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Journal Articles

Hydrogen permeation property of bulk cementite

Adachi, Nozomu*; Ueno, Haruki*; Onoe, Katsuhiko*; Morooka, Satoshi; Todaka, Yoshikazu*

ISIJ International, 61(8), p.2320 - 2322, 2021/08

 Times Cited Count:0

Journal Articles

Development of a membrane reactor with a closed-end silica membrane for nuclear-heated hydrogen production

Myagmarjav, O.; Tanaka, Nobuyuki; Nomura, Mikihiro*; Noguchi, Hiroki; Imai, Yoshiyuki; Kamiji, Yu; Kubo, Shinji; Takegami, Hiroaki

Progress in Nuclear Energy, 137, p.103772_1 - 103772_7, 2021/07

 Times Cited Count:1 Percentile:83.53(Nuclear Science & Technology)

Journal Articles

Kinetic and Fourier transform infrared studies on the thermal decomposition of sodium hydride

Kawaguchi, Munemichi

Journal of Physical Chemistry C, 125(22), p.11813 - 11819, 2021/06

Isothermal and constant heating thermogravimetry-differential thermal analysis (TG-DTA) and Fourier transform infrared spectrometer (FTIR) measurements have been performed for pre- and post-fired sodium hydride (NaH) in the temperature range of 500-700 K, respectively. Temperature dependence of NaH thermal decomposition rates obtained by the isothermal TGs showed an inflection point at around 620 K, which was caused by two kinds of hydrogen states (rapid diffusing and immobile hydrogen). In the FTIR spectra for the NaH and sodium (Na), the specific signals were observed at around 873.4, 1010.4, 1049.5 and 1125.7 cm$$^{-1}$$, and the integrated values of FTIR signals for post-fired NaH at below 550K and at above 698 K were comparable to those for pre-fired NaH and Na, respectively. Those for post-fired NaH at 602-667 K were the intermediate values of the pre-fired NaH and Na, which denoted that the Na-Na bonds haven't grown sufficiently and the hydrogen coexisted in metallic Na. In order to predict the practical kinetics of NaH thermal decomposition reaction, we suggested the simple kinetics model which assumed two kinds of rapidly diffusing and immobile hydrogen states. The simulation results revealed the inflection point in temperature dependence of the thermal decomposition rates accordingly because the transition from immobile hydrogen to rapid diffusing hydrogen crosses over at around 620 K.

Journal Articles

Evaluation of core material energy change during the in-vessel phase of Fukushima Daiichi Unit 3 based on observed pressure data utilizing GOTHIC code analysis

Sato, Ikken; Arai, Yuta*; Yoshikawa, Shinji

Journal of Nuclear Science and Technology, 58(4), p.434 - 460, 2021/04

 Times Cited Count:2 Percentile:95.57(Nuclear Science & Technology)

Journal Articles

High temperature gas-cooled reactors

Takeda, Tetsuaki*; Inagaki, Yoshiyuki; Aihara, Jun; Aoki, Takeshi; Fujiwara, Yusuke; Fukaya, Yuji; Goto, Minoru; Ho, H. Q.; Iigaki, Kazuhiko; Imai, Yoshiyuki; et al.

High Temperature Gas-Cooled Reactors; JSME Series in Thermal and Nuclear Power Generation, Vol.5, 464 Pages, 2021/02

As a general overview of the research and development of a High Temperature Gas-cooled Reactor (HTGR) in JAEA, this book describes the achievements by the High Temperature Engineering Test Reactor (HTTR) on the designs, key component technologies such as fuel, reactor internals, high temperature components, etc., and operational experience such as rise-to-power tests, high temperature operation at 950$$^{circ}$$C, safety demonstration tests, etc. In addition, based on the knowledge of the HTTR, the development of designs and component technologies such as high performance fuel, helium gas turbine and hydrogen production by IS process for commercial HTGRs are described. These results are very useful for the future development of HTGRs. This book is published as one of a series of technical books on fossil fuel and nuclear energy systems by the Power Energy Systems Division of the Japan Society of Mechanical Engineers.

