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Journal Articles

Cross section asymmetry of polarized $$gamma$$-ray elastic scattering

Omer, M.; Shizuma, Toshiyuki*; Koizumi, Mitsuo; Hajima, Ryoichi*; Hashimoto, Satoshi*; Miyamoto, Shuji*

LASTI Annual Report, 24, p.20 - 22, 2023/12

Journal Articles

Effect of nitrogen concentration on creep strength and microstructure of 9Cr-ODS ferritic/martensitic steel

Oka, Hiroshi*; Tanno, Takashi; Yano, Yasuhide; Otsuka, Satoshi; Kaito, Takeji; Hashimoto, Naoyuki*

Journal of Nuclear Materials, 572, p.154032_1 - 154032_8, 2022/12

 Times Cited Count:3 Percentile:66.21(Materials Science, Multidisciplinary)

9Cr oxide dispersion strengthened steels with slightly different nitrogen concentrations (0.0034 - 0.029 wt%) were prepared and their creep property at 973 K was investigated with microstructural characterization before and after the creep test. The creep strength decreased significantly as the nitrogen concentration increased. Microstructural observation revealed that, in the higher nitrogen concentration specimen, coarse Y-rich inclusions were found along the boundary between transformed ferrite region and residual ferrite region. The solubility difference of nitrogen in $$alpha$$ and $$gamma$$ phase would induce the localized increment of nitrogen concentration in the boundary region during the austenitizing process, resulting in the thermodynamic destabilization and subsequent coarsening of the dispersed oxide particles. The rows of creep voids were found near the rupture part of the crept specimen, suggesting that the coarse inclusions were the starting point of creep void formation and the subsequent premature fracture.

Journal Articles

Mesospheric ionization during substorm growth phase

Murase, Kiyoka*; Kataoka, Ryuho*; Nishiyama, Takanori*; Nishimura, Koji*; Hashimoto, Taishi*; Tanaka, Yoshimasa*; Kadokura, Akira*; Tomikawa, Yoshihiro*; Tsutsumi, Masaki*; Ogawa, Yasunobu*; et al.

Journal of Space Weather and Space Climate (Internet), 12, p.18_1 - 18_16, 2022/06

 Times Cited Count:1 Percentile:20.65(Astronomy & Astrophysics)

We identified two energetic electron precipitation (EEP) events during the growth phase of moderate substorms and estimated the mesospheric ionization rate for an EEP event for which the most comprehensive dataset from ground-based and space-born instruments was available. The mesospheric ionization signature reached below 70 km altitude and continued for ~15 min until the substorm onset, as observed by the PANSY radar and imaging riometer at Syowa Station in the Antarctic region. We also used energetic electron flux observed by the Arase and POES 15 satellites as the input for the air-shower simulation code PHITS to quantitatively estimate the mesospheric ionization rate. Combining the cutting-edge observations and simulations, we shed new light on the space weather impact of the EEP events during geomagnetically quiet times, which is important to understand the possible link between the space environment and climate.

Journal Articles

Impressions of the 3rd Joint Meeting of Japanese Society of Radiation Safety Management and Japan Health Physics Society

Watanabe, Yuki; Tsuji, Tomoya; Hirota, Seiko*; Hokama, Tomonori; Nakajima, Junya; Tsujiguchi, Takakiyo*; Kimura, Tatsuki*; Koike, Hiromi*; Nakamura, Kaori*; Kuwata, Haruka*; et al.

Hoken Butsuri (Internet), 57(1), p.54 - 64, 2022/03

no abstracts in English

Journal Articles

Anomalous radioisotope production for $$^{68}$$ZnO using polyethylene by accelerator neutrons

Tsukada, Kazuaki; Nagai, Yasuki*; Hashimoto, Shintaro; Minato, Futoshi; Kawabata, Masako*; Hatsukawa, Yuichi*; Hashimoto, Kazuyuki*; Watanabe, Satoshi*; Saeki, Hideya*; Motoishi, Shoji*

Journal of the Physical Society of Japan, 89(3), p.034201_1 - 034201_7, 2020/03

 Times Cited Count:2 Percentile:21.72(Physics, Multidisciplinary)

