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Journal Articles

Implementation of a new function for handling nuclear data of outgoing particles and residual excitation states in PHITS

Furuta, Takuya; Hashimoto, Shintaro; Ogawa, Tatsuhiko; Tanimura, Yoshihiko

Nuclear Instruments and Methods in Physics Research A, 1086, p.171320_1 - 171320_8, 2026/06

A new function to incorporate nuclear data libraries with outgoing particles plus residual nuclei in specific excitation states for neutron-induced reactions has been implemented in a Monte Carlo simulation code, Particle and Heavy Ion Transport code System (PHITS). With this function, accurate predictions of outgoing particle spectra and angular distributions according to the nuclear data libraries become possible, while accounting for production of residual nuclei and de-excitation gammas, conserving total energy and momentum in each event. This feature allows users to perform high-precision simulations of detector responses and radiation damage in materials.

Journal Articles

Journal Articles

Temperature effect on radiolytically generated hydrogen yield from a plutonium nitric acid aqueous solution

Toigawa, Tomohiro; Hotoku, Shinobu; Kumagai, Yuta; Abe, Yuma*; Oyama, Kanichi*; Fukaya, Hiroyuki; Ban, Yasutoshi; Kida, Takashi; Hasegawa, Satoshi*; Nakano, Masanao*; et al.

Journal of Nuclear Science and Technology, 63(3), p.322 - 327, 2026/03

 Times Cited Count:0 Percentile:0.00

The effect of temperature on hydrogen production generated from radiolysis was investigated to determine the associated implications for nuclear fuel reprocessing safety. The hydrogen yield from radiolysis of plutonium nitric acid solution was measured at temperatures up to the boiling temperature of the solution. The results showed no notable temperature dependence even under boiling conditions. The impact of solution agitation on hydrogen production was also assessed, which revealed minor differences in the hydrogen yield between static and agitated conditions at room temperature. These findings suggest that high temperatures or boiling the solution do not considerably enhance hydrogen generation, and provide crucial information for accurately modeling hydrogen risks under severe accidents.

JAEA Reports

Development of a high-resolution imaging camera for alpha dust and high-dose rate monitor (Contract research); FY2023 Nuclear Energy Science & Technology and Human Resource Development Project

Collaborative Laboratories for Advanced Decommissioning Science; Tohoku University*

JAEA-Review 2025-048, 56 Pages, 2026/02

JAEA-Review-2025-048.pdf:2.89MB

The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2023. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2022, this report summarizes the research results of the "Development of a high-resolution imaging camera for alpha dust and high-dose rate monitor" conducted in FY2023. The present study aims to develop a high-resolution imaging camera for alpha dust and a high-dose rate monitor. To realize the high-resolution imaging camera for alpha dust, we have developed novel scintillation materials with emission bands of 500-800 nm. Moreover, we have prepared several materials for the camera and software. We have also developed novel scintillation materials with emission bands of 650-1,000 nm, and simulation studies have been conducted for the high-dose-rate monitor system consisting of optical fiber. In addition, we demonstrated this monitoring system, and the dose-rate dynamic range was found to be 20 mSv/h to 1 kSv/h.

Journal Articles

Validation of ${it in situ}$ underwater radiation monitoring detector

Ji, W.*; Lee, E.*; Ji, Y.-Y.*; Ochi, Kotaro; Yoshimura, Kazuya; Funaki, Hironori; Sanada, Yukihisa

Nuclear Engineering and Technology, 58(2), p.103933_1 - 103933_6, 2026/02

We aimed to validate the performance of an in situ underwater radiation detector, MARK-U1 (Monitoring of Ambient Radiation of KAERI - Underwater), was used to estimate $$^{137}$$Cs activity concentration in river and reservoir sediment at predicted sites of contamination. Additionally, underwater core samples were collected to measure the radioactivity using a high-purity germanium (HPGe) detector. To estimate radioactivity, a conversion factor was derived by comparing the measured spectrum and $$^{137}$$Cs activity in the sample. A Monte Carlo N-Particle (MCNP) simulation was conducted to determine the effective source geometry for in situ measurement. The simulation results correlated well with the on-site MARK-U1 monitoring results, with a deviation of 31.62%. These findings validate the performance of the in situ detector. This device can therefore be used to estimate $$^{137}$$Cs activity concentration in the underwater sediment via on-site monitoring, without requiring sample collection.

