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Journal Articles

An Evaluation on Inelastic Thermal Neutron Scattering Cross-Section Data of Crystalline Graphite

Okita, Shoichiro; Abe, Yutaka*; Tasaki, Seiji*; Fukaya, Yuji

Radioisotopes, 73(3), p.233 - 240, 2024/11

Journal Articles

Magnetoelastic coupling for Fe-Ga thin films epitaxially grown on different substrates

Ding, H.*; Ito, Keita*; Endo, Yasushi*; Takanashi, Koki; Seki, Takeshi*

Journal of Physics D; Applied Physics, 57(38), p.385002_1 - 385002_10, 2024/09

 Times Cited Count:0 Percentile:0.00(Physics, Applied)

Journal Articles

High temperature nanoindentation of (U,Ce)O$$_{2}$$ compounds

Frazer, D.*; Saleh, T. A.*; Matsumoto, Taku; Hirooka, Shun; Kato, Masato; McClellan, K.*; White, J. T.*

Nuclear Engineering and Design, 423, p.113136_1 - 113136_7, 2024/07

 Times Cited Count:0 Percentile:0.00(Nuclear Science & Technology)

Nanoindentation based techniques can be employed on minute volumes of material to measure mechanical properties, including Young's modulus, hardness, and creep stress exponents. In this study, (U,Ce)O$$_{2}$$ solid solutions samples are used to develop elevated temperature nanoindentation and nanoindentation creep testing methods for use on mixed oxide fuels. Nanoindentation testing was performed on 3 separate (Ux-1,Cex)O$$_{2}$$ compounds ranging from x equals 0.1 to 0.3 at up to 800 $$^{circ}$$C: their Young's modulus, hardness, and creep stress exponents were evaluated. The Young's modulus decreases in the expected linear manner while the hardness decreases in the expected exponential manner. The nanoindentation creep experiments at 800 $$^{circ}$$C give stress exponent values, n=4.7-6.9, that suggests dislocation motion as the deformation mechanism.

Journal Articles

Inelastic neutron scattering study of magnon excitation by ultrasound injection in yttrium iron garnet

Shamoto, Shinichi; Akatsu, Mitsuhiro*; Chang, L.-J.*; Nemoto, Yuichi*; Ieda, Junichi

Applied Physics Letters, 124(11), p.112402_1 - 112402_5, 2024/03

 Times Cited Count:1 Percentile:57.87(Physics, Applied)

The magnon excitation by ultrasound injection in Y$$_3$$Fe$$_5$$O$$_{12}$$ is studied by inelastic neutron scattering. Both longitudinal and transverse ultrasound injections enhanced the inelastic neutron scattering intensity.

Journal Articles

Impact of interatomic structural characteristics of aluminosilicate hydrate on the mechanical properties of metakaolin-based geopolymer

Kim, G.*; Cho, S.-M.*; Im, S.*; Suh, H.*; Morooka, Satoshi; Shobu, Takahisa; Kanematsu, Manabu*; Machida, Akihiko*; Bae, S.*

Construction and Building Materials, 411, p.134529_1 - 134529_18, 2024/01

 Times Cited Count:7 Percentile:67.18(Construction & Building Technology)

Journal Articles

Magnetic layer thickness influence on magnetoelastic properties anisotropy in Co$$_{2}$$Fe$$_{0.4}$$Mn$$_{0.6}$$Si heusler alloy thin films

Nabialek, A.*; Chumak, O.*; Seki, Takeshi*; Takanashi, Koki; Baczewski, L. T.*; Szymczak, H.*

IEEE Transactions on Magnetics, 59(11), p.2501405_1 - 2501405_5, 2023/11

 Times Cited Count:2 Percentile:20.26(Engineering, Electrical & Electronic)

Journal Articles

Experimental evidence for the significance of optical phonons in thermal transport of tin monosulfide

Wu, P.*; Murai, Naoki; Li, T.*; Kajimoto, Ryoichi; Nakamura, Mitsutaka; Kofu, Maiko; Nakajima, Kenji; Xia, K.*; Peng, K.*; Zhang, Y.*; et al.

New Journal of Physics (Internet), 25(1), p.013032_1 - 013032_11, 2023/01

 Times Cited Count:0 Percentile:0.00(Physics, Multidisciplinary)

Journal Articles

Effect of magnesium silicate hydrate (M-S-H) formation on the local atomic arrangements and mechanical properties of calcium silicate hydrate (C-S-H); In situ X-ray scattering study

Kim, G.*; Im, S.*; Jee, H.*; Suh, H.*; Cho, S.*; Kanematsu, Manabu*; Morooka, Satoshi; Koyama, Taku*; Nishio, Yuhei*; Machida, Akihiko*; et al.

Cement and Concrete Research, 159, p.106869_1 - 106869_17, 2022/09

 Times Cited Count:25 Percentile:88.25(Construction & Building Technology)

Journal Articles

Rotation of complex ions with ninefold hydrogen coordination studied by quasielastic neutron scattering and first-principles molecular dynamics calculations

Omasa, Yoshinori*; Takagi, Shigeyuki*; Toshima, Kento*; Yokoyama, Kaito*; Endo, Wataru*; Orimo, Shinichi*; Saito, Hiroyuki*; Yamada, Takeshi*; Kawakita, Yukinobu; Ikeda, Kazutaka*; et al.

