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Teshigawara, Makoto; Ikeda, Yujiro*; Yan, M.*; Muramatsu, Kazuo*; Sutani, Koichi*; Fukuzumi, Masafumi*; Noda, Yohei*; Koizumi, Satoshi*; Saruta, Koichi; Otake, Yoshie*
Nanomaterials (Internet), 13(1), p.76_1 - 76_9, 2023/01
Times Cited Count:2 Percentile:54.89(Chemistry, Multidisciplinary)To enhance neutron intensity below cold neutrons, it is proposed that nanosized graphene aggregation could facilitate neutron coherent scattering under particle size conditions similar to nanodiamond. It might also be possible to use it in high neutron radiation conditions due to graphene's strong sp2 bonds. Using the RIKEN accelerator-driven compact neutron source and iMATERIA at J-PARC, we performed neutron measurement experiments, total neutron cross-section, and small-angle neutron scattering on nanosized graphene aggregation. The measured data revealed, for the first time, that nanosized graphene aggregation increased the total cross-sections and small-angle scattering in the cold neutron energy region, most likely due to coherent scattering, resulting in higher neutron intensities, similar to nanodiamond.
Harada, Masahide; Teshigawara, Makoto; Oi, Motoki; Oikawa, Kenichi; Takada, Hiroshi; Ikeda, Yujiro
Nuclear Instruments and Methods in Physics Research A, 1000, p.165252_1 - 165252_8, 2021/06
Times Cited Count:2 Percentile:34.88(Instruments & Instrumentation)This study explores high-energy neutron components of the extracted neutron beam at J-PARC pulsed neutron source using the foil activation method with threshold reactions. Foils of aluminum, gold, bismuth, niobium, and thulium were used to cover the neutron energy range from 0.3 MeV to 79.4 MeV. The experiment was performed using neutron beams of BL10 (NOBORU). The foils were irradiated by a neutron beam at 13.4 m from the moderator. To characterize high-energy neutron fields for irradiation applications, reaction rates in three different configurations with and without BC slit and Pb filter were examined. To compare the experiments with calculations given for the user, reaction rates for corresponding reactions were calculated by the PHITS code with the JENDL-3.2 and the JENDL dosimetry file. Although there was a systematic tendency in C/E (Calculation/Experiment) ratios for different threshold energies, which C/E ratio decreased as threshold energy increased up to 100 MeV, and all C/E ratios were in the range of 1.00.2. This indicated that high-energy neutron calculations were adequate for the analysis of experimental data for NOBORU users.
Matsumoto, Takahiro*; Sugimoto, Hidehiko*; Ohara, Takashi; Tokumitsu, Akio*; Tomita, Makoto*; Ikeda, Susumu*
Physical Review B, 103(24), p.245401_1 - 245401_9, 2021/06
Times Cited Count:0 Percentile:0(Materials Science, Multidisciplinary)Ma, B.*; Teshigawara, Makoto; Wakabayashi, Yasuo*; Yan, M.*; Hashiguchi, Takao*; Yamagata, Yutaka*; Wang, S.*; Ikeda, Yujiro*; Otake, Yoshie*
Nuclear Instruments and Methods in Physics Research A, 995, p.165079_1 - 165079_7, 2021/04
Times Cited Count:2 Percentile:34.88(Instruments & Instrumentation)We have optimized a cold neutron moderator to be operated at the RIKEN accelerator-driven compact neutron source. We selected a safe and easy to manage material, mesitylene, as the RANS cold moderator. An efficient moderator system was designed by studying and optimizing a coupled cold neutron moderator of mesitylene at 20 K with a polyethylene (PE) pre-moderator at room temperature in the slab geometry with Particle and Heavy Ion Transport code System (PHITS) simulations. The parameters of mesitylene and PE thickness, the reflector, and the shielding configuration were studied to increase cold neutron intensities. Consequently, an integrated cold neutron intensity of 1.1510n/cm/A at 2 m from the neutron-producing target was finally achieved, which was 12 times higher than that of the current PE moderator. The results showed attractive application prospect of mesitylene as cold neutron moderator material.
Kitazato, Kohei*; Milliken, R. E.*; Iwata, Takahiro*; Abe, Masanao*; Otake, Makiko*; Matsuura, Shuji*; Takagi, Yasuhiko*; Nakamura, Tomoki*; Hiroi, Takahiro*; Matsuoka, Moe*; et al.
