Interlaboratory comparison of electron paramagnetic resonance tooth enamel dosimetry with investigations of the dose responses of the standard samples

Toyoda, Shin*; Inoue, Kazuhiko*; Yamaguchi, Ichiro*; Hoshi, Masaharu*; Hirota, Seiko*; Oka, Toshitaka; Shimazaki, Tatsuya*; Mizuno, Hideyuki*; Tani, Atsushi*; Yasuda, Hiroshi*; et al.

Radiation Protection Dosimetry, 199(14), p.1557 - 1564, 2023/09

https://doi.org/10.1093/rpd/ncad150

Interlaboratory comparison studies are important for radiation dosimetry in order to demonstrate how the technique is universally available. The set of standard samples are examined in each participating laboratory in the present study. After a set of standard samples together with the samples with unknown doses, which were prepared in the same laboratory as the standard samples, are measured at a participating laboratory, those samples are sent to another participating laboratory for next measurement. There is some small difference observed in the sensitivity (the slope of the dose response line) of the standard samples while the differences in the obtained doses for the samples with unknown doses are rather systematic, implying that the difference is mostly due to the samples but not to measurements.

Long-term density-dependent groundwater flow analysis and its effect on nuclide migration for safety assessment of high-level radioactive waste disposal with consideration of interaction between fractures and matrix of rock formation in coastal crystalline groundwater systems

Park, Y.-J.*; Sawada, Atsushi; Ozutsumi, Takenori*; Tanaka, Tatsuya*; Hashimoto, Shuji*; Morita, Yutaka*

Proceedings of 3rd International Conference on Discrete Fracture Network Engineering (DFNE 2022) (Internet), 8 Pages, 2022/00

Safety analysis for underground disposal facilities for high-level radioactive waste requires thorough understanding of long-term groundwater flow and nuclide migration processes in geologic media. In the coastal subsurface systems, groundwater flow is defined by the complex interactions between freshwater of meteoric origin and denser saline water from the sea. In addition, sea levels are expected to fluctuate significantly due to a transgression and regression of the sea over the millions of years for safety analysis. This study presents long-term evolution of groundwater environment such as salinity concentration and flow velocity with focus of the interaction between fractures and matrix blocks in regional and near-field scale analysis framework for groundwater flow and nuclide migration for underground disposal facilities in hypothetical fractured crystalline coastal systems.

Study for development of the methodology for multi-scale hydrogeological modeling taking into account hydraulic heterogeneity caused by fracture network

Saegusa, Hiromitsu; Onoe, Hironori; Ishibashi, Masayuki; Tanaka, Tatsuya*; Abumi, Kensho*; Hashimoto, Shuji*; Bruines, P.*

JAEA-Research 2015-011, 59 Pages, 2015/10

JAEA-Research-2015-011.pdf:49.44MB

It is important to evaluate groundwater flow characteristics on several spatial scales for assessment of long-term safety on geological disposal of high-level radioactive wastes. An estimation of hydraulic heterogeneity caused by fracture network is significant for evaluation of the groundwater flow characteristics in the region of tens of meters square. Heterogeneity of equivalent hydraulic properties is needed to estimate for evaluation of the groundwater flow characteristics in the region of several km square. In order to develop the methodology for multi-scale hydrogeological modeling taking into account the hydraulic heterogeneity, spatial distribution of fractures and their hydraulic properties have been modeled using discrete fracture network (DFN) model. Then, hydrogeological continuum model taking into account the hydraulic heterogeneity has been estimated based on the DFN model. Through this study, the methodology for multi-scale hydrogeological modeling according to type of investigation data has been proposed.

Development of grouting technologies for HLW disposal in Japan, 4; Planning and results of in-situ grouting test

Tanaka, Tatsuya*; Uyama, Masao*; Ishida, Tomoko*; Nakanishi, Tatsuro; Onishi, Yuzo*

Proceedings of 7th Asian Rock Mechanics Symposium (ARMS-7) (USB Flash Drive), p.702 - 711, 2012/10

This paper describes the planning, material selection, execution and interpretation of the grout injection test carried out at the end of 2011 at the Grimsel Test Site (GTS) in Switzerland as part of grouting technology project of the Japan Atomic Energy Agency (JAEA). Based on the findings of the rockmass characterization part of the GTS grouting study (Nakanishi et al, 2012, Bruines et al., 2012), it was decided to perform the grout injection test in a 5 m interval with the highest expected hydraulic conductivity. During the grouting test the viscosity of the grout was continuously measured. Both the injected volume and pressure in the injection section were recorded. In the observation sections the pressure over time as well as the electric conductivity, which can be used to measure the arrival of the higher salinity silica grout, was recorded. As the grout reached the observation sections before the grout hardened the grout injection test was a success. The gathered data of the grouting test presents an important data set for further modeling efforts of the grouting process.

Development of grouting technologies for HLW disposal in Japan, 5; Development and application of numerical model for grout injection process during in-situ grouting test

Koyama, Tomofumi*; Katayama, Tatsuo*; Tanaka, Tatsuya*; Kuzuha, Yuji; Onishi, Yuzo*

Proceedings of 7th Asian Rock Mechanics Symposium (ARMS-7) (USB Flash Drive), p.712 - 720, 2012/10

Grouting is commonly used to decrease the hydraulic conductivity of the fractured rock masses and control the groundwater inflow. Since underground facilities were constructed in various geological conditions, different types of grout material and mixing/injection methods were developed for effective and economical grout injection. It is also important to evaluate the grout arrival distance and the range of altered hydraulic conductivity field after grout injection. However, the mechanism of grout injection process has not been clarified sufficiently yet due to complicated chemical and physical processes of grout. In this study, to simulate the grout injection process, the three-dimensional numerical model based on equivalent continuum approach was developed and applied to the in-situ grout injection tests at Grimsel test site, Switzerland. In the simulations, the injection pressure and/or injection rate was given as a boundary condition and total amount of injected grout (silica sol) was calculated. The simulation results were also compared with the ones obtained from in-situ measurements/monitoring and show qualitatively good agreement.

