Simultaneous determination of zircon crystallisation age and temperature; Common thermal evolution of mafic magmatic enclaves and host granites in the Kurobegawa granite, central Japan

Yuguchi, Takashi*; Yamazaki, Hayato*; Ishibashi, Kozue*; Sakata, Shuhei*; Yokoyama, Tatsunori; Suzuki, Satoshi*; Ogita, Yasuhiro; Sando, Kazusa*; Imura, Takumi*; Ono, Takeshi*

Journal of Asian Earth Sciences, 226, p.105075_1 - 105075_9, 2022/04

https://doi.org/10.1016/j.jseaes.2021.105075

Simultaneous determination of the U-Pb age of zircon and concentration of titanium in a single analysis spot, using inductively coupled plasma mass spectrometry with laser ablation sample introduction, produces paired age and temperature data of zircon crystallisation, potentially revealing time-temperature () histories for evolved magma. The Kurobegawa granite, central Japan, contains abundant mafic magmatic enclaves (MMEs). We applied this method to evaluate MMEs and their host (enclosing) granites. Cooling behaviour common to both MMEs and host rocks was found between 1.5 and 0.5 Ma. Rapid cooling from the zircon crystallisation temperature to the closure temperature of biotite K-Ar system was within 1 million year. Combining the obtained paths of MMEs and host rocks with petrological information can provide insights into magma chamber processes. This suggests that MME flotation, migration, and spread through the magma chamber ceased at 1.5-0.5 Ma, indicating the emplacement age of the Kurobegawa granitic pluton, as no large-scale reheating episodes have occurred since then.

The Study of oxidative stress status in the organs exposed to low dose/low dose-rate radiation (Contract research); FY2020 Nuclear Energy Science & Technology and Human Resource Development Project

Collaborative Laboratories for Advanced Decommissioning Science; Tohoku University*

JAEA-Review 2021-050, 82 Pages, 2022/01

The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2020. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2019, this report summarizes the research results of the "The study of oxidative stress status in the organs exposed to low dose/low dose-rate radiation" conducted in FY2020. The present study aims to investigate the biological effects of low dose/low dose-rate radiation exposure, which is of great social interest, on the oxidative stress status of individual organs and will contribute to the collection of scientific data in a dose range to be required. An interdisciplinary collaborative study discussed the correlation between radiation dose and the biological effect by analyzing the samples of wild Japanese macaques exposed to radiation due to the accident of Fukushima Daiichi Nuclear Power Station and of animal experiments.

Challenge to investigation of fuel debris in RPV by an advanced super dragon articulated robot arm (Contract research); FY2020 Nuclear Energy Science & Technology and Human Resource Development Project

Collaborative Laboratories for Advanced Decommissioning Science; Tokyo Institute of Technology*

JAEA-Review 2021-045, 65 Pages, 2022/01

JAEA-Review-2021-045.pdf:3.41MB

The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2020. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2019, this report summarizes the research results of the "Challenge to investigation of fuel debris in RPV by an advanced super dragon articulated robot arm" conducted in FY2020. The present study aims to develop the implementation techniques of the remote sensing method on a robot arm for monitoring the structure status in the reactor and the distribution of nuclear materials by a long-articulated robot arm with controlling and grasping the position and posture of the robot arm hand. In FY 2020, we have conducted fundamental operation check of the robot arm in the simulated environment, prototype construction of telescopic articulated arm and cable storage mechanism, investigation of drive wire specifications, improvement of LIBS probe, prototype construction of microchip

Research and development of radiation-resistant sensor for fuel debris by integrating advanced measurement technologies (Contract research); FY2020 Nuclear Energy Science & Technology and Human Resource Development Project

Collaborative Laboratories for Advanced Decommissioning Science; High Energy Accelerator Research Organization*