Journal Articles

Separation of Rh(III) and direct electrodeposition in phosphonium-based ionic liquids with electrochemical and spectroscopic analyses for extracted Rh(III) complex

Tokumitsu, Shun*; Matsumiya, Masahiko*; Sasaki, Yuji

Separation and Purification Technology, 382(Part 2), p.135631_1 - 135631_9, 2026/02

JAEA Reports

Introduction of classification considered as waste package for dismantling waste in JRTF

Nakajima, Ryota; Sakai, Tatsuya; Tani, Riku; Handa, Yuichi; Sunaoshi, Mizuho*; Inoue, Hidetaka*; Yamada, Satoshi; Shimizu, Osamu

JAEA-Technology 2025-012, 39 Pages, 2026/01

JAEA-Technology-2025-012.pdf:2.31MB

JAERI's Reprocessing Test Facility (JRTF) has transition to decommissioning since 1996 and inside the facility dismantled equipment and instrument. In the dismantling and removal work of glove boxes and other equipment, starting in October 2022, we prepared a "Manual for Separation of Dismantled Materials of JRTF" and carried out sorting and separation of the generated dismantled waste with the aim of producing waste package that meets the technical standards required for disposal to a landfill facility. This report describes the results and findings of sorting and separating the dismantled waste generated during the dismantling and removal work of glove boxes and other equipment in accordance with the "Manual for Separation of Dismantled Materials of JRTF".

JAEA Reports

Summaries of research and development activities by using supercomputer system of JAEA in FY2024 (April 1, 2024 - March 31, 2025)

HPC Technology Promotion Office, Center for Computational Science & e-Systems

JAEA-Review 2025-044, 140 Pages, 2026/01

JAEA-Review-2025-044.pdf:8.77MB

Japan Atomic Energy Agency (JAEA) conducts research and development (R&D) in various fields related to nuclear power as a comprehensive institution of nuclear energy R&Ds, and utilizes computational science and technology in many activities. Over the past 10 years or so, the publication of papers utilizing computational science and technology at JAEA has accounted for about 20 percent of the total publications each fiscal year. The supercomputer system of JAEA has become an important infrastructure to support computational science and technology. In FY2024, the system was utilized in R&D activities that were prioritized in the Fourth Medium- to Long-Term Plan, including contributing to carbon neutrality through the development of innovative technologies for improving safety, creating innovation by promoting diverse R&D related to nuclear science and technology, promoting R&D in response to the accident at TEPCO's Fukushima Daiichi Nuclear Power Station, steadily implementing technological developments for the treatment and disposal of high-level radioactive waste, and supporting nuclear safety regulatory administration and nuclear disaster prevention by promoting safety research for these purposes. This report presents a great number of R&D results accomplished by using the system in FY2024, as well as user support, operational records and overviews of the system, and so on.

Journal Articles

Residual stress relief effect in gradient structural steel and remaining life evaluation under stochastic fatigue loads

Qin, T. Y.*; Hu, F. F.*; Xu, P. G.; Zhang, R.*; Su, Y. H.; Ao, N.*; Li, Z. W.*; Shinohara, Takenao; Shobu, Takahisa; Wu, S. C.*

International Journal of Fatigue, 202, p.109233_1 - 109233_16, 2026/01

Journal Articles

Measurement of uranium and fission products in a spent fuel sample using fiber-optic laser-induced breakdown spectroscopy

Batsaikhan, M.; Oba, Hironori*; Karino, Takahiro; Akaoka, Katsuaki; Wakaida, Ikuo*; Iwata, Yoshihiro; Sakamoto, Kan*

Journal of Analytical Atomic Spectrometry, 21 Pages, 2026/00

JAEA Reports

Evaluation of the flow rate of leachate from near surface waste disposal facilities of radioactive wastes from research, industrial and medical facilities based on the latest knowledge

