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Oshima, Masumi*; Goto, Jun*; Hayakawa, Takehito*; Asai, Masato; Kin, Tadahiro*; Shinohara, Hirofumi*
Isotope News, (790), p.19 - 23, 2023/12
When analyzing samples that contain many radionuclides at various concentrations, such as radioactive waste or fuel debris, it is difficult to apply general spectrum analysis methods and is necessary to chemically separate each nuclide before quantifying it. The chemical separation is especially essential for analysis using a liquid scintillation counter (LSC). In this report, the authors explain the newly developed spectral determination method (SDM) in which the entire spectrum is fitted to quantify radioactivity of nuclides mixed in a sample. By applying the SDM to - and X-ray spectrum measured by LSC and -ray spectrum measured by Ge detector simultaneously, the authors demonstrated that radioactivity of 40 radionuclides mixed in a sample at concentrations varying by two orders could be quantified, which is useful to simplify chemical separation process in radionuclide quantification.
Urushidate, Tadayuki*; Yoda, Tomoyuki; Otani, Shuichi*; Yamaguchi, Toshio*; Kunii, Nobuaki*; Kuriki, Kazuki*; Fujiwara, Kenso; Niizato, Tadafumi; Kitamura, Akihiro; Iijima, Kazuki
JAEA-Review 2022-023, 8 Pages, 2022/09
After the accident of the Fukushima Daiichi Nuclear Power Station, the Japan Atomic Energy Agency has newly set up a laboratory in Fukushima and started measuring radioactivity concentrations of environmental samples. In October 2015, Fukushima Radiation Measurement Group has been accredited the ISO/IEC 17025 standard by the Japan Accreditation Board (JAB) as a testing laboratory for radioactivity analysis (Cs, Cs) based on Gamma-ray spectrometry with germanium semiconductor detectors. The laboratory has measured approximately 60,000 of various environmental samples at the end of March 2022. The laboratory quality control and measurement techniques have been accredited by regular surveillance of JAB. In September 2019, the laboratory renewed accreditation as a testing laboratory for radioactivity analysis.
Omer, M.; Shizuma, Toshiyuki*; Hajima, Ryoichi*; Koizumi, Mitsuo
Radiation Physics and Chemistry, 198, p.110241_1 - 110241_7, 2022/09
Times Cited Count:4 Percentile:63.92(Chemistry, Physical)Collaborative Laboratories for Advanced Decommissioning Science; National Institute of Advanced Industrial Science and Technology*
JAEA-Review 2021-026, 47 Pages, 2021/11
The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2020. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2019, this report summarizes the research results of the "Development of radiation hardened diamond image sensing devices" conducted in FY2020. The research objective of this project is to develop image sensing devices which work under the high radiation condition. The devices will be realized using radiation hardened diamond semiconductor devices as charge transfer devices and photodetectors. The research project has mainly two targets such as to confirm charge coupled devices operation on diamond unipolar devices and to characterize photo conductivity of diamond detectors.
Harada, Masahide; Sekijima, Mitsuaki*; Morikawa, Noriyuki*; Masuda, Shiho; Kinoshita, Hidetaka; Sakai, Kenji; Kai, Tetsuya; Kasugai, Yoshimi; Muto, Giichi*; Suzuki, Akio*; et al.
JPS Conference Proceedings (Internet), 33, p.011099_1 - 011099_6, 2021/03
In MLF at J-PARC, a unified mercury radioactivity monitor (UHAM) is installed to find an indication of failure of the mercury target and loop system by detecting radioactive materials leaked from the system with a -ray energy analysis with Germanium semi-conductor detectors (Ge detectors). It is composed of three units of sampling port and radiation monitors: (1) HAM for interstitial helium gas layer between the mercury vessel and surrounding water shroud of the mercury target, (2) CAM for atmosphere in the hot cell where the target loop is operated and (3) VAM for helium gas in the helium vessel where the target vessel is installed. Once any leakages of radioactive materials are detected, an alarm signal is issued immediately to the accelerator control system to stop beam operation. Software and hardware have been upgraded yearly. For example, two Ge detectors are used for HAM for redundancy, NaI Scintillation detectors are also used as supplemental for the Ge detector to keep availability of the system for high counting rate event. In April 2015, the UHAM activated when a small water coolant leakage from the water shroud of the mercury target occurred. VAM detected an abnormal increase of the counting rate in the helium vessel. It was also indicated that the measured radioactive nuclides were generated from the activation of the coolant (water) in the water shroud and not from the mercury.
Collaborative Laboratories for Advanced Decommissioning Science; National Institute of Advanced Industrial Science and Technology*
JAEA-Review 2020-027, 27 Pages, 2021/01
The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2019. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2019, this report summarizes the research results of the "Development of radiation hard diamond image sensing devices". The research objective of this project is to develop image sensing devices which work under the high radiation condition. The devices will be realized using radiation hard diamond semiconductor devices as charge transfer devices and photodetectors. The research project has mainly two targets such as to confirm charge coupled devices operation on diamond unipolar devices and to characterize photo conductivity of diamond detectors.