Journal Articles

Online measurement of the atmosphere around geopolymers under gamma irradiation

Cantarel, V.; Lambertin, D.*; Labed, V.*; Yamagishi, Isao

Journal of Nuclear Science and Technology, 58(1), p.62 - 71, 2021/01

 Times Cited Count:0 Percentile:0.01(Nuclear Science & Technology)

The gas production of wasteforms is a major safety concern for encapsulating active nuclear wastes. For geopolymers and cements, the H$$_{2}$$ produced by radiolytic processes is a key factor because of the large amount of water present in their porous structure. Herein, the gas composition evolution around geopolymers was monitored on line under $$^{60}$$Co gamma irradiation. Transient evolution of the hydrogen production yield was measured for samples with different formulations. The rate of its evolution and the final values are consistent with the presence of a chemical reaction of the pseudo-first order consuming hydrogen in the samples. The results show this phenomenon can significantly reduce the hydrogen source term of geopolymer wasteform provided their diffusion constant remains low. Lower hydrogen production rates and faster kinetics were observed with geopolymers formulations in which pore water pH was higher. Besides hydrogen production, a steady oxygen consumption was observed for all geopolymers samples. The oxygen consumption rates are proportional to the diffusion constants estimated in the modelization of hydrogen recombination by a pseudo first order reaction.

JAEA Reports

Interdisciplinary evaluation of biological effect of internal exposure by inhaling alpha-ray emitting nuclides represented by radon (Contract research); FY2019 Nuclear Energy Science & Technology and Human Resource Development Project

Collaborative Laboratories for Advanced Decommissioning Science; Okayama University*

JAEA-Review 2020-029, 55 Pages, 2020/12


JAEA/CLADS had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project in FY2019. Among the adopted proposals in FY2018, this report summarizes the research results of the "Interdisciplinary Evaluation of Biological Effect of Internal Exposure by Inhaling Alpha-ray Emitting Nuclides Represented by Radon" conducted in FY2019.

JAEA Reports

Assessment report on research and development activities in FY2019; Activity "Research and development on high temperature gas-cooled reactor and related heat application technology" (Interim report)

Sector of Fast Reactor and Advanced Reactor Research and Development

JAEA-Evaluation 2020-001, 128 Pages, 2020/08


Japan Atomic Energy Agency consulted with the "Evaluation Committee of Research Activities for High Temperature Gas-cooled Reactor (hereinafter referred to as "HTGR") and Related Hydrogen Production Technology" (hereinafter referred to as "Evaluation Committee"), which consists of specialists in the fields of the evaluation subjects of high temperature gas-cooled reactor and related heat application technology, for interim assessment in the 3rd Mid-and Long-Term Plan about the relevance of the management and research activities of the HTGR and related application technology during the period from April 2017 to March 2020. As a result, three members of the Evaluation Committee concluded a score of "S", and seven members of the Evaluation Committee concluded a score of "A". The interim assessment to research and development activities from April 2017 to March 2020 was concluded a score of "A". In addition, the Evaluation Committee recommended that the judgement to move to the construction phase of the HTTR-heat utilization test plant be made after 2 years, after the HTTR will be restarted and the thermal load fluctuation tests using HTTR will be carried out. This report lists the members of the Evaluation Committee and outlines the assessment item and the review process for procedure of the assessment. The assessment report which was issued by the Evaluation Committee is attached.

Journal Articles

Computational study on the spherical laminar flame speed of hydrogen-air mixtures

Trianti, N.; Motegi, Kosuke; Sugiyama, Tomoyuki; Maruyama, Yu

Proceedings of 2020 International Conference on Nuclear Engineering (ICONE 2020) (Internet), 9 Pages, 2020/08

Journal Articles

Modeling the processes of hydrogen isotopes interactions with solid surfaces

Chikhray, Y.*; Askerbekov, S.*; Kenzhin, Y.*; Gordienko, Y.*; Ishitsuka, Etsuo

Fusion Science and Technology, 76(4), p.494 - 502, 2020/05

 Times Cited Count:1 Percentile:42.23(Nuclear Science & Technology)

JAEA Reports

Interdisciplinary evaluation of biological effect of internal exposure by inhaling alpha-ray emitting nuclides represented by radon (Contract research); FY2018 Center of World Intelligence Project for Nuclear Science/Technology and Human Resource Development

Collaborative Laboratories for Advanced Decommissioning Science; Okayama University*

JAEA-Review 2019-024, 61 Pages, 2020/01


CLADS, JAEA, had been conducting the Center of World Intelligence Project for Nuclear Science/Technology and Human Resource Development (hereafter referred to "the Project") in FY2018. The Project aims to contribute to solving problems in nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2018, this report summarizes the research results of the "Interdisciplinary Evaluation of Biological Effect of Internal Exposure by Inhaling Alpha-ray Emitting Nuclides Represented by Radon". In the present study, the effect of alpha-ray emission in human body on the surrounding cells is estimated, and biological response to alpha-ray exposure is investigated at the whole organism level, by the evaluation method for radiation effects using radon that is an alpha-ray emitting nuclide, because there have been extensive studies on radon so far. From the obtained results, a model to evaluate the effect of internal exposure by alpha-ray emitting nuclides on health is constructed. Through these studies, we aim to form a research base by the interdisciplinary organic collaboration among research organizations.