Kitatani, Hikari; Ozone, Kenji; Nakata, Hisakazu

JAEA-Technology 2025-011, 57 Pages, 2025/12

JAEA-Technology-2025-011.pdf:5.32MB

Japan Atomic Energy Agency is responsible for near-surface disposal of research-related low-level radioactive waste and is considering two types of facilities: trench and concrete-pit. In safety assessment of such facilities, dose evaluation requires data on infiltration water. Evaluating infiltration involves uncertainties due to waste conditions and disposal environment. Therefore, in this report, a reference model was established based on the conceptual design conditions of near-surface disposal facilities, and leachate from the facilities was estimated by groundwater flow analysis, using applications by prior operators as reference and reflecting the latest knowledge for safety assessment. This allowed evaluation of how the hydraulic conductivity of each facility layer and surrounding soil affects leachate. Specifically, the 2D FEM groundwater flow code MIG2DF was used: trench facilities were evaluated assuming cover degradation, and concrete-pit facilities assuming salt effects in waste packages. Results showed that in trench facilities, deterioration of clay hydraulic conductivity increased inflow to the waste layer, especially when drainage layer conductivity decreased, as horizontal flow paths failed and infiltration into clay was promoted. In concrete-pit facilities, clay fracturing increased local flow and water through the waste layer. These results quantitatively demonstrate how changes in hydraulic conductivity of each layer affect leachate, providing useful insights for scenario development in safety assessment and for facility management.

JAEA Reports

Analytical study on stress behavior of core graphite components using simplified viscoelastic evaluation model

Saijo, Tomoaki; Shimazaki, Yosuke; Ishihara, Masahiro

JAEA-Technology 2025-010, 126 Pages, 2025/12

JAEA-Technology-2025-010.pdf:12.52MB

During the operation of the High Temperature Engineering Test Reactor (HTTR), thermal stress is generated in the graphite components. In addition, graphite exhibits dimensional shrinkage and creep deformation under neutron irradiation. As a result, residual stress remains in the graphite components during reactor shutdown. Therefore, in the design of the HTTR core graphite structures, stress analyses of the graphite components have previously been performed using the finite element analysis code VIENUS. In the HTTR, the graphite components are exposed to a wide range of temperature, from approximately 400$$^{circ}$$C to 1200$$^{circ}$$C, depending on their location. Consequently, irradiation-induced behaviors such as material property changes and irradiation shrinkage vary among the graphite components. On the other hand, since VIENUS code evaluates stress based on thermal fluid and heat conduction analysis results, it is not suitable for parametric studies. In this study, the influence of irradiation behavior on the stress behavior of graphite components in the wide temperature range (400$$^{circ}$$C to 1200$$^{circ}$$C) was analyzed using simplified viscoelastic evaluation model, consisting of two beam elements, to conduct efficient parametric studies. Operational stress exhibits two distinct patterns depending on whether the irradiation temperature is below or above 800$$^{circ}$$C, due to irradiation shrinkage. Residual stress approaches the thermal stress, preventing excessive increase even when irradiation shrinkage is large. Moreover good agreement in stress behavior trends was observed between the stress analysis results by the simplified viscoelastic evaluation model and VIENUS code. These results indicate that the simplified viscoelastic evaluation model is beneficial in simulating stress behavior.

JAEA Reports

Analysis of deposits inside "X-6 penetration" for the Unit 2 primary containment vessel at Fukushima Daiichi Nuclear Power Station

Yoneyama, Kai; Nitta, Ayako; Tanaka, Yasuyuki; Kodaka, Noriyasu; Kikuchi, Riku; Sakano, Takuma; Furuse, Takahiro; Sato, Soichi; Sambongi, Mitsuru; Tanaka, Kosuke

