be obtained at J-PARC (3-GeV proton + Hg). To check the validity of the unfolding, the unfolding with the Bi(n,xn) reactions and the response functions (JENDL/HE-2007 and TALYS) was applied. In our poster, we present the derivation of the spectrum and comparison with the spectrum with a Time-of-Flight technique.
Fujii, Daisuke; Iwanaka, Akihiro*; Tanaka, Mitsuru*
Physical Review D, 110(9), p.L091501_1 - L091501_8, 2024/11
Times Cited Count：2 Percentile：0.00(Astronomy & Astrophysics)The gravitational form factors (GFFs) of pions are calculated from a top-down holographic quantum chromodynamics (QCD) approach with momentum transfer dependence for the first time. It is important because the GFFs of hadrons have information on the internal stress distribution that may provide insight into the mechanism of how QCD forms hadrons. The forward limit value of this GFFs, i.e. the D-term, was also obtained. Furthermore, in this approach, we observe the so-called glueball dominance, in which pions have gravitational interactions via infinite glueball spectra.
Yee-Rendon, B.; Kondo, Yasuhiro; Tamura, Jun; Maekawa, Fujio; Meigo, Shinichiro
Proceedings of 21st Annual Meeting of Particle Accelerator Society of Japan (Internet), p.205 - 209, 2024/10
The Japan Atomic Energy Agency (JAEA) designs a 30-MW CW proton linear accelerator (linac) as a key component for the accelerator-driven subcritical system (ADS) project, aimed at nuclear waste management. The low energy beam transport (LEBT) in JAEA-ADS uses charge neutralization to minimize space-charge effects, which are the primary cause of beam loss in high-power accelerators. During commissioning and power ramp-up, precise control of the duty cycle is required for safety and machine protection; thus, a chopper system will be installed to manage the beam power. The chopper is located at the LEBT, to facilitate the disposal of the excess beam power, but its operation will affect the charge neutralization producing beam transients that could lead to beam loss. To shed light on this, we created a beam optics model for the chopper using an analytic approach to determine the required characteristics like voltage and dimensions, which was confirmed through TraceWin simulations. Subsequently, we analyzed the chopper's impact on space-charge compensation to evaluate the beam transients in the LEBT. This study reports the design of the chopper and its effects on beam performance for the JAEA-ADS LEBT.
Meigo, Shinichiro; Yamaguchi, Yuji
Proceedings of 21st Annual Meeting of Particle Accelerator Society of Japan (Internet), p.853 - 858, 2024/10
no abstracts in English
Pla
ais, A.*; Bouly, F.*; Froidefond, E.*; Lagniel, J.-M.*; Normand, G.*; Orduz, A. K.*; Yee-Rendon, B.; De Keukeleere, L.*; Van De Walle, J.*
Proceedings of 32nd Linear Accelerator Conference (LINAC 2024) (Internet), p.563 - 568, 2024/10
Reliability is an important feature for high power particle accelerators. This is particularly true for Accelerator-Driven Systems (ADS), for that every beam interruption can strongly affect the availability of the nuclear reactor. Many of these outages come from the loss of accelerating cavities or of their associated systems. Cavity failures can be compensated for by retuning other cavities of the linac. Finding the ideal compensation settings is however a difficult challenge that involves beam dynamics and multi-objective optimisation, and which raises very different issues according to the linac under study. For instance in the SPIRAL2 linac, a lot of cavities are mobilized for the compensation and the search space has a very high number of dimensions. Plus, it has quite low margins on the longitudinal acceptance. Linacs for ADS (such as the Japan Atomic Energy Agency ADS or MYRRHA) have a specific fault-tolerance design which facilitate the optimisation, but cavities have to be retuned in a few seconds. Hence we developed LightWin, a tool to automatically and systematically find compensation settings for every cavity failure of any given linac. In this study, we will present LightWin latest developments as well as the compensation strategies that we developed for SPIRAL2 and ADS linacs, both from a beam dynamics and a mathematical point of view.
Yee-Rendon, B.; Jameson, R. A.*; Okamura, Masahiro*; Li, C.*; Jiang, P.*; Maus, J. M.*
Proceedings of 32nd Linear Accelerator Conference (LINAC 2024) (Internet), p.492 - 495, 2024/10
LINACs is a simulation framework for designing optics and beam dynamics of charged particles in particle accelerators. LINACs is an open-source software that enables the user complete control over all design and simulation parameters of RFQs. This includes beam-driven design, fully 3D simulation using precise quadrupolar symmetry, and rigorous Poisson solution for external and space charge fields. The code can handle simultaneous particle beams with analytical input distributions and allows input beam scans. The software offers a relatively short running time and provides extensive analysis techniques. This work provides a historical overview of the code, presents results from RFQ models, and discusses future developments.
