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Journal Articles

Innovative powder production and granulation for advanced MOX fuel fabrication

Kurita, Tsutomu; Kato, Yoshiyuki; Yoshimoto, Katsunobu; Suzuki, Masahiro; Kihara, Yoshiyuki; Fujii, Kanichi

Proceedings of International Conference on Advanced Nuclear Fuel Cycle; Sustainable Options & Industrial Perspectives (Global 2009) (CD-ROM), p.94 - 102, 2009/09

With regard to advanced MOX fuel fabrication, a new concept in which one vessel especially designed to meet microwave de-nitration is utilized also for crushing and for granulation, without organic lubricant nor powder transfer across the processes, was introduced for innovative MOX powder production. In order to realize this concept, two attempts were made: A specially designed three blade impeller coupled with auxiliary blade. A uniquely shaped mixing blade coupled with an auxiliary blade having auto-orbital hybrid rotation. The mixing blade promotes the growth of particles, whereas the auxiliary blade suppresses the overgrowth by chopping larger particles. These granulators use a little water as binder. As a result, major diameter of granule 400-1000 micron and flow-ability 82-85 was obtained with fine WO$$_{3}$$ model powder. Therefore, a prospect to satisfy both desirable powder properties and simplified nuclear material production was opened, as well as improvement of working efficiency and cut down on costs.

Journal Articles

Flowability measurement of coarse particles using vibrating tube method

Ishii, Katsunori; Suzuki, Masahiro; Yamamoto, Takuma; Kihara, Yoshiyuki; Kato, Yoshiyuki; Kurita, Tsutomu; Yoshimoto, Katsunobu; Yasuda, Masatoshi*; Matsusaka, Shuji*

Journal of Chemical Engineering of Japan, 42(5), p.319 - 324, 2009/05

 Times Cited Count:7 Percentile:29.69(Engineering, Chemical)

The flowability of coarse particles has been experimentally investigated using the vibrating tube method, to evaluate the applicability of this method to MOX (mixed oxide of PuO$$_{2}$$ and UO$$_{2}$$) particles which are nuclear fuel used for electric power production. Five sizes of non-radioactive model particles, smaller than 850 micrometers, made of ZrO$$_{2}$$ were prepared, and the experiments were carried out using vibrating tubes with an outlet diameter from 2 to 4 mm. The outlet diameter significantly affected the flowability measurements. When using the tube with a 4-mm-outlet diameter, the flowability of all the model particles was successfully measured. The inclination angle of the tube, also, affected the flowability measurements. From the advantages of high sensitivity, short measurement time, simple structure, and easy operation, the vibrating tube method is expected to be applied to the remote flowability measurement of the MOX particles.

Journal Articles

Application of microwave heating to MOX fuel production and its contribution to Japanese energy strategy

Suzuki, Masahiro; Ishii, Katsunori; Yamamoto, Takuma; Kihara, Yoshiyuki; Kato, Yoshiyuki; Kurita, Tsutomu; Yoshimoto, Katsunobu; Fujii, Kanichi

Proceedings of Global Congress on Microwave Energy Applications (GCMEA 2008/MAJIC 1st), p.501 - 504, 2008/08

The natural resources, oil and uranium, would dry up around the midway of this century. FBR cycle most probably rescues this difficult situation. Mass production of MOX fuel for FBR, therefore, is the supreme subject to Japanese energy strategy. For this subject, we are attacking with Microwave heating technology. Up to present, we have succeeded to produce excellent PuO$$_{2}$$/UO$$_{2}$$ bulk, 2 kgMOX/batch, advancing toward the mass production target, 5 kgU/h for one batch.

JAEA Reports

Stabilization of simulated radioactive lead waste and simulated low level radioactive liquid waste using reformed sulfur (Joint research)

Sone, Tomoyuki; Sasaki, Toshiki; Miyamoto, Yasuaki; Yamaguchi, Hiromi; Inoue, Haruka*; Kihara, Tsuyoshi*; Takei, Yoshihisa*; Tatekawa, Takaiki*; Fukaya, Masaaki*; Iriya, Keishiro*; et al.