JAEA-Technology 2025-008, 44 Pages, 2025/12

JAEA-Technology-2025-008.pdf:4.3MB

At the TEPCO's Fukushima Daiichi Nuclear Power Station (1F), an investigation inside the reactors has been carried out. In order to safely carry out the decommissioning work such as fuel debris retrieval and building demolition, it is important to estimate the contamination in primary containment vessel for control the decommissioning planning and the worker radiation exposure levels. Therefore, the analysis of the deposit inside the penetration for the 1F Unit 2 primary containment vessel ("X-6 penetration") was performed to clarify the components and activity. The smears from the deposit were used for the analysis. Non-destructive analysis such as gamma-ray spectrometry, X-ray Fluorescence (XRF) and Scanning Electron Microscope-Energy dispersive X-ray spectroscopy (SEM-EDX) for the smear-samples were performed to determine the gamma-nuclides and the morphology of elements in the deposit. Furthermore, in order to evaluate the nuclides and nuclide composition of the deposit in detail, the smear-samples were dissolved and the quantitative analysis of gamma-nuclides, Sr-90, alpha-nuclides in the dissolved solution were conducted. The results (non-destructive analysis and quantitative analysis) were compared with the results of samples collected at different locations in the X-6 penetration in 2020. In the gamma-ray spectrometry as non-destructive analysis where the smears were analyzed directly, Co-60, Sb-125, Cs-134, Cs-137, Eu-154, Eu-155 and Am-241 were detected. In XRF results, Fe originating from construction material was detected as a major element and small amount of U and Zr originating from the fuel and fuel cladding were also detected. In SEM-EDX results, O and Fe were found as a major element of the deposit and U particles coexisting with Fe, Si, Cr, Ni and Zr were also found. These results were consistent with the SEM-EDX results of the samples collected in 2020. In radioactivity analysis, quantitative values for gamma-nuclides (Co-60, Sb-125, Cs-134, Cs-137, Eu-154, Eu-155), Sr-90, Pu-238, Pu-239+240, Am-241, Cm-244, U-235 and U-238 were obtained. Using the results, the ratios of radioactivity based on Cs-137 and U-238 were calculated. Both sets of the ratios were compared to the calculated value of the Unit 2 fuel composition from ORIGEN.

JAEA Reports

Design and characterisation of different characteristics of metakaolin-based geopolymer for fuel debris removal (Contract research); FY2023 Nuclear Energy Science & Technology and Human Resource Development Project

Collaborative Laboratories for Advanced Decommissioning Science; Hokkaido University*

JAEA-Review 2025-041, 79 Pages, 2025/12

JAEA-Review-2025-041.pdf:9.8MB

The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2023. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2023, this report summarizes the research results of the "Design and characterisation of different characteristics of metakaolin-based geopolymer for fuel debris removal" conducted in FY2023. This study aims to demonstrate the potential of metakaolin-based geopolymer, which has high fluidity and confinement performance, and incorporates neutron absorption capability through boron addition, for the stabilization and solidification of radioactive waste from fuel debris and contaminated water treatment. In this year, the research focused on the design and evaluation of metakaolin geopolymer with and without boron, the interaction between metakaolin-based geopolymer and Fe2O3 colloids, the characterization of geopolymer, and the property evaluation of simulated waste solidification samples. The influence of metakaolin's particle size and firing temperature on its leaching rate, and fluidity, hardening properties of geopolymer was investigated in detail. Additionally, the effects of boron addition in alkaline solution properties and extended hardening time were confirmed. In the interaction with colloids, the confinement of colloids and dimensional changes within the geopolymer were evaluated. Furthermore, solidification samples with simulated waste were prepared, and viscosity changes during the curing process were measured. Hardening time and temperature changes during curing were measured. Compression strength measurements and $$gamma$$-ray irradiation tests were also conducted, and through the measurement of hydrogen generation, important basic data on the properties of the solidified bodies were obtained. In research promotion, collaboration with Hokkaido University, JAEA, Sobueclay Co. Ltd., and the University of Sheffield was strengthened through regular meetings and data sharing, and plans for the following years were finalized. Additionally, a human resource development program was launched.