Physical Review Research (Internet), 4(3), p.033215_1 - 033215_9, 2022/09

Journal Articles

Revealing the ion dynamics in Li$$_{10}$$GeP$$_{2}$$S$$_{12}$$ by quasi-elastic neutron scattering measurements

Hori, Satoshi*; Kanno, Ryoji*; Kwon, O.*; Kato, Yuki*; Yamada, Takeshi*; Matsuura, Masato*; Yonemura, Masao*; Kamiyama, Takashi*; Shibata, Kaoru; Kawakita, Yukinobu

Journal of Physical Chemistry C, 126(22), p.9518 - 9527, 2022/06

 Times Cited Count:10 Percentile:54.98(Chemistry, Physical)

Journal Articles

Experimental analysis on dynamics of liquid molecules adjacent to particles in nanofluids

Hashimoto, Shunsuke*; Nakajima, Kenji; Kikuchi, Tatsuya*; Kamazawa, Kazuya*; Shibata, Kaoru; Yamada, Takeshi*

Journal of Molecular Liquids, 342, p.117580_1 - 117580_8, 2021/11

 Times Cited Count:4 Percentile:18.33(Chemistry, Physical)

Quasi-elastic neutron scattering (QENS) and pulsed-field-gradient nuclear magnetic resonance (PFGNMR) analyses of a nanofluid composed of silicon dioxide (SiO$$_{2}$$) nanoparticles and a base fluid of ethylene glycol aqueous solution were performed. The aim was to elucidate the mechanism increase in the thermal conductivity of the nanofluid above its theoretical value. The obtained experimental results indicate that SiO$$_{2}$$ particles may decrease the self-diffusion coefficient of the liquid molecules in the ethylene glycol aqueous solution because of their highly restricted motion around these nanoparticles. At a constant temperature, the thermal conductivity increases as the self-diffusion coefficient of the liquid molecules decreases in the SiO$$_{2}$$ nanofluids.

Journal Articles

Relevance of hydrogen bonded associates to the transport properties and nanoscale dynamics of liquid and supercooled 2-propanol

Zhai, Y.*; Luo, P.*; Nagao, Michihiro*; Nakajima, Kenji; Kikuchi, Tatsuya*; Kawakita, Yukinobu; Kienzle, P. A.*; Z, Y.*; Faraone, A.*

Physical Chemistry Chemical Physics, 23(12), p.7220 - 7232, 2021/03

 Times Cited Count:5 Percentile:25.90(Chemistry, Physical)

Journal Articles

Nanoscale relaxation in "Water-in-Salt" and "Water-in-Bisalt" electrolytes

Gonzal$'e$z, M. A.*; Borodin, O.*; Kofu, Maiko; Shibata, Kaoru; Yamada, Takeshi*; Yamamuro, Osamu*; Xu, K.*; Price, D. L.*; Saboungi, M.-L.*

Journal of Physical Chemistry Letters (Internet), 11(17), p.7279 - 7284, 2020/09

 Times Cited Count:22 Percentile:80.18(Chemistry, Physical)

Journal Articles

Segmental motions of proteins under non-native states evaluated using quasielastic neutron scattering

Fujiwara, Satoru*; Matsuo, Tatsuhito*; Sugimoto, Yasunobu*; Shibata, Kaoru

Journal of Physical Chemistry Letters (Internet), 10(23), p.7505 - 7509, 2019/12

 Times Cited Count:4 Percentile:18.38(Chemistry, Physical)

Characterization of the dynamics of disordered polypeptide chains is required to elucidate the behavior of intrinsically disordered proteins and proteins under non-native states related to the folding process. Here we develop a method using quasielastic neutron scattering, combined with small-angle X-ray scattering and dynamic light scattering, to evaluate segmental motions of proteins as well as diffusion of the entire molecules and local side-chain motions. We apply this method to RNase A under the unfolded and molten-globule (MG) states. The diffusion coefficients arising from the segmental motions are evaluated and found to be different between the unfolded and MG states. The values obtained here are consistent with those obtained using the fluorescence-based techniques. These results demonstrate not only feasibility of this method but also usefulness to characterize the behavior of proteins under various disordered states.

