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Journal Articles

Achievements and status of the STRAD project for radioactive liquid waste management

Arai, Yoichi; Watanabe, So; Nakahara, Masaumi; Funakoshi, Tomomasa; Hoshino, Takanori; Takahatake, Yoko; Sakamoto, Atsushi; Aihara, Haruka; Hasegawa, Kenta; Yoshida, Toshiki; et al.

Progress in Nuclear Science and Technology (Internet), 7, p.168 - 174, 2025/05

The Japan Atomic Energy Agency (JAEA) has been conducting a project named "Systematic Treatment of RAdioactive liquid waste for Decommissioning (STRAD)" project since 2018 for fundamental and practical studies for treating radioactive liquid wastes with complicated compositions. Fundamental studies have been conducted using genuine liquid wastes accumulated in a hot laboratory of the JAEA called the Chemical Processing Facility (CPF), and treatment procedures for all liquid wastes in CPF were successfully designed on the results obtained. As the next phase of the project, new fundamental and practical studies on primarily organic liquid wastes accumulated in different facilities of JAEA are in progress. This paper reviews the representative achievements of the STRAD project and introduces an overview of ongoing studies.

Journal Articles

Development of a dissolution method for analyzing the elemental composition of fuel debris using sodium peroxide fusion technique

Nakamura, Satoshi; Ishii, Sho*; Kato, Hitoshi*; Ban, Yasutoshi; Hiruta, Kenta; Yoshida, Takuya; Uehara, Hiroyuki; Obata, Hiroki; Kimura, Yasuhiko; Takano, Masahide

Journal of Nuclear Science and Technology, 62(1), p.56 - 64, 2025/01

 Times Cited Count:1 Percentile:57.00(Nuclear Science & Technology)

A dissolution method for analyzing the elemental composition of fuel debris using the sodium peroxide (Na$$_{2}$$O$$_{2}$$) fusion technique has been developed. Herein, two different types of simulated debris materials (such as solid solution of (Zr,RE)O$$_{2}$$ and molten core-concrete interaction products (MCCI)) were taken. At various temperatures, these debris materials were subsequently fused with Na$$_{2}$$O$$_{2}$$ in crucibles, which are made of different materials, such as Ni, Al$$_{2}$$O$$_{3}$$, Fe, and Zr. Then, the fused samples are dissolved in nitric acid. Furthermore, the effects of the experimental conditions on the elemental composition analysis were evaluated using inductively coupled plasma-atomic emission spectroscopy (ICP-AES), which suggested the use of a Ni crucible at 923 K as an optimum testing condition. The optimum testing condition was then applied to the demonstration tests with Three Mile Island unit-2 (TMI-2) debris in a shielded concrete cell, thereby achieving complete dissolution of the debris. The elemental composition of TMI-2 debris revealed by the proposed dissolution method has good reproducibility and has an insignificant contradiction in the mass balance of the sample. Therefore, this newly developed reproducible dissolution method can be effectively utilized in practical applications by dissolving fuel debris and estimating its elemental composition.

Journal Articles

Nanoscale visualization of crack tips inside molten corium-concrete interaction debris using 3D-FIB-SEM with multiphase positional misalignment correction

Miyata, Hokata*; Yoshida, Kenta*; Konashi, Kenji*; Du, Y.*; Kitagaki, Toru; Shobu, Takahisa; Shimada, Yusuke*

Microscopy, p.dfaf005_1 - dfaf005_10, 2025/00

 Times Cited Count:0 Percentile:0.00(Microscopy)

JAEA Reports

Annual report for FY2021 on the activities of Naraha Center for Remote Control Technology Development (April 1, 2021 - March 31, 2022)

Akiyama, Yoichi; Shibanuma, So; Yanagisawa, Kenichi*; Yamada, Taichi; Suzuki, Kenta; Yoshida, Moeka; Ono, Takahiro; Kawabata, Kuniaki; Watanabe, Kaho; Morimoto, Kyoichi; et al.