JAEA-Technology 2008-032, 25 Pages, 2008/03

JAEA-Technology-2008-032.pdf:5.54MB

Reformed sulfur (RS) is superior in water interception and acid resistance compared with cement. Therefore solidified wastes with RS should have the high resistance to leaching. Unconfined compressive strength test and leaching test using solidified simulated wastes containing lead contaminated with radioactive nuclides (Lead waste) with RS and solidified simulated low level radioactive liquid waste (LLLW) with RS were conducted to examine the applicability of reformed sulfur solidification method (RSSM) as solidification technique of Lead waste and LLLW. The results of these studies show that RSSM is effective technique for stabilization of lead compared with cement solidification method because solidified lead with RS has much stronger resistance to leaching of lead than solidified lead with cement. It also show that the applicability of RSSM as solidification technique of the waste containing lead oxide and LLLW is low because the resistance to leaching of solidified lead oxide with RS and of solidified simulated LLLW with RS were equal to or lower than those of solidified products with cement respectively.

Journal Articles

Journal Articles

Iodine behavior during dissolution process within NUCEF-BECKY

Kihara, Takehiro; Sakurai, Tsutomu*; *; Fujine, Sachio

Proc. of 5th Int. Nucl. Conf. on Recycling, Conditioning and Disposal (RECOD '98), 1, p.830 - 837, 1998/00

no abstracts in English

Journal Articles

Trapping and measuring radioiodine (iodine-129) in cartridge filters

Sakurai, Tsutomu; ; M.-L.Ye*; Kihara, Takehiro; Fujine, Sachio

Journal of Nuclear Science and Technology, 34(2), p.211 - 216, 1997/02

 Times Cited Count:16 Percentile:75.78(Nuclear Science & Technology)

no abstracts in English

Oral presentation

Feasibility study on powder flowability evaluation on simplified pelletizing MOX fuel fabrication process using vibrating capillary method; Influence of particle shape and diameter on flowability

Ishii, Katsunori; Suzuki, Masahiro; Yamamoto, Takuma; Kihara, Yoshiyuki; Matsusaka, Shuji*; Yasuda, Masatoshi*; Suna, Takayuki*; Kurita, Tsutomu; Kato, Yoshiyuki

no journal, , 

JAEA is developing simplified pelletizing MOX fuel fabrication process for fast breeder reactor. The final product of de-nitration, conversion and granulation process, are MOX fuel particles, of which diameter is hundres micrometer. These particles should have high flowability for easy handling in next process. The powder flowability is now evaluated by Carr's flowability index. In this oral presentation, the feasibility of powder flowability evaluation using vibrationg capillary method is investigated, employing ZrO$$_{2}$$ particles of shich parameters are diameter and particle shape (shapes are varied by gronding particle edge). Screening small particles under about 100 micrometer contribute best the improvement of powder flowability, screening small particle under 50 micrometer in the second, and rounding particle shape in the third.

Oral presentation

Relationship between outlet diameter of tube and mesurement range of particle diameter in vibrating tube method

Ishii, Katsunori; Suzuki, Masahiro; Yamamoto, Takuma; Kihara, Yoshiyuki; Kurita, Tsutomu; Kato, Yoshiyuki; Yasuda, Masatoshi*; Matsusaka, Shuji*; Yoshimoto, Katsunobu

no journal, , 

Particle flowability test using a vibrating tube with a tapered end was carried out to evaluate the applicability of this method to the analysis of MOX particles for nuclear fuel pellet fabrication. In this experiment, zirconia particles were used as model particles, which are less than 850 micrometers in diameter. The sample particles were prepared by mixing the particles with different sizes. The experimental results showed that stable fowability evaluation is possible for particles larger than 45 micrometers and less than 850 micrometres, adjusting outlet diameter of tube and inclination angle of tube.

