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Gu, G. H.*; Jeong, S. G.*; Heo, Y.-U.*; Harjo, S.; Gong, W.; Cho, J.*; Kim, H. S.*; 他4名*
Journal of Materials Science & Technology, 223, p.308 - 324, 2025/07
被引用回数:0 パーセンタイル:0.00(Materials Science, Multidisciplinary)Face-centered cubic (FCC) equi-atomic multi-principal element alloys (MPEAs) exhibit excellent mechanical properties from cryogenic to room temperatures. At room temperature, deformation is dominated by dislocation slip, while at cryogenic temperatures (CTs), reduced stacking fault energy enhances strain hardening with twinning. This study uses in-situ neutron diffraction to analyze the temperature-dependent deformation behavior of Al(CoNiV)
, a dual-phase (FCC/BCC) medium-entropy alloy (MEA). At liquid nitrogen temperature (LNT), deformation twinning in the FCC matrix leads to additional strain hardening through the dynamic Hall-Petch effect, giving the appearance of improved strengthening at LNT. In contrast, BCC precipitates show dislocation slip at both 77 K and 298 K, with temperature-dependent lattice friction stress playing a significant role in strengthening. The study enhances understanding of deformation behaviors and provides insights for future alloy design.
杉田 裕; 大野 宏和; Beese, S.*; Pan, P.*; Kim, M.*; Lee, C.*; Jove-Colon, C.*; Lopez, C. M.*; Liang, S.-Y.*
Geomechanics for Energy and the Environment, 42, p.100668_1 - 100668_21, 2025/06
国際共同プロジェクトDECOVALEX-2023は、数値解析を使用してベントナイト系人工バリアの熱-水-応力(または熱-水)相互作用を研究するためのタスクDとして、幌延人工バリア性能確認試験を対象とした。このタスクは、モデル化のために、1つの実物大の原位置試験と、補完的な4つの室内試験が選択された。幌延人工バリア性能確認試験は、人工的な地下水注入と組み合わせた温度制御非等温の試験であり、加熱フェーズと冷却フェーズで構成されている。6つの研究チームが、さまざまなコンピューターコード、定式化、構成法則を使用して、熱-水-応力または熱-水(研究チームのアプローチによって異なる)数値解析を実行した。
Go, G.*; Goli, D. P.*; 江崎 蘭世; Tserkovnyak, Y.*; Kim, S. K.*
Physical Review Research (Internet), 7(2), p.L022066_1 - L022066_7, 2025/06
It remains an open question whether or not the scalar spin chirality itself can exhibit a Hall-type transport. In this work, we show that the answer is yes: The scalar spin chirality is Hall-transported in Kagome ferromagnets and antiferromagnets under an external bias, engendering a phenomenon which we dub the scalar spin chirality Nernst effect. Our findings call for the need to lift the conventional assumption that the scalar spin chirality is a static quantity in order to discover the active roles of the scalar spin chirality in transport properties.
川崎 卓郎; 福田 竜生; 山中 暁*; 村山 一郎*; 加藤 孝典*; 馬場 将亮*; 橋本 英樹*; Harjo, S.; 相澤 一也; 田中 裕久*; et al.
Journal of Applied Physics, 137(9), p.094101_1 - 094101_7, 2025/03
被引用回数:0 パーセンタイル:0.00(Physics, Applied)Energy harvesting from waste heat can improve energy efficiency in society. This research investigated the structural behaviors of lead zirconate titanate-based ferroelectric ceramics using operando neutron diffraction measurements under the conditions of two energy-harvesting cycles that involve consideration of the temperature changes of automobile exhaust gas for achieving good harvesting efficiencies. Input and output electrical energies and neutron diffraction data were simultaneously collected. The obtained time-resolved neutron-diffraction intensity data indicate that the applied electric fields and temperature changes induced 90 domain rotation and lattice strain. These structural changes and their variations depending on cycle conditions, such as temperature changes, applied electric fields, and circuit switching, provide insight into the origins of the differences in the behaviors of electrical input/output energies in the cycles.
Cho, S. H.*; Cho, S. W.*; Lv, Z.*; 関根 由莉奈; Liu, S.*; Zhou, M.*; Nuxoll, R. F.*; Kanatzidis, E. E.*; Ghaffari, R.*; Kim, D.*; et al.
