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Journal Articles

High-temperature creep properties of 9Cr-ODS tempered martensitic steel and quantitative correlation with its nanometer-scale structure

Otsuka, Satoshi; Shizukawa, Yuta; Tanno, Takashi; Imagawa, Yuya; Hashidate, Ryuta; Yano, Yasuhide; Onizawa, Takashi; Kaito, Takeji; Onuma, Masato*; Mitsuhara, Masatoshi*; et al.

Journal of Nuclear Science and Technology, 60(3), p.288 - 298, 2023/03

 Times Cited Count:4 Percentile:76.47(Nuclear Science & Technology)

JAEA has been developing 9Cr-oxide dispersion strengthened (ODS) tempered martensitic steel(TMS) as a candidate material for the fuel cladding tubes of sodium-cooled fast reactors(SFRs). The reliable prediction of in-reactor creep-rupture strength is critical for implementing the 9Cr-ODS TMS cladding tube in the SFR. This study investigated the quantitative correlation between the creep properties of 9Cr-ODS TMS at 700 $$^{circ}$$C and the dispersions of nanosized oxides by analyzing the creep data and the material's nanostructure. The possibility of deriving a formula for estimating the in-reactor creep properties of 9Cr-ODS TMSs based on an analysis of the nanostructure of neutron-irradiated 9Cr-ODS TMSs was also discussed. The creep properties of 9Cr-ODS TMS at 700 $$^{circ}$$C closely correlated with the dispersion of nanosized oxide particles. The correlation between creep-rupture lives and nanosized oxide particle dispersion was determined using existing creep models. The elucidation of correlation between the stress exponent of secondary creep rate and the nanostructure is essential to enhance future modeling reliability and formulation.

Journal Articles

Micropores and mass transfer in the formation of myrmekites

Yuguchi, Takashi*; Yuasa, Haruka*; Izumino, Yuya*; Nakashima, Kazuo*; Sasao, Eiji; Nishiyama, Tadao*

American Mineralogist, 107(3), p.476 - 488, 2022/03

 Times Cited Count:2 Percentile:20.65(Geochemistry & Geophysics)

The methodology and interpretations in this study provide new insights into the mechanism of myrmekite formation in a granitic system. The presence of micropores in the myrmekites and this study clarified that the genesis of micropores is related to the formation of myrmekites in the Toki granite. The results led to an increased understanding of (1) an estimate of mass transfer between the reactant and product minerals, and the inflow and outflow of components with consideration of the volume change due to micropore formation, (2) the factor controlling the formation of micropores during myrmekitization, and (3) the sequential variations in the hydrothermal fluid chemistry during sub-solidus conditions. The micropores act as a migration pathway for hydrothermal fluid and thus enhance the mass transfer within a granitic body starting with the myrmekite formation and continuing through the present day and into the future.

Journal Articles

Critical slowing-down and field-dependent paramagnetic fluctuations in the skyrmion host EuPtSi; $$mu$$SR and NMR studies

Higa, Nonoka*; Ito, Takashi; Yogi, Mamoru*; Hattori, Taisuke; Sakai, Hironori; Kambe, Shinsaku; Guguchia, Z.*; Higemoto, Wataru; Nakashima, Miho*; Homma, Yoshiya*; et al.

Physical Review B, 104(4), p.045145_1 - 045145_7, 2021/07

 Times Cited Count:0 Percentile:0(Materials Science, Multidisciplinary)

Journal Articles

Study on oxidation model for Zircalloy-2 cladding in SFP accident condition

Nemoto, Yoshiyuki; Kaji, Yoshiyuki; Onizawa, Takashi*; Kanazawa, Toru*; Nakashima, Kazuo*; Tojo, Masayuki*

Proceedings of Annual Congress of the European Federation of Corrosion (EUROCORR 2018) (USB Flash Drive), 8 Pages, 2018/09

The authors proposed oxidation models based on oxidation data which previously obtained in high temperature oxidation tests on small sample of Zircalloy-2 (Zry2) cladding in dry air and in air/steam mixture environment. The oxidation models were implemented in computational fluid dynamics (CFD) code to analyse oxidation behavior of long cladding sample in hypothetical spent fuel pool (SFP) accident conditions. The oxidation tests were conducted using Zry2 cladding sample 500 mm in length. The oxide layer growth in dry air was well reproduced in the calculation using the oxidation model, meanwhile which in air/steam mixture was overestimated atmosphere composition change anticipated in the spent fuel rack during the accident, and its influence on the oxidation behaviour of the cladding were discussed in consideration of the oxidation model improvement.