We found anomalously large yields of $$^{67}$$Ga, $$^{66}$$Ga, $$^{rm 69m}$$Zn and $$^{64}$$Cu by neutron irradiation on a $$^{68}$$ZnO sample in a polyethylene shield. Neutron beams are generated from the $$^{9}$$Be($$d,n$$) reaction for 50 MeV deuterons. The yields obtained were more than 20 times larger than those in the unshielded sample. On the other hand, the yields of $$^{67}$$Ga, $$^{66}$$Ga, $$^{rm 69m}$$Zn and $$^{64}$$Cu from a metallic $$^{68}$$Zn sample and the yields of $$^{67}$$Cu, $$^{65}$$Ni and $$^{65}$$Zn from the $$^{68}$$ZnO and $$^{68}$$Zn samples were almost insensitive to the shield conditions. This finding would provide us a unique capability of accelerator neutrons to simultaneously produce a large amount of several radioisotopes, including proton induced reaction products, by using a single sample. The experimental data were compared with the yields estimated by using the Particle and Heavy Ion Transport code System and the result was discussed.

Journal Articles

Room temperature and low-field resonant enhancement of spin Seebeck effect in partially compensated magnets

Ramos, R.*; Hioki, Tomosato*; Hashimoto, Yusuke*; Kikkawa, Takashi*; Frey, P.*; Kreil, A. J. E.*; Vasyuchka, V. I.*; Serga, A. A.*; Hillebrands, B.*; Saito, Eiji

Nature Communications (Internet), 10, p.5162_1 - 5162_8, 2019/11

 Times Cited Count:24 Percentile:76.4(Multidisciplinary Sciences)

Journal Articles

First nuclear transmutation of $$^{237}$$Np and $$^{241}$$Am by accelerator-driven system at Kyoto University Critical Assembly

Pyeon, C. H.*; Yamanaka, Masao*; Oizumi, Akito; Fukushima, Masahiro; Chiba, Go*; Watanabe, Kenichi*; Endo, Tomohiro*; Van Rooijen, W. G.*; Hashimoto, Kengo*; Sakon, Atsushi*; et al.

Journal of Nuclear Science and Technology, 56(8), p.684 - 689, 2019/08

 Times Cited Count:12 Percentile:79.53(Nuclear Science & Technology)

This study demonstrates, for the first time, the principle of nuclear transmutation of minor actinide (MA) by the accelerator-driven system (ADS) through the injection of high-energy neutrons into the subcritical core at the Kyoto University Critical Assembly. The main objective of the experiments is to confirm fission reactions of neptunium-237 ($$^{237}$$Np) and americium-241 ($$^{241}$$Am), and capture reactions of $$^{237}$$Np. Subcritical irradiation of $$^{237}$$Np and $$^{241}$$Am foils is conducted in a hard spectrum core with the use of the back-to-back fission chamber that obtains simultaneously two signals from specially installed test ($$^{237}$$Np or $$^{241}$$Am) and reference (uranium-235) foils. The first nuclear transmutation of $$^{237}$$Np and $$^{241}$$Am by ADS soundly implemented by combining the subcritical core and the 100 MeV proton accelerator, and the use of a lead-bismuth target, is conclusively demonstrated through the experimental results of fission and capture reaction events.

Journal Articles

Time-resolved imaging of magnetoelastic waves by the cotton-mouton effect

Hioki, Tomosato*; Hashimoto, Yusuke*; Johansen, T. H.*; Saito, Eiji

Physical Review Applied (Internet), 11(6), p.061007_1 - 061007_5, 2019/06

 Times Cited Count:7 Percentile:36.99(Physics, Applied)

Journal Articles

Measurement and estimation of the $$^{99}$$Mo production yield by $$^{100}$$Mo($$n,2n$$)$$^{99}$$Mo

Minato, Futoshi; Tsukada, Kazuaki; Sato, Nozomi*; Watanabe, Satoshi*; Saeki, Hideya*; Kawabata, Masako*; Hashimoto, Shintaro; Nagai, Yasuki*

