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論文

Visualizing an ignition process of hydrogen jets containing sodium mist by high-speed imaging

土井 大輔; 清野 裕; 宮原 信哉*; 宇埜 正美*

Journal of Nuclear Science and Technology, 56(6), p.521 - 532, 2019/06

In severe accident scenarios for sodium-cooled fast reactors, it is desirable to gradually consume hydrogen generated by various ex-vessel phenomena without posting a challenge to containment integrity. An effective means is combustion of hydrogen jets containing sodium vapor and mist, but previous studies have been limited to determining ignition thresholds experimentally. The aim of this study was to visualize the ignition process in detail to investigate the ignition mechanism of hydrogen-sodium mixed jets. The ignition experiments of the hydrogen jet containing sodium mist were carried out under a condition of little turbulence. The ignition process was measured with an optical measurement system comprised of a high-speed camera and an image intensifier, and a spatial distribution of luminance was analyzed by image processing. Detail observation revealed that sodium mist particles burned as scattering sparks inside the jet and that hydrogen ignited around the mist particles. Additionally, the experimental results and a simple heat balance calculation indicated that the combustion heat of sodium mist particles could ignite the hydrogen as the heterogeneous ignition source in the fuel temperature range where the mist particle formation was promoted.

論文

An Interpretation of Fukushima-Daiichi Unit 3 plant data covering the two-week accident-progression phase based on correction for pressure data

佐藤 一憲

Journal of Nuclear Science and Technology, 56(5), p.394 - 411, 2019/05

福島第一3号機の圧力測定システムでは、運転中の蒸発/凝縮を補正するためにその一部に水柱が採用されている。これらの水柱の一部は事故条件下において蒸発し、正しい圧力データが示されていなかった。RPV(原子炉圧力容器), S/C(圧力抑制室)及びD/W(ドライウェル)の各圧力の比較を通し、水柱変化の効果を評価した。これによりRPV, S/C圧力データに対して水柱変化の効果の補正を行った。補正された圧力を用いて、事故進展中のRPV, S/C, D/W間のわずかな圧力差を評価した。この情報を、3号機の水位、CAMS(格納系雰囲気モニタリングシステム)および環境線量率などのデータとともに活用し、RPVおよびPCVの圧力上昇・下降および放射性物質の環境への放出に着目して事故進展挙動の解釈を行った。RPV内およびRPV外の燃料デブリのドライアウトはこれらの圧力低下を引き起こしている可能性がある一方、S/Cからペデスタルに流入したS/C水がペデスタルに移行した燃料デブリによって加熱されたことがPCV加圧の原因となっている。ペデスタル移行燃料デブリの周期的な再冠水とそのドライアウトは、最終的なデブリの再冠水まで数回の周期的な圧力変化をもたらしている。

論文

Validation study of initiating phase evaluation method for the core disruptive accident in an SFR

石田 真也; 川田 賢一; 深野 義隆

Proceedings of 27th International Conference on Nuclear Engineering (ICONE-27) (Internet), 10 Pages, 2019/05

高速炉の安全研究の分野では炉心損傷事故(CDA)が評価上重要な課題であるとして、当該事故に関する評価手法の研究開発が進められて来ている。その中でSAS4AはCDAの起因過程(IP)の事象進展を評価するために開発が進められている解析コードである。本研究ではSAS4Aの信頼性向上のため、PIRT手法を適用したSAS4Aの検証を行った。SAS4Aの検証は、(1) CDAの代表的な事象であるULOFに対する評価指標(FOM)の選択、(2) ULOFに関連する物理現象の抽出、(3)物理現象のランク付け、(4)評価マトリクスの構築、(5)評価マトリクスに基づく試験解析、という流れで実施し、これによりSAS4Aの信頼性向上を図ることができた。

論文

Study on loss-of-cooling and loss-of-coolant accidents in spent fuel pool, 1; Overview

加治 芳行; 根本 義之; 永武 拓; 吉田 啓之; 東條 匡志*; 後藤 大輔*; 西村 聡*; 鈴木 洋明*; 大和 正明*; 渡辺 聡*

Proceedings of 27th International Conference on Nuclear Engineering (ICONE-27) (Internet), 8 Pages, 2019/05

