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排気中$$^{14}$$Cモニタリング手法の検証(再評価)と高度化への提言

Re-Evaluation of a Method for Monitoring Airborne$$^{14}$$C Discharge and its Contribution to Development of an Advanced Method

小嵐 淳   ; 井坂 圭輔*; 横田 友和*; 小沢 友康*; 三上 智   ; 秋山 聖光; 小林 博英 

Koarashi, Jun; Isaka, Keisuke*; Yokota, Tomokazu*; Kozawa, Tomoyasu*; Mikami, Satoshi; Akiyama, Kiyomitsu; Kobayashi, Hirohide

より安定で信頼性が高く、効率的な排気中$$^{14}$$Cのモニタリング手法を確立することを目的として、現在東海再処理施設で実施しているモニタリング手法の基礎となる捕集・測定技術および放出評価法に関する試験・検討を行った。得られた結果に基づいてモニタリング手法を再評価し、現在のモニタリング手法の妥当性を検証するとともに、手法の高度化へ向けた技術的要件を提示した。

Some investigations were made for re-evaluating collection and measurement techniques in an airborne $$^{14}$$C discharge monitoring at the Tokai reprocessing plant (TRP), which include (1)collection efficiency of CO$$_{2}$$ in a carbon sampler using monoethanolamine as CO$$_{2}$$ absorbent;(2)affect of incorporating tritiated water into the carbon sampler on quantitative estimation of $$^{14}$$C activity in airborne effluent; (3)affect of leakage in air sampling on evaluating airborne $$^{14}$$C discharge; and (4)determination of chemical forms of $$^{14}$$C in airborne release from the TRP. The results presented not only the validity of the TRP's monitoring method, but also the technical aspects required for establishing a more reliable and effective monitoring method.

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