Intruder configurations in Ne at the transition into the island of inversion; Detailed structure study of Ne

Wang, H.*; Yasuda, Masahiro*; Kondo, Yosuke*; Nakamura, Takashi*; Tostevin, J. A.*; Ogata, Kazuyuki*; Otsuka, Takaharu*; Poves, A.*; Shimizu, Noritaka*; Yoshida, Kazuki; et al.

Physics Letters B, 843, p.138038_1 - 138038_9, 2023/08

https://doi.org/10.1016/j.physletb.2023.138038

Detailed -ray spectroscopy of the exotic neon isotope Ne has been performed using the one-neutron removal reaction from Ne. Based on an analysis of parallel momentum distributions, a level scheme with spin-parity assignments has been constructed for Ne and the negative-parity states are identified for the first time. The measured partial cross sections and momentum distributions reveal a significant intruder p-wave strength providing evidence of the breakdown of the N = 20 and N = 28 shell gaps. Only a weak, possible f-wave strength was observed to bound final states. Large-scale shell-model calculations with different effective interactions do not reproduce the large p-wave and small f-wave strength observed experimentally, indicating an ongoing challenge for a complete theoretical description of the transition into the island of inversion along the Ne isotopic chain.

Development of technologies for enhanced analysis accuracy of fuel debris; Summary results of the 2020 fiscal year (Subsidy program for the project of decommissioning and contaminated water management)

Ikeuchi, Hirotomo; Koyama, Shinichi; Osaka, Masahiko; Takano, Masahide; Nakamura, Satoshi; Onozawa, Atsushi; Sasaki, Shinji; Onishi, Takashi; Maeda, Koji; Kirishima, Akira*; et al.

JAEA-Technology 2022-021, 224 Pages, 2022/10

JAEA-Technology-2022-021.pdf:12.32MB

A set of technology, including acid dissolving, has to be established for the analysis of content of elements/nuclides in the fuel debris samples. In this project, a blind test was performed for the purpose of clarifying the current level of analytical accuracy and establishing the alternative methods in case that the insoluble residue remains. Overall composition of the simulated fuel debris (homogenized powder having a specific composition) were quantitatively determined in the four analytical institutions in Japan by using their own dissolving and analytical techniques. The merit and drawback for each technique were then evaluated, based on which a tentative flow of the analyses of fuel debris was constructed.

Stabilization treatment of nuclear fuel material contained with organic matter

Senzaki, Tatsuya; Arai, Yoichi; Yano, Kimihiko; Sato, Daisuke; Tada, Kohei; Ogi, Hiromichi*; Kawanobe, Takayuki*; Ono, Shimpei; Nakamura, Masahiro; Kitawaki, Shinichi; et al.

JAEA-Testing 2022-001, 28 Pages, 2022/05

JAEA-Testing-2022-001.pdf:2.33MB

In preparation for the decommissioning of Laboratory B of the Nuclear Fuel Cycle Engineering Laboratory, the nuclear fuel material that had been stored in the glove box for a long time was moved to the Chemical Processing Facility (CPF). This nuclear fuel material was stored with sealed by a polyvinyl chloride (PVC) bag in the storage. Since it was confirmed that the PVC bag swelled during storage, it seems that any gas was generated by radiolysis of the some components contained in the nuclear fuel material. In order to avoid breakage of the PVC bag and keep it safety for long time, we began the study on the stabilization treatment of the nuclear fuel material. First, in order to clarify the properties of nuclear fuel material, radioactivity analysis, component analysis, and thermal analysis were carried out. From the results of thermal analysis, the existence of organic matter was clarified. Then, ion exchange resin with similar thermal characteristics was selected and the thermal decomposition conditions were investigated. From the results of these analyzes and examinations, the conditions for thermal decomposition of the nuclear fuel material contained with organic matter was established. Performing a heat treatment of a small amount of nuclear fuel material in order to confirm the safety, after which the treatment amount was scaled up. It was confirmed by the weight change after the heat treatment that the nuclear fuel material contained with organic matter was completely decomposed.

Quantitative analysis of Zr adsorbed on IDA chelating resin using Micro-PIXE

Arai, Yoichi; Watanabe, So; Ono, Shimpei; Nomura, Kazunori; Nakamura, Fumiya*; Arai, Tsuyoshi*; Seko, Noriaki*; Hoshina, Hiroyuki*; Kubota, Toshio*

QST-M-23; QST Takasaki Annual Report 2018, P. 59, 2020/03

https://repo.qst.go.jp/records/79251

C ages and calendar years of Japanese nails measured with accelerator mass spectrometry

Nagata, Kazahiro*; Furunushi, Yasuko*; Matsubara, Akihiro*; Kokubu, Yoko; Nakamura, Toshio*

Tetsu To Hagane, 105(4), p.488 - 491, 2019/04

https://doi.org/10.2355/tetsutohagane.TETSU-2018-137

The Japanese nails had been produced by the traditional ironmaking way of Tatara until the Edo period since the late of 6 Century. The quality of the Japanese nails is affected from steel produced by Tatara in each age. The C ages of 3 Japanese nails collected at shrines and temples at their repair were measured with accelerator mass spectrometry and calibrated to calendar years. Each C age provided plural calendar year periods with definite probabilities, and one of the periods determined in comparison with the history of temples and their repair records. The production ages of nails used in the Daibutuden of the Todaiji temple, the living quarters of the Manjuin temple and the Zaoudo of the Yoshino-Kongoji temple are before 1692, the 12 Century and before 1592, respectively, when they were repaired or reconstructed.