JAEA-Review 2023-015, 60 Pages, 2023/09

JAEA-Review-2023-015.pdf:4.78MB

Naraha Center for Remote Control Technology Development (NARREC) was established in Japan Atomic Energy Agency to promote a decommissioning work of Fukushima Daiichi Nuclear Power Station (Fukushima Daiichi NPS). NARREC consists of a Full-scale Mock-up Test Building and Research Management Building. Various test facilities are installed in these buildings for the decommissioning work of Fukushima Daiichi NPS. These test facilities are intended to be used for various users, such as companies engaged in the decommissioning work, research and development institutions, educational institutions and so on. The number of NARREC facility uses was 84 in FY2021. We participated booth exhibitions and presentations on the decommissioning related events. Moreover, we also contributed to the development of human resources by supporting the 6th Creative Robot Contest for Decommissioning. As a new project, "Narahakko Children's Classroom" was implemented for elementary school students in Naraha Town. This report summarizes the activities of NARREC in FY2021, such as the utilization of facilities and equipment of NARREC, the development of remote-control technologies for supporting the decommissioning work, arrangement of the remote-control machines for emergency response, and training for operators by using the machines.

Journal Articles

Experiences in dismantlement of gloveboxes for wet recovery and other use that are contaminated with nuclear fuel materials

Kitamura, Akihiro; Hirano, Hiroshi*; Yoshida, Masato; Takeuchi, Kentaro

Hoken Butsuri (Internet), 58(2), p.76 - 90, 2023/08

The alpha contaminated gloveboxes have been dismantled for over 20 years in Plutonium Fuel Fabrication Facility. The so called wet recovery equipment gloveboxes, which recover plutonium and uranium from scrap fuel by dissolving and extracting processes, were chosen as the priority gloveboxes to be dismantled. These gloveboxes and other gloveboxes in the same room were size reduced and removed up until 2022. Also, non-radioactive ancillary facility and non-radioactive giant glovebox were removed from 2007 to 2010 for ease of glovebox dismantling activities that follows and for making waste storage spaces. Several incidents were occurred and recidivism prevention measures were implemented on each occasion. In this report, glovebox dismantling activities we conducted in the past 20 years are reviewed and lessons we have learned are summarized.

Journal Articles

Report on participation in the 6th Asian and Oceanic Congress on Radiation Protection

Yoshitomi, Hiroshi; Manabe, Kentaro; Ochi, Kotaro; Kono, Takahiko; Sasaki, Michiya*; Yoshida, Hiroko*

Hoken Butsuri (Internet), 58(2), p.105 - 111, 2023/08

This article gives the report on participation in the 6th Asian and Oceanic Congress on Radiation Protection (AOCRP6), which was held in Mumbai, India on between February 7th and 11th, 2023.

Journal Articles

Development of nondestructive elemental analysis system for Hayabusa2 samples using muonic X-rays

Osawa, Takahito; Nagasawa, Shunsaku*; Ninomiya, Kazuhiko*; Takahashi, Tadayuki*; Nakamura, Tomoki*; Wada, Taiga*; Taniguchi, Akihiro*; Umegaki, Izumi*; Kubo, Kenya*; Terada, Kentaro*; et al.

ACS Earth and Space Chemistry (Internet), 7(4), p.699 - 711, 2023/04

 Times Cited Count:7 Percentile:72.47(Chemistry, Multidisciplinary)

The concentrations of carbon and other major elements in asteroid samples provide very important information on the birth of life on the Earth and the solar-system evolution. Elemental analysis using muonic X-rays is one of the best analytical methods to determine the elemental composition of solid materials, and notably, is the only method to determine the concentration of light elements in bulk samples in a non-destructive manner. We developed a new analysis system using muonic X-rays to measure the concentrations of carbon and other major elements in precious and expectedly tiny samples recovered from the asteroid Ryugu by spacecraft Hayabusa2. Here we report the development process of the system in 4 stages and their system configurations, The analysis system is composed of a stainless-steel analysis chamber, an acrylic glove box for manipulating asteroid samples in a clean environment, and Ge semiconductor detectors arranged to surround the analysis chamber. The performance of the analysis system, including the background level, which is crucial for the measurement, was greatly improved from the first stage to the later ones. Our feasibility study showed that the latest model of our muonic X-ray analysis system is capable of determining the carbon concentration in Hayabusa2's sample model with an uncertainty of less than 10 percent in a 6-day measurement.

