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Journal Articles

Hot cell equipment improvement effortsat Analytical Laboratory in Tokai Reprocessing Plant

Ishibashi, Atsushi; Masui, Kenji; Goto, Yuichi; Yamamoto, Masahiko; Taguchi, Shigeo; Ishikawa, Satoshi*; Ishikawa, Tomoya*

Nihon Hozen Gakkai Dai-19-Kai Gakujutsu Koenkai Yoshishu, p.18 - 21, 2023/08

An inner-box typed hot cell for analysis of highly radioactive samples has been operated for about 40 years in Tokai Reprocessing Plant since its installation in 1980. During the operation of analytical hot cell, improvement and upgrades including auxiliary equipment have been performed, in addition to keep the equipment in proper condition through periodic inspections and maintenance. This paper describes about these efforts for analytical hot cell and its results.

Journal Articles

Development of a local exhaust device for removal of radioactive waste from glove-box for handling nuclear fuel materials

Ishibashi, Atsushi; Saegusa, Yu; Aoya, Juri; Yamamoto, Masahiko; Taguchi, Shigeo; Kuno, Takehiko

Nihon Hozen Gakkai Dai-18-Kai Gakujutsu Koenkai Yoshishu, p.241 - 244, 2022/07

no abstracts in English

Journal Articles

Fast nuclear-spin conversion of H$$_{2}$$ trapped and polarized in a CO$$_{2}$$ matrix

Yamakawa, Koichiro; Ishibashi, Atsuki*; Namiyoshi, Toshinobu*; Azuma, Yuichi*; Arakawa, Ichiro*

Physical Review B, 102(4), p.041401_1 - 041401_5, 2020/07

 Times Cited Count:2 Percentile:12.54(Materials Science, Multidisciplinary)

JAEA Reports

Report on analytical activities in potentially hazardous materials mitigation measures at the Plutonium Conversion Development Facility; 2015.12 $$sim$$ 2016.10

Horigome, Kazushi; Taguchi, Shigeo; Ishibashi, Atsushi; Inada, Satoshi; Kuno, Takehiko; Surugaya, Naoki

JAEA-Technology 2017-008, 14 Pages, 2017/05

JAEA-Technology-2017-008.pdf:1.15MB

The plutonium solution had been converted into MOX powder to mitigate the potential hazards of storage plutonium solution such as hydrogen generation at the Plutonium Conversion Development Facility. The plutonium conversion operations had been started in April, 2014, and had been finished in July, 2016. With respect to the samples taken from the conversion process, about 2,200 items of plutonium/uranium solutions and MOX powders had been analyzed for the operation control in the related analytical laboratories at the Tokai Reprocessing Plant. This paper describes the reports on analytical activities and related maintenance works in the analytical laboratories conducted from December, 2015 to October, 2016.

JAEA Reports

Report on analytical activities in potentially hazardous materials mitigation measures at the Plutonium Conversion Development Facility; 2014.4 $$sim$$ 2015.12

Horigome, Kazushi; Suzuki, Hisanori; Suzuki, Yoshimasa; Ishibashi, Atsushi; Taguchi, Shigeo; Inada, Satoshi; Kuno, Takehiko; Surugaya, Naoki

JAEA-Technology 2016-026, 21 Pages, 2016/12

JAEA-Technology-2016-026.pdf:1.14MB

In order to mitigate potential hazards of storage plutonium in solution such as hydrogen generation, conversion of plutonium solution into MOX powder has been carried out since 2014 in the Plutonium Conversion Development Facility. With respect to the samples taken from the conversion process, about 3500 items of plutonium/uranium solutions and MOX powders have been analyzed for the operation control in the related analytical laboratories at the Tokai Reprocessing Plant. This paper describes the reports on analytical activities and related maintenance works in the analytical laboratories conducted from April 2014 to December 2015.

Journal Articles

Maintenance experiences at analytical laboratory at the Tokai Reprocessing Plant

Suzuki, Hisanori; Nagayama, Tetsuya; Horigome, Kazushi; Ishibashi, Atsushi; Kitao, Takahiko; Surugaya, Naoki

Nihon Hozen Gakkai Dai-11-Kai Gakujutsu Koenkai Yoshishu, p.214 - 219, 2014/07

The Tokai Reprocessing Plant (TRP) is developing the technology to recover uranium and plutonium from spent nuclear fuel. There is an analytical laboratory which was built in 1978, as one of the most important facilities for process and material control analyses at the TRP. Samples taken from each process are analyzed by various analytical methods using hot cells, glove boxes and hume-hoods. A large number of maintenance work have been so far done and different types of experience have been accumulated. This paper describes our achievements in the maintenance activities at the analytical laboratory at the TRP.