本研究では、使用済燃料プール(SFP)の事故時における燃料被覆管の酸化モデル及びSFPに設置されたスプレイの冷却性能を評価するための数値シミュレーション手法を開発した。これらをMAAPやSAMPSONのようなシビアアクシデント(SA)解析コードに組み込み、SFPの事故時解析を実施した。数値流体力学コードを用いた解析を実施し、SA解析コードの結果と比較することにより、SFP事故の詳細を検討した。さらに、3次元臨界解析手法を開発し、SFPにおける使用済燃料のより安全な燃料配置について検討した。

論文

Chemical reaction kinetics dataset of Cs-I-B-Mo-O-H system for evaluation of fission product chemistry under LWR severe accident conditions

宮原 直哉; 三輪 周平; 堀口 直樹; 佐藤 勇*; 逢坂 正彦

Journal of Nuclear Science and Technology, 56(2), p.228 - 240, 2019/02

 パーセンタイル:100(Nuclear Science & Technology)

軽水炉シビアアクシデント時のソースターム評価における核分裂生成物(FP)化学挙動評価モデルを高度化するため、FP化学データベース「ECUME」の初版を構築した。ECUMEには、代表的な事故シーケンスにおける主要な化学反応と、その実効的な化学反応速度定数を実装する計画である。初版においては、300-3000Kの温度領域におけるCs-I-B-Mo-O-H系の主要化学種に対し、それらの生成に係る化学反応の速度定数を文献調査または第一原理に基づく理論計算によって整備した。構築した化学反応データセットを用いた解析の一例として化学反応解析を実施した結果、1000Kにおいて有意な化学反応速度の効果が見られた。また、平衡に至った後の化学組成を化学平衡計算の結果と比較したところ、代表的なCs-I-B-Mo-O-H系化学種に対して良く整合する結果が得られた。これらの結果から、構築したデータセットは、速度論の考慮が必要なシビアアクシデント時のCs-I-B-Mo-O-H系FP化学挙動評価のために有用であるとの結論を得た。

論文

Characterization of the VULCANO test products for fuel debris removal from the Fukushima Daiichi Nuclear Power Plant

北垣 徹; 池内 宏知; 矢野 公彦; 荻野 英樹; Haquet, J.-F.*; Brissonneau, L.*; Tormos, B.*; Piluso, P.*; 鷲谷 忠博

Progress in Nuclear Science and Technology (Internet), 5, p.217 - 220, 2018/11

Characterization of the fuel debris is required to develop fuel debris removal tools for the decommissioning of Fukushima Daiichi Nuclear Power Plant (1F). In this study, the VULCANO MCCI test, VBS-U4, was selected as 1F similar conditions and the characteristics of the samples were examined. In the molten pool sample, the round-edged corium-rich oxides region, with diameters of 1-10 mm, is surrounded by a concrete-rich oxide region. It shows convection of the molten pool. Other samples also show the features of the MCCI progression. The main chemical forms of the samples are SiO$$_{2}$$, (U,Zr)O$$_{2}$$, Fe and so on. The microstructure of the samples is heterogeneous structure composed of these phases. The difference in Vickers hardness between the metallic phases and the oxide phases is a distinctive characteristic. It can be noted that the heterogeneous distribution of metallic phases in 1F MCCI products interrupt with the removal operation such as by damaging the core-boring bit.

論文

Evaluation of chemical speciation of iodine and cesium considering fission product chemistry in reactor coolant system

石川 淳; Zheng, X.; 塩津 弘之; 杉山 智之; 丸山 結

Proceedings of Asian Symposium on Risk Assessment and Management 2018 (ASRAM 2018) (USB Flash Drive), 6 Pages, 2018/10

