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Takeda, Takeshi
JAEA-Data/Code 2025-005, 106 Pages, 2025/06
JAEA has been creating input data for pressurized water reactor (PWR) analysis with RELAP5/MOD3.3 code, mainly based on design information for the four-loop PWR's Tsuruga Power Station Unit-2 as the reference reactor of the Large Scale Test Facility (LSTF). The cold leg large-break loss-of-coolant accident (LBLOCA) calculation in the flamework of the BEMUSE program is cited as a representative OECD/NEA activity related to the PWR analysis. The new regulatory requirements for PWRs in Japan include the event of loss of recirculation functions from emergency core cooling system (ECCS) in the cold leg LBLOCA. This event should be evaluated the effectiveness of measures against severe core damage. The input data for this study were made preparations to analyze the PWR LBLOCA, which is one of the design basis accidents that should be postulated in the safety design. This report describes the main features of the input data for the PWR LBLOCA analysis. The PWR model comprised a reactor vessel, pressurizer (PZR), hot legs, steam generators (SGs), SG secondary-side system, crossover legs, cold legs, and ECCS. A four-loop PWR was simulated by two loops in the LBLOCA calculation. Specifically, loop-A attached with the PZR corresponded to three loops, and loop-B mounted with the break was equal to one loop. The nodalization schemes of the PWR components were referred to those of the LSTF components. Moreover, interpretations were added to the main input data for the PWR LBLOCA analysis, and further information such as the basis for determining the input data was provided. In addition, transient analysis was performed employing the prepared input data for the loss of ECCS recirculation functions event. The present transient analysis was confirmed to be appropriate generally by comparing with the calculation in the previous study using the RELAP5/MOD3.3 code. Furthermore, sensitivity analyses were executed exploiting the RELAP5/MOD3.3 code to clarify the effects of a discharge coefficient through the break and water injection flow rate of the alternative recirculation on the fuel rod cladding surface temperature. This report explains the results of the sensitivity analyses within the defined ranges, which complement some of the content of the previous study's calculation for the loss of ECCS recirculation functions event.
Fukuda, Kodai; Obara, Toru*; Suyama, Kenya
Nuclear Technology, 211(5), p.963 - 973, 2025/05
Times Cited Count:0 Percentile:0.00(Nuclear Science & Technology)elik, Y.*; Stankovskiy, A.*; Iwamoto, Hiroki; Iwamoto, Yosuke; Van den Eynde, G.*
Annals of Nuclear Energy, 212, p.111048_1 - 111048_12, 2025/03
Times Cited Count:1 Percentile:57.00(Nuclear Science & Technology)Fukuda, Kodai; Obara, Toru*
Nuclear Technology, 12 Pages, 2025/00
Collaborative Laboratories for Advanced Decommissioning Science; Tokyo Institute of Technology*
JAEA-Review 2024-010, 112 Pages, 2024/08
The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2022. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2021, this report summarizes the research results of the "Uncertainty reduction of the FPs transport mechanism and debris degradation behavior and evaluation of the reactor contamination of debris state on the basis of the accident progression scenario of Fukushima Daiichi Nuclear Power Station Unit 2 and 3" conducted in FY2022. The present study aims to elucidate the cause of the high dosage under shield plug by clarification of to the cesium behavior of migration, adhesion to structure and deposition as well as evaluate the properties of metal-rich debris predeceasing melted through the materials science approach based on the most probable scenario of accident progression of Unit 2 and 3. In this fiscal year, the followings were achieved.
Tanabe, Kosuke*; Komeda, Masao; Toh, Yosuke; Kitamura, Yasunori*; Misawa, Tsuyoshi*; Tsuchiya, Kenichi*; Sagara, Hiroshi*
Scientific Reports (Internet), 14, p.18828_1 - 18828_10, 2024/08
Times Cited Count:0 Percentile:0.00(Multidisciplinary Sciences)Hayashi, Hirokazu; Minato, Kazuo*
Electrochemistry (Internet), 92(4), p.043020_1 - 043020_5, 2024/04
Times Cited Count:0 Percentile:0.00(Electrochemistry)The electrochemical behavior of neptunium in NaCl-2CsCl melt at 823-923 K was investigated by cyclic voltammetry, differential pulse voltammetry, and open-circuit chronopotentiometry after polarization. The results show that Np ions are reduced to Np metal by a two-step mechanism via Np
ions in NaCl-2CsCl melt. The diffusion coefficients of Np
and Np
ions were determined from cyclic voltammograms. The apparent standard potentials of Np
/Np
and Np
/Np
redox couples have been determined to be E
(Np
/Np
) = -3.353 + 7.67
10
T, and E
(Np
/Np
) = -1.175 + 4.99
10
T vs. Cl
/Cl
(V), respectively. The activity coefficients of Np
and Np
ions were also determined using the reported data on the Gibbs free energy of formation for NpCl
and NpCl
in supercooled liquid state.