Kitayama, Yoshiharu; Terasaka, Yuta; Sato, Yuki; Torii, Tatsuo
Proceedings of International Youth Nuclear Congress 2020 (IYNC 2020) (Internet), 4 Pages, 2020/05
Kurihara, Momo*; Yasutaka, Tetsuo*; Aono, Tatsuo*; Ashikawa, Nobuo*; Ebina, Hiroyuki*; Iijima, Takeshi*; Ishimaru, Kei*; Kanai, Ramon*; Karube, Jinichi*; Konnai, Yae*; et al.
Journal of Radioanalytical and Nuclear Chemistry, 322(2), p.477 - 485, 2019/11
Times Cited Count:4 Percentile:37.41(Chemistry, Analytical)We assessed the repeatability and reproducibility of methods for determining low dissolved radiocesium concentrations in freshwater in Fukushima. Twenty-one laboratories pre-concentrated three of 10 L samples by five different pre-concentration methods (prussian-blue-impregnated filter cartridges, coprecipitation with ammonium phosphomolybdate, evaporation, solid-phase extraction disks, and ion-exchange resin columns), and activity of radiocesium was measured. The z-scores for all of the Cs results were within 2, indicating that the methods were accurate. The relative standard deviations (RSDs) indicating the variability in the results from different laboratories were larger than the RSDs indicating the variability in the results from each separate laboratory.
Kai, Tetsuya; Hiroi, Kosuke; Su, Y. H.; Shinohara, Takenao; Parker, J. D.*; Matsumoto, Yoshihiro*; Hayashida, Hirotoshi*; Segawa, Mariko; Nakatani, Takeshi; Oikawa, Kenichi; et al.
Physics Procedia, 88, p.306 - 313, 2017/06
Times Cited Count:5 Percentile:88.13(Instruments & Instrumentation)Mikami, Satoshi; Matsuda, Norihiro; Ando, Masaki; Kinase, Sakae; Kitano, Mitsuaki; Kawase, Keiichi; Matsumoto, Shinichiro; Yamamoto, Hideaki; Saito, Kimiaki
Radioisotopes, 64(9), p.589 - 607, 2015/09
This article presents the features of regional distributions and temporal changes in air dose rate and radionuclide deposition densities in Fukushima on the basis of analyses on large-scale environmental monitoring results using diverse methods. The continuity of decontamination effects is discussed according to repeated monitoring data after the decontamination model project. Further, some examples are shown on the projection of air dose rates together with the ecological half lives for different land uses.
Tsuda, Shuichi; Yoshida, Tadayoshi; Ando, Masaki; Matsuda, Norihiro; Mikami, Satoshi; Tanigaki, Minoru*; Okumura, Ryo*; Takamiya, Koichi*; Sato, Nobuhiro*; Seki, Akiyuki; et al.
Radioisotopes, 64(4), p.275 - 289, 2015/04
This article provides practically useful information on air dose rate measurements in the environments. The basic requirements for the accurate measurements are described giving actual data. The characteristics and some measured results are shown for reliable methods which are widely used in the environmental radiation measurements. Further, information is given on internet sites where air dose rates and related data obtained by official organizations can be browsed.
Nakamura, Tatsuya; Katagiri, Masaki; Chen, Y. E.*; Ukibe, Masahiro*; Okubo, Masataka*
Nuclear Instruments and Methods in Physics Research A, 559(2), p.766 - 768, 2006/04
Times Cited Count:13 Percentile:65.10(Instruments & Instrumentation)We have been developing a position-sensitive neutron detector, which exhibits a high spatial resolution of the order of 10 microns and high detection efficiency. The analysis on the pulse-heights or on the time-delay between the STJs gives incident positions of the neutrons. In this paper, the response of the STJs/LBO neutron detector measured using a cold neutron beam is presented. The two STJs have the same size of 50 50 m and their distance is 1.3 mm. The count intensity in the correlation map varied depending on the incident position of the neutron beam which gives an evidence for the position-sensitivity of the detector. These experimental results were qualitatively understood by a simple solid-angle model.
Kondo, Keitaro; Takagi, Satoshi*; Murata, Isao*; Miyamaru, Hiroyuki*; Takahashi, Akito*; Kubota, Naoyoshi; Ochiai, Kentaro; Nishitani, Takeo
Fusion Engineering and Design, 81(8-14), p.1527 - 1533, 2006/02
Times Cited Count:14 Percentile:67.66(Nuclear Science & Technology)In a fusion reactor development, double-differential charged-particle emission cross sections(DDXc) are necessary to estimate nuclear heating and material damages of candidate materials irradiated with neutrons. Especially in light nuclei such as Be, Li, and C, nuclear reactions are complicated and difficult to estimate energy spectra of emitted particles based only on theoretical calculations Therefore development of a new technique for precise measurements of DDXc is quite important. Recently we successfully developed a new spectrometer for measurement of DDXc using a pencil-beam DT neutron source of FNS in JAERI. In the present study we carried out measurements of DDXc of Be, C, F, and Al using the spectrometer. The present technique was valid from the result of measurement for the Al(n,x) reactions. Slight differences appeared between measured data and evaluation or previous experimental values for Be(n,x) reactions at backward scattering angle and in lower energy region.