JAEA-Review 2021-042, 115 Pages, 2022/01

JAEA-Review-2021-042.pdf:5.18MB

The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2020. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2018, this report summarizes the research results of the "Research and development of radiation-resistant sensor for fuel debris by integrating advanced measurement technologies" conducted from FY2018 to FY2020. Since the final year of this proposal was FY2020, the results for three fiscal years were summarized. The present study aims to in-situ measure and analyze the distribution status and criticality of flooded fuel debris. For this purpose, we construct a neutron measurement system by developing compact diamond neutron sensor and integrated circuit whose radiation resistance was improved by circuit design. Along with the multi-phased array sonar and the acoustic sub-bottom profiling (SBP) system, the neutron measurement system will be installed in the ROV (developed by

Analysis of risk reduction effect of supposed steam condenser implementation as accident measure for accident of evaporation to dryness by boiling of reprocessed high level liquid waste

Yoshida, Kazuo; Tamaki, Hitoshi; Hiyama, Mina*

JAEA-Research 2021-013, 20 Pages, 2022/01

JAEA-Research-2021-013.pdf:2.35MB

An accident of evaporation to dryness by boiling of high level liquid waste (HLLW) is postulated as one of the severe accidents caused by the loss of cooling function at a fuel reprocessing plant. In this case, volatile radioactive materials, such as ruthenium (Ru) are released from the tanks with water and nitric-acid mixed vapor into atmosphere. An idea has been proposed to implement a steam condenser as an accident countermeasure. This measure is expected to prevent nitric acid steam diffusing in facility building and to increase gaseous Ru trapping ratio into condensed water. A simulation study has been carried out with a hypothetical typical facility building to analyze the efficiency of steam condenser. In this study, SCHERN computer code simulates chemical behaviors of Ru in nitrogen oxide, nitric acid and water mixed vapor based on the conditions obtained from simulation with thermal-hydraulic computer code MELCOR. The effectiveness of steam condenser has been analyzed quantitively in preventing mixed vapor diffusion and gaseous Ru trapping effect. Some issues to be solved in analytical model has been also clarified in this study.

Measurement of nuclide production cross sections for proton-induced reactions on Mn and Co at 1.3, 2.2, and 3.0 GeV

Takeshita, Hayato*; Meigo, Shinichiro; Matsuda, Hiroki*; Iwamoto, Hiroki; Nakano, Keita; Watanabe, Yukinobu*; Maekawa, Fujio

Nuclear Instruments and Methods in Physics Research B, 511, p.30 - 41, 2022/01

https://doi.org/10.1016/j.nimb.2021.10.016

Nuclide production cross sections for proton-induced reactions on Mn and Co at incident energies of 1.3, 2.2, and 3.0 GeV were measured by the activation method at the J-PARC. In total, 143 production cross sections of reaction products were obtained. Among them, the cross sections of Mn(p,X)S and Mn(p,X)Ar were measured for the first time. The stable proton beam and well established beam monitoring system contributed to the reduction of the systematic uncertainties to typically less than 5%, which was better than those of the previous data. To examine the prediction capabilities of spallation reaction models and evaluated data library, the measured data were compared with the spallation reaction models in PHITS (INCL4.6/GEM, etc.), INCL++/ABLA07, and the JENDL/HE-2007 library. The comparison of the mean square deviation factors indicated that both INCL4.6/GEM and JENDL/HE-2007 showed better agreement with the measured data than the others.

Evaluation of the minimum critical amount for heterogeneous lattice systems composed of fuel rods utilized in low-power water-moderated research and test reactors by using continuous-energy Monte Carlo code MVP with JENDL-4.0