Morphology-controlled synthesis of Mo compounds from a nitric acid solution by the microwave heating and/or Zr-addition

Osaka, Masahiko; Tanaka, Kosuke; Sekine, Shinichi; Akutsu, Yoko; Suzuki, Tatsuya*; Mimura, Hitoshi*

Journal of Nuclear Materials, 427(1-3), p.384 - 388, 2012/08

https://doi.org/10.1016/j.jnucmat.2012.05.022

Morphology-controlled synthesis of Mo compounds from a nitric acid solution by microwave heating was investigated for effective utilizations of Mo fission product from a high level nuclear waste. The microwave heating method was revealed to greatly accelerate crystallization and crystal growth of the synthesized powder. Addition of a small amount of Zr stabilized synthesis of a hexagonal-MoO powder. Furthermore, the microwave heating with Zr-addition has synthesized a specific urchin-like shaped hexagonal-MoO crystal having a good crystallinity. The present methods would be useful for effective utilization of Mo from high level nuclear waste in terms of their practicability and ability to the morphology control.

The JAEA grouting test at the Grimsel test site; Site characterization of a fractured rockmass and preparation of DFN model and its equivalent continuous porous media model

Bruines, P.*; Tanaka, Tatsuya*; Koyama, Tomofumi*; Kishi, Hirokazu; Nakanishi, Tatsuro; Onishi, Yuzo*

Proceedings of 2012 ISRM International Symposium; Rock Engineering and Technology for Sustainable Underground Construction (EUROCK 2012) (USB Flash Drive), 15 Pages, 2012/05

To better understand the grouting process and the effect of grouting on the performance of a nuclear waste repository, the Japanese Atomic Energy Agency (JAEA) has initiated a grouting test carried out in the fractured granite of the Grimsel Test Site (GTS) located in the Swiss Alps. This paper describes the characterization of the rock mass, how the data obtained has been used to make a discrete fracture network (DFN) model and how an up-scaled equivalent continuous porous media (ECPM) model for the purpose of numerical simulation of the grout injection process is generated. The generated DFN model and the up-scaled ECPM model was able to reproduce the measured fracture characteristics (e.g. orientation, density) as well as the hydraulic behavior observed in the field (e.g. transmissivity distribution, anisotropy, heterogeneity) and has proven to be suitable for modeling grouting behavior.

Development of grouting technologies for geological disposal of high level waste in Japan, 1; Preliminary study for in-situ grout injection test in crystalline rock mass test site

Nakanishi, Tatsuro; Fujita, Tomoo; Tsuda, Hidenori; Tanaka, Tatsuya*; Uyama, Masao*; Onishi, Yuzo*

Dai-41-Kai Gamban Rikigaku Ni Kansuru Shimpojiumu Koenshu (CD-ROM), p.71 - 76, 2012/01

Grouting technology is fundamental to the safe and efficient construction of underground facilities for the geological disposal of high level waste in Japan. The Japan Atomic Energy Agency has been developing grouting materials and technologies with consideration to the long term chemical interactions between the grout material and the natural barrier rock mass. An in-situ grout injection test has been carried out at the Grimsel Test Site to optimize grouting design.

Development of grouting technologies for geological disposal of high level waste in Japan, 2; Hydrogeological descriptive modeling by discrete fracture network in crystalline rock mass test site

Tanaka, Tatsuya*; Bruines, P.*; Abumi, Kensho*; Hashimoto, Shuji*; Kuzuha, Yuji; Onishi, Yuzo*

Dai-41-Kai Gamban Rikigaku Ni Kansuru Shimpojiumu Koenshu (CD-ROM), p.77 - 82, 2012/01

This study aims to establish grouting techniques and evaluation of the effects of grouting in the geological environment of crystalline rock. A hydrogeological model has been generated using discrete fracture networks based on the data obtained by the short-borehole investigation campaign performed at at Grimsel test site in Switzerland to support the design of planned in-situ grouting test. The equivalent porous media with the consideration of hydraulic heterogeneity has been created from the DFN (Discrete Fracture Network) in order to be provided for the simulation of the grout injection process. Uncertainties and remaining issues associated with the assumption in interpreting the data and its modeling were addressed in a systematic way.

Reformation of hazardous wastes into useful supporting materials for fast reactor fuels

Osaka, Masahiko; Miwa, Shuhei; Tanaka, Kosuke; Akutsu, Yoko; Ikeda, Kaoru*; Mimura, Hitoshi*; Suzuki, Tatsuya*; Usuki, Toshiyuki; Yano, Toyohiko*

Annals of Nuclear Energy, 38(12), p.2661 - 2666, 2011/10

https://doi.org/10.1016/j.anucene.2011.07.030

Novel concepts for effective utilization of molybdenum (Mo) from nuclear waste and magnesium silicates from hazardous asbestos wastes are proposed. A fast reactor cycle scheme that incorporates each material is described in the present paper. Basic studies on some fundamental technologies for the present cycle are given. Basic separation aspects for Mo by using LIX63 micro capsules and tertiary pyridine resin were investigated. A simple chemical synthesis route for Mo precursor powder from Mo containing HNO solution was tested. Effects of impurities in recovered Mo on sintering behavior were experimentally investigated.