Nature Astronomy (Internet), 5(3), p.246 - 250, 2021/03
Times Cited Count:43 Percentile:96.93(Astronomy & Astrophysics)Here we report observations of Ryugu's subsurface material by the Near-Infrared Spectrometer (NIRS3) on the Hayabusa2 spacecraft. Reflectance spectra of excavated material exhibit a hydroxyl (OH) absorption feature that is slightly stronger and peak-shifted compared with that observed for the surface, indicating that space weathering and/or radiative heating have caused subtle spectral changes in the uppermost surface. However, the strength and shape of the OH feature still suggests that the subsurface material experienced heating above 300 C, similar to the surface. In contrast, thermophysical modeling indicates that radiative heating does not increase the temperature above 200 C at the estimated excavation depth of 1 m, even if the semimajor axis is reduced to 0.344 au. This supports the hypothesis that primary thermal alteration occurred due to radiogenic and/or impact heating on Ryugu's parent body.
Oi, Motoki; Teshigawara, Makoto; Harada, Masahide; Ikeda, Yujiro
Journal of Nuclear Science and Technology, 56(7), p.573 - 579, 2019/07
Times Cited Count:0 Percentile:0.01(Nuclear Science & Technology)In pulsed neutron sources, a neutron absorber called decoupler is attached to the moderator to sharpen the neutron pulses for achieving good neutron energy resolutions. Cadmium and boron carbide (BC) are widely used as the decoupler materials. However, it is difficult to use BC in MW-class spallation neutron sources owing to high burn-up, which decreases cut-off energy and increase of helium gas swelling. To solve these issues, we introduce the concept of pre-decoupler to reduce neutron absorption in the BC decoupler, which is sandwiched by appropriate neutron absorption materials. Then, we study impacts of the pre-decouplers on BC decoupler in terms of burn-up by performing simplified model calculations. It is shown that neutron absorption in BC is reduced by 60% by using a Cd pre-decoupler without neutron intensity penalty. Moreover, helium gas swelling in BC is restrained to be one-third of the value when not using the pre-decoupler.
Teshigawara, Makoto; Tsuchikawa, Yusuke*; Ichikawa, Go*; Takata, Shinichi; Mishima, Kenji*; Harada, Masahide; Oi, Motoki; Kawamura, Yukihiko*; Kai, Tetsuya; Kawamura, Seiko; et al.
Nuclear Instruments and Methods in Physics Research A, 929, p.113 - 120, 2019/06
Times Cited Count:16 Percentile:86.05(Instruments & Instrumentation)A nano-diamond is an attractive neutron reflection material below cold neutron energy. The total neutron cross section of a nano-diamond was derived from a neutron transmission measurement over the neutron energy range of 0.2 meV to 100 meV because total neutron cross section data were not available. The total cross section of a nano-diamond with particle size of approximately 5 nm increased with a decrease in neutron energy to 0.2 meV. It was approximately two orders of magnitude larger than that of graphite at 0.2 meV. The contribution of inelastic scattering to the total cross section was to be shown negligible small at neutron energies of 1.2, 1.5, 1.9, 2.6, and 5.9 meV in the inelastic neutron scattering measurement. Moreover, small-angle neutron scattering measurements of the nano-diamond showed a large scattering cross section in the forward direction for low neutron energies.
Harada, Masahide; Teshigawara, Makoto; Oi, Motoki; Klinkby, E.*; Zanini, L.*; Batkov, K.*; Oikawa, Kenichi; Toh, Yosuke; Kimura, Atsushi; Ikeda, Yujiro
Nuclear Instruments and Methods in Physics Research A, 903, p.38 - 45, 2018/09
Times Cited Count:10 Percentile:67.52(Instruments & Instrumentation)Mikake, Shinichiro; Ikeda, Koki; Matsui, Hiroya; Tsuji, Masakuni*; Nishigaki, Makoto*
Doboku Gakkai Rombunshu, C (Chiken Kogaku) (Internet), 74(1), p.76 - 91, 2018/03
Pre-grouting of shafts and galleries had been conducted during the construction of MIU in the aspect of reducing water inflow. After excavating GL.-500m gallery, a post-grouting was performed on section of the pre-excavation grouting area under high water pressure condition (max: 4MPa). The post-grouting experiment was performed outside of the pre-grouting zone with designs, applying colloidal silica grouting material and complex dynamic grouting. It was estimated that the inflow after post-grouting was reduced by 1/100 of the case that pre- and post-grouting were not performed. These results indicate that the applied combined pre- and post-grouting methodology is effective in reducing water inflow and it can be applicable under high water pressure condition. Then, this paper states the theoretical evaluation of relationship between reduction of hydraulic conductivity and the grouting zone is very convenient and useful for grouting design and estimate of water inflow.
Teshigawara, Makoto; Ikeda, Yujiro; Oi, Motoki; Harada, Masahide; Takada, Hiroshi; Kakishiro, Masanori*; Noguchi, Gaku*; Shimada, Tsubasa*; Seita, Kyoichi*; Murashima, Daisuke*; et al.