Sasaki, Yuto*; Sano, Aaru; Sasaki, Shinji; Iwamoto, Nobuyuki; Ouchi, Kazuki; Kitatsuji, Yoshihiro; Takaki, Naoyuki*; Maeda, Shigetaka
Journal of Nuclear Science and Technology, 61(4), p.509 - 520, 2024/04
Times Cited Count:5 Percentile:73.39(Nuclear Science & Technology)Ac is attracting attention as an alpha-emitting medical radioisotope. Since its demand is expected to increase, domestic production of
Ac is required from the viewpoint of Japan's medical research and economic security. To establish the technical bases for the
Ac production, JAEA has evaluated the radioactivity that can be produced in the experimental fast reactor Joyo and designed the concept that upgrades the existing facilities for transporting the irradiated target from Joyo to a neighboring PIE facility rapidly. Efficient
Ac Separation from
Ra irradiated in a fast reactor was studied. Ba and La were used as alternatives to Ra and Ac, respectively. By using DGA resin as an adsorbent, it can be expected that Ra and impurities generated by irradiation will be removed and Ac will be isolated. This study has revealed that Joyo can sufficiently produce
Ac as a raw material for pharmaceuticals.
Konno, Chikara
JAEA-Conf 2023-001, p.143 - 146, 2024/02
I modified NJOY2016.67 to produce photonuclear ACE files which can be used in MCNP6.2 and PHITS3.27 and produced the ACE file of the JENDL-5 photonuclear sub-library. Simple test calculations with the produced ACE file supported that the produced ACE file had no serious problems.
Pyeon, C. H.*; Katano, Ryota; Oizumi, Akito; Fukushima, Masahiro
Nuclear Science and Engineering, 197(11), p.2902 - 2919, 2023/11
Times Cited Count:2 Percentile:46.61(Nuclear Science & Technology)Sample reactivity and void reactivity experiments are carried out in the solid-moderated and solid-reflected cores at the Kyoto University Critical Assembly (KUCA) with the combined use of aluminum (Al), lead (Pb) and bismuth (Bi) samples, and Al spacers simulating the void. MCNP6.2 eigenvalue calculations together with JENDL-4.0 provide good accuracy of sample reactivity with the comparison of experimental results; also experimental void reactivity is attained by using MCNP6.2 together with JENDL-4.0 and ENDF/B-VII.1 with a marked accuracy of relative difference between experiments and calculations. Uncertainty quantification of sample reactivity and void reactivity is acquired by using the sensitivity coefficients based on MCNP6.2/ksen and covariance library data of SCALE6.2 together with ENDF/B-VII.1, arising from the impact of uncertainty induced by Al, Pb and Bi cross sections. A series of reactivity analyses with the Al spacer simulating the void demonstrates the means of analyzing the void in the solid-moderated and solid-reflected cores at KUCA
Konno, Chikara; Ota, Masayuki*; Kwon, Saerom*; Onishi, Seiki*; Yamano, Naoki*; Sato, Satoshi*
Journal of Nuclear Science and Technology, 60(9), p.1046 - 1069, 2023/09
Times Cited Count:8 Percentile:92.35(Nuclear Science & Technology)JENDL-5 was validated from a viewpoint of shielding applications under the Shielding Integral Test Working Group of the JENDL Committee. The following benchmark experiments were selected: JAEA/FNS in-situ experiments, Osaka Univ./OKTAVIAN TOF experiments, ORNL/JASPER sodium experiments, NIST iron experiment and QST/TIARA experiments. These experiments were analyzed with MCNP and nuclear data libraries (JENDL-5, JENDL-4.0 or JENDL-4.0/HE, ENDF/B-VIII.0 and JEFF-3.3). The analysis results demonstrate that JENDL-5 is comparable to or better than JENDL-4.0 or JENDL-4.0/HE, ENDF/B-VIII.0 and JEFF-3.3.
Maruyama, Yu; Sugiyama, Tomoyuki*; Shimada, Asako; Lind, T.*; Bentaib, A.*; Sogalla, M.*; Pellegrini, M.*; Albright, L.*; Clayton, D.*
Proceedings of 20th International Topical Meeting on Nuclear Reactor Thermal Hydraulics (NURETH-20) (Internet), p.4782 - 4795, 2023/08
Kimura, Yoshiki; Tsuchiya, Kenichi*
Radioisotopes, 72(2), p.121 - 139, 2023/07
Rapid and precise radioisotope identification in the scene of nuclear detection and nuclear security incidents is one of the challenging issues for the prompt response on the detection alarm or the incidents. A radioisotope identification algorithm using a deep artificial neural network model applicable to handheld gamma-ray detectors has been proposed in the present paper. The proposed algorithm automatically identifies gamma-emitting radioisotopes based on the count contribution ratio (CCR) from each of them estimated by the deep artificial neural network model trained by simulated gamma-ray spectra. The automated radioisotope identification algorithm can support first responders of nuclear detection and nuclear security incidents without sufficient experience and knowledge in radiation measurement. The authors tested the performance of the proposed algorithm using two different types of deep artificial neural network models in application to handheld detectors having high or low energy resolution. The proposed algorithm showed high performance in identifying artificial radioisotopes for actually measured gamma-ray spectra. It was also confirmed that the algorithm is applicable to identifying U and automated uranium categorization by analyzing estimated CCRs by the deep artificial neural network models. The authors also com-pared the performance of the proposed algorithm with a conventional radioisotope identification method and discussed promising ways to improve the performance of the algorithm using the deep artificial neural network.