Japan Atomic Energy Agency is pursuing the development and application of the methodologies on fission product (FP) chemistry for source term analysis by using integrated severe accident analysis code THALES2/KICHE. Generally, specific chemical forms of iodine and cesium such as cesium iodide (CsI) and cesium hydroxide (CsOH) were assumed in the source term analysis for light water reactors using an integrated severe accident analysis code. The accident at the Fukushima Dai-ichi Nuclear Power Station leads possible chemical effects of B$$_{4}$$C control materials and atmosphere on chemical speciation of iodine and cesium such as cesium metaborate (CsBO$$_{2}$$) and hydrogen iodide (HI). The difference of chemical speciation affects not only the FP behavior in the reactor coolant system (RCS) and transport to containment but also pH value of the suppression pool water in the containment. The pH value is one of the influential factors on the release of gaseous iodine (I$$_{2}$$ and organic iodine) from containment liquid phase. In the present study, the improvement of the THALES2/KICHE code in terms of FP chemistry in RCS was performed and applied to source term analysis for severe accidents at a boil water reactor with Mark-I containment vessel. This paper discusses the chemical speciation of iodine and cesium, and FP behavior and transport to containment.

論文

Creep deformation analysis of a pipe specimen based on creep damage evaluation method

勝山 仁哉; 山口 義仁; Li, Y.

Proceedings of 26th International Conference on Nuclear Engineering (ICONE-26) (Internet), 6 Pages, 2018/07

過酷な条件下における原子炉機器の破損挙動を評価するための手法の整備が重要となっている。我々は、有限要素法を用いて、高温下における機器のクリープ変形及び損傷挙動を評価するための手法の整備を進めている。本研究では、COSSALベンチマーク解析の一環として、我々が整備したクリープ損傷評価手法の検証を行うことを目的に、大型管状試験体に対する損傷評価を行った。その結果、材料の損傷を考慮したクリープ構成則が最も精度がよいことなどを示した。

論文

Three-dimensional numerical study on pool stratification behavior in molten corium-concrete interaction (MCCI) with MPS method

Li, X.; 佐藤 一憲; 山路 哲史*; Duan, G.*

Proceedings of 26th International Conference on Nuclear Engineering (ICONE-26) (Internet), 8 Pages, 2018/07

溶融コリウム・コンクリート相互作用(MCCI)は軽水炉の仮想的シビアアクシデント時の後期フェーズにおいて炉容器外で生じる可能性のある重要事象である。本研究では、MPS法を用いてKITによって実施された模擬物質による成層化溶融プールの実験COMET-L3に対する3次元解析を行った。コリウム/クラスト/コンクリート間の伝熱は粒子間の熱伝導モデルで模擬した。さらに、ケイ酸系コンクリートではケイ酸系析出物の効果によって軸方向と径方向の浸食が異なる可能性が既往研究から示唆されていることから、2つの異なる解析ケースを実施した。解析の結果、MCCIにおいて金属コリウムは酸化物コリウムと全く異なるコンクリート浸食パターンを示しており、アクシデントマネジメントにおける格納系境界の溶融貫通時間の評価に考慮する必要があることが分かった。

論文

Influence of chemical speciation in reactor cooling system on pH of suppression pool during BWR severe accident

塩津 弘之; 石川 淳; 杉山 智之; 丸山 結

Journal of Nuclear Science and Technology, 55(4), p.363 - 373, 2018/04

 パーセンタイル:100(Nuclear Science & Technology)

The influences of chemical speciation for Cs-I-Te-Mo-Sn-B-C-O-H system, simulating a state in the reactor cooling system (RCS) of BWR, on pH of the suppression chamber (S/C) water pool were analytically investigated with PHREEQC code. Major conditions were chosen on the basis of the outputs from a BWR severe accident analysis by THALES2 code and chemical thermodynamic analysis with VICTORIA2.0 code. The chemical thermodynamic analysis showed that the chemical speciation of important volatile FPs, Cs and I, was strongly influenced by Mo and B$$_{4}$$C control material. As a consequence, pH of the S/C water pool was predicted to range from approximately 6 to 10, depending on the fraction of volatile FPs transported from the RCS to the S/C water pool and the H$$_{2}$$/H$$_{2}$$O ratio associated with the oxygen potential. It was implied that the formation of volatile I species such as I$$_{2}$$ in the S/C water pool was larger by 3 orders at the lowest pH than that at the highest pH.

