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論文

Pulsed muon facility of J-PARC MUSE

下村 浩一郎*; 幸田 章宏*; Pant, A. D.*; 砂川 光*; 藤森 寛*; 梅垣 いづみ*; 中村 惇平*; 藤原 理賀; 反保 元伸*; 河村 成肇*; et al.

Interactions (Internet), 245(1), p.31_1 - 31_6, 2024/12

J-PARC Muon Facility: MUSE (Muon Science Establishment) is responsible for the inter-university user program and the operation, maintenance, and construction of the muon beamlines, namely D-line, S-line, U-line, and H-line, along with the muon source at J-PARC Materials and Life Science Facility (MLF). In this paper, recent developments are briefly presented.

論文

$$^{149}$$Sm synchrotron-radiation-based M$"{o}$ssbauer spectroscopy of Sm-based heavy fermion compounds

筒井 智嗣; 東中 隆二*; 水牧 仁一朗*; 小林 義男*; 中村 仁*; 伊藤 孝; 依田 芳卓*; 松田 達磨*; 青木 勇二*; 佐藤 英行*

Interactions (Internet), 245(1), p.9_1 - 9_10, 2024/12

$$^{149}$$Sm synchrotron-radiation-based M$"{o}$ssbauer spectroscopy has been applied to Sm-based heavy fermion intermetallics, Sm$$Tr_2$$Al$$_{20}$$ ($$Tr$$ = Ti, V and Cr) and SmOs$$_{4}$$Sb$$_{12}$$. The isomer shifts obtained demonstrate that the Sm valence states in these compounds are intermediate. Since the difference of the isomer shifts in 22.502 keV $$^{149}$$Sm M$"{o}$ssbauer effect between Sm$$^{2+}$$ and Sm$$^{3+}$$ state is comparable to the 2nd order Doppler shift, consideration of the 2nd order Doppler shift is required to precisely discuss Sm valence state through the shifts of the M$"{o}$ssbauer spectra. In addition, the plots of the isomer shifts obtained by the M$"{o}$ssbauer spectroscopy against the Sm valence states estimated from Sm L-edge X-ray absorption spectroscopy exhibit a linear correlation except for that in SmOs$$_4$$Sb$$_{12}$$. This implies that the origin of the intermediate valence state in SmOs$$_4$$Sb$$_{12}$$ differs from that in Sm$$Tr_2$$Al$$_{20}$$ ($$Tr$$ = Ti, V and Cr).

論文

Muon spin relaxation in mixed perovskite (LaAlO$$_3$$)$$_x$$(SrAl$$_{0.5}$$Ta$$_{0.5}$$O$$_3$$)$$_{1-x}$$ with $$xsimeq 0.3$$

伊藤 孝; 髭本 亘; 幸田 章宏*; 中村 惇平*; 下村 浩一郎*

Interactions (Internet), 245(1), p.25_1 - 25_7, 2024/12

We report on muon spin relaxation ($$mu^+$$SR) measurements in a mixed perovskite compound, (LaAlO$$_3$$)$$_{x}$$(SrAl$$_{0.5}$$Ta$$_{0.5}$$O$$_3$$)$$_{1-x}$$ with $$xsimeq 0.3$$ (LSAT), which is widely used as a single-crystalline substrate for thin film deposition. In zero applied field (ZF), muon depolarization due to the distribution of nuclear dipole fields was observed in the temperature range from 4 K to 270 K. Interestingly, $$mu^+$$SR time spectra in ZF maintained a Gaussian-like feature over the entire range, while the depolarization rate exhibited a monotonic decrease with increasing temperature. This behavior may be attributed to the thermally activated diffusion of muons between a few adjacent sites within a confined space of the angstrom scale, where the motionally averaged local field that each muon experiences can remain non-zero and result in maintaining the Gaussian-like line shape. The spatial distribution of electrostatic potential at lattice interstices evaluated via density functional theory calculations suggests that such a restriction of muon diffusion paths can be caused by the random distribution of cations with different nominal valences in the mixed perovskite lattice.

論文

$$^{149}$$Sm synchrotron-radiation-based M$"{o}$ssbauer and $$mu^+$$SR studies of Sm$$_3$$Ru$$_4$$Ge$$_{13}$$

筒井 智嗣; 伊藤 孝; 中村 仁*; 吉田 実生*; 小林 義男*; 依田 芳卓*; 中村 惇平*; 幸田 章宏*; 東中 隆二*; 青木 大*; et al.