Lab on a Chip, 9 Pages, 2025/00
被引用回数:0 パーセンタイル:0.00(Biochemical Research Methods)アミノ酸は体内のタンパク質合成と代謝プロセスに不可欠な物質である。本研究では、運動中の汗からのアミノ酸損失について定量的に調べることを目的とした。汗中のアミノ酸含有量をリアルタイムで分析するため、測定のための技術基盤としてウェアラブルなマイクロ流体システムを構築した。定量分析を実現するため、ウェアラブルデバイスに蛍光アッセイを組み込み、さらにスマートフォンベースの画像化技術を統合させたシステムを開発した。
Sarenac, D.*; Gorbet, G.*; Clark, C. W.*; Cory, D. G.*; Ekinci, H.*; Henderson, M. E.*; Huber, M. G.*; Hussey, D. S.*; Kapahi, C.*; Kienzle, P. A.*; et al.
Physical Review Research (Internet), 6(3), p.L032054_1 - L032054_8, 2024/09
Neutron interferometry has played a distinctive role in fundamental science and characterization of materials. Moir neutron interferometers are candidate next-generation instruments: they offer microscopy-like magnification of the signal, enabling direct camera recording of interference patterns across the full neutron wavelength spectrum. Here we demonstrate the extension of phase-grating moir
interferometry to two-dimensional geometries. Our measurements of phase topologies and gravitationally induced phase shifts are in good agreement with theory.
Nguyen, T.-D.*; Singh, C.*; Kim, Y. S.*; Han, J. H.*; Lee, D.-H.*; Lee, K.*; Harjo, S.; Lee, S. Y.*
Journal of Materials Research and Technology, 31, p.1547 - 1556, 2024/07
被引用回数:3 パーセンタイル:41.92(Materials Science, Multidisciplinary)This study investigates the mechanical properties of a friction-stir-welded (FSW) AA6061-T6 aluminum alloy at ultra-low temperature (ULT) of 20 K. In-situ neutron diffraction and orientation imaging microscopy were employed to compare the tensile deformation behavior of the base metal (BM) and heat-affected zone (HAZ) in the FSW aluminum plate. The results demonstrate that compared to room-temperature (RT), ULT induces a significant improvement in tensile strength and ductility in both the BM and HAZ. The enhanced mechanical properties in BM at ULT result from a more homogeneous deformation than occurs at RT. On the other hand, HAZ at ULT exhibits an even lower yield strength than at RT, but the strain hardening rate (SHR) is the most significant among the alloys, leading to a tensile strength of 346 MPa and the highest ductility of 46.8%. The lowest yield strength corresponds to the lowest-hardness zones in HAZ, caused by dissolved/coarsened precipitates during the FSW process.
Kim, Y. S.*; Chae, H.*; Lee, D.-Y.*; Han, J. H.*; Hong, S.-K.*; Na, Y. S.*; Harjo, S.; 川崎 卓郎; Woo, W.*; Lee, S.-Y.*
Materials Science & Engineering A, 899, p.146453_1 - 146453_7, 2024/05
被引用回数:4 パーセンタイル:63.37(Nanoscience & Nanotechnology)This work focused on the mechanical properties and serration-involved deformation behavior of advanced alloys at 15 K. Evolution of stacking faults and -martensite improved the mechanical performance of CoCrNi alloys, and significant strain-induced martensite transformation of DED-SS316L led to superior strength and strain hardening. A magnitude in stress drop was governed by dislocation density, phase type, and lattice defects, irrespective of processing method. FCC {200} notably was influenced recovery behavior after stress drop, and the contribution of strain energy density by serration on tensile toughness was the greatest for HR-CoCrNi.
大沢 直樹*; Kim, S.-Y.*; 久保田 真彦*; Wu, H.*; 渡部 創; 伊藤 辰也; 永石 隆二
Nuclear Engineering and Technology, 56(3), p.812 - 818, 2024/03
被引用回数:2 パーセンタイル:57.00(Nuclear Science & Technology)An impregnated silica-based adsorbent was prepared by combining HONTA extractant, Crea extractant, and macroporous silica polymer composite particles (SiO-P). The performance of platinum-group metals adsorption and separation on prepared (HONTA + Crea)/SiO
-P adsorbent was assessed by batch-adsorption and chromatographic separation studies. (HONTA + Crea)/SiO
-P adsorbent showed high adsorption performance of Pd(II) owing to an affinity between Pd(II) and Crea extractant based on the Hard and Soft Acids and Bases theory. The chromatographic experiment showed that Pd(II) was recovered entirely from the feed solution using 0.2 M thiourea in 0.1 M HNO
. Possibility of recovery of Zr(IV), Mo(VI), and Re(VII) was also observed using the (HONTA + Crea)/SiO
-P adsorbent.
