Effect of grain refinement on cracks occurring in SUS304L stainless steel under nuclear reactor operating conditions

Hirota, Noriaki; Takeda, Ryoma; Ide, Hiroshi; Tsuchiya, Kunihiko; Kobayashi, Yoshinao*

Nuclear Materials and Energy (Internet), 45, p.102009_1 - 402009_10, 2025/12

https://doi.org/10.1016/j.nme.2025.102009

Using SUS304L stainless steel, which is employed in reactor structural components, the effects of grain refinement on stress corrosion cracking occurring under nuclear reactor operating conditions were investigated. As a result, after conducting slow strain rate testing (SSRT) in air and nuclear reactor operating environments, a comparison of the tensile properties of SUS304L with the same grain size revealed that elongation significantly decreased with increasing grain size under nuclear reactor operating conditions. In SSRT conducted in air, the -value obtained from the Hall-Petch relationship was lower than the conventional values. Observations showed the absence of cracks on SUS304L with 0.59 and 1.52 m grains; however, SUS304L with larger grains exhibited rougher fracture surfaces and side cracks. Thin oxide films were formed on SUS304L with 0.59 m and 1.52 m grains, while SUS304L with coarse grains of 28.4 m or larger enabled the formation of oxide films with over 2 m thickness. CrO films were formed on SUS304L with 0.59 m, 1.52 m, and 28.4 m, while CrO and Fe based oxides were formed on SUS304L with 39.5 m and 68.6 m. Crystal orientation analysis revealed linear surface layers without cracks in the -phase for SUS304L with 0.59 m and 1.52 m. In materials with Larger grain sizes, surface irregularities and cracks were observed in the -phase. In fine-grained SUS304L, lattice diffusion caused uniform O diffusion in the -phase, resulting in the formation of a thin CrO layer that suppressed cracks. In coarse-grained SUS304L, grain boundary diffusion caused Fe oxide formation at the grain boundaries, weakening them, and supersaturated O led to the formation of thick films comprising CrO and Fe-based oxides, resulting in peeling and cracking.

Current status and future prospects of the Horonobe International Project (HIP), 4; Task C: Full-scale Engineering Barrier System (EBS) dismantling experiment

Ono, Hirokazu

Genshiryoku Bakkuendo Kenkyu (CD-ROM), 31(2), p.140 - 143, 2024/12

https://nuce.aesj.or.jp/jnuce/vol31/jnuce-vol31-2-p140-143.pdf

In the geological disposal of high-level radioactive waste, after emplacement of an EBS, the near-field environment is affected by processes such as heat release from the waste, groundwater infiltration into the EBS, swelling and deformation of the buffer material, and chemical reactions between groundwater and minerals. It is crucial to develop simulation codes to evaluate such coupled thermal-hydraulic-stress-chemical (THMC) processes for safety assessment of geological disposal. The full-scale vertical-emplacement EBS experiment (Horonobe EBS experiment) has been undertaken in the 350 m gallery of the Horonobe Underground Research Laboratory (URL) with the Horonobe geological environment. In the Horonobe EBS experiment, various sensors were installed in the buffer and backfill material to obtain the data required to evaluate coupled THMC processes in near-field. In Task C of the Horonobe International Project (HIP), the dismantling experiment of the Horonobe EBS experiment will be carried out and the data obtained from this experiment will be used to understand the coupled processes and to evaluate the simulation code.

Development of a radiation tolerant laser-induced breakdown spectroscopy system using a single crystal micro-chip laser for remote elemental analysis

Tamura, Koji; Nakanishi, Ryuzo; Oba, Hironori; Karino, Takahiro; Shibata, Takuya; Taira, Takunori*; Wakaida, Ikuo

Journal of Nuclear Science and Technology, 61(8), p.1109 - 1116, 2024/08

https://doi.org/10.1080/00223131.2023.2298485

Consideration on roles and relationship between observations/measurements and model predictions for environmental consequence assessments for nuclear facilities

Togawa, Orihiko; Okura, Takehisa; Kimura, Masanori

JAEA-Review 2022-049, 76 Pages, 2023/01

JAEA-Review-2022-049.pdf:3.74MB

Before construction and after operation of nuclear facilities, environmental consequence assessments are conducted for normal operation and an emergency. These assessments mainly aim at confirming safety for the public around the facilities and producing relief for them. Environmental consequence assessments are carried out using observations/ measurements by environmental monitoring and/or model predictions by calculation models, sometimes using either of which and at other times using both them, according to the situations and necessities. First, this report investigates methods, roles, merits/demerits and relationship between observations/measurements and model predictions which are used for environmental consequence assessments of nuclear facilities, especially holding up a spent nuclear fuel reprocessing plant at Rokkasho, Aomori as an example. Next, it explains representative examples of utilization of data on observations/measurements and results on model predictions, and considers points of attention at using them. Finally, the report describes future direction, for example, improvements of observations/measurements and model predictions, and fusion of both them.

Design of microchannel suitable for packing with anion exchange resins; Uranium separation from seawater containing a large amount of cesium

Ouchi, Kazuki; Tsukahara, Takehiko*; Brandt, A.*; Muto, Yuki*; Nabatame, Nozomi*; Kitatsuji, Yoshihiro

Analytical Sciences, 37(12), p.1789 - 1794, 2021/12

https://doi.org/10.2116/analsci.21P110

We attempted to scale down a separation process of uranium (U) using the microchip column loaded with anion exchange resin to develop safety and waste-reducing separation technique. The ideal separation performance of U was obtained by the properly design of a microchannel. The concentration of U in seawater as a real-world sample could be quantified with the prepared microchip column. It indicates that the microchip column is sufficiently practical. Compared to separation of U with a general column, the column size was successfully scaled down to 1/5000.