Nuclear Materials and Energy (Internet), 14, p.14 - 21, 2018/01
Times Cited Count:0 Percentile:0.01(Nuclear Science & Technology)We developed an Au-In-Cd (AuIC) decoupler material to reduce induced radioactivity instead of Ag-In-Cd one, which has a cut off energy of 1eV. In order to implement it into an actual moderator-reflector assembly, a number of critical engineering issues need to be resolved with regard to large-sized bonding between AuIC and A5083 alloys by the hot isostatic pressing process. We investigated this process in terms of the surface conditions, sizes, and heat capacities of large AuIC alloys. We also show a successful implementation of an AuIC decoupler into a reflector assembly, resulting in a remarkable reduction of radioactivity by AuIC compared to AIC without sacrificing neutronic performance.
Aso, Tomokazu; Teshigawara, Makoto; Hasegawa, Shoichi; Aoyagi, Katsuhiro*; Muto, Hideki*; Nomura, Kazutaka*; Takada, Hiroshi; Ikeda, Yujiro
JAEA-Technology 2017-021, 75 Pages, 2017/08
Liquid hydrogen is employed as a cold neutron moderator material at the spallation neutron source of Materials and Life science experimental Facility of Japan Proton Accelerator Research Complex (J-PARC). From January 2015, it became observable that the differential pressure between heat exchangers and an 80 K adsorber (ADS) in a helium refrigerator system increased with operating time. In November 2015, the differential pressure rise became more significant, leading to degrade the refrigerating performance in cooling liquid hydrogen. In order to investigate the cause of the abnormal differential pressure rise between the heat exchangers and the ADS, we carried out visual inspection inside the heat exchangers and analyzed the impurities contained in the helium gas. Unfortunately, we could not identify the impurities causing the performance degradation, but observed a trace of oil in the inlet piping of the heat exchanger. Based on investigations of the abnormal events occurred in the refrigerators with similar refrigerating capacity at other facilities, we took measures that cleaning the heat exchangers with Freon and replacing the ADS with new one. As a result, the differential pressure rise phenomenon was removed to recover the performance. We have detected oil from the Freon used for cleaning the heat exchangers and at a felt supporting charcoal packed in the ADS. In particular, oil was accumulated in membranous form onto the felt at the entrance side in the ADS. The amount of oil contained in the helium gas was about 10 ppb or so, less than the design value, in the helium refrigerator. However, the oil accumulated onto the felt in the ADS through long operating period may cause abnormal differential pressure rise, leading to the performance degradation of the helium refrigerator. Further study is needed to specify the cause more clearly.
Ohgama, Kazuya; Ikeda, Kazumi*; Ishikawa, Makoto; Kan, Taro*; Maruyama, Shuhei; Yokoyama, Kenji; Sugino, Kazuteru; Nagaya, Yasunobu; Oki, Shigeo
Proceedings of 2017 International Congress on Advances in Nuclear Power Plants (ICAPP 2017) (CD-ROM), 10 Pages, 2017/04
Yamauchi, Kunihito; Okano, Jun; Shimada, Katsuhiro; Omori, Yoshikazu; Terakado, Tsunehisa; Matsukawa, Makoto; Koide, Yoshihiko; Kobayashi, Kazuhiro; Ikeda, Yoshitaka; Fukumoto, Masahiro; et al.
JAEA-Technology 2015-053, 36 Pages, 2016/03
The superconducting Satellite Tokamak machine "JT-60SA" under construction in Naka Fusion Institute is an international collaborative project between Japan (JA) and Europe (EU). The contributions for this project are based on the supply of components, and thus European manufacturer shall conduct the installation, commissioning and tests on Naka site. This means that Japan Atomic Energy Agency (JAEA) had a quite difficult issue to manage the works by European workers and their safety although there is no direct contract. This report describes the approaches for the work and safety managements, which were agreed with EU after the tough negotiation, and then the completed on-site works for Quench Protection Circuits (QPC) as the first experience for EU in JT-60SA project. With the help of these approaches by JAEA, the EU works for QPC were successfully completed with no accident, and a great achievement was made for both EU and JA.
Yoshida, Masahiro*; Ishii, Kenji; Naka, Makoto*; Ishihara, Sumio*; Jarrige, I.*; Ikeuchi, Kazuhiko*; Murakami, Yoichi*; Kudo, Kazutaka*; Koike, Yoji*; Nagata, Tomoko*; et al.