Journal Articles

Defect analysis of matrix damage in reactor pressure vessel steel using WB-STEM

Yoshida, Kenta*; Toyama, Takeshi*; Inoue, Koji*; Nagai, Yasuyoshi*; Shimodaira, Masaki

Materia, 62(3), p.154 - 158, 2023/03

no abstracts in English

Journal Articles

Evaluation of indoor air dose rate based on Cs-137 depth distribution in surrounding artificially paved surfaces surveyed 10 years after the Fukushima Daiichi Nuclear Power Plant accident

Kobayashi, Hikaru*; Suto, Masahito*; Otsuki, Kentaro*; Yoshimura, Kazuya; Yoshida, Hiroko*

Japan Architectural Review (Internet), 6(1), p.e12353_1 - e12353_12, 2023/00

Journal Articles

End-to-end simulations and error studies of the J-PARC muon linac

Takeuchi, Yusuke*; Tojo, Junji*; Yamanaka, T.*; Nakazawa, Yuga*; Iinuma, Hiromi*; Kondo, Yasuhiro; Kitamura, Ryo; Morishita, Takatoshi; Cicek, E.*; Ego, Hiroyasu*; et al.

Proceedings of 31st International Linear Accelerator Conference (LINAC 2022) (Internet), p.562 - 564, 2022/10

A muon linac is under development for future muon g-2/EDM experiments at J-PARC. The linac provides a 212 MeV muon beam to an MRI-type compact storage ring. After the initial acceleration using the electrostatic field created by mesh and cylindrical electrodes, the muons are accelerated using four types of radio-frequency accelerators. To validate the linac design as a whole, end-to-end simulations were performed using General Particle Tracer. In addition, error studies were performed to investigate the effects on beam and spin dynamics of various errors in the accelerator components and input beam distribution. This paper describes the results of the end-to-end simulations and error studies.

Journal Articles

High-power test of an APF IH-DTL prototype for the muon linac

Nakazawa, Yuga*; Iinuma, Hiromi*; Iwata, Yoshiyuki*; Cicek, E.*; Ego, Hiroyasu*; Futatsukawa, Kenta*; Kawamura, Naritoshi*; Mibe, Tsutomu*; Mizobata, Satoshi*; Otani, Masashi*; et al.

Proceedings of 31st International Linear Accelerator Conference (LINAC 2022) (Internet), p.275 - 278, 2022/09

We conducted a high-power test of a prototype cavity of a 324-MHz inter-digital H-mode drift tube linac (IH-DTL) for the muon g-2/EDM experiment at J-PARC. This prototype cavity (short-IH) was developed to verify the fabrication methodology for the full-length IH cavity with a monolithic DT structure. After 40 h of conditioning, the short-IH has been stably operated with an RF power of 88 kW, which corresponds to 10% higher accelerating field than the design field (E0) of 3.0 MV/m. In addition, the thermal characteristics and frequency response were measured, verifying that the experimental data was consistent with the three-dimensional model. In this paper, the high-power tests of this IH-DTL for muon acceleration are described.

Journal Articles

The Muon linac project at J-PARC

Kondo, Yasuhiro; Kitamura, Ryo; Fuwa, Yasuhiro; Morishita, Takatoshi; Moriya, Katsuhiro; Takayanagi, Tomohiro; Otani, Masashi*; Cicek, E.*; Ego, Hiroyasu*; Fukao, Yoshinori*; et al.

Proceedings of 31st International Linear Accelerator Conference (LINAC 2022) (Internet), p.636 - 641, 2022/09

The muon linac project for the precise measurement of the muon anomalous magnetic and electric dipole moments, which is currently one of the hottest issues of the elementary particle physics, is in progress at J-PARC. The muons from the J-PARC muon facility are once cooled to room temperature, then accelerated up to 212 MeV with a normalized emittance of 1.5 $$pi$$ mm mrad and a momentum spread of 0.1%. Four types of accelerating structures are adopted to obtain the efficient acceleration with a wide beta range from 0.01 to 0.94. The project is moving into the construction phase. We already demonstrated the re-acceleration scheme of the decelerated muons using a 324-MHz RFQ in 2017. The high-power test of the 324-MHz Interdigital H-mode (IH) DTL using a prototype cavity was performed in 2021. The fabrication of the first module of 14 modules of the 1296-MHz Disk and Washer (DAW) CCL will be done to confirm the production process. Moreover, the final design of the travelling wave accelerating structure for the high beta region is also proceeding. In this paper, the recent progress toward the realization of the world first muon linac will be presented.