Journal Articles

Characterization of the PTW 34031 ionization chamber (PMI) at RCNP with high energy neutrons ranging from 100 - 392 MeV

Theis, C.*; Carbonez, P.*; Feldbaumer, E.*; Forkel-Wirth, D.*; Jaegerhofer, L.*; Pangallo, M.*; Perrin, D.*; Urscheler, C.*; Roesler, S.*; Vincke, H.*; et al.

EPJ Web of Conferences, 153, p.08018_1 - 08018_5, 2017/09

 Times Cited Count:0 Percentile:0.03(Nuclear Science & Technology)

At CERN, gas-filled ionization chambers PTW-34031 (PMI) are commonly used in radiation fields including neutrons, protons and $$gamma$$-rays. A response function for each particle is calculated by the radiation transport code FLUKA. To validate a response function to high energy neutrons, benchmark experiments with quasi mono-energetic neutrons have been carried out at RCNP, Osaka University. For neutron irradiation with energies below 200 MeV, very good agreement was found comparing the FLUKA simulations and the measurements. In addition it was found that at proton energies of 250 and 392 MeV, results calculated with neutron sources underestimate the experimental data due to a non-negligible gamma component originating from the target $$^{7}$$Li(p,n)Be reaction.

Journal Articles

Gamma radiation resistance of spin Seebeck devices

Yagmur, A.*; Uchida, Kenichi*; Ihara, Kazuki*; Ioka, Ikuo; Kikkawa, Takashi*; Ono, Madoka*; Endo, Junichi*; Kashiwagi, Kimiaki*; Nakashima, Tetsuya*; Kirihara, Akihiro*; et al.

Applied Physics Letters, 109(24), p.243902_1 - 243902_4, 2016/12

 Times Cited Count:3 Percentile:14.8(Physics, Applied)

Thermoelectric devices based on the spin Seebeck effect (SSE) were irradiated with gamma ($$gamma$$) rays with the total dose of around 3$$times$$10$$^{5}$$ Gy in order to investigate the $$gamma$$-radiation resistance of the devices. To demonstrate this, Pt/Ni$$_{0.2}$$Zn$$_{0.3}$$Fe$$_{2.5}$$O$$_{4}$$/Glass and Pt/Bi$$_{0.1}$$Y$$_{2.9}$$Fe$$_{5}$$O$$_{12}$$/Gd$$_{3}$$Ga$$_{5}$$O$$_{12}$$ SSE devices were used. We confirmed that the thermoelectric, magnetic, and structural properties of the SSE devices are not affected by the $$gamma$$-ray irradiation. This result demonstrates that SSE devices are applicable to thermoelectric generation even in high radiation environments.

JAEA Reports

Current status of a decommissioning project in the Enrichment Engineering Facilities; Results in the first-half of the fiscal year of 2014

Matsumoto, Takashi; Morimoto, Yasuyuki; Takahashi, Nobuo; Takata, Masaharu; Yoshida, Hideaki; Nakashima, Shinichi; Ishimori, Yuu

JAEA-Technology 2015-036, 60 Pages, 2016/01

JAEA-Technology-2015-036.pdf:9.15MB

The Enrichment Engineering Facilities of the Ningyo-toge Environmental Engineering Center was constructed in order to establish the technical basis of the uranium enrichment plant in Japan. Uranium enrichment tests, using natural and reprocessed uranium, were carried out from 1979 to 1990 at two types of plants in the facilities. UF$$_{6}$$ handling equipment and Supplemental equipment in these plants are intended to be dismantled by 2019 in order to make places for future projects, for example, inventory investigation, precipitation treatment, etc. This report shows the basic plan of this decommissioning project and presents the current state of dismantling in the first-half of the fiscal year of 2014, with indicating its schedule, procedure, situation, results, and so on. The dismantled materials generated amounted to 37 mesh containers and 199 drums, and the secondary waste generated amounted to 271.4 kg.