Oral presentation

Discussion on optimization of microwave heating for MOX fuel production

Kato, Yoshiyuki; Kurita, Tsutomu; Matsumoto, Masaki; Suzuki, Masahiro; Ishii, Katsunori; Yamamoto, Takuma; Kihara, Yoshiyuki; Yoshimoto, Katsunobu; Fujii, Kanichi

no journal, , 

An earlier accomplishment of FBR(fast breeder reactor) fuel cycle is the supreme subject from the point of view on the protection of environment by suppressing the green house effect as well as saving the oil. Microwave heating (MH) is employed as the MOX (mixed oxides U-Pu) production process in the main stream of FBR cycle. Thus, we are the optimization of MH method. We will describe the practical work of MOX fuel production which recycles the consumed nuclear fuel containing both U and Pu. The MH is employed to solidify the mixed solution by evaporating nitric acid and water. We call this processing de-nitration. The physical, mechanical, and chemical characteristics of the products are analyzed, being thereby discussed the contribution of the MH technology to the MOX fuel production. And, optimization of MH is discussed from the view point of design of MH oven, regulation of MH power, and combination with several auxiliary heating sources.

Oral presentation

Development of simplified pellet fuel production technology, 2; Processing technology for de-nitration conversion based on microwave heating

Kato, Yoshiyuki; Kimura, Yuichi; Isomae, Hidemi; Kurita, Tsutomu; Yoshimoto, Katsunobu; Makino, Takayoshi; Suzuki, Masahiro; Kihara, Yoshiyuki

no journal, , 

no abstracts in English

Oral presentation

Development of simplified pellet fuel production technology, 4; Unified technology of de-nitration conversion and granulation

Kurita, Tsutomu; Kato, Yoshiyuki; Yoshimoto, Katsunobu; Ishii, Katsunori; Suzuki, Masahiro; Kihara, Yoshiyuki

no journal, , 

no abstracts in English

Oral presentation

Development of simplified pellet fuel production technology, 3; Mass production technology for De-nitration conversion based on microwave heating

Ishii, Katsunori; Yamamoto, Takuma; Suzuki, Masahiro; Kihara, Yoshiyuki; Kato, Yoshiyuki; Kurita, Tsutomu; Yoshimoto, Katsunobu; Yoshimura, Tadahiro*

no journal, , 

To confirm the prospect of the simplified pellet production technology, JAEA is developing mass production technology for de-nitration conversion based on microwave heating. Base on the experimental result, the suitable processes for the mass production, are selected.

Oral presentation

Development of simplified pellet fuel production technology, 1; Ongoing works and future subjects

Suzuki, Masahiro; Ishii, Katsunori; Kihara, Yoshiyuki; Kurita, Tsutomu; Yoshimoto, Katsunobu; Okita, Takatoshi; Kashimura, Motoaki; Kato, Masato; Namekawa, Takashi; Fujii, Kanichi

no journal, , 

In FaCT project, we have set major six technologies for success of simplified pellet fuel fabrication. Our schedule on the technical fundamental technology should be completed by 2010, being transferred to the development of a technology for tele-command operation of mass production and facility maintenance until 2015. In this time, we will report current states of FaCT project as well as future plan.

Oral presentation

Experiment to reduce sample amount in vibrating tube method

Ishii, Katsunori; Suzuki, Masahiro; Yamamoto, Takuma; Kihara, Yoshiyuki; Kurita, Tsutomu; Kato, Yoshiyuki; Yoshimoto, Katsunobu; Yasuda, Masatoshi*; Matsusaka, Shuji*

no journal, , 

The feasibility study on applyiing the vibrating tube method to the MOX powder for FBR fuel production has been carried out. it is favorable to reduce the sample amount for effective flowability measurement. In this study, the possibility to reduce the sample amount in the vibrating tube method was investigated, analizing the influence of the sample amount on flowability profiles.

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