Journal Articles

Fabrication and low-power test of disk-and-washer cavity for muon acceleration

Takeuchi, Yusuke*; Tojo, Junji*; Nakazawa, Yuga*; Kondo, Yasuhiro; Kitamura, Ryo; Morishita, Takatoshi; Cicek, E.*; Ego, Hiroyasu*; Futatsukawa, Kenta*; Kawamura, Naritoshi*; et al.

Proceedings of 13th International Particle Accelerator Conference (IPAC 22) (Internet), p.1534 - 1537, 2022/06

The muon g-2/EDM experiment is under preparation at Japan Proton Accelerator Research Complex (J-PARC), and the muon linear accelerator for the experiment is being developed. A Disk-and-Washer (DAW) cavity will be used for the medium-velocity part of the accelerator, and muons will be accelerated from $$v/c$$ = $$beta$$ = 0.3 to 0.7 with the operating frequency of 1.296 GHz. Machining, brazing, and low-power measurements of a prototype cell reflecting the design of the first tank of DAW were performed to identify fabrication problems. Several problems were identified, such as misalignment of washers during brazing, and some measures will be taken in the actual tank fabrication. In this paper, the results of the prototype cell fabrication will be reported.

Journal Articles

${it In situ}$ TEM observation and MD simulation of frank partial dislocation climbing in Al-Cu alloy

Chen, J.*; Yoshida, Kenta*; Suzudo, Tomoaki; Shimada, Yusuke*; Inoue, Koji*; Konno, Toyohiko*; Nagai, Yasuyoshi*

Materials Transactions, 63(4), p.468 - 474, 2022/04

 Times Cited Count:3 Percentile:23.47(Materials Science, Multidisciplinary)

In situ electron irradiation using high-resolution transmission electron microscopy (HRTEM) was performed to visualize the Frank loop evolution in aluminium-copper (Al-Cu) alloy with an atomic-scale spatial resolution of 0.12 nm. The ${it in situ}$ HRTEM observation along the [110] direction of the FCC-Al lattice, Frank partial dislocation bounding an intrinsic stacking fault exhibited an asymmetrical climb along the $$<$$112$$>$$ direction opposed to those in the reference pure Al under an electron irradiation, with a corresponding displacement-per-atom rate of 0.055-0.120 dpa/s. The asymmetrical climb of the partial dislocation was described as pinning effects due to Cu-Cu bonding in Guinier-Preston zones by a molecular dynamics simulation.

Journal Articles

Dissolution and precipitation behaviors of zircon under the atmospheric environment

Kitagaki, Toru; Yoshida, Kenta*; Liu, P.*; Shobu, Takahisa

npj Materials Degradation (Internet), 6(1), p.13_1 - 13_8, 2022/02

 Times Cited Count:2 Percentile:12.90(Materials Science, Multidisciplinary)

Journal Articles

Nonmagnetic-magnetic transition and magnetically ordered structure in SmS

Yoshida, Shogo*; Koyama, Takehide*; Yamada, Haruhiko*; Nakai, Yusuke*; Ueda, Koichi*; Mito, Takeshi*; Kitagawa, Kentaro*; Haga, Yoshinori

Physical Review B, 103(15), p.155153_1 - 155153_5, 2021/04

 Times Cited Count:1 Percentile:4.81(Materials Science, Multidisciplinary)

Journal Articles

Morphological reproductive characteristics of testes and fertilization capacity of cryopreserved sperm after the Fukushima accident in raccoon (${it Procyon lotor}$)

Komatsu, Kazuki*; Iwasaki, Tsugumi*; Murata, Kosuke*; Yamashiro, Hideaki*; Goh, V. S. T.*; Nakayama, Ryo*; Fujishima, Yohei*; Ono, Takumi*; Kino, Yasushi*; Shimizu, Yoshinaka*; et al.

Reproduction in Domestic Animals, 56(3), p.484 - 497, 2021/03

 Times Cited Count:13 Percentile:83.05(Agriculture, Dairy & Animal Science)

We have established an archive system of livestock and wild animals from the surrounding ex-evacuation zone. Wildlife within the alert zone have been exposed to low-dose-rate (LDR) radiation for a long and continuous time. In this study, we analysed the morphological characteristics of the testes and in vitro fertilization (IVF) capacity of cryopreserved sperm of raccoons from the ex-evacuation zone of the FDNPP accident. This study revealed that the chronic and LDR radiation exposure associated with the FDNPP accident had no adverse effect on the reproductive characteristics and functions of male raccoons.