JAEA Reports

Laboratory testing of rock core samples from pre-excavation grouting area at Mizunami Underground Research Laboratory

Uyama, Masao*; Hitomi, Takashi*; Nakashima, Satoru*; Sato, Toshinori; Sanada, Hiroyuki; Aoyagi, Yoshiaki

JAEA-Research 2015-010, 67 Pages, 2015/10

JAEA-Research-2015-010.pdf:32.34MB
JAEA-Research-2015-010-appendix(CD-ROM).zip:528.25MB

Japan Atomic Energy Agency has been conducting a research project on (Grouting Technology Development for the Radioactive Waste Repository) funded by Ministry of Economy, Trade and Industry (METI), Japan. As a part of the project, various investigations were carried out in the -200m Refuge Niche where pre-excavation grouting was performed and the distribution of the injected grouting material, also the effectiveness of grouting penetration for reduction of groundwater inflow were confirmed As the continuation of these investigations, chemical influences of grouting material on the rock mass were determined through (Laboratory testing of rock core samples from pre-excavation grouting area at Mizunami Underground Research Laboratory). Specifically, core samples were obtained by check boring at where infiltration solidification of the grouting material was expected, and X-ray florescent analysis and Transmission Electron Microscope observation were performed focused on the contact parts of the grouting material and rock mass in fractures. As a result, the chemical influences of grouting material on the rock mass were identified.

Journal Articles

Activation, Radiation shielding materials

Sukegawa, Atsuhiko; Iida, Hiromasa*; Itoga, Toshio*; Okumura, Keisuke; Kai, Tetsuya; Konno, Chikara; Nakashima, Hiroshi; Nakamura, Takashi*; Ban, Shuichi*; Yashima, Hiroshi*; et al.

Hoshasen Shahei Handobukku; Kisohen, p.299 - 356, 2015/03

no abstracts in English

Journal Articles

Measurement of neutron energy spectra behind shields for quasi-monoenergetic neutrons generated by 246-MeV and 389-MeV protons using a Bonner sphere spectrometer

Matsumoto, Tetsuro*; Masuda, Akihiko*; Nishiyama, Jun*; Harano, Hideki*; Iwase, Hiroshi*; Iwamoto, Yosuke; Hagiwara, Masayuki*; Satoh, Daiki; Yashima, Hiroshi*; Nakane, Yoshihiro; et al.

Progress in Nuclear Science and Technology (Internet), 4, p.332 - 336, 2014/04

Recently, many high-energy accelerators are used for various fields. Shielding data for high-energy neutrons are therefore very important from the point of view of radiation protection in high energy accelerator facilities. However, the shielding experimental data for high energy neutrons above 100 MeV are very poor both in quality and in quantity. In this study, neutron penetration spectral fluence and ambient dose through iron and concrete shields were measured with a Bonner sphere spectrometer (BSS). Quasi-monoenergetic neutrons were produced by the $$^{7}$$Li(p,xn) reaction by bombarding a 1-cm thick Li target with 246-MeV and 389-MeV protons in the Research Center for Nuclear Physics (RCNP) of the Osaka University. Shielding materials are iron blocks with a thickness from 10 cm to 100 cm and concrete blocks with a thickness from 25 cm to 300 cm.

Journal Articles

Shielding benchmark experiment using hundreds of MeV quasi-monoenergetic neutron source by a large organic scintillator

Hagiwara, Masayuki*; Iwase, Hiroshi*; Iwamoto, Yosuke; Satoh, Daiki; Matsumoto, Tetsuro*; Masuda, Akihiko*; Yashima, Hiroshi*; Nakane, Yoshihiro; Nakashima, Hiroshi; Sakamoto, Yukio; et al.

