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Modeling the processes of hydrogen isotopes interactions with solid surfaces

Chikhray, Y.*; Askerbekov, S.*; Kenzhin, Y.*; Gordienko, Y.*; 石塚 悦男

Fusion Science and Technology, 76(4), p.494 - 502, 2020/05

 被引用回数:0 パーセンタイル:100(Nuclear Science & Technology)

The investigation of the mechanisms and dynamics of hydrogen isotopic interaction with solid surfaces (metals, ceramics, graphites, eutectics) in temperature and pressure ranges is important not only for the correct prediction of each isotope's evolution but also for substantiation of the safe operation of hydrogen-facing structural materials. The interaction of the hydrogen isotopes mix with the surface of solid metal or liquid eutectics is a complicated multistage H-D-T-O-solid interacting process depending on material property, environment, and the solid's surface parameters. To better understand the mechanisms of hydrogen isotopes interchange at a solid surface and to identify the limiting stages in the sorption-desorption processes, a reactor experiment of neutron irradiation was conducted with lithium-containing eutectics as tritium-generating media under the external flow of hydrogen. This work presents the model and results of its application to fitting the experimental results of tritium yield from the lithium-lead eutectics Pb$$_{83}$$Li$$_{17}$$under thermal neutrons irradiation at the IVG.1M reactor in Kazakhstan. The elaborated model and the approach used were also applied to the simulation of high temperature gas cooled reactor graphite corrosion in water vapors.


Promising neutron irradiation applications at the high temperature engineering test reactor

Ho, H. Q.; 本多 友貴*; 濱本 真平; 石井 俊晃; 高田 昌二; 藤本 望*; 石塚 悦男

Journal of Nuclear Engineering and Radiation Science, 6(2), p.021902_1 - 021902_6, 2020/04

High temperature engineering test reactor (HTTR), a prismatic type of the HTGR, has been constructed to establish and upgrade the basic technologies for the HTGRs. Many irradiation regions are reserved in the HTTR to be served as a potential tool for an irradiation test reactor in order to promote innovative basic researches such as materials, fusion reactor technology, and radiation chemistry and so on. This study shows the overview of some possible irradiation applications at the HTTRs including neutron transmutation doping silicon (NTD-Si) and iodine-125 ($$^{125}$$I) productions. The HTTR has possibility to produce about 40 tons of doped Si-particles per year for fabrication of spherical silicon solar cell. Besides, the HTTR could also produce about 1.8$$times$$10$$^{5}$$ GBq/year of $$^{125}$$I isotope, comparing to 3.0$$times$$10$$^{3}$$ GBq of total $$^{125}$$I supplied in Japan in 2016.


燃料デブリ取り出しを容易にするゲル状充填材の開発(委託研究); 平成30年度英知を結集した原子力科学技術・人材育成推進事業

廃炉国際共同研究センター; 大阪大学*

JAEA-Review 2019-029, 36 Pages, 2020/02




Mitigation of cavitation damage in J-PARC mercury target vessel

直江 崇; 木下 秀孝; 粉川 広行; 涌井 隆; 若井 栄一; 羽賀 勝洋; 高田 弘

JPS Conference Proceedings (Internet), 28, p.081004_1 - 081004_6, 2020/02



On the hydrogen production of geopolymer wasteforms under irradiation

Cantarel, V.; 有阪 真; 山岸 功

Journal of the American Ceramic Society, 102(12), p.7553 - 7563, 2019/12

 被引用回数:0 パーセンタイル:100(Materials Science, Ceramics)

放射性廃棄物固化において、固化体からの水素発生は安全上の主要な懸念事項である。ジオポリマー材で固化する場合、材の多孔質構造中に多量の水が存在するため、水の放射線分解による水素発生が重要な因子となる。本研究では、ジオポリマー材単独またはゼオライト(模擬廃棄物)を含むジオポリマー固化体を、水飽和度と試料サイズを変えて$$^{60}$$Co $$gamma$$線で照射し、水素放出量を測定した。試料が塊状でサイズが大きく(円筒形40cm長)かつ水で飽和している場合(円筒形40cm長)の水素ガス放出量は1.9$$times$$10$$^{-10}$$ mol/Jであり、粉末試料の放出量2.2$$times$$10$$^{-8}$$ mol/Jよりも2桁小さかった。測定結果をジオポリマー中での水素の発生、再結合および拡散挙動を考慮したモデルにより解釈した。ジオポリマー中の拡散係数が既知であれば、モデルは水素放出量を水飽和度の関数として再現でき、試料サイズ40cmまでの放出量を予測できることがわかった。


Conceptual design of direct $$^{rm 99m}$$Tc production facility at the high temperature engineering test reactor

Ho, H. Q.; 石田 大樹*; 濱本 真平; 石井 俊晃; 藤本 望*; 高木 直行*; 石塚 悦男

Nuclear Engineering and Design, 352, p.110174_1 - 110174_7, 2019/10

 被引用回数:0 パーセンタイル:100(Nuclear Science & Technology)