Journal Articles

On the hydrogen production of geopolymer wasteforms under irradiation

Cantarel, V.; Arisaka, Makoto; Yamagishi, Isao

Journal of the American Ceramic Society, 102(12), p.7553 - 7563, 2019/12

 Times Cited Count:5 Percentile:50.87(Materials Science, Ceramics)

The hydrogen gas (H$$_{2}$$) production of wasteforms is a major safety concern for encapsulating nuclear wastes. For geopolymers, the H$$_{2}$$ produced by radiolytic processes is a key factor because of the large amount of water present in their porous structure. Herein, the hydrogen production was measured under $$^{60}$$Co gamma irradiation. The effect of water saturation and sample size were studied for pure geopolymers, or using zeolites as an example waste. When geopolymer monolithic samples were large and saturated by water, the hydrogen released was measured up to two orders of magnitude lower with a 40 cm long cylinder samples (1.9$$times$$10$$^{-10}$$ mol/J) than a sample in powder form (2.2$$times$$10$$^{-8}$$ mol/J). To interpret results, a simple model was used, considering only hydrogen production, a potential recombination and its diffusion in the geopolymer matrix. Knowing the diffusion constant of the matrix, the model was able to reproduce the evolution of the hydrogen release as a function of the water saturation level and predict the evolution when sample size is increased up to 40 cm.

Journal Articles

Isotope and plasma size scaling in ion temperature gradient driven turbulence

Idomura, Yasuhiro

Physics of Plasmas, 26(12), p.120703_1 - 120703_5, 2019/12

 Times Cited Count:2 Percentile:28.55(Physics, Fluids & Plasmas)

This Letter presents the impacts of the hydrogen isotope mass and the normalized gyroradius $$rho^*$$ on L-mode like hydrogen (H) and deuterium (D) plasmas dominated by ion temperature gradient driven (ITG) turbulence using global full-f gyrokinetic simulations. In ion heated numerical experiments with adiabatic electrons, the energy confinement time shows almost no isotope mass dependency, and is determined by Bohm like $$rho^*$$ scaling. Electron heated numerical experiments with kinetic electrons show clear isotope mass dependency caused by the isotope effect on the collisional energy transfer from electrons to ions, and the H and D plasmas show similar ion and electron temperature profiles at an H to D heating power ratio of $$sim 1.4$$. The normalized collisionless ion gyrokinetic equations for H and D plasmas become identical at the same $$rho^*$$, and collisions weakly affect ITG turbulence. Therefore, the isotope mass dependency is mainly contributed by the $$rho^*$$ scaling and the heating sources.

Journal Articles

Comparison of experimental and simulation results on catalytic HI decomposition in a silica-based ceramic membrane reactor

Myagmarjav, O.; Tanaka, Nobuyuki; Nomura, Mikihiro*; Kubo, Shinji

International Journal of Hydrogen Energy, 44(59), p.30832 - 30839, 2019/11

 Times Cited Count:7 Percentile:42.22(Chemistry, Physical)

JAEA Reports

Improvement of accumulator in cryogenic hydrogen system used for 1-MW pulsed spallation neutron source

Aso, Tomokazu; Tatsumoto, Hideki*; Otsu, Kiichi*; Kawakami, Yoshihiko*; Komori, Shinji*; Muto, Hideki*; Takada, Hiroshi

JAEA-Technology 2019-013, 77 Pages, 2019/09


At Materials and Life Science experimental Facility (MLF) of the Japan Proton Accelerator Research Complex (J-PARC), a 1-MW pulsed spallation neutron source is equipped with a cryogenic hydrogen system which circulates liquid hydrogen (20 K and 1.5 MPa) to convert high energy neutrons generated at a mercury target to cold neutrons at three moderators with removing nuclear heat of 3.8 kW deposited there. The cryogenic system includes an accumulator with a bellows structure in order to absorb pressure fluctuations generated by the nuclear heat deposition in the system. Welded inner bellows of the first accumulator was failured during operation, forcing us to improve the accumulator to have sufficient pressure resistance and longer life-time. We have developed elemental technologies for manufacturing welded bellows of the accumulator by a thick plate with high pressure resistance, succeeding to find optimum welding conditions. We fabricated a prototype bellows block and carried out an endurance test by adding a pressure change of 2 MPa repeatedly. As a result, the prototype bellows was successfully in use exceeding the design life of 10,000 times. Since distortions given during welding and assembling affect functionality and lifetime of the bellows, we set the levelness of each element of the bellows as within 0.1$$^{circ}$$. The improved accumulator has already been in operation for about 25,000 hours as of January 2019, resulting that the number of strokes reached to 16,000. In July 2018, we demonstrated that the accumulator could suppress the pressure fluctuation generated by the 932 kW beam injection as designed. As current operational beam power is 500 kW, the current cryogenic hydrogen system could be applicable for stable operation at higher power in the future.