Progress in Nuclear Science and Technology (Internet), 4, p.327 - 331, 2014/04

We have developed several hundreds of MeV p-$$^{7}$$Li quasi-monoenergetic neutron fields in the Research Center for Nuclear Physics (RCNP), Osaka University, Japan. In this study, we extended the measurements to higher energy with a p-$$^{7}$$Li quasi-monoenergetic neutron source, which was produced from a 1.0-cm-thick lithium target bombarded with 246 and 389 MeV protons, using a larger NE213 scintillator of 25.4-cm in diameter and 25.4-cm in thickness. The large NE213 have good energy resolution for high energy neutrons, because it can stop recoil protons up to 180 MeV. The measured data are compared with the Monte-Carlo codes (PHITS with JENDL-HE data library) in the energy spectra, time spectra and the attenuation length of the peak neutrons. This comparison shows good agreement between experiments and calculations. The attenuation length estimated from the well-fitted curves with single exponential form will be useful for the practical shielding design of high energy accelerator facilities.

Journal Articles

Response measurement of various neutron dose equivalent monitors in 134-387 MeV neutron fields

Nakane, Yoshihiro; Hagiwara, Masayuki*; Iwamoto, Yosuke; Iwase, Hiroshi*; Satoh, Daiki; Sato, Tatsuhiko; Yashima, Hiroshi*; Matsumoto, Tetsuro*; Masuda, Akihiko*; Nunomiya, Tomoya*; et al.

Progress in Nuclear Science and Technology (Internet), 4, p.704 - 708, 2014/04

no abstracts in English

Journal Articles

Activation detector measurements at the hadron absorber of the NuMI neutrino beamline at Fermilab

Matsuda, Norihiro; Kasugai, Yoshimi; Matsumura, Hiroshi*; Iwase, Hiroshi*; Toyoda, Akihiro*; Yashima, Hiroshi*; Sekimoto, Shun*; Oishi, Koji*; Sakamoto, Yukio*; Nakashima, Hiroshi; et al.

Progress in Nuclear Science and Technology (Internet), 4, p.337 - 340, 2014/04

The Neutrinos at the Main Injector (NuMI) at Fermilab produces intense neutrino beam to investigate the phenomena of the neutrino mixing and oscillation. The Hadron Absorber, consists of thick blocks of aluminum, iron and concrete, is placed at the end of decay volume as a dump for primary proton and secondary particles generated in NuMI. In order to estimate the shielding effect, the reaction rate measurements with activation detector were carried out on the back surface of the absorber. The induced activities in the detectors were measured by analyzing their $$gamma$$-ray spectra using HPGe detectors. Two kind of peak was showed on two-dimensional distributions of obtained reaction rates at right angle to the beam direction. One was strong peaks at the both horizontal side. And, another smaller was at the top. It was concluded that these peaks were the results of particles streaming through the gaps in the Hadron Absorber shielding.

Journal Articles

Fitting method for spectrum deduction in high-energy neutron field induced by GeV-protons using experimental reaction-rate data

Kasugai, Yoshimi; Matsuda, Norihiro; Sakamoto, Yukio; Nakashima, Hiroshi; Yashima, Hiroshi*; Matsumura, Hiroshi*; Iwase, Hiroshi*; Hirayama, Hideo*; Mokhov, N.*; Leveling, A.*; et al.

Reactor Dosimetry; 14th International Symposium (ASTM STP 1550), p.675 - 689, 2012/08

Under the collaborative study project of JASMIN, shielding experiments has been carried out using the anti-proton target station (Pbar) of Fermilab. In the experiment, the multi-foil activation technique was utilized, and the neutron spectra in high-energy region between 1 and 100 MeV were deduced by using the "fitting method", which is newly developed. In this method, we made an assumption that neutron energy spectra could be expressed with a simple function. The validity of the fitting method was confirmed by comparison with the results of the unfolding method and the theoretical calculations. Finally, it was found that there are simple correlations between reaction rates and the adjusting parameters in the fitting function. The correlations are useful for estimating the adjusting parameters easily, and a neutron spectrum in the high-energy region can be deduced from a set of reaction-rate data without the complicated calculations of unfolding.