This study proposed a conceptual design of direct $$^{rm 99m}$$Tc production facility from a natural MoO$$_{3}$$ target at the high temperature engineering test reactor (HTTR). $$^{rm 99m}$$Tc is produced by a beta decay of $$^{99}$$Mo, which is formed via the $$^{98}$$Mo(n,$$gamma$$)$$^{99}$$Mo reaction. $$^{rm 99m}$$Tc is then extracted from the MoO$$_{3}$$ target by sublimation method to take advantage of the high temperature of the HTTR core. The foremost advantage of this concept is that the MoO$$_{3}$$ target is heated up inside the reactor without pulling out for external electric heating, and as a result, $$^{rm 99m}$$Tc could be extracted directly during irradiation. With 1 kg of MoO$$_{3}$$ target, the HTTR could produce about 6.8$$times$$10$$^{8}$$ MBq of $$^{rm 99m}$$Tc activity in comparison with 3.0$$times$$10$$^{8}$$ MBq of total $$^{rm 99m}$$Tc supplied in Japan in 2017.


Irradiation growth behavior of improved Zr-based alloys for fuel cladding

天谷 政樹; 垣内 一雄; 三原 武

Proceedings of International Nuclear Fuel Cycle Conference / Light Water Reactor Fuel Performance Conference (Global/Top Fuel 2019) (USB Flash Drive), p.1048 - 1056, 2019/09

New fuel cladding alloys of which composition was changed from conventional ones have been developed by nuclear fuel vendors and utilities. Since the irradiation growth of fuel cladding is one of the most important parameters which determine the dimensional stability of fuel rod and/or fuel assembly during normal operation, the irradiation growth behavior of the improved Zr-based alloys for light-water reactor fuel cladding was investigated. The coupon specimens were prepared from fuel cladding tubes with various kinds of improved Zr-based alloys. The specimens were loaded into test rigs and had been irradiated in the Halden reactor in Norway under several coolant temperature conditions up to a fast-neutron fluence of $$sim$$7.8$$times$$10$$^{21}$$ (n/cm$$^{2}$$, E $$>$$ 1 MeV). Irradiation conditions such as specimen temperatures had been continuously monitored during the irradiation. During and after the irradiation, the amount of irradiation growth of each specimen was evaluated as a part of the interim and final inspections. The effect of the difference in alloy composition on the amount of irradiation growth seemed insignificant if the other conditions e.g. the final heat treatment condition at fabrication and the irradiation temperature were the same.


Development of remote sensing technique using radiation resistant optical fibers under high-radiation environment

伊藤 主税; 内藤 裕之; 石川 高史; 伊藤 敬輔; 若井田 育夫

JPS Conference Proceedings (Internet), 24, p.011038_1 - 011038_6, 2019/01



Mechanical properties database of reactor pressure vessel steels related to fracture toughness evaluation

飛田 徹; 西山 裕孝; 鬼沢 邦雄

JAEA-Data/Code 2018-013, 60 Pages, 2018/11


原子炉圧力容器の健全性を判断する上で、破壊靱性をはじめとする材料の機械的特性は重要な情報となる。本レポートは、日本原子力研究開発機構が取得した中性子照射材を含む原子炉圧力容器鋼材の機械的特性、具体的には引張試験, シャルピー衝撃試験, 落重試験及び破壊靱性試験の公開データをまとめたものである。対象とした材料は、初期プラントから最新プラント相当の不純物含有量及び靱性レベルで製造されたJIS SQV2A(ASTM A533B Class1)相当の5種類の原子炉圧力容器鋼である。また母材に加え、原子炉圧力容器の内張りとして用いられている2種類のステンレスオーバーレイクラッド材の機械的特性データについても記載した。これらの機械的特性データは、材料ごとにグラフで整理するとともに今後のデータの活用しやすさを考慮して表形式でリスト化した。


Feasibility study of large-scale production of iodine-125 at the high temperature engineering test reactor

Ho, H. Q.; 本多 友貴*; 濱本 真平; 石井 俊晃; 藤本 望*; 石塚 悦男

Applied Radiation and Isotopes, 140, p.209 - 214, 2018/10

 被引用回数:2 パーセンタイル:48.87(Chemistry, Inorganic & Nuclear)

The feasibility of a large-scale iodine-125 production from natural xenon gas at high-temperature gas-cooled reactors was investigated. A high-temperature engineering test reactor, which is located in Japan, was used as a reference HTGR reactor in this study. First, a computer code based on a Runge-Kutta method was developed to calculate the quantities of isotopes arising from the neutron irradiation of natural xenon gas target. This code was verified with a good agreement with a reference result. Next, optimization of irradiation planning was carried out. As results, with 4 days of irradiation and 8 days of decay, the $$^{125}$$I production could be maximized and the $$^{126}$$I contamination was within an acceptable level. The preliminary design of irradiation channels at the HTTR was also optimized. The case with 3 irradiation channels and 20-cm diameter was determined as the optimal design, which could produce approximately 180,000 GBq per year of $$^{125}$$I production.