Yee-Rendon, B.; Kondo, Yasuhiro; Tamura, Jun; Maekawa, Fujio; Meigo, Shinichiro
Proceedings of 32nd Linear Accelerator Conference (LINAC 2024) (Internet), p.488 - 491, 2024/10
The Japan Atomic Energy Agency (JAEA) is designing a 30-MW CW proton linear accelerator (linac) for nuclear waste transmutation. Space-charge is the primary challenge in achieving low losses and high beam quality for high-power accelerators, especially at low energy levels where space-charge forces are greater. To counteract the space-charge effects, the low-energy beam transport (LEBT) uses a magnetostatic design to enable the neutralization of the beam charge, the so-called space charge compensation. The neutralization is an accumulation process that reaches a charge balance between the main beam and the opposite ionized particles. However, this equilibrium is destroyed by the chopper system used during beam ramping. During those transient regimes, the beam optics conditions are not optimal for the beam, producing considerable degradation that can end in serious damage to the accelerator. Thus, analysis of beam behavior at these periods is essential to develop a robust design and an efficient operation of the JAEA-ADS linac. This study presents the beam dynamics of neutralization build-up and chopper operation for the JAEA-ADS LEBT.
Nishihara, Kenji; Sugawara, Takanori; Fukushima, Masahiro; Iwamoto, Hiroki; Katano, Ryota; Abe, Takumi
Proceedings of International Conference on Nuclear Fuel Cycle (GLOBAL2024) (Internet), 4 Pages, 2024/10
A pilot plant for the accelerator-driven system is proposed as a scaled-down version of a lead-bismuth cooled ADS with 800 MW thermal output for transmutation of minor actinides. In this presentation, the design policy of the pilot plant is presented.
Arai, Yoichi; Watanabe, So; Watanabe, Masayuki; Arai, Tsuyoshi*; Katsuki, Kenta*; Agou, Tomohiro*; Fujikawa, Hisaharu*; Takeda, Keisuke*; Fukumoto, Hiroki*; Hoshina, Hiroyuki*; et al.
Nuclear Instruments and Methods in Physics Research B, 554, p.165448_1 - 165448_10, 2024/09
Times Cited Count：0 Percentile：0.00(Instruments & Instrumentation)Shibata, Hiroki; Saito, Hiroaki; Hayashi, Hirokazu; Takano, Masahide
Nihon Genshiryoku Gakkai Wabun Rombunshi (Internet), 23(3), p.74 - 80, 2024/08
Partitioning and transmutation of minor actinides techniques have been developed to reduce the radiotoxicity and volume in the high-level radioactive wastes. Minor actinide nitride fuel has been chosen as a candidate for transmutation of long-lived nuclides by accelerator-driven system. Understanding irradiation behavior of nitride fuel is important for its design and development, however, experimental data on irradiation tests of actinide nitrides and these solid solutions are scarce. Recently, in JAEA, nitride fuel performance analysis module based on light water reactor fuel performance code, FEMAXI-7, has been developed to simulate irradiation behavior of the nitride fuel. In this study, performance analysis was carried out focusing on the pellet-cladding mechanical interaction (PCMI), which was pointed out as the most effective factor for the fuel safety during irradiation. Simulation results show that PCMI does not cause the creep rupture of the cladding.
Yamagishi, Isao; Hato, Shinji*; Nishihara, Kenji; Tsubata, Yasuhiro; Sagawa, Yusuke*
JAEA-Data/Code 2024-002, 63 Pages, 2024/07
JAEA-Data-Code-2024-002.pdf:2.91MB
JAEA-Data-Code-2024-002-appendix(CD-ROM).zip:9.42MB
Adsorption columns filled with zeolite are used to treat contaminated water containing radioactive cesium generated by the Fukushima Daiichi Nuclear Power Station accident. As the contaminated water treatment progresses, the radioactive cesium in the adsorption column becomes highly concentrated, and the adsorption column becomes a high radiation source. To evaluate the radiation effects such as decay heat and radiolytic hydrogen production in the adsorption column, the concentration of radioactive cesium in the adsorption column is necessary, but since it is difficult to evaluate the concentration by measurement, it is estimated by simulation. In this research, a zeolite column adsorption dynamics simulation (Zeolite Adsorption Column: ZAC) code was developed to calculate the concentration of radioactive materials such as radioactive cesium in a zeolite filled adsorption column when they are injected into the column. The code was validated through comparison of calculation results with existing codes and experimental results of small column tests. This report presents the details of the model, the handling of the code, and the validity of the results for the developed code.