Interactions (Internet), 245(1), p.55_1 - 55_9, 2024/12

$$^{149}$$Sm SR-based M$"{o}$ssbauer and muon spin relaxation ($$mu^+$$SR) spectroscopies have been applied to Sm$$_3$$Ru$$_4$$Ge$$_{13}$$. The temperature dependence of the $$^{149}$$Sm SR-based M$"{o}$ssbauer spectra in the paramagnetic state implies the presence of dynamical nuclear Zeeman and/or quadrupole interactions. The time differential $$mu^+$$SR spectra also exhibit a marked temperature dependence in the paramagnetic state, indicating the presence of magnetic fluctuation in Sm$$_3$$Ru$$_4$$Ge$$_{13}$$ at least. These results in the present work infer that the dynamical hyperfine interactions observed using the mutually complementary spectroscopic methods are connected with the mechanism of the heavy fermion behavior in Sm$$_3$$Ru$$_4$$Ge$$_{13}$$.

論文

Evaluation of analytical uncertainty in quantitative determination of elements; The Case of boron

墨田 岳大*; 大澤 崇人; Chiu, I.-H.; 池田 篤史

Analytica Chimica Acta, 1329, p.343256_1 - 343256_10, 2024/11

The uncertainty including accuracy and precision is the most vital factor that determines the overall quality of quantitative analysis. The objectives of this study are (1) to investigate the analytical uncertainty of a prompt gamma-ray analysis (PGA), a chemical interference-free method in principle, on the quantitative analysis of boron and (2) to evaluate the applicability of inductively coupled plasma optical emission spectrometry (ICP-OES), a common technique for quantitative elemental analysis including boron. PGA provided analytical quantity that is equivalent to the true quantity. The analytical uncertainty in both methods was adequately evaluated by comparing the results from PGA and ICP-OES for a series of boron-containing materials with different physical/chemical properties and the major sources of uncertainty in both methods are specified. The evaluation concept demonstrated in this study could be beneficial to a wide range of analytical chemistry.

論文

Magnetoelastic coupling for Fe-Ga thin films epitaxially grown on different substrates

Ding, H.*; 伊藤 啓太*; 遠藤 恭*; 高梨 弘毅; 関 剛斎*

Journal of Physics D; Applied Physics, 57(38), p.385002_1 - 385002_10, 2024/09

 被引用回数:0 パーセンタイル:0.00(Physics, Applied)

This paper reports the systematic study on the structure, magnetic properties and magnetoelastic properties for the Fe$$_{100-x}$$Ga$$_{x}$$ (001) thin films epitaxially grown on the different substrates of GaAs(001) and MgO(001) using the sputtering technique. The alloy composition dependence of effective magnetoelastic coupling coefficient B$$_{eff}$$ along the FeGa [110] direction indicated that the largest magnetoelastic coupling was obtained for the Fe-Ga layer with x = 30 grown on the MgO substrate. Considering the results of structural analysis and magnetization measurement, the different crystallite sizes depending on the kind of substrate may give rise to the different magnetoelastic coupling strengths between the Fe-Ga layers on the MgO and the GaAs. The magnetostriction along the FeGa [111] direction was also estimated with the assumption of plausible elastic property of Fe-Ga, and showed the values comparable to the reported value of bulk Fe-Ga. This means the large magnetostriction can be obtained even for the Fe-Ga thin films epitaxially grown not only on the GaAs(001) but also on the MgO(001). The findings in this work will give a guideline for designing spintronic applications with a Fe-Ga layer exhibiting a large magnetoelastic coupling.

論文

Chiral gauge field in fully spin-polarized magnetic Weyl semimetal with magnetic domain walls

小沢 耀弘*; 荒木 康史; 野村 健太郎*

Journal of the Physical Society of Japan, 93(9), p.094704_1 - 094704_9, 2024/09

 被引用回数:0 パーセンタイル:0.00(Physics, Multidisciplinary)

磁性ワイル半金属における磁化の変調は、運動量空間におけるワイル点位置のシフトを引き起こし、ワイルフェルミオンに対して実効的なカイラリティ依存のゲージ場として働く。本研究では、完全スピン偏極したワイル強磁性体Co$$_{3}$$Sn$$_{2}$$S$$_{2}$$において、このような磁化誘起カイラルゲージ場の効果を取り扱う。磁化と結合した積層カゴメ格子上で定義したCo$$_{3}$$Sn$$_{2}$$S$$_{2}$$の強束縛模型を用いて、運動量空間におけるワイル点の位置(カイラルゲージ場に相当)の磁化方向依存性を計算した。これを用いて、磁壁構造が存在する場合に、カイラルゲージ場の空間構造から生じるカイラル磁場を評価した。その結果磁壁存在下では、ワイルフェルミオンに対してランダウ量子化を強く引き起こすほどの、数百テスラという巨大なカイラル磁場が生じることが導出された。このような巨大カイラル磁場は、従来の磁性体スピントロニクスにおけるスピン起電力に相当する、磁壁の運動による電荷ポンピングを誘起することも予想される。