Scientific Reports (Internet), 6, p.23611_1 - 23611_8, 2016/03
Times Cited Count:1 Percentile:11.46(Multidisciplinary Sciences)Niwa, Hideharu*; Saito, Makoto*; Kobayashi, Masaki*; Harada, Yoshihisa*; Oshima, Masaharu*; Moriya, Shogo*; Matsubayashi, Katsuyuki*; Nabae, Yuta*; Kuroki, Shigeki*; Ikeda, Takashi; et al.
Journal of Power Sources, 223, p.30 - 35, 2013/02
Times Cited Count:18 Percentile:50.94(Chemistry, Physical)To design non-platinum, inexpensive, but high performance carbon-based cathode catalysts for polymer electrolyte fuel cells, it is important to elucidate the active site for oxygen reduction reaction (ORR). However, it is difficult to directly identify the active site by applying conventional structural or electronic probes to such complex systems. Here, we used C 1 X-ray absorption spectroscopy (XAS) to observe electronic structure of carbon in iron phthalocyanine-based catalysts, and found a signature of edge exposure below the edge, whose intensity is well correlated with the ORR activity. These results demonstrate that C 1 XAS can be used to characterize the ORR activity of carbon-based cathode catalysts in terms of the edge exposure.
Kobayashi, Masaki*; Niwa, Hideharu*; Saito, Makoto*; Harada, Yoshihisa*; Oshima, Masaharu*; Ofuchi, Hironori*; Terakura, Kiyoyuki*; Ikeda, Takashi; Koshigoe, Yuka*; Ozaki, Junichi*; et al.
Electrochimica Acta, 74, p.254 - 259, 2012/07
Times Cited Count:52 Percentile:80.98(Electrochemistry)The electronic structure of the residual metal atoms in FePc-based carbon catalysts, prepared by pyrolyzing a mixture of FePc and phenolic resin polymer at 800C, before and after acid washing have been investigated using XAFS spectroscopy to clarify the role of Fe in the ORR activity. The decomposition analyses for the XAFS spectra reveal that the composition ratio of each Fe component is unaltered by the acid washing, indicating that the residual Fe components were removed by the acid washing irrespective of their chemical states. Because the oxygen reduction potential was approximately unchanged by the acid washing, the residual Fe itself does not seem to contribute directly to the ORR activity. The residual Fe can act as a catalyst to accelerate the growth of the sp carbon network during pyrolysis. The results imply that light elements are components of the ORR active sites in the FePc-based carbon catalysts.
Sasaki, Takuo*; Suzuki, Hidetoshi*; Inagaki, Makoto*; Ikeda, Kazuma*; Shimomura, Kenichi*; Takahashi, Masamitsu; Kozu, Miwa*; Hu, W.; Kamiya, Itaru*; Oshita, Yoshio*; et al.
IEEE Journal of Photovoltaics, 2(1), p.35 - 40, 2012/01
Times Cited Count:5 Percentile:22.57(Energy & Fuels)Kubo, Makoto*; Mikake, Shinichiro; Ikeda, Koki; Yamamoto, Masaru
Kisoko, 39(9), p.82 - 85, 2011/09
Japan Atomic Energy Agency (JAEA)'s task is to provide the scientific and technical basis for safe geological disposal of high-level radioactive waste. This involves researches on development and improvement of techniques for characterization of the deep geological environment and a wide range of engineering for deep underground application in crystalline rock at "Mizunami Underground Research Laboratory". This report describes the summary of construction.
Takeuchi, Ryuji; Kosaka, Hiroshi; Sato, Atsuya*; Tomiyama, Shingo*; Kageyama, Soichiro*; Ikeda, Makoto*
JAEA-Research 2011-008, 77 Pages, 2011/06
Subsurface water balance observation is a kind of methods in order to estimate a recharge rate. Results of the observation are affected by the various factors such as the scale, the topography, a geological feature, the climate. Therefore, the observation in the regional scale is necessary at many basins. The purpose of this study is to confirm the applicability of the method for the evaluation of runoff volume, which is one of parameters to evaluate the recharge rate by surface water balance observation, by geomorphometry and statistical analyses using digital elevation model (DEM). The runoff index which is the original indicator to evaluate the degree of flow rate on a catchment was calculated by the comparison between the result of geomorphometry and statistics analyses, and the observed data of river flow rate in the monitoring stations. Using this index, the flow rate of the Hiyoshi River was evaluated. The evaluated flow rate was about 60% against the observed flow rate.
Ikeda, Makoto; Munakata, Masahiro; Sakai, Ryutaro; Kimura, Hideo; Jia, H.*; Matsuba, Hisashi*
Nihon Chikasui Gakkai 2011-Nen Shunki Koenkai Koen Yoshi, p.86 - 91, 2011/05
no abstracts in English