Journal Articles

Mass production of Nb$$_{3}$$Sn conductors for ITER toroidal field coils in Japan

Takahashi, Yoshikazu; Isono, Takaaki; Hamada, Kazuya; Nunoya, Yoshihiko; Nabara, Yoshihiro; Matsui, Kunihiro; Hemmi, Tsutomu; Kawano, Katsumi; Koizumi, Norikiyo; Oshikiri, Masayuki; et al.

IEEE Transactions on Applied Superconductivity, 22(3), p.4801904_1 - 4801904_4, 2012/06

 Times Cited Count:7 Percentile:41.31(Engineering, Electrical & Electronic)

Japan Atomic Energy Agency is the first to start the mass production of the TF conductors in Phase IV in March 2010 among the 6 parties who are procuring TF conductors in the ITER project. The conductor is cable-in-conduit conductor with a central spiral. A total of 900 Nb$$_{3}$$Sn strands and 522 copper strands are cabled around the central spiral and then wrapped with stainless steel tape whose thickness is 0.1 mm. Approximately 60 tons of Nb$$_{3}$$Sn strands were manufactured by the two suppliers in December 2010. This amount corresponds to approximately 55% of the total contribution from Japan. Approximately 30% of the total contribution from Japan was completed as of February 2011. JAEA is manufacturing one conductor per month under a contract with two Japanese companies for strands, one company for cabling and one company for jacketing. This paper summarizes the technical developments including a high-level quality assurance. This progress is a significant step in the construction of the ITER machine.

Journal Articles

XUV-FEL spectroscopy; He two-photon ionization cross-sections

Sato, Takahiro*; Iwasaki, Atsushi*; Ishibashi, Kazuki*; Okino, Tomoya*; Yamanouchi, Kaoru*; Adachi, Junichi*; Yagishita, Akira*; Yazawa, Hiroki*; Kannari, Fumihiko*; Aoyama, Makoto; et al.

Europhysics News, 42(5), P. 10, 2011/09

The resonant and non-resonant two-photon single ionization processes of He were investigated using intense free electron laser light in the extreme ultraviolet (XUV) region (53.4-61.4 nm) covering the 1s-2p and 1s-3p resonant transitions of He. On the basis of the dependences of the yield of He$$^{+}$$ on the XUV light-field intensity at 53.4, 58.4, 56.0 and 61.4 nm, the absolute values of the two-photon ionization cross sections of He at the four different wavelengths and their dependence on the light-field intensity were determined for the first time.

Journal Articles

Determination of the absolute two-photon ionization cross section of He by an XUV free electron laser

Sato, Takahiro*; Iwasaki, Atsushi*; Ishibashi, Kazuki*; Okino, Tomoya*; Yamanouchi, Kaoru*; Adachi, Junichi*; Yagishita, Akira*; Yazawa, Hiroki*; Kannari, Fumihiko*; Aoyama, Makoto; et al.

Journal of Physics B; Atomic, Molecular and Optical Physics, 44(16), p.161001_1 - 161001_5, 2011/08

 Times Cited Count:36 Percentile:83.28(Optics)

The resonant and non-resonant two-photon single ionization processes of He were investigated using intense free electron laser light in the extreme ultraviolet (XUV) region (53.4-61.4 nm) covering the 1s-2p and 1s-3p resonant transitions of He. On the basis of the dependences of the yield of He$$^{+}$$ on the XUV light-field intensity at 53.4, 58.4, 56.0 and 61.4 nm, the absolute values of the two-photon ionization cross sections of He at the four different wavelengths and their dependence on the light-field intensity were determined for the first time.

JAEA Reports

Precise and accurate determination of plutonium by controlled-potential coulometry and its uncertainty evaluation

Yamamoto, Masahiko; Ishibashi, Atsushi; Nagayama, Tetsuya; Surugaya, Naoki; Kurosawa, Akira; Hiyama, Toshiaki

JAEA-Technology 2010-040, 28 Pages, 2010/12

JAEA-Technology-2010-040.pdf:0.97MB

Precise analysis of plutonium is necessary for material control and safeguards in nuclear facility. Thus, controlled-potential coulometry, which yields absolute results and high precision, was applied for the determination of plutonium. The coulometry system and sample pretreatment procedures were optimized following ISO12183:2005. Plutonium sample prepared from NBL CRM-126 Pu metal was measured and agreed well with certified value. For spike preparation of isotope dilution mass spectrometry (IDMS), plutonium solution was prepared from MOX powder. Plutonium content was 15.5995 mgPu/g. The uncertainty was calculated by ISO/BIPM Guide to the Expression of Uncertainties in Measurements. The relative expanded uncertainty was 0.023% with confidence interval of 95%. The results were in good agreement with those obtained by IDMS. Thus the proposed coulometry method was successfully applied for the determination of plutonium at the highest level of precision and accuracy.