Journal of the Physical Society of Japan, 86(11), p.114803_1 - 114803_6, 2017/11

 Times Cited Count:10 Percentile:56.7(Physics, Multidisciplinary)

We have measured the yield of $$^{99}$$Mo, the mother nuclide of $$^{99m}$$Tc used in nuclear diagnostic procedure. $$^{99}$$Mo was produced by $$^{100}$$Mo($$n$$,$$2n$$)$$^{99}$$Mo using neutrons with thermal energy up to about 40 MeV, provided by C($$d$$,$$n$$). The $$^{99}$$Mo yield agrees with an estimated yield with the use of the latest data of C($$d$$,$$n$$) and the evaluated cross section given in the JENDL. Based on this, a new calculation was carried out to produce $$^{99}$$Mo to seek for a good economical condition. Various conditions such as the $$^{100}$$MoO$$_{3}$$ sample mass, the distance between the carbon target and the sample, the radius of the deuteron beam, and the neutron irradiation time were considered. The calculated $$^{99}$$Mo yield indicates that about 30% of the $$^{99}$$Mo demand in Japan can be fulfilled with a single accelerator. The elusion of $$^{99m}$$Tc from the $$^{99}$$Mo twice per day would meet about 50% of the $$^{99}$$Mo demand.

Journal Articles

Hierarchically self-organized dissipative structures of filler particles in poly(styrene-$$ran$$-butadiene) rubbers

Yamaguchi, Daisuke; Yuasa, Takeshi*; Sone, Takuo*; Tominaga, Tetsuo*; Noda, Yohei*; Koizumi, Satoshi*; Hashimoto, Takeji*

Macromolecules, 50(19), p.7739 - 7759, 2017/10

 Times Cited Count:14 Percentile:48.33(Polymer Science)

We elucidated the spatial distribution of filler particles in cross-linked poly(styrene-$$ran$$-butadiene) rubbers (SBR) developed under a typical fillers/rubbers compounding process as one of dissipative structures formed under a stress field imposed on the given system. The dispersion state of the fillers in SBR was clarified on the basis of hierarchical structures consisting of five structure levels. More specifically, it has the following characteristics depending on the specific interactions: Small, compact clusters build up compact mass-fractal structures, while large, loose clusters build up open mass-fractal structures.

Journal Articles

Proposal for selective isotope transmutation of long-lived fission products using quasi-monochromatic $$gamma$$-ray beams

Hayakawa, Takehito; Miyamoto, Shuji*; Hajima, Ryoichi; Shizuma, Toshiyuki; Amano, So*; Hashimoto, Satoshi*; Misawa, Tsuyoshi*

Journal of Nuclear Science and Technology, 53(12), p.2064 - 2071, 2016/12

 Times Cited Count:6 Percentile:43.12(Nuclear Science & Technology)

We have proposed a new selective isotope transmutation method using photonuclear reactions with quasi-monochromatic $$gamma$$-ray beams. This method is based on the fact that the particle threshold of a long-lived fission product (LLFP) such as $$^{93}$$Zr, $$^{107}$$Pd, or $$^{79}$$Se is lower than those of stable isotopes of the same chemical element. Therefore, this method has an excellent advantage that LLFPs cannot, in principle, be produced newly even if the target materials include stable isotopes in addition to a LLFP. Laser Compton scattering $$gamma$$-ray sources and neutron capture $$gamma$$-rays in nuclear reactors are candidates for this method.

Journal Articles

Overview of the PHITS code and application to nuclear data; Radiation damage calculation for materials

Iwamoto, Yosuke; Sato, Tatsuhiko; Niita, Koji*; Hashimoto, Shintaro; Ogawa, Tatsuhiko; Furuta, Takuya; Abe, Shinichiro; Kai, Takeshi; Matsuda, Norihiro; Iwase, Hiroshi*; et al.

