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Novel critical behavior of magnetization in URhSi; Similarities to the uranium ferromagnetic superconductors UGe$$_2$$ and URhGe

URhSiの新奇な磁気臨界現象; ウラン系強磁性超伝導物質UGe$$_2$$とURhGeとの類似性

立岩 尚之; 芳賀 芳範; 山本 悦嗣

Tateiwa, Naoyuki; Haga, Yoshinori; Yamamoto, Etsuji

ウラン系強磁性物質URhSiについて、強磁性転移温度$$T_{rm C}$$近辺で磁気測定を行い、臨界現象の研究を行った。自発磁化の温度依存に関する臨界指数$$beta$$、磁化率の指数$$gamma$$$$T_{rm C}$$における磁化に関する指数$$delta$$を、修正アロットプロットとスケーリング理論等を用いて決定した。URhSiの強磁性状態は一軸磁気異方性が大きいものの、臨界指数は三次元イジングモデルから期待されるもの($$beta$$ = 0.325, $$gamma$$ = 1.241, and $$delta$$ = 4.82)とは異なることが明らかにされた。URhSiの臨界指数($$beta$$ = 0.300 $$pm$$ 0.002, $$gamma$$ = 1.00 $$pm$$ 0.02, and $$delta$$ = 4.32 $$pm$$ 0.04)は、ウラン系強磁性超伝導物質UGe$$_2$$とURhGeと類似している。URhSiの静的磁性と動的磁性をウラン系強磁性超伝導物質と対比させ議論する。

We study the critical behavior of dc magnetization in the uranium ferromagnet URhSi around the ferromagnetic phase transition at $$T_{rm C}{,}{sim}{,}$$10 K. The critical exponent $$beta$$ for the spontaneous magnetization below $$T_{rm C}$$, $$gamma$$ for the magnetic susceptibility, and $$delta$$ for the magnetic isotherm at $$T_{rm C}$$ have been determined as $$beta$$ = 0.300 $$pm$$ 0.002, $$gamma$$ = 1.00 $$pm$$ 0.02, and $$delta$$ = 4.32 $$pm$$ 0.04 by the scaling analysis and the critical isotherm analysis. Magnetization has strong uniaxial magnetic anisotropy in the ferromagnetic state of URhSi. However, the universality class of the critical phenomenon does not belong to the 3D Ising system ($$beta$$ = 0.325, $$gamma$$ = 1.241, and $$delta$$ = 4.82). The obtained exponents in URhSi are similar to those in uranium ferromagnetic superconductors UGe$$_2$$ and URhGe. We discuss the static and dynamical magnetic properties of URhSi in comparison with those in UGe$$_2$$, URhGe and UCoGe.

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パーセンタイル:100

分野:Materials Science, Multidisciplinary

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