Collaborative Laboratories for Advanced Decommissioning Science; Shinshu University*
JAEA-Review 2023-053, 87 Pages, 2024/05
JAEA-Review-2023-053.pdf:4.67MB
The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2022. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2020, this report summarizes the research results of the "Development of environmental mitigation technology with novel water purification agents" conducted from FY2020 to FY2022. The present study aims to develop a reusable adsorbent for strontium ions with high adsorption property to contribute to the improvement of the treatment process of radioactive contaminated water generated by the Great East Japan Earthquake. As a result, reusable adsorbent materials showing excellent Sr adsorption performances were developed. The current adsorbent materials for strontium are extremely expensive and single use, so the storage and disposal of massive generation of waste have become a major problem.
Saito, Shigeru; Meigo, Shinichiro; Makimura, Shunsuke*; Hirano, Yukinori*; Tsutsumi, Kazuyoshi*; Maekawa, Fujio
JAEA-Technology 2023-025, 48 Pages, 2024/03
JAEA-Technology-2023-025.pdf:3.11MB
JAEA has been developing Accelerator-Driven Systems (ADS) for research and development of nuclear transmutation using accelerators in order to reduce the volume and hazardousness of high-level radioactive waste generated by nuclear power plants. In order to prepare the material irradiation database necessary for the design of ADS and to study the irradiation effects in Lead-Bismuth Eutectic (LBE) alloys, a proton irradiation facility is under consideration at J-PARC. In this proton irradiation facility, 250 kW proton beams will be injected into the LBE spallation target, and irradiation tests under LBE flow will be performed for candidate structural materials for ADS. Furthermore, semiconductor soft-error tests, medical RI production, and proton beam applications will be performed. Among these, Post Irradiation Examination (PIE) of irradiated samples and RI separation and purification will be carried out in the PIE facility to be constructed near the proton irradiation facility. In this PIE facility, PIE of the equipment and samples irradiated in other facilities in J-PARC will also be performed. This report describes the conceptual study of the PIE facility, including the items to be tested, the test flow, the facilities, the test equipment, etc., and the proposed layout of the facility.
Li, N.*; Sun, Y.*; Nakajima, Kunihisa; Kurosaki, Ken*
Journal of Nuclear Science and Technology, 61(3), p.343 - 353, 2024/03
Times Cited Count：1 Percentile：27.70(Nuclear Science & Technology)During the Fukushima Daiichi nuclear power plant (1F) accident, an overwhelming amount of the cesium remaining in the pressure vessel could have been deposited onto 304 stainless steel (SS304) steam separators and dryers, both with large surface areas. During 1F's decommissioning, the deposited cesium is a safety hazard as it can generate radioactive dust. However, the cohesive and adhesive strengths of CsOH-chemisorbed oxide scales are yet to be defined. In this study, we investigated how CsOH-chemisorption affects the cohesive and adhesive strengths between oxide scales and SS304 substrates with a scratch tester. The scratch test results revealed that the cohesive strengths of the oxide scales decreased after CsOH-chemisorption, while adhesive failure could not be reached.
Yee-Rendon, B.; Kondo, Yasuhiro; Tamura, Jun; Maekawa, Fujio; Meigo, Shinichiro
Proceedings of 20th Annual Meeting of Particle Accelerator Society of Japan (Internet), p.545 - 549, 2023/11
The Japan Atomic Energy Agency (JAEA) is proposing a 30-MW proton linear accelerator (linac) for the application of accelerator-driven subcritical system (ADS) technology to achieve nuclear waste transmutation. A major challenge for the JAEA-ADS linac is the efficient transport of a 35 keV proton beam from the ion source to the radio-frequency quadrupole. In order to achieve this goal, we have optimized a magnetostatic low energy beam transport (LEBT) consisting of two solenoids to reduce the transmission of high-charge ions generated by the source and minimize the growth of proton emittance, while taking into account various space-charge compensation scenarios. In this report, we present the optical design and discuss the multiparticle tracking results of the JAEA-ADS LEBT.
Plaais, A.*; Bouly, F.*; Yee-Rendon, B.
Proceedings of 14th International Particle Accelerator Conference (IPAC 23) (Internet), p.4097 - 4100, 2023/09
Reliability in high power hadron accelerators is a major issue, particularly for Accelerator Driven Systems (ADS). For example, the Japan Atomic Energy Agency (JAEA) ADS maximum frequency of beam trips longer than 5 min was set to 42 per year. A significant number of breakdowns are caused by the failure of accelerating cavities or by their associated systems. Hence, we studied how these can be effectively reduced. To this end, we developed the numerical tool LightWin that aims to determine the compensation settings for any superconducting (SC) linac automatically and systematically. This tool has been successfully used for the MYRRHA SC linac. In this work, we applied LightWin to compensate for several failure scenarios involving the last section of the JAEA ADS linac and compared the associated retuned settings and beam performance to those found in a previous study with TraceWin.