JAEA-Conf 2016-004, p.63 - 69, 2016/09

A general purpose Monte Carlo Particle and Heavy Ion Transport code System, PHITS, is being developed through the collaboration of several institutes. PHITS can deal with the transport of nearly all particles, including neutrons, protons, heavy ions, photons, and electrons, over wide energy ranges using various nuclear reaction models and data libraries. PHITS users apply the code to various research and development fields such as nuclear technology, accelerator design, medical physics, and cosmic-ray research. This presentation briefly summarizes the physics models implemented in PHITS, and introduces some new models such as muon-induced nuclear reaction model and a $$gamma$$ de-excitation model EBITEM. We will also present the radiation damage cross sections for materials, PKA spectra and kerma factors calculated by PHITS under the IAEA-CRP activity titled "Primary radiation damage cross section."

Journal Articles

Complete $$^{40}$$Ar resetting in an ultracataclasite by reactivation of a fossil seismogenic fault along the subducting plate interface in the Mugi M$'e$lange of the Shimanto accretionary complex, southwest Japan

Tonai, Satoshi*; Ito, Shun*; Hashimoto, Yoshitaka*; Tamura, Hajimu; Tomioka, Naotaka*

Journal of Structural Geology, 89, p.19 - 29, 2016/08

 Times Cited Count:16 Percentile:48.38(Geosciences, Multidisciplinary)

We used the K-Ar ages of clay-sized mineral grains to investigate the timing of activity on the fossil seismogenic Minami-Awa Fault. The K-Ar ages from matrix shale of the m$'e$lange range from 85 to 48 Ma and decrease with decreasing amount of detrital mica. In contrast, the K-Ar ages of an ultracataclasite within the fault core are significantly younger, ranging from 29 to 23 Ma, and are unrelated to grain size. This indicates that $$^{40}$$Ar diffused completely from the ultracataclasite between 29 and 23 Ma. The diffusion of $$^{40}$$Ar in the ultracataclasite was probably caused by frictional heating or high-temperature fluid migration that occurred when the fault was reactivated. The results indicate that seismogenic faults that separate tectonic m$'e$lange from coherent strata in accretionary complex may slip, not only during accretion, but also long after accretion.

Journal Articles

Development of numerical simulation system for thermal-hydraulic analysis in fuel assembly of sodium-cooled fast reactor

Ohshima, Hiroyuki; Uwaba, Tomoyuki; Hashimoto, Akihiko*; Imai, Yasutomo*; Ito, Masahiro*

AIP Conference Proceedings 1702, p.040011_1 - 040011_4, 2015/12

A numerical simulation system, which consists of a deformation analysis program and three kinds of thermal-hydraulics analysis programs, is being developed in Japan Atomic Energy Agency in order to offer methodologies to clarify thermal-hydraulic phenomena in fuel assemblies of sodium-cooled fast reactors under various operating conditions including fuel deformation. This paper gives a summary of numerical methods of component programs of the system and their validation studies.

Journal Articles

Overview of particle and heavy ion transport code system PHITS

Sato, Tatsuhiko; Niita, Koji*; Matsuda, Norihiro; Hashimoto, Shintaro; Iwamoto, Yosuke; Furuta, Takuya; Noda, Shusaku; Ogawa, Tatsuhiko; Iwase, Hiroshi*; Nakashima, Hiroshi; et al.

Annals of Nuclear Energy, 82, p.110 - 115, 2015/08

 Times Cited Count:35 Percentile:94.59(Nuclear Science & Technology)

The general purpose Monte Carlo Particle and Heavy Ion Transport code System, PHITS, is being developed through a collaboration of several institutes in Japan and Europe. The Japan Atomic Energy Agency is responsible for managing the entire project. PHITS can deal with the transport of nearly all particles, including neutrons, protons, heavy ions, photons, and electrons, over wide energy ranges using various nuclear reaction models and data libraries. This paper briefly summarizes the physics models implemented in PHITS, and introduces some important functions useful for particular purposes, such as an event generator mode and beam transport functions.

