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JAEA Reports

Analysis of the radioactivity concentrations in radioactive waste generated from JRR-3, JRR-4 and JRTF facilities

Tobita, Minoru*; Konda, Miki; Omori, Takeshi*; Nabatame, Tsutomu*; Onizawa, Takashi*; Kurosawa, Katsuaki*; Haraga, Tomoko; Aono, Ryuji; Mitsukai, Akina; Tsuchida, Daiki; et al.

JAEA-Data/Code 2022-007, 40 Pages, 2022/11

JAEA-Data-Code-2022-007.pdf:1.99MB

Radioactive wastes generated from nuclear research facilities in Japan Atomic Energy Agency are planning to be buried in the near surface disposal field. Therefore, it is required to establish the method to evaluate the radioactivity concentrations of radioactive wastes until the beginning of disposal. In order to contribute to this work, we collected and analyzed concrete, ash, ceramic and brick samples generated from JRR-3, JRR4 and JRTF facilities. In this report, we summarized the radioactivity concentrations of 24 radionuclides ($$^{3}$$H, $$^{14}$$C, $$^{36}$$Cl, $$^{41}$$Ca, $$^{60}$$Co, $$^{63}$$Ni, $$^{90}$$Sr, $$^{94}$$Nb, $$^{99}$$Tc, $$^{rm 108m}$$Ag, $$^{129}$$I, $$^{137}$$Cs, $$^{133}$$Ba, $$^{152}$$Eu, $$^{154}$$Eu, $$^{rm 166m}$$Ho, $$^{234}$$U, $$^{238}$$U, $$^{238}$$Pu, $$^{239}$$Pu, $$^{240}$$Pu, $$^{241}$$Am, $$^{243}$$Am, $$^{244}$$Cm) which were obtained from radiochemical analysis of the samples in fiscal years 2020-2021.

Journal Articles

Rabi-oscillation spectroscopy of the hyperfine structure of muonium atoms

Nishimura, Shoichiro*; Torii, Hiroyuki*; Fukao, Yoshinori*; Ito, Takashi; Iwasaki, Masahiko*; Kanda, Sotaro*; Kawagoe, Kiyotomo*; Kawall, D.*; Kawamura, Naritoshi*; Kurosawa, Noriyuki*; et al.

Physical Review A, 104(2), p.L020801_1 - L020801_6, 2021/08

 Times Cited Count:13 Percentile:84.11(Optics)

Journal Articles

Present status of J-PARC linac

Oguri, Hidetomo; Hasegawa, Kazuo; Ito, Takashi; Chishiro, Etsuji; Hirano, Koichiro; Morishita, Takatoshi; Shinozaki, Shinichi; Ao, Hiroyuki; Okoshi, Kiyonori; Kondo, Yasuhiro; et al.

Proceedings of 11th Annual Meeting of Particle Accelerator Society of Japan (Internet), p.389 - 393, 2014/10

no abstracts in English

Journal Articles

Recent progress in the energy recovery linac project in Japan

Sakanaka, Shogo*; Akemoto, Mitsuo*; Aoto, Tomohiro*; Arakawa, Dai*; Asaoka, Seiji*; Enomoto, Atsushi*; Fukuda, Shigeki*; Furukawa, Kazuro*; Furuya, Takaaki*; Haga, Kaiichi*; et al.

Proceedings of 1st International Particle Accelerator Conference (IPAC '10) (Internet), p.2338 - 2340, 2010/05

Future synchrotron light source using a 5-GeV energy recovery linac (ERL) is under proposal by our Japanese collaboration team, and we are conducting R&D efforts for that. We are developing high-brightness DC photocathode guns, two types of cryomodules for both injector and main superconducting (SC) linacs, and 1.3 GHz high CW-power RF sources. We are also constructing the Compact ERL (cERL) for demonstrating the recirculation of low-emittance, high-current beams using above-mentioned critical technologies.