Journal Articles

${it In situ}$ WB-STEM observation of dislocation loop behavior in reactor pressure vessel steel during post-irradiation annealing

Du, Y.*; Yoshida, Kenta*; Shimada, Yusuke*; Toyama, Takeshi*; Inoue, Koji*; Arakawa, Kazuto*; Suzudo, Tomoaki; Milan, K. J.*; Gerard, R.*; Onuki, Somei*; et al.

Materialia, 12, p.100778_1 - 100778_10, 2020/08

In order to ensure the integrity of the reactor pressure vessel in the long term, it is necessary to understand the effects of irradiation on the materials. In this study, irradiation-induced dislocation loops were observed in neutron-irradiated reactor pressure vessel specimens during annealing using our newly developed WB-STEM. It was confirmed that the proportion of $$<100>$$ loops increased with increasing annealing temperature. We also succeeded in observing the phenomenon that two $$frac{1}{2}$$$$<111>$$ loops collide into a $$<100>$$ loop. Moreover, a phenomenon in which dislocation loops decorate dislocations was also observed, and the mechanism was successfully explained by molecular dynamics simulation.

Journal Articles

How different is the core of $$^{25}$$F from $$^{24}$$O$$_{g.s.}$$ ?

Tang, T. L.*; Uesaka, Tomohiro*; Kawase, Shoichiro; Beaumel, D.*; Dozono, Masanori*; Fujii, Toshihiko*; Fukuda, Naoki*; Fukunaga, Taku*; Galindo-Uribarri, A.*; Hwang, S. H.*; et al.

Physical Review Letters, 124(21), p.212502_1 - 212502_6, 2020/05

 Times Cited Count:18 Percentile:73.39(Physics, Multidisciplinary)

The structure of a neutron-rich $$^{25}$$F nucleus is investigated by a quasifree ($$p,2p$$) knockout reaction. The sum of spectroscopic factors of $$pi 0d_{5/2}$$ orbital is found to be 1.0 $$pm$$ 0.3. The result shows that the $$^{24}$$O core of $$^{25}$$F nucleus significantly differs from a free $$^{24}$$O nucleus, and the core consists of $$sim$$35% $$^{24}$$O$$_{rm g.s.}$$, and $$sim$$65% excited $$^{24}$$O. The result shows that the $$^{24}$$O core of $$^{25}$$F nucleus significantly differs from a free $$^{24}$$O nucleus. The result may infer that the addition of the $$0d_{5/2}$$ proton considerably changes the neutron structure in $$^{25}$$F from that in $$^{24}$$O, which could be a possible mechanism responsible for the oxygen dripline anomaly.

Journal Articles

Re-acceleration of ultra cold muon in J-PARC Muon Facility

Kondo, Yasuhiro; Hasegawa, Kazuo; Morishita, Takatoshi; Otani, Masashi*; Futatsukawa, Kenta*; Kawamura, Naritoshi*; Mibe, Tsutomu*; Yamazaki, Takayuki*; Yoshida, Mitsuhiro*; Kitamura, Ryo*; et al.

Proceedings of 9th International Particle Accelerator Conference (IPAC '18) (Internet), p.5041 - 5046, 2018/06

J-PARC is developing the reacceleration system of the ultra slow (30 meV) muon (USM) obtained by two-photon laser resonant ionization of muonium atoms. The muon beam thus obtained has low emittance, meeting the requirement for the g-2/EDM experiment. J-PARC E34 experiment aims to measure the muon anomalous magnetic moment (g-2) with a precision of 0.1 ppm and search for EDM with a sensitivity to $$10^{-21}$$ e cm. The USM's are accelerated to 212 MeV by using a muon dedicated linac to be a ultra cold muon beam. The muon LINAC consists of an RFQ, a inter-digital H-mode DTL, disk and washer coupled cell structures, and disk loaded structures. Proof of the slow muon acceleration scheme is an essential step to realize the world first muon linac. In October 2017, we have succeeded to accelerate slow negative muoniums generated using a simpler muonium source to 89 keV. In this talk, present design of the muon linac and the result of the world first muon acceleration experiment are reported.

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