JAEA Reports

A Study on the methodology for rational treatment/disposal of contaminated concrete waste considering volume reduction of waste (Contract research); FY2023 Nuclear Energy Science & Technology and Human Resource Development Project

Collaborative Laboratories for Advanced Decommissioning Science; Hokkaido University*

JAEA-Review 2025-037, 103 Pages, 2025/12

JAEA-Review-2025-037.pdf:7.28MB

The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2023. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2023, this report summarizes the research results of the "A study on the methodology for rational treatment/disposal of contaminated concrete waste considering volume reduction of waste" conducted in FY2023. The present study aims to evaluate rational waste management strategies incorporating reuse and recycling focusing on radioactive concrete waste, which will be massively generated from dismantling. Feasibility and challenges of aggregate recycling are considered assuming a typical recycled aggregate production technique, based on the characteristics of the concrete. In 2023, the migration behaviors of radionuclides and ions in cementitious materials having interfacial transition zones (ITZ) were investigated through diffusion and leaching experiments using radioactive and non-radioactive tracers and modeled by random walk particle tracking method with a sampling technique using a probabilistic distribution model for two media with an interface. Properties of surrogate contaminated concrete samples prepared by immersing in Cs solution were examined. Migration of ions was studied for surrogate contaminated aggregates and recycled concrete using the surrogate. In addition, surrogate waste package was prepared using by-product powder to study mechanical and chemical properties as well as leaching behavior of radionuclides. Information on properties of the contaminated concrete and tools to estimate the amount of concrete were organized in order to evaluate different waste management scenarios incorporating reuse/recycling.

Journal Articles

A Methodology for the design of non-uniform core configurations in the modified STACY facility

Dechenaux, B.*; Brovchenko, M.*; Araki, Shohei; Gunji, Satoshi; Suyama, Kenya

Annals of Nuclear Energy, 223, p.111555_1 - 111555_11, 2025/12

 Times Cited Count:0 Percentile:0.00(Nuclear Science & Technology)

Journal Articles

Development of nano-sized graphene flowers as neutron reflectors; Intensify neutron beam caused by coherent scattering

Teshigawara, Makoto; Ikeda, Yujiro*; Muramatsu, Kazuo*; Sutani, Koichi*; Kimijima, Koichi*; Fukuzumi, Masafumi*; Noda, Yohei*; Koizumi, Satoshi*; Kawamura, Yuji*; Saruta, Koichi; et al.

Canadian Journal of Physics, 103(12), p.1225 - 1231, 2025/12

 Times Cited Count:0 Percentile:0.00

Science using neutrons in the nanometer (nm) wavelength region as probes is expanding into a wide range of fields, from basic research in materials and life science to industrial applications. Dramatic increase in the intensity of the beam source is required to drive such research. We have focused on coherent scattering caused by nano-sized particle aggregations to increase the intensity of neutron beams. Nanodiamond is being vigorously researched and developed with the aim of practical application. On the other hand, we have focused on graphene, which has higher van der Waals forces by an order of magnitude and stronger bonding, sp2, between carbons than nanodiamond. This is expected to lead to its processability into a lumped for and to adapt to higher radiation fields. By promoting chemical vapor deposition (CVD), we have established a technique to form nano-sized graphene (called graphene flower) with a shape similar to a sunflower flower. In this talk, we report on the neutron scattering properties that contribute to the coherent scattering of the newly developed graphene flower.

Journal Articles

Prediction analysis of the development of the excavation damaged zone around the gallery excavated at 500 m depth at Horonobe Underground Research Laboratory

Aoyagi, Kazuhei; Tamura, Tomonori; Ozaki, Yusuke; Ishii, Eiichi; Motoshima, Takayuki*; Sugawara, Kentaro*

Dai-51-Kai Gamban Rikigaku Ni Kansuru Shimpojiumu Koen Rombunshu(Internet), p.119 - 124, 2025/12

In a high-level radioactive waste disposal, it is important to understand the extent of the Excavation Damaged Zone (EDZ) because it can be one of the factors to determine whether disposal galleries or pits can be excavated or not in the design or construction phases. In this study, we performed a hydro-mechanical coupling analysis to simulate the three-dimensional excavation of the twin galleries which were excavated at a depth of 500 m in the Horonobe Underground Research Laboratory. The analysis revealed that the EDZ was developed 1.5-2.0 m from the gallery wall. The stress acting on the shotcrete was within the ultimate limit state. Based on these results, we estimated that the stability of the twin galleries will be maintained, despite the relatively large extent of the EDZ.

Journal Articles

None

Koizumi, Mitsuo; Yogo, Akifumi*

Isotope News, (802), p.11 - 14, 2025/12

no abstracts in English

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