Journal Articles

Development of special rotor for centrifugal separation of isotopes in solid pure metals

Ono, Masao; Sueyoshi, Masanori*; Okayasu, Satoru; Hao, T.; Esaka, Fumitaka; Osawa, Takahito; Iguchi, Yusuke*; Mashimo, Tsutomu

Review of Scientific Instruments, 80(8), p.083908_1 - 083908_6, 2009/08

 Times Cited Count:3 Percentile:17.76(Instruments & Instrumentation)

A prototype rotor with 2 grooves for the multi-stage centrifugal isotope separation in solid state was developed to test a new idea. This idea is based on the sedimentation of constitutional atoms in solid. In the performance test using indium specimen, it is verified that the developed rotor can receive all injected molten-indium droplets from an automatic raw-material feeding system even at the high rotational speed of 97,000 r.p.m. without the loss of rotational stability, and the received indium specimens can be transferred in/between 2 grooves through the plastic flow under the influence of strong centrifugal force even in the solid state. The isotope ratio of centrifuged indium specimens was analyzed employing the Secondary Ion Mass Spectrometry (SIMS), and it is confirmed that intended isotope separation by the centrifugation is realized in the solid state.

JAEA Reports

The Outline of investigation on integrity of JMTR concrete structures, cooling system and utility facilities

Ebisawa, Hiroyuki; Hanakawa, Hiroki; Asano, Norikazu; Kusunoki, Hidehiko; Yanai, Tomohiro; Sato, Shinichi; Miyauchi, Masaru; Oto, Tsutomu; Kimura, Tadashi; Kawamata, Takanori; et al.

JAEA-Technology 2009-030, 165 Pages, 2009/07

JAEA-Technology-2009-030.pdf:69.18MB

The condition of facilities and machinery used continuously were investigated before the renewal work of JMTR on FY 2007. The subjects of investigation were reactor building, primary cooling system tanks, secondary cooling system piping and tower, emergency generator and so on. As the result, it was confirmed that some facilities and machinery were necessary to repair and others were used continuously for long term by maintaining on the long-term maintenance plan. JMTR is planed to renew by the result of this investigation.

Journal Articles

Isotope fractionation due to sedimentation of atoms in centrifuged indium-lead alloy

Ono, Masao; Iguchi, Yusuke*; Okayasu, Satoru; Esaka, Fumitaka; Kobayashi, Katsura*; Hao, T.; Bagum, R.*; Osawa, Takahito; Fujii, Kimio; Nakamura, Eizo*; et al.

Defect and Diffusion Forum, 289-292, p.63 - 68, 2009/04

The atomic-scale graded structure of In-Pb alloy was formed by an ultracentrifuge experiment under conditions that a gravitational field of 0.81$$times$$10$$^{6}$$ G for 100 hours at 150 $$^{circ}$$C in solid state in our previous study. The isotope ratio measurements were performed on the centrifuged sample with secondary ion mass spectrometer (SIMS). $$^{206}$$Pb/$$^{208}$$Pb and $$^{207}$$Pb/$$^{208}$$Pb isotope ratio changed with negative gradient in the direction of centrifugal force approximately 1.5% and 0.8%, respectively. And three-isotope diagram of $$^{206}$$Pb/$$^{208}$$Pb versus $$^{207}$$Pb/$$^{208}$$Pb proved that the isotope fluctuation depends on isotopic mass difference. These results showed that the strong gravitational field not only affected on the inter-diffusion but also on self-diffusion in this alloy as causing isotope fractionation effect, and the isotope fractionation was dependent on mass-difference.

Journal Articles

Mass-dependent isotopic fractionation of a solid tin under a strong gravitational field

Osawa, Takahito; Ono, Masao; Esaka, Fumitaka; Okayasu, Satoru; Iguchi, Yusuke*; Hao, T.; Magara, Masaaki; Mashimo, Tsutomu

EPL; A Letters Journal Exploring the Frontiers of Physics, 85(6), p.64001_1 - 64001_5, 2009/03

 Times Cited Count:6 Percentile:41.57(Physics, Multidisciplinary)

Pure tin metals were centrifuged at 1$$times$$$$10^6$$ $$g$$ and at 220 $$^{circ}$$C for 100 hours, 0.40$$times$$$$10^6$$ $$g$$ at 220-230 $$^{circ}$$C for 24 hours, and 0.25$$times$$$$10^6$$ $$g$$ at 220 $$^{circ}$$C for 24 hours. Their isotopic compositions were measured by a secondary ion mass spectrometer (SIMS). $$^{116}$$Sn/$$^{120}$$Sn and $$^{124}$$Sn/$$^{120}$$Sn ratios of the 1.02$$times$$$$10^6$$ $$g$$ sample were considerably different than the initial compositions, and the magnitude of isotopic fractionation reached 2.6%. A three-isotope diagram of $$^{116}$$Sn/$$^{120}$$Sn versus $$^{124}$$Sn/$$^{120}$$Sn shows conclusively that isotopic fractionation caused by a gravitational field depended only on isotopic mass.