Occupation sites and valence states of Co dopants in (La, Co)-codoped M-type Sr ferrite; Fe and Co nuclear magnetic resonance studies

Sakai, Hironori; Hattori, Taisuke; Tokunaga, Yo; Kambe, Shinsaku; Ueda, Hiroaki*; Tanioku, Yasuaki*; Michioka, Chishiro*; Yoshimura, Kazuyoshi*; Takao, Kenta*; Shimoda, Aiko*; et al.

Physical Review B, 98(6), p.064403_1 - 064403_10, 2018/08

https://doi.org/10.1103/PhysRevB.98.064403

To specify preferential occupation sites of Co substituents and to clarify charge and spin states of Co ions in (La, Co)-cosubstituted hexagonal magnetoplumbite-type (M-type) Sr ferrite, Fe and Co nuclear magnetic resonance (NMR) spectra are measured under zero and external magnetic fields using powdered and single crystalline specimens. To a considerable degree, the charge compensation between La and Co works in the equal (La, Co)-codoped case, where more than half of the Co ions are considered to be present in the minority spin sites at the center of the oxygen tetrahedra, with the = 3/2 state carrying a small orbital moment owing to spin-orbit interaction. The remaining small number of high-spin Co ( = 3/2, = 1) ions with unquenched orbital moments would be distributed to the other octahedral , , and sites.

AMS radiocarbon age of the Kurodake pyroclastic-flow deposit in Kuju volcanic group, SW Japan

Okuno, Mitsuru*; Nagaoka, Shinji*; Kokubu, Yoko; Nakamura, Toshio*; Kobayashi, Tetsuo*

Fukuoka Daigaku Rigaku Shuho, 48(1), p.1 - 5, 2018/03

http://id.nii.ac.jp/1316/00004368/

Kuju volcanic group, located in central Kyushu, Japan, consists of over twenty volcanoes (lava domes as well as small stratovolcanoes). The Kurodake is largest lava dome with a volume of 1.6 km, and generated Kurodake pyroclastic-flow (Kj-Kd) and ash-fall (Kj-KdA) deposits. To refine age of the Kurodake eruption, we conducted radiocarbon dating of a charcoal fragment in the Kj-Kd with an AMS system at Tono Geoscience Center, JAEA. The obtained C date, 150540 BP, can correspond to 1310-1423 cal BP (probability= 74.6%), 1430-1442 cal BP (2.4%) and 1456-1521 cal BP (23.0%) in 2 confidence level. The medium probability date, 1391 cal BP, is consistent with the stratigraphy and gives the reliable age for the Kj-Kd.

AMS radiocarbon dates of pyroclastic-flow deposits on the southern slope of the Kuju Volcanic Group, Kyushu, Japan

Okuno, Mitsuru*; Nagaoka, Shinji*; Kokubu, Yoko; Nakamura, Toshio*; Kobayashi, Tetsuo*

Radiocarbon, 59(2), p.483 - 488, 2017/00

https://doi.org/10.1017/RDC.2016.66

We present here results of AMS C dating to refine the history of the middle and western parts of the Kuju Volcanic Group, located in middle Kyushu, Japan, which consists of more than 20 lava domes and cones. C dating has conducted by AMS (JAEA-AMS-TONO) under the Common-Use Facility Program of JAEA. The Handa PF deposits, which are products of the largest eruption of the group, were dated to 53.5 ka BP. The Shirani and Muro PF deposits, which are block-and-ash flows, were dated to 44 to 50 cal ka BP and 3539 cal ka BP, respectively. These ages can be correlated with the TL ages for the lava domes. Therefore, both TL and C methods can be useful tools in establishing the eruptive sequence of lava domes and pyroclastic flows. This study also demonstrates that these eruptive activities occurred after the Handa pfl, the biggest eruption during the last 150 kyrs without a significant time interval.

Development of human resource capacity building assistance for nuclear security

Noro, Naoko; Nakamura, Yo; Hirai, Mizuki; Kobayashi, Naoki; Kawata, Norio; Naoi, Yosuke

Proceedings of 18th International Symposium on the Packaging and Transport of Radioactive Materials (PATRAM 2016) (DVD-ROM), 7 Pages, 2016/09

The paper describes the methdologies ISCN has adopted to develop its training curricula on nuclear security. ISCN has been working closely with the international partners to build its own capacity, especially with the Sandia National Laboratories of the United States. The paper then focuses on the joint course development between IAEA and ISCN on the International Training Course on Transport Security which ISCN hosted in 2015.

Basic Radiation Knowledge for School Education Course; Nuclear Technology Seminar 2014 (Contract program)

Watanabe, Yoko; Arai, Nobuyoshi; Sawada, Makoto; Kanaizuka, Seiichi; Shimada, Mayuka*; Ishikawa, Tomomi*; Nakamura, Kazuyuki

JAEA-Review 2015-026, 38 Pages, 2015/11

JAEA-Review-2015-026.pdf:10.55MB

JAEA has conducted Nuclear Technology Seminar for Asian countries which plan to introduce NPP, in order to increase the number of engineers and specialists. The Nuclear Technology Seminar on the Basic Radiation Knowledge for School Education Course was launched in 2012 due to increased recognition of the dissemination of the basic knowledge of radiation in public and education sectors as an important issue in the aftermath of the Fukushima Dai-ichi NPP Accident. In response to the requests of past participants, a new exercise "Joint experiment with high school students" was introduced from 2014 to provide an international learning experience for the course participants and the local Japanese students. A new learning material was also developed to help participants to study the basics of radiation in English. All the course activities including the details of preparatory process and course evaluation were described in this report.