Journal Articles

Response measurement of a Bonner sphere spectrometer for high-energy neutrons

Masuda, Akihiko*; Matsumoto, Tetsuro*; Harano, Hideki*; Nishiyama, Jun*; Iwamoto, Yosuke; Hagiwara, Masayuki*; Satoh, Daiki; Iwase, Hiroshi*; Yashima, Hiroshi*; Nakamura, Takashi*; et al.

IEEE Transactions on Nuclear Science, 59(1), p.161 - 166, 2012/02

 Times Cited Count:12 Percentile:66.47(Engineering, Electrical & Electronic)

In this study, responses of Bonner sphere spectrometer (BSS) for 245 and 388 MeV neutrons was measured at RCNP, Osaka University. The neutrons are generated in the $$^{7}$$Li(p,n) reaction and its spectra consist of a high-energy peak and a continuum down to the low energy. Therefore, the observed counts of BSS caused by the continuum need to be subtracted. Adjusting a Li target angle and a collimator position, 0 deg and 30 deg component of generated neutron are available. While the 0 deg component contains both the peak and the continuum, the 30 deg component is considered to contain only the continuum. Therefore, the response of the peak is obtained. The spectra were measured using the time-of-flight (TOF) method with a NE213 scintillator.

Journal Articles

Dependence of fracture geometry and spatial variation in pressure on hydraulic conductivity in rock fractures

Kishida, Kiyoshi*; Hosoda, Takashi*; Sawada, Atsushi; Sato, Hisashi; Nakashima, Shinichiro*; Yasuhara, Hideaki*

Harmonising Rock Engineering and the Environment, p.1327 - 1330, 2011/10

Although it is generally known that a natural rock fracture indicates a complex aperture distribution, the fracture is an ideal representation of the parallel plate model. The cubic law is applied to evaluate the hydraulic properties of fractured rock. From several previous research works, it is known that the cubic law can be applied when the Reynolds number is less than 1.0 and that the advection term can basically be ignored in such fracture flows. In this research work, two-dimensional seepage flow analyses, using the authors' proposed 2D model which is considered with the advection term, are carried out for single fracture hydro-conductivity experiments under conditions which allow for the application of the cubic law. From the numerical results, the validity of the 2D model is discussed along with the local Reynolds number and the application of the cubic law.

Journal Articles

Evaluation of dose rate reduction in a spacecraft compartment due to additional water shield

Sato, Tatsuhiko; Niita, Koji*; Shurshakov, V. A.*; Yarmanova, E. N.*; Nikolaev, I. V.*; Iwase, Hiroshi*; Sihver, L.*; Mancusi, D.*; Endo, Akira; Matsuda, Norihiro; et al.

Cosmic Research, 49(4), p.319 - 324, 2011/08

 Times Cited Count:11 Percentile:60.27(Engineering, Aerospace)

HZE particle transport codes are the indispensable tool in the shielding design of spacecrafts. We are therefore developing a general-purpose Monte Carlo code PHITS, which can deal with the transports of all kinds of hadrons and heavy ions with energies up to 200 GeV/n in 3-dimensional phase spaces. The applicability of PHITS to space researches has been well verified by comparing the neutron spectra in spacecrafts calculated by the code with the corresponding experimental data. Recently, PHITS was employed in the estimation of radiation fields in the Russian Service Module in ISS. The results of the estimation indicate that PHITS can reproduce experimental data of the dose reduction rates due to water shielding attached on the wall of the Russian crew cabin fairly well. The details of the calculation procedures will be given in the presentation, together with the results of other applications of PHITS to the space exploration.

Journal Articles

Shielding experiments under JASMIN collaboration at Fermilab, 4; Measurement and analyses of high-energy neutron spectra in the anti-proton target station

Matsuda, Norihiro; Kasugai, Yoshimi; Sakamoto, Yukio; Nakashima, Hiroshi; Matsumura, Hiroshi*; Iwase, Hiroshi*; Kinoshita, Norikazu*; Hirayama, Hideo*; Yashima, Hiroshi*; Mokhov, N.*; et al.