Journal Articles

Isotope fluctuation in indium-lead alloy induced by solid centrifugation

Ono, Masao; Iguchi, Yusuke*; Okayasu, Satoru; Esaka, Fumitaka; Kobayashi, Katsura*; Hao, T.; Bagum, R.*; Osawa, Takahito; Fujii, Kimio; Nakamura, Eizo*; et al.

Journal of Nuclear Science and Technology, 45(Suppl.6), p.108 - 110, 2008/09

 Times Cited Count:1 Percentile:10.01(Nuclear Science & Technology)

The atomic-scale graded structure of In-Pb alloy was formed by an ultracentrifuge experiment under conditions that a gravitational field of 810,000 G for 100 hours at 150$$^{circ}$$C (solid state) in our previous study. The isotope fluctuation on this sample was measured using secondary ion mass spectrometer (SIMS). The ratio both $$^{208}$$Pb/$$^{206}$$Pb and $$^{115}$$In/$$^{113}$$In changed with positive gradient in the direction of centrifugal force approximately 1.2%. These isotope fluctuations were larger than that of starting state of natural state (In$$<$$0.2%, Pb$$<$$0.1%). These show that the sedimentation of isotopes occurred by solid centrifugation in this alloy, although achieved concentration gradients were small.

Journal Articles

The Influence of nitrate on dissolution behavior of cement hydrates

Fujita, Hideki*; Negishi, Kumi*; Osawa, Tsutomu*; Honda, Akira

Semento, Konkurito Rombunshu, (61), p.262 - 269, 2008/02

The influence of sodium nitrate on dissolution of cement hydrates was investigated by flow through experiment. Dissolution of portlandite was accelerated in NaNO$$_{3}$$ solution of 1 mol dm$$^{-3}$$ than in ion exchanged water. The acceleration of portlandite dissolution attributed to impact of ionic strength on the activities of aqueous species, because Ca concentration in 1 mol kg$$^{-1}$$ NaNO$$_{3}$$ solution equilibrated with portlandite was estimated to be 1.5 times as high as that in pure water. After flow through experiment, compressive strength fell down and porosity was higher than blank test using pure water. However low permeabilities were contradictory kept during NaNO$$_{3}$$ solution flowing. Dense existence of Na was possible to cause the low permeability during NaNO$$_{3}$$ solution flowing.

JAEA Reports

Isopleths of surface air concentration and surface air kerma rate due to a radioactive cloud released from a stack, 3

Tachibana, Haruo; Kikuchi, Masamitsu; Sekita, Tsutomu; Yamaguchi, Takenori; Oeda, Mikihiro*; Kurosawa, Naohiro*

JAERI-Data/Code 2004-010, 19 Pages, 2004/06

JAERI-Data-Code-2004-010.pdf:1.92MB
JAERI-Data-Code-2004-010-appendix(CD-ROM).zip:12.12MB

This report is a revised edition of "Isopleths of Surface Air Concentration and Surface Air Absorbed Dose Rate due to a Radioactive Cloud Released from a Stack(II)"(JAERI-M 90-206) and based on the revised Nuclear Safety Guidelines reflected the ICRP1990 Recommendation. Characteristics of this report are the use of Air Karma Rate (Gy/h) unit instead of Air Absorbed Dose Rate (Gy/h) unit, and the records of isopleths of surface air concentration and surface air karma rate on CD-ROM. These recorded data on CD-ROM can be printed out on paper and/or pasted on digital map by personal computer.

