Validation of underwater radiation monitoring detector

Ji, W.*; Lee, E.*; Ji, Y.-Y.*; Ochi, Kotaro; Yoshimura, Kazuya; Funaki, Hironori; Sanada, Yukihisa

Nuclear Engineering and Technology, 58(2), p.103933_1 - 103933_6, 2026/02

https://doi.org/10.1016/j.net.2025.103933

We aimed to validate the performance of an in situ underwater radiation detector, MARK-U1 (Monitoring of Ambient Radiation of KAERI - Underwater), was used to estimate Cs activity concentration in river and reservoir sediment at predicted sites of contamination. Additionally, underwater core samples were collected to measure the radioactivity using a high-purity germanium (HPGe) detector. To estimate radioactivity, a conversion factor was derived by comparing the measured spectrum and Cs activity in the sample. A Monte Carlo N-Particle (MCNP) simulation was conducted to determine the effective source geometry for in situ measurement. The simulation results correlated well with the on-site MARK-U1 monitoring results, with a deviation of 31.62%. These findings validate the performance of the in situ detector. This device can therefore be used to estimate Cs activity concentration in the underwater sediment via on-site monitoring, without requiring sample collection.

A Methodology for the design of non-uniform core configurations in the modified STACY facility

Dechenaux, B.*; Brovchenko, M.*; Araki, Shohei; Gunji, Satoshi; Suyama, Kenya

Annals of Nuclear Energy, 223, p.111555_1 - 111555_11, 2025/12

https://doi.org/10.1016/j.anucene.2025.111555

Gamma-ray spectral deconvolution using an unsupervised deep learning model for radioisotope identification with CsI(Tl) spectrometer for field use

Kimura, Yoshiki; Yamaguchi, Tomoki

Radioisotopes, 74(3), p.251 - 264, 2025/11

https://doi.org/10.3769/radioisotopes.740301

Radioisotope identification (RIID) by gamma-ray spectral analysis has been widely used, and accurate identification of radioisotopes is an important issue in various fields. Handheld instruments are commonly used for on-site RIID but often suffer from limited performance. This paper proposes a spectral deconvolution using unsupervised neural network models for RIID with handheld instruments in field use. This approach allows optimization of the neural network for deconvolution based on a measured spectrum combined with an energy-broadening matrix, and it does not require extensive training datasets or the precise modeling of the detector and measurement conditions. The performance of the proposed approach was examined in simulated and measured spectra, assuming the measurements of several radioisotopes with CsI(Tl) spectrometers. It was demonstrated that the unsupervised neural network models can improve the peak resolution more significantly compared to conventional deconvolution algorithms and contribute to RIID performance in the low energy resolution spectra.

Development of passive wireless communication systems operatable under inferior-wireless environment with obstacles (Contract research); FY2023 Nuclear Energy Science & Technology and Human Resource Development Project

Collaborative Laboratories for Advanced Decommissioning Science; Yokohama National University*

JAEA-Review 2025-025, 90 Pages, 2025/10

JAEA-Review-2025-025.pdf:5.59MB

The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2023. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2022, this report summarizes the research results of the "Development of passive wireless communication systems operatable under inferior-wireless environment with obstacles" conducted in FY2023. This study aims to develop a wireless communication system for obstacle-dense environments by designing base stations, sensor nodes (SN), positioning algorithms, and wireless area formation methods for electromagnetic wave-shielded regions. Key outcomes are as follows: For direction-finding with high-performance antennas, triangulation positioning accuracy was evaluated, and a sensor information demodulation system was built. SNs with frequency-scanning analog and frequency-fixed digital methods achieved communication distances of 6-8 meters and wireless charging of 1-2 V in 3-15 minutes at 6 meters. Diode characteristics remained unchanged after 1,000 Gy radiation. Positioning algorithms using multipath tomography were validated with a high-resolution measurement system in the lab. Simulations with reactor building CAD diagrams optimized node numbers and arrangements. Wireless coverage in electromagnetic wave-shielded regions was tested using a composite antenna (patch array and waveguide), achieving a range of approximately 1.5 meters.

Establishment of characterization method for small fuel debris using the world's first isotope micro imaging apparatus (Contract research); FY2023 Nuclear Energy Science & Technology and Human Resource Development Project

Collaborative Laboratories for Advanced Decommissioning Science; Kogakuin University*

JAEA-Review 2025-013, 111 Pages, 2025/10

JAEA-Review-2025-013.pdf:7.49MB

The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2023. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2021, this report summarizes the research results of the "Establishment of characterization method for small fuel debris using the world's first isotope micro imaging apparatus" conducted from FY2021 to FY2023. The present study aims to obtain, for the first time in the world, the important data necessary for clarifying the retrieval of small amounts of fuel debris, and to evaluate and examine them. The isotope microimaging apparatus (developed by Kogakuin University) introduced at the JAEA Fuel Monitoring Facility (FMF) can obtain local quantitative data such as isotope composition while processing cross-sections of radioactive micro-samples, which can be used to determine the properties of fuel debris. In FY2021, we improved the isotope microimaging apparatus introduced to the JAEA FMF to accommodate high radiation dose samples. In FY2022, we maintained the isotope microimaging apparatus at the JAEA FMF and succeeded in analyzing real particles containing uranium. In FY2023, we completed development to automate and remotely perform analysis routines using a prototype machine at Kogakuin University. At the JAEA FMF, although manual operations were involved, we succeeded in analyzing each Cs isotope from real particles by resonance ionization. In Nagoya University, we improved the RIMS apparatus to investigate the difference in electronic state caused by ion beam sputtering. And we succeeded in obtaining resonance ionization signals from neutral particles generated by ion beam sputtering. At the JAEA CLADS, they investigated the ionization scheme for important nuclides Nd and Gd. Those proposed ionization schemes were examined at Kogakuin University.