論文

熱水力安全評価基盤技術高度化戦略マップ2017; 軽水炉の継続的な安全性向上に向けたアプローチ

糸井 達哉*; 岩城 智香子*; 大貫 晃*; 木藤 和明*; 中村 秀夫; 西田 明美; 西 義久*

日本原子力学会誌, 60(4), p.221 - 225, 2018/04

日本原子力学会熱流動部会は福島第一原子力発電所(1F)事故の教訓を基にした分野のロードマップの改訂(ローリング)を進め、2018年3月に「熱水力安全評価基盤技術高度化戦略マップ2017(熱水力ロードマップ2017)」を策定した。世界最高水準の安全性の実現とその継続的改善を図るため、安全裕度向上策及び人材育成に必要なニーズとシーズのマッチングを考慮して選定・詳述された2015年版の技術課題を見直すと共に、主要な技術課題の実施状況の記載、「軽水炉安全技術・人材ロードマップ」との対応状況の明示、計算科学技術部会の協力による1F事故の原因ともなった外的事象対応の記述の改訂など、記載が大幅に充実された。その概要をまとめる。

論文

Thermophysical properties of stainless steel containing 5mass%-B$$_{4}$$C in the solid phase

高井 俊秀; 古川 智弘; 山野 秀将

Proceedings of 2018 International Congress on Advances in Nuclear Power Plants (ICAPP 2018) (CD-ROM), p.1007 - 1013, 2018/04

This study describes estimation results of thermophysical properties of stainless steel containing 5mass% boron carbide (5mass%B$$_{4}$$C-SS) in the solid state. 5mass%B$$_{4}$$C-SS eutectic sample was synthesized using a hot press method. Homogeneity of the sample was evaluated by chemical composition analysis, metal structure observation, and micro X-ray diffraction (XRD). Specific gravity and specific heat were evaluated up to 1000$$^{circ}$$C. These measurements proved that the specific gravity in our sample was lowered and the temperature dependence of the specific gravity, along with the elevation of temperature, became gradual compared to that of grade type 316L stainless steel (SUS316L) used as a reactor material by addition of B$$_{4}$$C. The specific heat became slightly higher than that of SUS316L by addition of B$$_{4}$$C and showed similar temperature dependence up to 800$$^{circ}$$C.

論文

Behavior of cesium molybdate, Cs$$_{2}$$MoO$$_{4}$$, in severe accident conditions, 1; Partitioning of Cs and Mo among gaseous species

Do, Thi Mai Dung*; Sujatanond, S.*; 小川 徹

Journal of Nuclear Science and Technology, 55(3), p.348 - 355, 2018/03

 パーセンタイル:100(Nuclear Science & Technology)

シビアアクシデント時のセシウム挙動理解のために、水素-水蒸気環境におけるCs$$_{2}$$MoO$$_{4}$$の高温化学を調べた。Cs$$_{2}$$MoO$$_{4}$$-MoO$$_{3}$$疑似二元系をRedlich-Kister型の熱化学モデルで記述した。モデルの検証のために、Cs$$_{2}$$MoO$$_{4}$$の蒸発損失速度を熱天秤で乾燥及び湿潤アルゴン雰囲気下で測定し、解析により正確に予測評価できることを示した。同モデルを用いて、全電源喪失によるBWR炉心損傷時のCs及びMoの気相化学種間での分配を評価した。

論文

人材育成の観点から見た福島第一原子力発電所の過酷事故対応の教訓

吉澤 厚文*; 大場 恭子; 北村 正晴*

日本機械学会論文集(インターネット), 83(856), p.17-00263_1 - 17-00263_17, 2017/12

This research aims to develop capability of on-site staffs that can respond to beyond design basis accident in the sophisticater socio-technical system, in which ensuring safety has been more complicated. The authors focused on the actions to prevent the accident progression undertaken by on-site staffs, which were hardly evaluated in existing accident analyses and reports. With reference to the concept of resilience engineering, "Responding" of the four cornerstones was particularly analyzed. Based on the precedent studies, causal factors of modeling "Responding" where pointed out the importance of "Attitude" that is a new lesson learned from on-site response at the accident. In addition, new lessons learned on improvement of skills indicated the limit of the concept of risk removal type safety as a safety goal that human is defined as "a safety hazard element". This led the necessity of the success expansion type of safety as a new safety goal that human is defined as "a resource necessary for system flexibility and resilience". Thus, new lessons learned successfully derived introduced for human resource development of the next generation to lead technologies in the society.