論文

Dramatic elastic response at the critical end point in UTe$$_2$$

Vali$v{s}$ka, M.*; Haidamak, T.*; Cabala, A.*; Posp$'i$$v{s}$il, J.*; Bastien, G.*; Sechovsk$'y$, V.*; Prokle$v{s}$ka, J.*; 柳澤 達也*; Opletal, P.; 酒井 宏典; et al.

Physical Review Materials (Internet), 8(9), p.094415_1 - 094415_9, 2024/09

 被引用回数:0

Elastic responses at the metamagnetic transition in UTe$$_2$$ are studied at high field. The elastic anomaly becomes the strongest at the critical-end-point. Similar behavior was also observed in another metamagnet UCoAl, suggesting a universal elastic response triggered by critical magnetic fluctuations.

論文

なぜ漆は真っ黒になるのか?; 日本の伝統技術を最先端科学技術へ

南川 卓也

化学, 79(8), p.48 - 52, 2024/08

漆は、耐水性・耐薬品性に優れた稀有な天然塗料である。生漆にごく微量の鉄を加えると、非常に美しい漆黒が作り出されることが古くから知られている。しかし現代でも漆の構造や反応はほとんど解明されておらず、鉄を加えると何故黒色になるかも明らかにされていない。本研究では、黒漆が黒色になる原因を性質の異なる量子ビームを用いることで分析した。その結果、黒漆は生漆と全く違うナノ構造を持ち、その構造の違いで色が変化することが明らかになった。この結果は、長年にわたって謎であった漆膜の構造解析が初めて成功した結果である。本解説では、この研究を解説するとともに、化学系の大学生を対象にしているため、この研究がどのように進められてきたのかなども説明するものである。

論文

スピン軌道相互作用による創発インダクタンス

家田 淳一; 荒木 康史; 山根 結太*

固体物理, 59(8), p.403 - 410, 2024/08

In recent years, "emergent inductors" using current-induced magnetization dynamics in magnetic nanostructures have been discovered, opening the way to power control in the nanoscale, which was previously impossible. We review the spin-orbit interaction phenomenon for emergent inductors.

論文

Octupolar edge state in an $$e_g$$ orbital system on a square lattice

久保 勝規

Physical Review B, 110(7), p.075110_1 - 075110_7, 2024/08

 被引用回数:0 パーセンタイル:0.00(Materials Science, Multidisciplinary)

A tight-binding model for $$e_g$$ orbitals on a square lattice is investigated. We consider only the nearest-neighbor hopping and the model is characterized by two hopping parameters, $$t_1$$ and $$t_2$$. There are Dirac points in the electronic band structure and the type of the Dirac points (type-I or type-II) depends on the ratio $$t_2/t_1$$. For the case of the type-I Dirac points, edge states appear for a lattice with edges perpendicular to the $$[11]$$ direction. The edge states at a certain momentum along the edges have octupole moments with opposite signs between the right and left edges. Thus, these edge states can be called helical octupolar edge states. This study bridges the research fields of topological phenomena and multipole physics.

論文

Nuclear structure properties of $$^{193-200}$$Hg isotopes within large-scale shell model calculations

Sahoo, S.*; Srivastava, P. C.*; 清水 則孝*; 宇都野 穣

Physical Review C, 110(2), p.024306_1 - 024306_16, 2024/08

 被引用回数:0 パーセンタイル:0.00(Physics, Nuclear)

G行列をもとにした有効相互作用であるKHEE相互作用を用いて、$$^{193-200}$$Hgの低励起状態の殻模型計算を行った。偶偶核の$$8^+$$$$10^+$$$$12^+$$の励起エネルギーが近いことなど、イラスト状態のエネルギー準位をよく再現した。また、$$2^+$$の電気四重極モーメントが正の値であることも再現し、オブレート変形していることを確かめた。イラスト状態間の$$E2$$遷移が一部強く抑制されているという現象について調べ、配位の変化によるものであることを示した。

論文

Reevaluation of structures in $$^{70}$$Se from combined conversion-electron and $$gamma$$-ray spectroscopy

Smallcombe, J.; Garnsworthy, A. B.*; Korten, W.*; Singh, P.*; Muir, D.*; Pr$'o$chniak, L.*; Ali, F. A.*; Andreoiu, C.*; Ansari, S.*; Ball, G. C.*; et al.