Journal Articles

Complexation of lutetium-177 with bifunctional chelators in the presence of Mg, Cu, and Yb

Watanabe, Satoshi; Hashimoto, Kazuyuki; Ishioka, Noriko

JAEA-Review 2014-050, JAEA Takasaki Annual Report 2013, P. 102, 2015/03

Journal Articles

Overview of particle and heavy ion transport code system PHITS

Iwamoto, Yosuke; Sato, Tatsuhiko; Niita, Koji*; Matsuda, Norihiro; Hashimoto, Shintaro; Furuta, Takuya; Noda, Shusaku; Ogawa, Tatsuhiko; Iwase, Hiroshi*; Nakashima, Hiroshi; et al.

JAEA-Conf 2014-002, p.69 - 74, 2015/02

A general purpose Monte Carlo Particle and Heavy Ion Transport code System, PHITS, is being developed through the collaboration of several institutes in Japan and Europe. PHITS can deal with the transport of nearly all particles, including neutrons, protons, heavy ions, photons, and electrons, over wide energy ranges using various nuclear reaction models and data libraries. All components of PHITS such as its source, executable and data-library files are assembled in one package and then distributed to many countries. More than 1,000 researchers apply the code to various research and development fields such as nuclear technology, accelerator design, medical physics, and cosmic-ray research. This presentation briefly summarizes the physics models implemented in PHITS, and introduces some important functions for specific applications, such as an event generator mode and a radiation damage calculation function.

Journal Articles

Lutetium-177 complexation of DOTA and DTPA in the presence of competing metals

Watanabe, Satoshi; Hashimoto, Kazuyuki; Ishioka, Noriko

Journal of Radioanalytical and Nuclear Chemistry, 303(2), p.1519 - 1521, 2015/02

 Times Cited Count:10 Percentile:64.26(Chemistry, Analytical)

As basic studies of bifunctional chelating agent for $$^{177}$$Lu-labeled antibodies, $$^{177}$$Lu complexation of DOTA and DTPA was investigated by the addition of competing metals, Ca(II), Fe(II) and Zn(II). From comparison of competing metals, the inhibition by competing metals on the $$^{177}$$Lu complexation was in the order of Ca(II) $$<$$ Fe(II) $$<$$ Zn(II) and Ca(II) $$<$$ Zn(II) $$<$$ Fe(II) as DOTA and DTPA, respectively. For comparison between DOTA and DTPA, the susceptibility to the inhibition on $$^{177}$$Lu complexation by all the three competing metals was DTPA $$<$$ DOTA. Therefore, it was found that DTPA is advantageous for $$^{177}$$Lu complexation compared with DOTA in the presence of Ca(II), Fe(II) and Zn(II), and that the elimination of Fe from $$^{177}$$Lu solution is especially effective because the $$^{177}$$Lu complexation of DTPA is highly inhibited by Fe(II).

Journal Articles

Improvement of photonuclear reaction model below 140 MeV in the PHITS code

Noda, Shusaku; Hashimoto, Shintaro; Sato, Tatsuhiko; Fukahori, Tokio; Chiba, Satoshi*; Niita, Koji*

Journal of Nuclear Science and Technology, 52(1), p.57 - 62, 2015/01

 Times Cited Count:14 Percentile:72.94(Nuclear Science & Technology)

The author improved the photonuclear reaction model in the PHITS code for incident photon energy below 140 MeV. There are three major improvements: (1) JENDL Photonuclear Data File (JENDL/PD-2004) is adopted to determine the total reaction cross section, (2) the evaporation model for the giant resonance of some light nuclei is modified considering the isospin selection rule, and (3) the quasideuteron disintegration process is implemented in the JAERI Quantum Molecular Dynamics model. The improved PHITS code can contribute to various practical applications such as neutron dose estimation in X-ray therapy.

Journal Articles

Production of highly purified no-carrier-added $$^{177}$$Lu for radioimmunotherapy

Watanabe, Satoshi; Hashimoto, Kazuyuki; Watanabe, Shigeki; Iida, Yasuhiko*; Hanaoka, Hirofumi*; Endo, Keigo*; Ishioka, Noriko

Journal of Radioanalytical and Nuclear Chemistry, 303(1), p.935 - 940, 2015/01

 Times Cited Count:11 Percentile:67.09(Chemistry, Analytical)

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