Development on high-power spallation neutron sources with liquid metals

二川 正敏

Proceedings of 13th International Symposium on Advanced Science and Technology in Experimental Mechanics (13th ISEM'18) (USB Flash Drive), 6 Pages, 2018/10



Feasibility study of new applications at the high-temperature gas-cooled reactor

Ho, H. Q.; 本多 友貴*; 濱本 真平; 石井 俊晃; 高田 昌二; 藤本 望*; 石塚 悦男

Proceedings of 9th International Topical Meeting on High Temperature Reactor Technology (HTR 2018) (USB Flash Drive), 6 Pages, 2018/10

Besides the electricity generation and hydrogen production, HTGRs have many advantages for thermal neutron irradiation applications such as stable operation in longterm, large space available for irradiation target, and high thermal neutron economy. This study summarized the feasibility of new irradiation applications at the HTGRs including neutron transmutation doping silicon and I-125 productions. The HTTR located in Japan was used as a reference HTGR in this study. Calculation results show that HTTR could irradiate about 40 tons of doped Si particles per year for fabrication of spherical silicon solar cell. Besides, the HTTR could also produce about 1.8x105 GBq in a year of I-125, comparing to 3.0x103 GBq of total I-125 supplied in Japan in 2016.


Investigation of irradiated properties of extended burnup TRISO fuel

Shaimerdenov, A.*; Gizatulin, S.*; Kenzhin, Y.*; Dyussambayev, D.*; 植田 祥平; 相原 純; 柴田 大受

Proceedings of 9th International Topical Meeting on High Temperature Reactor Technology (HTR 2018) (USB Flash Drive), 6 Pages, 2018/10



Modeling and simulation of redistribution of oxygen-to-metal ratio in MOX

廣岡 瞬; 加藤 正人; 渡部 雅

Transactions of the American Nuclear Society, 118, p.1624 - 1626, 2018/06



Sound speeds in and mechanical properties of (U,Pu)O$$_{2-x}$$

廣岡 瞬; 加藤 正人

Journal of Nuclear Science and Technology, 55(3), p.356 - 362, 2018/03

 被引用回数:1 パーセンタイル:70.85(Nuclear Science & Technology)

密度, O/MおよびPu含有率をパラメータとして、MOXの音速測定を行った。これらのパラメータの影響はそれぞれ一次関数でよくフィッティングすることができ、MOXの音速を評価するフィッティング式が得られた。得られた音速のデータから機械物性が評価され、例として、密度低下によりヤング率は急激に低下する結果が得られた。また、過去に報告されている熱膨張のデータを用いることにより、ヤング率の温度依存性を評価した。温度上昇によりヤング率が低下し、文献値とよく一致する結果が得られた。


Irradiation performance of sodium-bonded control rod for the fast breeder reactor

佐々木 新治; 前田 宏治; 古屋 廣高*

Journal of Nuclear Science and Technology, 55(3), p.276 - 282, 2018/03

 被引用回数:1 パーセンタイル:70.85(Nuclear Science & Technology)

The lifetime of control rods is limited by the absorber (B$$_{4}$$C pellets)-cladding mechanical interaction (ACMI). Therefore, sodium (Na)-bonded control rods were developed for long-life control rods. Na-bonded control rods have been irradiated in the experimental fast breeder reactor, JOYO MK-III, and the diametrical changes of the Na-bonded absorber pins after the irradiation were measured in detail. In this paper, these detailed measurements were compared with the results obtained in helium (He)-bonded control rods with and without the shroud tube in a wide burn-up range. From the comparison, it was concluded that the Na-bonded absorber pins are very effective for achieving long-life control rods.


Evaluation of crack growth rates and microstructures near the crack tip of neutron-irradiated austenitic stainless steels in simulated BWR environment

知見 康弘; 笠原 茂樹; 瀬戸 仁史*; 橘内 裕寿*; 越石 正人*; 西山 裕孝

Proceedings of 18th International Conference on Environmental Degradation of Materials in Nuclear Power Systems - Water Reactors, Vol.2, p.1039 - 1054, 2018/00

 被引用回数:0 パーセンタイル:100



Effect of chloride ion on corrosion behavior of SUS316L-grade stainless steel in nitric acid solutions containing seawater components under $$gamma$$-ray irradiation

佐野 雄一; 安倍 弘; 竹内 正行; 飯嶋 静香; 内田 直樹

Journal of Nuclear Materials, 493, p.200 - 206, 2017/09

 被引用回数:4 パーセンタイル:36.05(Materials Science, Multidisciplinary)



Geopolymers and their potential applications in the nuclear waste management field; A Bibliographical study

Cantarel, V.; 本岡 隆文; 山岸 功

JAEA-Review 2017-014, 36 Pages, 2017/06




Evaluation of irradiation-induced point defect migration energy during neutron irradiation in modified 316 stainless steel

関尾 佳弘; 山県 一郎; 赤坂 尚昭; 坂口 紀史*

Proceedings of International Conference on Fast Reactors and Related Fuel Cycles; Next Generation Nuclear Systems for Sustainable Development (FR-17) (USB Flash Drive), 8 Pages, 2017/06


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