論文

Application of Bayesian approaches to nuclear reactor severe accident analysis

Zheng, X.; 玉置 等史; 塩津 弘之; 杉山 智之; 丸山 結

Proceedings of Asian Symposium on Risk Assessment and Management 2017 (ASRAM 2017) (USB Flash Drive), 11 Pages, 2017/11

Nuclear reactor severe accident simulation involves uncertainties, which may result from incompleteness of modeling of accident scenarios, selection of alternative models and unrealistic setting of parameters during the numerical simulation, etc. Both deterministic and probabilistic methods are required to reach reasonable estimation of risk for severe accidents. Computational codes are widely used for the deterministic accident simulations. Bayesian approaches, including both parametric and nonparametric, are applied to the simulation-based severe accident researches at Japan Atomic Energy Agency (JAEA). In the paper, an overview of these research activities is introduced: (1) Dirichlet process models, a nonparametric Bayesian approach, are applied to source term uncertainty and sensitivity analyses; (2) Gaussian process models are applied to the optimization for operations of severe accident countermeasures; (3) Nonparametric models, include models based on Dirichlet process and K-nearest neighbors algorithm, are built to predict the chemical forms of fission products. Simplified models are integrated into the integral severe accident code, THALES2/KICHE; (4) We have also launched the research of dynamic probabilistic risk assessment (DPRA), and because a great number of accident scenarios will be generated during DPRA, Bayesian approaches would be useful for the boosting of computational efficiency.

論文

Neutron resonance analysis for nuclear safeguards and security applications

Paradela, C.*; Heyse, J.*; Kopecky, S.*; Schillebeeckx, P.*; 原田 秀郎; 北谷 文人; 小泉 光生; 土屋 晴文

EPJ Web of Conferences (Internet), 146, p.09002_1 - 09002_4, 2017/09

 パーセンタイル:100

Neutron-induced reactions can be used to study the properties of nuclear materials in the field of nuclear safeguards and security. The elemental and isotopic composition of these materials can be determined by using the presence of resonance structures in the reaction cross sections as fingerprints. This idea is the basis of two non-destructive analytical techniques which have been developed at the GELINA neutron time-of-flight facility of the JRC-IRMM: Neutron Resonance Capture Analysis (NRCA) and Neutron Resonance Transmission Analysis (NRTA). A full quantitative validation of the NRTA technique was obtained by determining the areal densities of enriched reference samples used for safeguards applications with an accuracy better than 1%. Moreover, a combination of NRTA and NRCA has been proposed for the characterisation of particle-like debris of melted fuel formed in severe nuclear accidents. In order to deal with the problems due to the diversity in shape and size of these samples and the presence of strong absorbing matrix materials, new capabilities have been implemented in the resonance shape analysis code REFIT. They have been validated by performing a blind test in which the elemental abundance of a combined sample composed of unknown quantities of materials such as cobalt, tungsten, rhodium or gold was determined with accuracies better than 2%.

論文

Prediction of chemical effects of Mo and B on the Cs chemisorption onto stainless steel

Di Lemma, F. G.; 山下 真一郎; 三輪 周平; 中島 邦久; 逢坂 正彦

Energy Procedia, 127, p.29 - 34, 2017/09

 パーセンタイル:100

シビアアクシデント時における炉内のステンレス鋼へのセシウム(Cs)化学吸着挙動に関して、Csと化合物を形成すると考えられるモリブデン(Mo)及びホウ素(B)の影響を評価した。化学平衡計算を用いてCs化学吸着により生成される化合物の安定性を評価し、Mo及びBの影響を予測した。Moが存在する場合、一部はCs$$_{2}$$MoO$$_{4}$$として吸着する可能性が示された。一方、Cs化学吸着に与えるBの影響は小さいことが示された。以上の予測結果より、今後の研究においてMoの影響に対する考慮が必要であることがわかった。

