Uncertainty reduction of the FPs transport mechanism and debris degradation behavior and evaluation of the reactor contamination of debris state on the basis of the accident progression scenario of Fukushima Daiichi Nuclear Power Station Unit 2 and 3 (Contract research); FY2023 Nuclear Energy Science & Technology and Human Resource Development Project

Collaborative Laboratories for Advanced Decommissioning Science; Institute of Science Tokyo*

JAEA-Review 2025-012, 96 Pages, 2025/10

JAEA-Review-2025-012.pdf:3.99MB

JAEA/CLADS had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). Among the adopted proposals in FY2021, this report summarizes the research results of the "Uncertainty reduction of the FPs transport mechanism and debris degradation behavior and evaluation of the reactor contamination of debris state on the basis of the accident progression scenario of Fukushima Daiichi Nuclear Power Station unit 2 and 3" conducted from FY2021 to FY2023. The present study aims to elucidate the cause of the high dosage under shield plug by clarification of to the cesium behavior of migration, adhesion to structure and deposition as well as evaluate the properties of metal-rich debris predeceasing melted through the materials science approach based on the most probable scenario of accident progression of Unit 2 and 3. Through three years investigation, chemi-absorption configuration of Cs has been elucidated to change with acidity of steel surface during oxidation in humid atmosphere and CsO trapping compound as well as penetration depth have found to be importantly considered. For metallic debris, solid oxidation was found to be controlled by FeO formation and molten state was found to tend to preferentially yield ZrO resulting in formation of slate structure during solidification. Present findings obtained are contributing to better improve the accuracy of accident progression scenario in FDNPP in viewpoint of backward analysis.

Input data preparation for PWR large-break LOCA analysis with RELAP5/MOD3.3 code

Takeda, Takeshi

JAEA-Data/Code 2025-005, 106 Pages, 2025/06

JAEA-Data-Code-2025-005.pdf:2.93MB

JAEA has been creating input data for pressurized water reactor (PWR) analysis with RELAP5/MOD3.3 code, mainly based on design information for the four-loop PWR's Tsuruga Power Station Unit-2 as the reference reactor of the Large Scale Test Facility (LSTF). The cold leg large-break loss-of-coolant accident (LBLOCA) calculation in the flamework of the BEMUSE program is cited as a representative OECD/NEA activity related to the PWR analysis. The new regulatory requirements for PWRs in Japan include the event of loss of recirculation functions from emergency core cooling system (ECCS) in the cold leg LBLOCA. This event should be evaluated the effectiveness of measures against severe core damage. The input data for this study were made preparations to analyze the PWR LBLOCA, which is one of the design basis accidents that should be postulated in the safety design. This report describes the main features of the input data for the PWR LBLOCA analysis. The PWR model comprised a reactor vessel, pressurizer (PZR), hot legs, steam generators (SGs), SG secondary-side system, crossover legs, cold legs, and ECCS. A four-loop PWR was simulated by two loops in the LBLOCA calculation. Specifically, loop-A attached with the PZR corresponded to three loops, and loop-B mounted with the break was equal to one loop. The nodalization schemes of the PWR components were referred to those of the LSTF components. Moreover, interpretations were added to the main input data for the PWR LBLOCA analysis, and further information such as the basis for determining the input data was provided. In addition, transient analysis was performed employing the prepared input data for the loss of ECCS recirculation functions event. The present transient analysis was confirmed to be appropriate generally by comparing with the calculation in the previous study using the RELAP5/MOD3.3 code. Furthermore, sensitivity analyses were executed exploiting the RELAP5/MOD3.3 code to clarify the effects of a discharge coefficient through the break and water injection flow rate of the alternative recirculation on the fuel rod cladding surface temperature. This report explains the results of the sensitivity analyses within the defined ranges, which complement some of the content of the previous study's calculation for the loss of ECCS recirculation functions event.

Built-in physics models and proton-induced nuclear data validation using MCNP, PHITS, and FLUKA; Impact on the shielding design for proton accelerator facilities

elik, Y.*; Stankovskiy, A.*; Iwamoto, Hiroki; Iwamoto, Yosuke; Van den Eynde, G.*

Annals of Nuclear Energy, 212, p.111048_1 - 111048_12, 2025/03

https://doi.org/10.1016/j.anucene.2024.111048

Uncertainty reduction of the FPs transport mechanism and debris degradation behavior and evaluation of the reactor contamination of debris state on the basis of the accident progression scenario of Fukushima Daiichi Nuclear Power Station Unit 2 and 3 (Contract research); FY2022 Nuclear Energy Science & Technology and Human Resource Development Project

Collaborative Laboratories for Advanced Decommissioning Science; Tokyo Institute of Technology*

JAEA-Review 2024-010, 112 Pages, 2024/08

JAEA-Review-2024-010.pdf:6.49MB

The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2022. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2021, this report summarizes the research results of the "Uncertainty reduction of the FPs transport mechanism and debris degradation behavior and evaluation of the reactor contamination of debris state on the basis of the accident progression scenario of Fukushima Daiichi Nuclear Power Station Unit 2 and 3" conducted in FY2022. The present study aims to elucidate the cause of the high dosage under shield plug by clarification of to the cesium behavior of migration, adhesion to structure and deposition as well as evaluate the properties of metal-rich debris predeceasing melted through the materials science approach based on the most probable scenario of accident progression of Unit 2 and 3. In this fiscal year, the followings were achieved.