Journal Articles

Development of a TES microcalorimeter for spectroscopic measurement of LX-rays emitted by transuranium elements

Maehata, Keisuke*; Nakamura, Keisuke*; Yasumune, Takashi*; Ishibashi, Kenji*; Takasaki, Koji; Tanaka, Keiichi*; Odawara, Akikazu*; Nagata, Atsushi*

Journal of Nuclear Science and Technology, 47(3), p.308 - 313, 2010/03

 Times Cited Count:5 Percentile:35.66(Nuclear Science & Technology)

A phase transition edge sensor (TES) microcalorimeter was developed for the energy dispersive measurement of LX-ray photons emitted from transuranium elements. The phase transition temperature of the TES was designed to be 200 mK by using bilayer structure of Au of 120 nm thick and Ti of 50 nm thick. The Au layer of 5.0 $$mu$$m thick was deposited on the Au/Ti bilayer for absorption efficiency of 50% and counting rate of 100 counts per second in the detection of LX-ray photons with the energy from 10 to 20 keV. The TES microcalorimeter was operated for the detection of LX-ray photons emitted from $$^{241}$$Am, $$^{238}$$Pu and $$^{239}$$Pu sources. The decay time constant of 180 $$mu$$s of detection signal pulses allowed the TES microcalorimeter operating with the counting rate higher than 100 counts per second. The energy resolution was obtained to be 50 eV of FWHM value for a peak corresponding to $$^{237}$$Np L$$beta$$$$_{1}$$ X-ray of 17.75 keV.

Journal Articles

Determination of Plutonium in High Active Liquid Waste by Spectrophotometry using Dysprosium as an Internal Standard

Kitao, Takahiko; Jitsukata, Shu*; Sato, Soichi; Ikeda, Hisashi ; Atsushi, Ishibashi,; Surugaya, Naoki

SYMPOSIUM ON SAFEGUARDS AND NUCLEAR MATERIAL MANAGEMENT, 0 Pages, 2001/00

None

Oral presentation

Measurement technology for safeguards analysis at the Tokai reprocessing plant

Yamamoto, Masahiko; Surugaya, Naoki; Taguchi, Shigeo; Ishibashi, Atsushi; Horigome, Kazushi; Yamazaki, Hitoshi; Ogura, Hiroshi; Watahiki, Hiromi; Watanabe, Masahisa; Kurosawa, Akira; et al.

no journal, , 

no abstracts in English

Oral presentation

Precise determination of plutonium by controlled-potential coulometry and its uncertainty estimation

Yamamoto, Masahiko; Ishibashi, Atsushi; Nagayama, Tetsuya; Surugaya, Naoki; Kurosawa, Akira

no journal, , 

no abstracts in English

Oral presentation

Training of chemical analysis technique of radioactive materials in actual field

Masaki, Yuji*; Miyauchi, Hironari*; Taguchi, Shigeo; Horigome, Kazushi; Ishibashi, Atsushi; Yamamoto, Masahiko; Masui, Kenji; Nishida, Naoki; Kuno, Takehiko; Surugaya, Naoki

no journal, , 

Reprocess the technology development center has longtime experience for the handling of the radiation and perform support aiming at the acquisition of the spot analysis technique about the radioactive nuclear material handling in response to a demand out of the mechanism.

Oral presentation

Nuclear spin conversion of H$$_2$$ trapped in solid CO$$_2$$

Yamakawa, Koichiro; Namiyoshi, Toshinobu*; Ishibashi, Atsuki*; Arakawa, Ichiro*

no journal, , 

We detected weak infrared absorption by H$$_{2}$$ trapped and polarized in solid CO$$_{2}$$ and evaluated the strength of the local electric field just in the solid. By analyzing the time evolution of the spectrum, we determined the conversion rates of H$$_{2}$$ to examine the effect of the electric field on the conversion.

Oral presentation

Nuclear spin conversion of hydrogen trapped in condensed layers of carbon dioxide

Yamakawa, Koichiro; Ishibashi, Atsuki*; Namiyoshi, Toshinobu*; Arakawa, Ichiro*

no journal, , 

The mechanism of the interconvertion between the nuclear spin isomers has been attracted much interest recently. In the present work, we detected the weak infrared absorption by hydrogen molecules polarized in the condensed layers of carbon dioxide and measured the rate of the nuclear spin conversion to discuss its mechanism.

17 (Records 1-17 displayed on this page)
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