Journal Articles

Validating polarization effects in $$gamma$$-rays elastic scattering by Monte Carlo simulation

Omer, M.; Hajima, Ryoichi*

New Journal of Physics (Internet), 21(11), p.113006_1 - 113006_10, 2019/11

AA2019-0407.pdf:0.73MB

 Times Cited Count:6 Percentile:43.86(Physics, Multidisciplinary)

Journal Articles

Proposal of laser-induced ultrasonic guided wave for corrosion detection of reinforced concrete structures in Fukushima Daiichi Nuclear Power Plant decommissioning site

Furusawa, Akinori; Takenaka, Yusuke; Nishimura, Akihiko

Applied Sciences (Internet), 9(17), p.3544_1 - 3544_12, 2019/09

 Times Cited Count:9 Percentile:55.64(Chemistry, Multidisciplinary)

Remote-controlled, non-destructive testing is necessary to detect corrosion of the reinforced concrete structures at the Fukushima Daiichi Nuclear Power Plant (NPP) de-commissioning site. This work aims to demonstrate that laser-induced ultrasonic guided wave technology can be applied to achieve this task. Hence, accelerated electrolytic corrosion is performed on a reinforced concrete specimen fabricated by embedding a steel rod into mortar. Waveforms of the laser-induced ultrasonic guided wave on the rod are measured with a previously employed piezoelectric transducer (PZT) probe, for each fixed corrosion time. Based on the results of Fourier and wavelet transforms of the waveforms, issues concerning the detection and extent of rebar corrosion are discussed. It is exhibited that the changes in bonding strength due to corrosion are distinguishable in the frequency domain of the ultrasonic signal.

Journal Articles

Dynamic properties of human $$alpha$$-synuclein related to propensity to amyloid fibril formation

Fujiwara, Satoru*; Kono, Fumiaki*; Matsuo, Tatsuhito*; Sugimoto, Yasunobu*; Matsumoto, Tomoharu*; Narita, Tetsuhiro*; Shibata, Kaoru

Journal of Molecular Biology, 431(17), p.3229 - 3245, 2019/08

 Times Cited Count:15 Percentile:51.31(Biochemistry & Molecular Biology)

$$alpha$$-synuclein ($$alpha$$Syn) is an intrinsically disordered protein (IDP) with unknown function. $$alpha$$Syn is known to form amyloid fibrils, which are implicated with the pathogenesis of Parkinson's disease and other synucleinopathies. Elucidating the mechanism of fibril formation of $$alpha$$Syn is therefore important for understanding the mechanism of the pathogenesis of these diseases. Here, using the quasielastic neutron scattering (QENS) and small-angle X-ray scattering (SAXS) techniques, we investigated the dynamic and structural properties of $$alpha$$Syn. These results imply that fibril formation of $$alpha$$Syn requires not only the enhanced local motions but also the segmental motions such that the proper inter-molecular interactions are possible.

Journal Articles

Real time and real space analysis for coherent QENS and its application to liquid bismuth

Kikuchi, Tatsuya*; Kawakita, Yukinobu

Physica B; Condensed Matter, 567, p.51 - 54, 2019/08

 Times Cited Count:0 Percentile:0.00(Physics, Condensed Matter)

Journal Articles

Measurement of neutron scattering cross section of nano-diamond with particle diameter of approximately 5 nm in energy range of 0.2 meV to 100 meV

Teshigawara, Makoto; Tsuchikawa, Yusuke*; Ichikawa, Go*; Takata, Shinichi; Mishima, Kenji*; Harada, Masahide; Oi, Motoki; Kawamura, Yukihiko*; Kai, Tetsuya; Kawamura, Seiko; et al.

Nuclear Instruments and Methods in Physics Research A, 929, p.113 - 120, 2019/06

 Times Cited Count:21 Percentile:89.29(Instruments & Instrumentation)

A nano-diamond is an attractive neutron reflection material below cold neutron energy. The total neutron cross section of a nano-diamond was derived from a neutron transmission measurement over the neutron energy range of 0.2 meV to 100 meV because total neutron cross section data were not available. The total cross section of a nano-diamond with particle size of approximately 5 nm increased with a decrease in neutron energy to 0.2 meV. It was approximately two orders of magnitude larger than that of graphite at 0.2 meV. The contribution of inelastic scattering to the total cross section was to be shown negligible small at neutron energies of 1.2, 1.5, 1.9, 2.6, and 5.9 meV in the inelastic neutron scattering measurement. Moreover, small-angle neutron scattering measurements of the nano-diamond showed a large scattering cross section in the forward direction for low neutron energies.

Journal Articles

Thermal and mechanical properties of CeO$$_{2}$$

Suzuki, Kiichi; Kato, Masato; Sunaoshi, Takeo*; Uno, Hiroki*; Carvajal-Nunez, U.*; Nelson, A. T.*; McClellan, K. J.*

Journal of the American Ceramic Society, 102(4), p.1994 - 2008, 2019/04

 Times Cited Count:50 Percentile:92.86(Materials Science, Ceramics)

The fundamental properties of CeO$$_{2}$$ were assessed using a range of experimental techniques. The oxygen potential of CeO$$_{2}$$ was measured by the thermogravimetric technique, and a numerical fit for the oxygen potential of CeO$$_{2}$$ is derived based on defect chemistry. Mechanical properties of CeO$$_{2}$$ were obtained using sound velocity measurement, resonant ultrasound spectroscopy and nanoindentation. The obtained mechanical properties of CeO$$_{2}$$ are then used to evaluate the Debye temperature and Gruneisen constant. The heat capacity and thermal conductivity of CeO$$_{2}$$ were also calculated using the Debye temperature and the Gruneisen constant. Finally, the thermal conductivity was calculated based upon laser flash analysis measurements. This result demonstrates that the thermal conductivity has strong dependence upon material purity.

154 (Records 1-20 displayed on this page)