Electrochemical behavior of neptunium in NaCl-2CsCl melt

Hayashi, Hirokazu; Minato, Kazuo*

Electrochemistry (Internet), 92(4), p.043020_1 - 043020_5, 2024/04

https://doi.org/10.5796/electrochemistry.23-69159

The electrochemical behavior of neptunium in NaCl-2CsCl melt at 823-923 K was investigated by cyclic voltammetry, differential pulse voltammetry, and open-circuit chronopotentiometry after polarization. The results show that Np ions are reduced to Np metal by a two-step mechanism via Np ions in NaCl-2CsCl melt. The diffusion coefficients of Np and Np ions were determined from cyclic voltammograms. The apparent standard potentials of Np/Np and Np/Np redox couples have been determined to be E(Np/Np) = -3.353 + 7.6710T, and E(Np/Np) = -1.175 + 4.9910 T vs. Cl/Cl (V), respectively. The activity coefficients of Np and Np ions were also determined using the reported data on the Gibbs free energy of formation for NpCl and NpCl in supercooled liquid state.

Processing of JENDL-5 photonuclear sublibrary

Konno, Chikara

JAEA-Conf 2023-001, p.143 - 146, 2024/02

https://doi.org/10.11484/jaea-conf-2023-001

I modified NJOY2016.67 to produce photonuclear ACE files which can be used in MCNP6.2 and PHITS3.27 and produced the ACE file of the JENDL-5 photonuclear sub-library. Simple test calculations with the produced ACE file supported that the produced ACE file had no serious problems.

JENDL-5 benchmark test for shielding applications

Konno, Chikara; Ota, Masayuki*; Kwon, Saerom*; Onishi, Seiki*; Yamano, Naoki*; Sato, Satoshi*

Journal of Nuclear Science and Technology, 60(9), p.1046 - 1069, 2023/09

https://doi.org/10.1080/00223131.2022.2164372

JENDL-5 was validated from a viewpoint of shielding applications under the Shielding Integral Test Working Group of the JENDL Committee. The following benchmark experiments were selected: JAEA/FNS in-situ experiments, Osaka Univ./OKTAVIAN TOF experiments, ORNL/JASPER sodium experiments, NIST iron experiment and QST/TIARA experiments. These experiments were analyzed with MCNP and nuclear data libraries (JENDL-5, JENDL-4.0 or JENDL-4.0/HE, ENDF/B-VIII.0 and JEFF-3.3). The analysis results demonstrate that JENDL-5 is comparable to or better than JENDL-4.0 or JENDL-4.0/HE, ENDF/B-VIII.0 and JEFF-3.3.

Radioisotope identification algorithm using deep artificial neural network for supporting nuclear detection and first response on nuclear security incidents

Kimura, Yoshiki; Tsuchiya, Kenichi*

Radioisotopes, 72(2), p.121 - 139, 2023/07

https://doi.org/10.3769/radioisotopes.72.121

Rapid and precise radioisotope identification in the scene of nuclear detection and nuclear security incidents is one of the challenging issues for the prompt response on the detection alarm or the incidents. A radioisotope identification algorithm using a deep artificial neural network model applicable to handheld gamma-ray detectors has been proposed in the present paper. The proposed algorithm automatically identifies gamma-emitting radioisotopes based on the count contribution ratio (CCR) from each of them estimated by the deep artificial neural network model trained by simulated gamma-ray spectra. The automated radioisotope identification algorithm can support first responders of nuclear detection and nuclear security incidents without sufficient experience and knowledge in radiation measurement. The authors tested the performance of the proposed algorithm using two different types of deep artificial neural network models in application to handheld detectors having high or low energy resolution. The proposed algorithm showed high performance in identifying artificial radioisotopes for actually measured gamma-ray spectra. It was also confirmed that the algorithm is applicable to identifying U and automated uranium categorization by analyzing estimated CCRs by the deep artificial neural network models. The authors also com-pared the performance of the proposed algorithm with a conventional radioisotope identification method and discussed promising ways to improve the performance of the algorithm using the deep artificial neural network.

Uncertainty reduction of the FPs transport mechanism and debris degradation behavior and evaluation of the reactor contamination of debris state on the basis of the accident progression scenario of Fukushima Daiichi Nuclear Power Station Unit 2 and 3 (Contract research); FY2021 Nuclear Energy Science & Technology and Human Resource Development Project

Collaborative Laboratories for Advanced Decommissioning Science; Tokyo Institute of Technology*

JAEA-Review 2022-053, 89 Pages, 2023/02

JAEA-Review-2022-053.pdf:3.47MB

The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2021. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2021, this report summarizes the research results of the "Uncertainty reduction of the FPs transport mechanism and debris degradation behavior and evaluation of the reactor contamination of debris state on the basis of the accident progression scenario of Fukushima Daiichi Nuclear Power Station Unit 2 and 3" conducted in FY2021. The present study aims to elucidate the cause of the high dosage under shield plug by clarification of to the cesium behavior of migration, adhesion to structure and deposition as well as evaluate the properties of metal-rich debris predeceasing melted through the materials science approach based on the most probable scenario of accident progression of Unit 2 and 3. In this fiscal year, the followings were achieved.

Calculation of shutdown gamma distribution in the high temperature engineering test reactor

Ho, H. Q.; Ishii, Toshiaki; Nagasumi, Satoru; Ono, Masato; Shimazaki, Yosuke; Ishitsuka, Etsuo; Goto, Minoru; Simanullang, I. L.*; Fujimoto, Nozomu*; Iigaki, Kazuhiko

Nuclear Engineering and Design, 396, p.111913_1 - 111913_9, 2022/09

https://doi.org/10.1016/j.nucengdes.2022.111913