Tazaki, Makiko
Nihon Genshiryoku Gakkai-Shi ATOMO, 65(3), p.183 - 186, 2023/03
no abstracts in English
Collaborative Laboratories for Advanced Decommissioning Science; Tokyo Institute of Technology*
JAEA-Review 2022-053, 89 Pages, 2023/02
The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2021. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2021, this report summarizes the research results of the "Uncertainty reduction of the FPs transport mechanism and debris degradation behavior and evaluation of the reactor contamination of debris state on the basis of the accident progression scenario of Fukushima Daiichi Nuclear Power Station Unit 2 and 3" conducted in FY2021. The present study aims to elucidate the cause of the high dosage under shield plug by clarification of to the cesium behavior of migration, adhesion to structure and deposition as well as evaluate the properties of metal-rich debris predeceasing melted through the materials science approach based on the most probable scenario of accident progression of Unit 2 and 3. In this fiscal year, the followings were achieved.
Sato, Takumi; Nagae, Yuji; Kurata, Masaki; Quaini, A.*; Guneau, C.*
CALPHAD; Computer Coupling of Phase Diagrams and Thermochemistry, 79, p.102481_1 - 102481_11, 2022/12
Times Cited Count:1 Percentile:7.57(Thermodynamics)Ho, H. Q.; Ishii, Toshiaki; Nagasumi, Satoru; Ono, Masato; Shimazaki, Yosuke; Ishitsuka, Etsuo; Goto, Minoru; Simanullang, I. L.*; Fujimoto, Nozomu*; Iigaki, Kazuhiko
Nuclear Engineering and Design, 396, p.111913_1 - 111913_9, 2022/09
Times Cited Count:1 Percentile:14.76(Nuclear Science & Technology)Ho, H. Q.; Ishitsuka, Etsuo; Iigaki, Kazuhiko
Recent Contributions to Physics, 82(3), p.16 - 20, 2022/09
Nagata, Hiroshi; Otsuka, Kaoru; Omori, Takazumi; Ide, Hiroshi
JAEA-Technology 2022-017, 113 Pages, 2022/08
Japan Materials Testing Reactor (JMTR) was decided as a one of decommission facilities in April 2017. The activation activity of radioactive materials remaining in the reactor facility was evaluated in order to submit the decommissioning plan to the Nuclear Regulation Authority. Total activation activity was 9.310
Bq after the permanent shutdown of reactor, 2.7
10
Bq after 21 years, 1.0
10
Bq after 40 years and 2.4
10
Bq after 100 years. The structure with high activation activity was the core structural materials in JMTR such as beryllium frame, aluminum reflector, etc., and the material was stainless steel, beryllium, etc. The ratio of nuclides to the total amount of activated radioactivity was highest in H-3 until about 40 years after the reactor shutdown, and then in Ni-63. For reference, the radioactivity level was classified based on the results of the obtained radioactivity concentration. The ratio of the weight of each radioactivity level to the total weight was 0.3-0.4% (10-13t) for L1, 0.0-0.4% (0-14t) for L2, 1.0-1.2% (32-39t) for L3 and 98.0-98.7% (about 3200t) for CL until 100 years after the reactor shutdown. It was found that those classified as CL account for more than 90% of the total. When treating and disposing of radioactive waste, evaluation will be carried out based on appropriate methods, including evaluation results of secondary pollutants.
Kirishima, Akira*; Akiyama, Daisuke*; Kumagai, Yuta; Kusaka, Ryoji; Nakada, Masami; Watanabe, Masayuki; Sasaki, Takayuki*; Sato, Nobuaki*
Journal of Nuclear Materials, 567, p.153842_1 - 153842_15, 2022/08
Times Cited Count:9 Percentile:79.01(Materials Science, Multidisciplinary)To understand the chemical structure and stability of nuclear fuel debris consisting of UO, Zr, and Stainless Steel (SUS) generated by the Fukushima Daiichi Nuclear Power Plant accident in Japan in 2011, simulated debris of the UO
-SUS-Zr system and other fundamental component systems were synthesized and characterized. The simulated debris were synthesized by heat treatment for 1 to 12 h at 1600
C, in inert (Ar) or oxidative (Ar + 2% O
) atmospheres.
Np and
Am tracers were doped for the leaching tests of these elements and U from the simulated debris. The characterization of the simulated debris was conducted by XRD, SEM-EDX, Raman spectroscopy, and M
ssbauer spectroscopy, which provided the major uranium phase of the UO
-SUS-Zr debris was the solid solution of U
O
(s.s.) with Zr(IV) and Fe(II) regardless of the treatment atmosphere. The long-term immersion test of the simulated debris in pure water and that in seawater revealed the macro scale crystal structure of the simulated debris was chemically very stable in the wet condition for a year or more. Furthermore, the leaching test results showed that the actinide leaching ratios of U, Np, Am from the UO
-SUS-Zr debris were very limited and less than 0.08 % for all the experiments in this study.