Yanagisawa, Hiroshi

JAEA-Technology 2021-023, 190 Pages, 2021/11

JAEA-Technology-2021-023.pdf:5.25MB

Computational analyses on nuclear criticality characteristics were carried out for heterogeneous lattice systems composed of water moderator and fuel rods utilized in lowpower research and test reactors, in which the depletion of fuel due to burnup is relatively small, by using the continuous-energy Monte Carlo code MVP Version 2 with the evaluated nuclear data library JENDL-4.0. In the analyses, the minimum critical number of fuel rods was evaluated using calculated neutron multiplication factors for the heterogeneous systems of the uranium dioxide fuel rod in the Static Experiments Critical Facility (STACY) and the Tank-type Critical Assembly (TCA), and the uranium-zirconium hydride fuel rod in the Nuclear Safety Research Reactor (NSRR). In addition, six sorts of the ratio of reaction rates, which are components of neutron multiplication factors, were calculated in the analyses to explain the variation of neutron multiplication factors with the ratio of water moderator to fuel volume in a unit fuel rod cell. Those results of analyses are considered to be useful for the confirmation of reasonableness and validity of criticality safety measures as data showing criticality characteristics for water-moderated heterogeneous lattice systems composed of the existing fuel rods in research and test reactors, of which criticality data are not sufficiently provided by the Criticality Safety Handbook.

Development of radiation hardened diamond image sensing devices (Contract research); FY2020 Nuclear Energy Science & Technology and Human Resource Development Project

Collaborative Laboratories for Advanced Decommissioning Science; National Institute of Advanced Industrial Science and Technology*

JAEA-Review 2021-026, 47 Pages, 2021/11

JAEA-Review-2021-026.pdf:2.16MB

The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2020. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2019, this report summarizes the research results of the "Development of radiation hardened diamond image sensing devices" conducted in FY2020. The research objective of this project is to develop image sensing devices which work under the high radiation condition. The devices will be realized using radiation hardened diamond semiconductor devices as charge transfer devices and photodetectors. The research project has mainly two targets such as to confirm charge coupled devices operation on diamond unipolar devices and to characterize photo conductivity of diamond detectors.

Consideration on utilization of atmospheric dispersion models for a nuclear emergency preparedness and response

Togawa, Orihiko; Okura, Takehisa; Kimura, Masanori; Nagai, Haruyasu

JAEA-Review 2021-021, 61 Pages, 2021/11

JAEA-Review-2021-021.pdf:3.72MB

Triggered by the Fukushima Daiichi Nuclear Power Station accident, there have been a lot of arguments among various situations and levels about utilization of atmospheric dispersion models for a nuclear emergency preparedness and response. Most of these arguments, however, were alternative and extreme discussions on whether predictions by computational models could be applied or not for protective measures in a nuclear emergency, and it was hard to say that these arguments were politely conducted, based on scientific verification in an emergency response. It was known, on the other hand, that there were not a few potential users of atmospheric dispersion models and/or calculation results by the models within the Japan Atomic Energy Agency (JAEA) and outside. However, they seemed to have a lack of understanding and a misunderstanding on proper use of different kinds of atmospheric dispersion models. This report compares an outline of models and calculation method in atmospheric dispersion models for a nuclear emergency preparedness and response, with a central focus on the models which have been developed and used in the JAEA. Examples of calculations by these models are also described in the report. This report aims at contributing to future consideration and activities for potential users of atmospheric dispersion models within the JAEA and outside.

Experimental analysis on dynamics of liquid molecules adjacent to particles in nanofluids

Hashimoto, Shunsuke*; Nakajima, Kenji; Kikuchi, Tatsuya*; Kamazawa, Kazuya*; Shibata, Kaoru; Yamada, Takeshi*

Journal of Molecular Liquids, 342, p.117580_1 - 117580_8, 2021/11

https://doi.org/10.1016/j.molliq.2021.117580

Quasi-elastic neutron scattering (QENS) and pulsed-field-gradient nuclear magnetic resonance (PFGNMR) analyses of a nanofluid composed of silicon dioxide (SiO) nanoparticles and a base fluid of ethylene glycol aqueous solution were performed. The aim was to elucidate the mechanism increase in the thermal conductivity of the nanofluid above its theoretical value. The obtained experimental results indicate that SiO particles may decrease the self-diffusion coefficient of the liquid molecules in the ethylene glycol aqueous solution because of their highly restricted motion around these nanoparticles. At a constant temperature, the thermal conductivity increases as the self-diffusion coefficient of the liquid molecules decreases in the SiO nanofluids.