Journal Articles

Formation mechanisms of insoluble Cs particles observed in Kanto district four days after Fukushima Daiichi NPP accident

Hidaka, Akihide

Journal of Nuclear Science and Technology, 56(9-10), p.831 - 841, 2019/09

 Times Cited Count:3 Percentile:44.1(Nuclear Science & Technology)

The insoluble Cs particles (Type A) were firstly observed in Tsukuba-city on the morning of March 15. The particles have been considered to be generated in RPV of Unit 2 by evaporation/condensation based on the measured $$^{134}$$Cs/$$^{137}$$Cs ratio and the core temperatures of each unit. However, the Type A particles with smaller diameter than the Type B particles of Unit 1 origin, are covered by almost pure silicate glass and have a trace of the quenching. This indicates that the particles could have been generated due to the melting of the HEPA filter in SGTS by the fire of H$$_{2}$$ detonation at Unit 3, and atomization followed by quenching of the molten materials by air blast of the explosion. Although the particles were mostly dispersed to the sea because of the wind direction, some of them deposited onto the lower elevation of R/B at Unit 3, could have been subsequently re-suspended and released into the environment, by the steam flow in the R/B caused by restart of the Unit 3 core cooling water injection at 2:30 of March 15.

Journal Articles

Estimation of hydrogen gas production at transient criticality in uranyl nitrate solution

Yoshida, Ryoichiro; Yamane, Yuichi; Abe, Hitoshi

Proceedings of International Nuclear Fuel Cycle Conference / Light Water Reactor Fuel Performance Conference (Global/Top Fuel 2019) (USB Flash Drive), p.408 - 414, 2019/09

In a criticality accident, it is known that some kinds of radiolysis gases are generated mainly due to kinetic energy of fission fragments. Hydrogen gas (H$$_{2}$$) is one of them, which is able to initiate explosion. The rate of H$$_{2}$$ generation and its total amount can be estimated from the number of fission per second if its G value is known. In this study, it was tried to estimate G value of hydrogen gas (G(H$$_{2}$$)) by using the H$$_{2}$$ concentration measured as time-series data in Transient Experiment Critical Facility (TRACY) which was carried out by Japan Atomic Energy Agency. There was time lag in the measured H$$_{2}$$ concentration from its generation. To overcome those problems, measured profile of H$$_{2}$$ concentration was reproduced based on a hypothetical model and its total amount was evaluated. Based on the model, the obtained G(H$$_{2}$$) was 1.2.

Journal Articles

CFD analysis of hydrogen flame acceleration with burning velocity models

Motegi, Kosuke; Trianti, N.; Matsumoto, Toshinori; Sugiyama, Tomoyuki; Maruyama, Yu

Proceedings of 18th International Topical Meeting on Nuclear Reactor Thermal Hydraulics (NURETH-18) (USB Flash Drive), p.4324 - 4335, 2019/08

Journal Articles

Research and development on membrane IS process for hydrogen production using solar heat

Myagmarjav, O.; Iwatsuki, Jin; Tanaka, Nobuyuki; Noguchi, Hiroki; Kamiji, Yu; Ioka, Ikuo; Kubo, Shinji; Nomura, Mikihiro*; Yamaki, Tetsuya*; Sawada, Shinichi*; et al.

International Journal of Hydrogen Energy, 44(35), p.19141 - 19152, 2019/07

 Times Cited Count:1 Percentile:68.51(Chemistry, Physical)

Journal Articles

Visualizing an ignition process of hydrogen jets containing sodium mist by high-speed imaging

Doi, Daisuke; Seino, Hiroshi; Miyahara, Shinya*; Uno, Masayoshi*

Journal of Nuclear Science and Technology, 56(6), p.521 - 532, 2019/06

 Times Cited Count:1 Percentile:0.01(Nuclear Science & Technology)

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