Implementation of a low-activation Au-In-Cd decoupler into the J-PARC 1 MW short pulsed spallation neutron source

Teshigawara, Makoto; Ikeda, Yujiro; Oi, Motoki; Harada, Masahide; Takada, Hiroshi; Kakishiro, Masanori*; Noguchi, Gaku*; Shimada, Tsubasa*; Seita, Kyoichi*; Murashima, Daisuke*; et al.

Nuclear Materials and Energy (Internet), 14, p.14 - 21, 2018/01

https://doi.org/10.1016/j.nme.2018.02.001

We developed an Au-In-Cd (AuIC) decoupler material to reduce induced radioactivity instead of Ag-In-Cd one, which has a cut off energy of 1eV. In order to implement it into an actual moderator-reflector assembly, a number of critical engineering issues need to be resolved with regard to large-sized bonding between AuIC and A5083 alloys by the hot isostatic pressing process. We investigated this process in terms of the surface conditions, sizes, and heat capacities of large AuIC alloys. We also show a successful implementation of an AuIC decoupler into a reflector assembly, resulting in a remarkable reduction of radioactivity by AuIC compared to AIC without sacrificing neutronic performance.

Effects of irradiation on mechanical properties of HIP-bonded reduced-activation ferritic/martensitic steel F82H first wall

Furuya, Kazuyuki; Wakai, Eiichi; Miyamoto, Kenji*; Akiba, Masato; Sugimoto, Masayoshi

Journal of Nuclear Materials, 367-370(1), p.494 - 499, 2007/08

https://doi.org/10.1016/j.jnucmat.2007.03.011

A partial mock-up of a breeding blanket structure made of F82H steel has been successfully fabricated. In this study, microstructural observation and EDX analysis of the HIP interfaces were performed, and effects of irradiation on mechanical properties of the HIP-bonded region were also examined. Neutron irradiation was performed up to about 2 dpa at about 523 K. After the irradiation, tensile test was performed at temperatures of 295 and 523 K. The HIP interfaces possessed many precipitates, and enriched peak spectrum of chromium was detected from the precipitates. In addition, aspect of the spectrum was qualitatively equivalent to that of MC in grain boundaries of F82H steel. In result, the HIP boundary has many MC which were generally seen in grain boundaries of F82H steel. Rupture did not occur in the HIP interface. In result, it can be mentioned that bondability is maintained under the irradiation and testing conditions. The strength and elongation of the HIP-bonded region decreased somewhat in comparison with the results of an IEA standard steel.

Neutron irradiation effect on mechanical properties of SS/SS HIP joint materials for ITER shielding blankets

Yamada, Hirokazu*; Sato, Satoshi; Mori, Kensuke*; Nagao, Yoshiharu; Takada, Fumiki; Kawamura, Hiroshi

Fusion Engineering and Design, 81(1-7), p.631 - 637, 2006/02

https://doi.org/10.1016/j.fusengdes.2005.07.012

This study estimated the neutron irradiation effect with 1.5 dpa on the mechanical properties of the SS/SS HIP joint materials jointed in the standard HIP joint condition. Results of this study showed that the HIP process in the standard HIP condition could make SS/SS HIP joint material of which tensile properties was equivalent to that of the SS base material. In addition, the effect of surface roughness at the HIP joint material on the mechanical properties of SS/SS HIP joint material was estimated.

Cladding technique for development of Ag-In-Cd decoupler

Teshigawara, Makoto; Harada, Masahide; Saito, Shigeru; Kikuchi, Kenji; Kogawa, Hiroyuki; Ikeda, Yujiro; Kawai, Masayoshi*; Kurishita, Hiroaki*; Konashi, Kenji*

Journal of Nuclear Materials, 343(1-3), p.154 - 162, 2005/08

https://doi.org/10.1016/j.jnucmat.2004.08.036

For decoupled and poisoned moderator, a thermal neutron absorber, i.e., decoupler, is located around the moderator to give neutron beam with a short decay time. A B4C decoupler is already utilized, however, it is difficult to use in a MW class source because of He void swelling and local heating by (n,a) reaction. Therefore, a Ag-In-Cd (AIC) alloy which gives energy-dependence of macroscopic neutron cross section like that of BC was chosen. However, from heat removal and corrosion protection points of view, AIC is needed to bond between an Al alloy (A6061-T6), which is the structural material of a moderator. An AIC plate is divided into a Ag-In (15wt%) and Ag-Cd (35wt%) plate to extend the life time, shorten by burn up of Cd. We performed bonding tests by HIP (Hot Isostatic Pressing). We found out that a better HIP condition was holding at 803 K, 100 MPa for 1 h for small test pieces (f20mm). Though a hardened layer is found in the bonding layer, the rupture strength of the bonding layer is more than 20 MPa, which is less than that of the design stress.

Fabrication of model for fusion nuclear first wall made from F82H steel by HIP method and the metallurgical and mechanical properties

Furuya, Kazuyuki

JAERI-Research 2004-013, 165 Pages, 2004/09

JAERI-Research-2004-013.pdf:53.73MB

no abstracts in English