Physical Review C, 110(2), p.024318_1 - 024318_16, 2024/08

 被引用回数:0 パーセンタイル:0.00(Physics, Nuclear)

In the selenium isotopes various shape phenomena are present, in particular the emergence of a dominant oblate deformation in the most neutron-deficient isotopes has been observed. The scenario of shape coexisting oblate and prolate bands has been proposed across the isotopic chain, with the crossing point of such bands being located near $$^{70}$$Se, where no coexistence has yet been identified. To determine the presence or absence of any low-lying $$0^+$$ state in $$^{70}$$Se, confirm the level structure, and interpret the nuclear deformation with theoretical models. A combined internal conversion electron and $$gamma$$-ray spectroscopy study was undertaken with the SPICE and TIGRESS spectrometers at the TRIUMF-ISAC-II facility. Nuclear models were provided by the Generalised Triaxial Rotor Model (GTRM) and the collective Generalised Bohr Hamiltonian (GBH). Despite a comprehensive search, no evidence was found for the existence of a $$0^+$$ state below 2 MeV in $$^{70}$$Se. Significant discrepancies to the previously established positive parity level scheme were found. GBH calculations using UNEDF1 mass parameters were found to reproduce the revised low-lying level structure well. $$^{70}$$Se does not have a well defined axial shape. The 2$$_2^{+}$$ state at 1601 keV resembles a quasi-$$gamma$$ excitation rather than a member of a shape coexisting band; the presence of such a band is all but ruled out.

論文

Magnonic $$varphi$$ Josephson junctions and synchronized precession

仲田 光樹; Zou, J.*; Klinovaja, J.*; Loss, D.*

Physical Review Research (Internet), 6(3), p.033207_1 - 033207_11, 2024/08

We uncover theoretically that a surprisingly rich dynamics can emerge in magnetic junctions due to intrinsic non-local damping, using analytical and numerical methods. In particular, under microwave pumping, we show that coherent spin precession in the right and left insulating ferromagnet (FM) of the junction becomes synchronized by non-local damping and thereby a magnonic analog of the $$varphi$$ Josephson junction emerges, where $$varphi$$ stands here for the relative precession phase of right and left FM in the stationary limit. Remarkably, $$varphi$$ decreases monotonically from $$ pi$$ to $$pi/2$$ as the magnon-magnon interaction, arising from spin anisotropies, increases. Moreover, we also find a magnonic diode effect giving rise to rectification of magnon currents. Our predictions are readily testable with current device and measurement technologies at room temperatures.

論文

Spectroscopy of deeply bound orbitals in neutron-rich Ca isotopes

Li, P. J.*; 宇都野 穣; 吉田 数貴; 他85名*

Physics Letters B, 855, p.138828_1 - 138828_11, 2024/08

 被引用回数:0 パーセンタイル:0.00(Astronomy & Astrophysics)

We report on the first measurement of unbound states in $$^{53}$$Ca and $$^{55}$$Ca, populated from $$^{54,56}$$Ca$$(p,pn)$$ reactions. Orbital angular momentum $$l$$ assignments were extracted from momentum distributions calculated with the distorted wave impulse approximation (DWIA). The resonances at 5516(41) keV in $$^{53}$$Ca and 6000(250) keV in $$^{55}$$Ca indicate a significant $$l$$ = 3 component, providing the first experimental evidence for the $$nu 0f_{7/2}$$ single-particle strength of unbound hole states in the neutron-rich Ca isotopes. The observed excitation energies and cross-sections point towards extremely localized and well separated strength distributions, with some fragmentation for the $$nu 0f_{7/2}$$ orbital in $$^{55}$$Ca. These results are in good agreement with predictions from shell-model calculations using the effective GXPF1Bs interaction and ab initio calculations and diverge markedly from the experimental distributions in the nickel isotones at Z = 28.

論文

Development of a non-destructive carbon quantification method in iron by negative muon lifetime measurement

二宮 和彦*; 久保 謙哉*; 稲垣 誠*; 吉田 剛*; 竹下 聡史*; 反保 元伸*; 下村 浩一郎*; 河村 成肇*; Strasser, P.*; 三宅 康博*; et al.