Yamasoto, Kotaro; Tsutsumi, Masahiro; Oishi, Tetsuya*; Yoshizawa, Michio; Yoshida, Makoto
Nuclear Instruments and Methods in Physics Research A, 550(3), p.609 - 615, 2005/09
Times Cited Count:5 Percentile:40.67(Instruments & Instrumentation)A phoswich detector composed of a thin plate CsI(Tl) scintillator and a plastic scintillator (BC-400) has been designed and evaluated to improve the sensitivity in the low-energy region of large-area plastic scintillation detector. Applicability of the CsI(Tl)/Plastic phoswich detector was examined on radioactivity measurement of massive and large-area materials. The rise-time discrimination technique was applied in order to further improve the minimum detectable activity in the low-energy region. On the basis of the estimation of minimum detectable activity, it was made clear that the energy range of large-area plastic scintillation detector can be expanded down to a few tens of keV by adding a thin plate CsI(Tl) scintillator.
Kawasaki, Katsuya
Hoken Butsuri, 40(1), p.56 - 60, 2005/03
The centralized radioactivity measurement system has been used to carry out intensively measurements of a large number and variety of samples that are necessary for the control of radioactivity in the facilities of the JAERI Tokai Establishment and its environment. The operation of the system started in 1981, and presently the system processes more than 20,000 samples a year. However, the computers of the system have aged so much that the manufacturer's support and stable operation are no longer sure. Therefore, we renewed and restructured the computer system in 2003. A client-server system was adopted in the new system. The information of samples can be registered through the intranet. The clients can also confirm the progress of processing of their samples and browse the analytical results from their own computers. The renewed system can provide some convenience functions to the clients. This report is introduced about the centralized radioactivity measurement system.
Kawasaki, Katsuya; Mochizuki, Kaoru*; Suzuki, Takehiko; Kinouchi, Nobuyuki
JAERI-Tech 2004-070, 50 Pages, 2004/12
The centralized radioactivity measurement system has been used to carry out intensively measurements of a large number and variety of samples that are necessary for the control of radioactivity in the facilities of the JAERI Tokai Establishment and its environment. The operation of the system started in 1981, and presently the system processes more than 20,000 samples a year. However, the computers of the system have aged so much that the manufacturer's support and stable operation are no longer sure. Therefore, we renewed and restructured the computer system in 2003. A client-server system was adopted in the new system. The information of samples can be registered through the intranet. The clients can also confirm the progress of processing of their samples and browse the analytical results from their own computers. The renewed system can provide some convenience functions to the clients.
Saegusa, Jun; Kawasaki, Katsuya; Mihara, Akira; Ito, Mitsuo; Yoshida, Makoto
Applied Radiation and Isotopes, 61(6), p.1383 - 1390, 2004/12
Times Cited Count:29 Percentile:84.78(Chemistry, Inorganic & Nuclear)no abstracts in English
Yamagishi, Hideshi; Nakamura, Tatsuya; Soyama, Kazuhiko; Masaoka, Sei; Aizawa, Kazuya
Review of Scientific Instruments, 75(7), p.2340 - 2345, 2004/07
Times Cited Count:9 Percentile:45.56(Instruments & Instrumentation)A new instrument system with the capability of secondary-particle discrimination (InSPaD) was studied for the development of two-dimensional neutron detectors (2D-ND) filled with helium-3 gas and with high spatial resolution. The InSPaD can discriminate between the tracks of a proton and a triton created in the nuclear reaction He(,) by simply setting the level of discriminators appropriately in each signal channel, and the system exhibits a high spatial resolution, high counting rate, low background, and stability. The simulations of the 2D-ND equipped with the InSPaD revealed spatial resolutions of 0.46 mm in full width at half maximum for a 10% mixture of CH with helium-3 at 0.3 MPa. The results of neutron-detection experiments using a microstrip gas chamber, including the range of the secondary particles and the pulse-height distribution, agreed well with the simulated results, indicating the feasibility of the InSPaD.
Ito, Haruhiko; Homma, Kenzo; Itabashi, Yukio; Tabata, Toshio; Akashi, Kazutomo; Inaba, Yukio; Kumahara, Hajime; Takahashi, Kunihiro; Kitajima, Toshio; Yokouchi, Iichiro
JAERI-Review 2003-024, 76 Pages, 2003/10
no abstracts in English
Kanno, Ikuo*; Yoshihara, Fumiki*; Nouchi, Ryo*; Sugiura, Osamu*; Murase, Yasuhiro*; Nakamura, Tatsuya; Katagiri, Masaki
Review of Scientific Instruments, 74(9), p.3968 - 3973, 2003/09
Times Cited Count:18 Percentile:65.44(Instruments & Instrumentation)junction-type radiation detectors were fabricated with an InSb substrate. The detectors had 1000 times higher resistances than the ones of the previously reported Schottky-type detectors. The output pulses of the preamplifier were analyzed from the point of view of the contribution of electrons and holes. The energy spectra of Am alpha particles were measured at operating temperatures of up to 115 K. The inherent voltage of the detector was estimated.