Journal Articles

Oxygen and Hydrogen Isotopic Ratios of the Anomalously Discharged Groundwater after the 1995 Kobe Earthquake in Awaji Island, Japan

Osawa, Hideaki; Sato, Tsutomu*; Sakai, Ryutaro; Osawa, Hideaki; Kodama, Toshio*

Nihon Suimon Kagakkai-Shi, 29(1), p.13 - 24, 1999/00

None

Oral presentation

Isotope fractionation due to sedimentation of atoms in centrifuged indium-lead alloy

Ono, Masao; Iguchi, Yusuke*; Okayasu, Satoru; Esaka, Fumitaka; Kobayashi, Katsura*; Hao, T.; Bagum, R.*; Osawa, Takahito; Fujii, Kimio; Nakamura, Eizo*; et al.

no journal, , 

The atomic-scale graded structure of In-Pb alloy was formed by an ultracentrifuge experiment under conditions that a gravitational field of 0.81$$times$$10$$^{6}$$G for 100 hours at 150 $$^{circ}$$C in solid state in our previous study. The isotope ratio measurements were performed on the centrifuged sample with secondary ion mass spectrometer (SIMS, CAMECA IMS-6f). Both $$^{115}$$In/$$^{113}$$In and $$^{208}$$Pb/$$^{206}$$ isotope ratio changed with negative gradient in the direction of centrifugal force approximately 1.2% showing the tendency that the heavy $$^{115}$$In isotope ($$^{208}$$Pb isotope) abundance increased and light $$^{113}$$In isotope ($$^{206}$$Pb isotope) abundance decreased in the direction of centrifugal force. This showed that the isotope fractionation effect due to sedimentation of atoms occurred in this alloy by ultracentrifuge experiment.

Oral presentation

Isotopic fractionation of tin under extremely strong centrifugal force field

Osawa, Takahito; Ono, Masao; Esaka, Fumitaka; Okayasu, Satoru; Iguchi, Yusuke*; Hao, T.; Mashimo, Tsutomu

no journal, , 

Pure tin metals were centrifuged at 1,0200,000G and at 220$$^{circ}$$C for 100 hours, 400,000 G at 220-230$$^{circ}$$C for 24 hours, and 250,000G at 220$$^{circ}$$C for 24 hours. Their isotopic compositions were measured by a secondary ion mass spectrometer (SIMS). 116Sn/120Sn and 124Sn/120Sn ratios of the 1,0200,000G sample were considerably different than the initial compositions, and the magnitude of isotopic fractionation reached 2.6%. A three-isotope diagram of 116Sn/120Sn versus 124Sn/120Sn shows conclusively that isotopic fractionation caused by a gravitational field depended on isotopic mass.

Oral presentation

Centrifugal isotope separation in solid or liquid

Ono, Masao; Hao, T.; Okayasu, Satoru; Esaka, Fumitaka; Osawa, Takahito; Iguchi, Yusuke*; Mashimo, Tsutomu

no journal, , 

no abstracts in English

Oral presentation

Risk communication for the acceptance of irradiated food

Ichikawa, Mariko*; Iizuka, Tomoko*; Gamo, Emi*; Kobori, Emiko*; Shibuya, Michiko*; Shibosawa, Hisako*; Chiba, Etsuko*; Yokoyama, Tsutomu*; Fukutomi, Fumitake*; Todoriki, Setsuko*; et al.

no journal, , 

no abstracts in English

Oral presentation

Isotopic fractionation of a solid tin under a ultra-strong centrifugal force field

Osawa, Takahito; Ono, Masao; Esaka, Fumitaka; Okayasu, Satoru; Mashimo, Tsutomu*

no journal, , 

no abstracts in English

Oral presentation

Isotopic fractionation of a solid tin under a ultra-strong centrifugal force field

Osawa, Takahito; Ono, Masao; Esaka, Fumitaka; Okayasu, Satoru; Mashimo, Tsutomu*

no journal, , 

no abstracts in English

Oral presentation

Isotope fractionation in AgI super-ionic conductor by centrifugation

Ono, Masao; Okayasu, Satoru; Iguchi, Yusuke*; Esaka, Fumitaka; Ishitsuka, Etsuo; Osawa, Takahito; Ogata, Yudai; Mashimo, Tsutomu*

no journal, , 

Oral presentation

Research and development on preceding processing methods for contaminated water management waste at Fukushima Daiichi Nuclear Power Station, 43; Crystallization of amorphous phases formed in Alkali Activated Material solidified body

Kobayashi, Yutaro*; Osawa, Norihisa*; Haga, Kazuko*; Kaneda, Yoshihisa*; Chaerun Raudhatul, I.*; Sato, Tsutomu*; Taniguchi, Takumi; Kuroki, Ryoichiro; Osugi, Takeshi

no journal, , 

no abstracts in English

22 (Records 1-20 displayed on this page)