Journal of Radioanalytical and Nuclear Chemistry, 333(7), p.3445 - 3450, 2024/07

 被引用回数:0 パーセンタイル:0.00(Chemistry, Analytical)

A novel nondestructive light element analysis method for bulk materials using muon beams was demonstrated. This method is based on the lifetime measurement of muons in a material and performed by measuring muon-decay electrons and identifying elements using the atomic number based on muon lifetimes. Muon irradiation on pure iron and two steel samples with known carbon contents was conducted to prepare a calibration curve for the quantitative analysis. We also performed a muon lifetime measurement for a Japanese sword and successfully determined its carbon content as 0.51 wt% using the calibration curve, without sample destruction.

論文

Single-shot laser-driven neutron resonance spectroscopy for temperature profiling

Lan, Z.*; 有川 安信*; Mirfayzi, S. R.*; Morace, A.*; 早川 岳人*; 佐藤 博隆*; 加美山 隆*; Wei, T.*; 巽 湧太*; 小泉 光生; et al.

Nature Communications (Internet), 15, p.5365_1 - 5365_7, 2024/07

The temperature measurement of material inside of an object is one of the key technologies for control of dynamical processes. For this purpose, various techniques such as laser-based thermography and phase-contrast imaging thermography have been studied. However, it is, in principle, impossible to measure the temperature of an element inside of an object using these techniques. One of the possible solutions is measurements of Doppler brooding effect in neutron resonance absorption (NRA). Here we present a method to measure the temperature of an element or an isotope inside of an object using NRA with a single neutron pulse of approximately 100 ns width provided from a high-power laser. We demonstrate temperature measurements of a tantalum (Ta) metallic foil heated from the room temperature up to 617 K. Although the neutron energy resolution is fluctuated from shot to shot, we obtain the temperature dependence of resonance Doppler broadening using a reference of a silver (Ag) foil kept to the room temperature. A free gas model well reproduces the results. This method enables element(isotope)-sensitive thermometry to detect the instantaneous temperature rise in dynamical processes.

論文

Room-temperature flexible manipulation of the quantum-metric structure in a topological chiral antiferromagnet

Han, J.*; 内村 友宏*; 荒木 康史; Yoon, J.-Y.*; 竹内 祐太郎*; 山根 結太*; 金井 駿*; 家田 淳一; 大野 英男*; 深見 俊輔*

Nature Physics, 20(7), p.1110 - 1117, 2024/07

 被引用回数:2 パーセンタイル:87.91(Physics, Multidisciplinary)

量子状態の幾何学的構造を特徴づける基礎的な量として、「量子計量」と「ベリー曲率」が存在する。ベリー曲率は、凝縮系において多種の重要な現象に寄与することが知られている。一方、量子計量も新たなトポロジカル物理現象の起源となることが予想されているが、特に常温常圧下においては、その効果はほとんど探索されていない。本研究では、トポロジカルカイラル反強磁性体Mn$$_{3}$$Snと白金の接合系を用い、界面でのナノスピン構造を介して、電子系の量子計量構造の制御に成功した。ベリー曲率ではなく量子計量特有の効果として、時間反転反対称でかつ電子散乱に対して頑強な、二次非線形ホール効果を測定した。更に、界面スピン構造は弱磁場及び界面スピン軌道相互作用によって急峻に変調されるため、量子計量構造も鋭敏に制御可能であることを示した。本研究成果により、量子状態に内在する量子計量構造を活用したトポロジカル物理現象が室温環境下でも可能になり、且つ応用面においても非線形素子を構築する助けとなることが期待される。

論文

Theory of the inverse Rashba-Edelstein effect induced by thermal spin injection

細川 海慈*; 山 正樹*; 松尾 衛; 加藤 岳生*

Physical Review B, 110(3), p.035309_1 - 035309_12, 2024/07

 被引用回数:0 パーセンタイル:0.00(Materials Science, Multidisciplinary)

Our result provides an important foundation for an accurate analysis of the inverse Rashba-Edelstein effect induced by thermal spin injection.

論文

Significance of the refraction effect on the $$p-d$$ elementary process in the ($$p,pd$$) reaction

吉田 数貴; 茶園 亮樹*; 緒方 一介*

Physical Review C, 110(1), p.014617_1 - 014617_9, 2024/07

 被引用回数:0 パーセンタイル:0.00(Physics, Nuclear)

In the present work, we investigate the deuteron refraction effect in the exclusive ($$p,pd$$) reactions. The refraction effect on the $$p-d$$ elementary process is taken into account by the local semiclassical approximation to the distorted waves. The results are compared with those obtained with the asymptotic momentum approximation, which is standardly applied to the distorted wave impulse approximation framework. It is shown that the refraction effect drastically changes the energy sharing distribution of the $$^{16}$$O($$p,pd$$)$$^{14}$$N reaction at 101.3 MeV and gives a better agreement with experimental data.

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