論文

Development of the severe accident evaluation method on second coolant leakages from the PHTS in a loop-type sodium-cooled fast reactor

山田 文昭; 今泉 悠也; 西村 正弘; 深野 義隆; 有川 晃弘*

Proceedings of 25th International Conference on Nuclear Engineering (ICONE-25) (CD-ROM), 10 Pages, 2017/07

ループタイプ・ナトリウム冷却高速原型炉の設計基準事故(DBA)を超える除熱機能喪失の一つとして、2箇所の1次冷却材漏えいによる原子炉容器液位確保機能喪失(LORL)のシビアアクシデント(SA)評価手法を開発した。2ヶ所の1次冷却材漏えいは、DBAの出力運転中の1ヶ所の1次冷却材漏えいに伴う原子炉停止後の低温停止中に、別ループの1次冷却系配管において2ヶ所目の漏えいが発生し、過度に原子炉容器(RV)液位が低下し、LORLに至る可能性がある。本論文では、想定される漏えい部位の組合せから、厳しいRV液位となる代表事故シーケンスの選定、RVへの冷却材ナトリウムの汲み上げ、1次主冷却系のサイフォンブレークによるRV内冷却材ナトリウムの汲み出し停止の液位確保策、RV液位を過度計算するプログラム、液位計算プログラムを用いた代表事故シーケンスのRV液位挙動を示した。評価の結果、DBAを超える2ヶ所の1次冷却材漏えいに対して、2ヶ所目漏えいに対する液位確保策により崩壊熱除去運転に必要なRV液位が確保され、除熱機能喪失を防止できることを明らかにした。

論文

Fluid dynamic analysis on hydrogen deflagration in vertical flow channel with annular obstacles

松本 俊慶; 佐藤 允俊; 杉山 智之; 丸山 結

Proceedings of 25th International Conference on Nuclear Engineering (ICONE-25) (CD-ROM), 6 Pages, 2017/07

Hydrogen combustion including deflagration and detonation could become a significant threat to the integrity of containment vessel or reactor building in a severe accident of nuclear power stations. In the present study, numerical analyses were carried out for the ENACCEF No.153 test to develop computational techniques to evaluate the flame acceleration phenomenon during the hydrogen deflagration. This experiment investigated flame propagation in the hydrogen-air premixed gas in a vertical channel with flow obstacles. The reactingFoam solver of the open source CFD code, OpenFOAM, was used for the present analysis. Nineteen elementary chemical reactions were considered for the overall process of the hydrogen combustion. For a turbulent flow, renormalization group (RNG) k-e two-equation model was used in combination with wall functions. Three manners of nodalization were applied and its influences on the flame propagation acceleration were discussed.

論文

Preliminary analysis of the post-disassembly expansion phase and structural response under unprotected loss of flow accident in prototype sodium cooled fast reactor

小野田 雄一; 松場 賢一; 飛田 吉春; 鈴木 徹

Mechanical Engineering Journal (Internet), 4(3), p.16-00597_1 - 16-00597_14, 2017/06

For the prototype sodium-cooled fast reactor, MONJU, the mechanical energy and structural response under energetics caused by neutronic power excursion during Unprotected Loss of Flow accident (ULOF) were preliminarily analyzed. The objective of this study is to demonstrate the integrity of the reactor vessel against the mechanical load induced by the energetics. Conservative energy production was assumed in order to confirm the robustness of the safety design of MONJU. Mechanical energy was evaluated with the code in which mechanistic modelling of core expansion was implemented. The mechanical energy, which were obtained by analyzing the expanding behavior of core materials after energetics, were about one order of magnitude below the thermodynamic work potential calculated by assuming isentropic expansion of the fuel vapor to one atmosphere, which was often used as an indicator to express the severity of the energetics. Structural integrity was then evaluated with coupled fluid-structure dynamics code using the obtained mechanical energy. No or very small circumferential residual strain of the reactor vessel was evaluated in most analytical cases, and even in the most conservative energy production case, the residual strain was only 0.008 % so that the integrity of the reactor vessel is maintained. The result obtained in the present study shows that MONJU has enough robustness against the mechanical load under energetics.

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