Journal of the Korean Physical Society, 59(2), p.2055 - 2058, 2011/08

 Times Cited Count:0 Percentile:0(Physics, Multidisciplinary)

It is important to obtain neutron spectra and its intensity on shielding experiment. Deduction of high-energy neutron spectra were done using fitting and unfolding methods based on the shielding data obtained at the anti-proton (pbar) target station in Fermilab. The neutron spectra for fitting method is useful to be easily obtained and the values gave reasonable results compared with nuclear data. Therefore, that for unfolding methods included inconsistency. Furthermore, the deduced neutron spectra were verified through the calculation analyses by PHITS code.

Journal Articles

Manufacturability and strength assessment of modified 9Cr-1Mo steel products for Japan sodium cooled fast reactor components, 2; Long thin-walled tubes with small diameter

Wakai, Takashi; Onizawa, Takashi; Obara, Satoshi; Nakashima, Takashi*; Yokoyama, Tetsuo*; Iseda, Atsuro*; Ogumo, Shinya*; Futagami, Satoshi*

Tainetsu Kinzoku Zairyo Dai-123-Iinkai Kenkyu Hokoku, 52(2), p.171 - 181, 2011/07

To enhance the economic competitiveness, high-Cr ferritic steels are adopted as the structural materials for JSFR, because the steels have both excellent high temperature strength and thermal properties. Among the high-Cr ferritic steels, modified 9Cr-1Mo steel (compatible to ASTM A213 T91) is a candidate of the structural material for the demonstration facility of JSFR, because the steel has superior microstructure stability at elevated temperature for long time. As for the steam generator tubes, to enhance the safety, straight double-walled tubes will be employed. In this study, the following technical issues were investigated; (1) Industrial manufacturability of thin-walled small bore tubes made of modified 9Cr-1Mo steel, (2) performance demonstration of the thin-walled small bore tubes, (3) industrial manufacturability of double-walled tubes using the thin-walled small bore tubes and (4) extraction of technical problems to manufacture the double-walled tubes for the JSFR steam generator. As a result, thin-walled small bore tubes made of modified 9Cr-1Mo steel were successfully manufactured by using the existing industrial facilities, up to 17m in length. The mechanical properties of the tubes satisfy the requirements from plant designing, as well as those from the material strength standards. Further, double walled tubes were also manufactured, up to 15m in length. The surface conditions of the tubes and the contact pressure between inner and outer tubes should be optimized.

Journal Articles

Characterisation of quadi-monoenergetic neutron energy spectra using $$^{7}$$Li(p,n) reactions at 246-389 MeV

Iwamoto, Yosuke; Hagiwara, Masayuki*; Satoh, Daiki; Iwase, Hiroshi*; Yashima, Hiroshi*; Itoga, Toshiro*; Sato, Tatsuhiko; Nakane, Yoshihiro; Nakashima, Hiroshi; Sakamoto, Yukio; et al.

Proceedings of 10th Meeting of the Task Force on Shielding Aspects of Accelerators, Targets and Irradiation Facilities (SATIF-10), p.53 - 61, 2011/03

The neutron energy spectra penetrating 10 to 100 cm thick iron and 25 to 200 cm thick concrete shields have been measured using 138, 243 and 387 MeV quasi-monoenergetic neutron sources at the Research Center for Nuclear Physics (RCNP) facility, Osaka University. The source neutrons were produced from a 1 cm thick lithium target bombarded with 140, 245 and 388 MeV protons. Two types of NE213 liquid organic scintillators and Bonner ball neutron spectrometers were used for the neutron energy spectrum measurement. The TOF and unfolding methods were applied to estimate the energy spectra behind the shield in the peak energy region and continuous energy region, respectively. We have also measured the neutron energy spectra and angular distribution of the source neutron above 1 MeV in the angular range from 0$$^{circ}$$ to 30$$^{circ}$$ with the TOF method. All measured data were compared with the PHITS Monte Carlo calculations.

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