Weathering promotes the sorption of radiocesium in mafic minerals of river sediments in the Fukushima Prefecture, Japan

Hagiwara, Hiroki; Watanabe, Yusuke; Konishi, Hiromi*; Funaki, Hironori; Fujiwara, Kenso; Iijima, Kazuki

Applied Geochemistry, 190, p.106490_1 - 106490_10, 2025/10

https://doi.org/10.1016/j.apgeochem.2025.106490

Oxygen potential and oxygen diffusion data for guiding the manufacture of MOX fuel for fast neutron reactors

Vauchy, R.; Horii, Yuta; Hirooka, Shun; Akashi, Masatoshi; Sunaoshi, Takeo*; Nakamichi, Shinya; Saito, Kosuke

Journal of Nuclear Materials, 616, p.156115_1 - 156115_16, 2025/10

https://doi.org/10.1016/j.jnucmat.2025.156115

Research on radioactive aerosol control and decontamination at Fukushima Daiichi Nuclear Power Station Decommissioning (Contract research); FY2023 Nuclear Energy Science & Technology and Human Resource Development Project

Collaborative Laboratories for Advanced Decommissioning Science; The University of Tokyo*

JAEA-Review 2025-015, 73 Pages, 2025/09

JAEA-Review-2025-015.pdf:5.9MB

The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2023. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2021, this report summarizes the research results of the "Research on radioactive aerosol control and decontamination at Fukushima Daiichi Nuclear Power Station decommissioning" conducted from FY2021 to FY2023. The present study aims to develop a safe laser decontamination system that integrates advanced particle detection and characterization systems with aerosol dispersion control, in collaboration with UK researchers. For aerosol dispersion control, new containment methods ranging from simple mechanical containment hoods to optical laser shields are jointly investigated. The Japanese team will develop a radioactive dispersion control method based on the use of water mist and water spray to reduce radiation risks during laser cutting and decontamination applications. Based on data on aerosol particles provided by the UK team, the potential to enhance aerosol scrubbing efficiency will be explored. Additionally, the effect of charge enhancement will be evaluated. The UK team will develop laser-based aerosol containment methods and conducting experiments to improve the condensation of aerosol particles and mist in spray scrubbing. The development of aerosol removal technologies and strategies will be carried out through comprehensive experimental and computational studies. Experiments will be conducted at UTARTS facility to verify simultaneous operations such as laser decontamination, cutting, and spray operations. Aerosol measurements will also be performed to obtain high spatial resolution data that can better validate CFD models. In the final year, mock-up tests will be conducted to verify the system's operation and decontamination performance at full scale, evaluating the decontamination system developed through this research.

Clarification of debris formation conditions on the basis of the sampling data and experimental study using simulated fuel debris and reinforcement of the analytical results of severe accident scenario (Contract research); FY2023 Nuclear Energy Science & Technology and Human Resource Development Project

Collaborative Laboratories for Advanced Decommissioning Science; University of Fukui*

JAEA-Review 2025-007, 120 Pages, 2025/09

JAEA-Review-2025-007.pdf:8.13MB

The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2023. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station (1F), Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2021, this report summarizes the research results of the "Clarification of debris formation conditions on the basis of the sampling data and experimental study using simulated fuel debris and reinforcement of the analytical results of severe accident scenario" conducted from FY2021 to FY2023. The present study aims to clarify the debris formation mechanism and utilize the results to refine the accident scenario. In the backward analysis of oxide debris formation, we prepared simulated fuel particles by the aerodynamic levitation method and ejection of melted oxides from a tungsten pipe with a small hole and summarized the relationship between preparation conditions and the properties of the particles. We also demonstrated the formation of simulated fuel debris obtained by the sampling in 1F and clarified the difference between the experimental results and thermodynamic calculation. From the estimation of mixing, melting and solidified states of metallic debris, it was found that the formation of thin reaction layer suppresses the damage of SUS in spite of Zr content around 1000 C, and we quantify the elution rate of BC and Zircaloy to the melted SUS. We extended reaction rate data between various pressure vessel with SUS and Zr and welding parts and suggested reaction rate equation for large scale experiment. We also estimated the failure behavior of lower plenum of pressure vessel and outflow behavior of melt. Furthermore, we estimated transition behavior of Uranium melt to metallic debris melt in the re-melting process of predropped metallic debris. As the experimental techniques in the future, we prepared the semi-melted debris from oxide and metals and analyzed the reaction products and discussed the formation of simulated debris with a small amount of uranium oxide using a CCIM furnace and the aerodynamic levitation method.

Simple technique for the preparation of uranium-impregnated porous silica particles and their application as working standard particles for analysis of the safeguards environmental samples

Tomita, Jumpei; Tomita, Ryohei; Suzuki, Daisuke; Yasuda, Kenichiro; Miyamoto, Yutaka

Journal of Nuclear Science and Technology, 12 Pages, 2025/09

https://doi.org/10.1080/00223131.2025.2557376