Linh, B. D.*; Corsi, A.*; Gillibert, A.*; Obertelli, A.*; Doornenbal, P.*; Barbieri, C.*; Duguet, T.*; Gmez-Ramos, M.*; Holt, J. D.*; Hu, B. S.*; et al.
Physical Review C, 109(3), p.034312_1 - 034312_15, 2024/03
被引用回数:2 パーセンタイル:58.81(Physics, Nuclear)理化学研究所RIビームファクトリーにて中性子過剰核Arビームからの1中性子ノックアウト反応実験を行い、
Arのエネルギー準位および分光学的因子を導出した。特に、第一励起状態の
への分光学的因子が大きいことから、始状態の
Arの基底状態において中性子が
軌道を多く占めていることがわかった。これは、中性子数32がよい魔法数として知られる
Caとは異なった性質であり、カルシウムからアルゴンへと陽子が2個減ることで閉殻構造が大きく崩れることが明らかになった。
Park, P.*; Cho, W.*; Kim, C.*; An, Y.*; Kang, Y.-G.*; Avdeev, M.*; Sibille, R.*; 飯田 一樹*; 梶本 亮一; Lee, K. H.*; et al.
Nature Communications (Internet), 14, p.8346_1 - 8346_9, 2023/12
被引用回数:21 パーセンタイル:84.93(Multidisciplinary Sciences)The triangular lattice antiferromagnet (TLAF) has been the standard paradigm of frustrated magnetism for several decades. The most common magnetic ordering in insulating TLAFs is the 120 structure. However, a new triple-
chiral ordering can emerge in metallic TLAFs, representing the short wavelength limit of magnetic skyrmion crystals. We report the metallic TLAF Co
TaS
as the first example of tetrahedral triple-
magnetic ordering with the associated topological Hall effect (non-zero
). We also present a theoretical framework that describes the emergence of this magnetic ground state, which is further supported by the electronic structure measured by angle-resolved photoemission spectroscopy. Additionally, our measurements of the inelastic neutron scattering cross section are consistent with the calculated dynamical structure factor of the tetrahedral triple-
state.
Yang, D. S.*; Wu, Y.*; Kanatzidis, E. E.*; Avila, R.*; Zhou, M.*; Bai, Y.*; Chen, S.*; 関根 由莉奈; Kim, J.*; Deng, Y.*; et al.
Materials Horizons, 10(11), p.4992 - 5003, 2023/09
被引用回数:12 パーセンタイル:79.80(Chemistry, Multidisciplinary)本論文では、ハード及びソフトハイブリッド材料システムでの3Dプリントによって形成されたマイクロ流体ネットワーク、統合バルブ、およびマイクロスケール光学キュベットにより、汗成分に対してその場で分光および蛍光分析した成果を紹介する。一連の試験により、これらのマイクロキュベットシステムが汗中の銅、塩化物、グルコースの濃度と汗のpHを実験室レベルの精度と感度で評価できることが実証された。
Chen, S.*; Browne, F.*; Doornenbal, P.*; Lee, J.*; Obertelli, A.*; 角田 佑介*; 大塚 孝治*; 茶園 亮樹*; Hagen, G.*; Holt, J. D.*; et al.
Physics Letters B, 843, p.138025_1 - 138025_7, 2023/08
被引用回数:9 パーセンタイル:85.35(Astronomy & Astrophysics)Scからの1陽子ノックアウト反応を用いて、
Caと
Caのガンマ崩壊を観測した。
Caでは1456(12)keVの
線遷移が、
Caでは1115(34)keVの遷移が観測された。どちらの遷移も暫定的に
と割り当てられた。有効核子間相互作用をわずかに修正した広い模型空間での殻模型計算では、
準位エネルギー、2中性子分離エネルギー、反応断面積が実験とよく一致し、N=34閉殻の上に新しい殻が形成されていることを裏付けた。その構成要素である
と
軌道はほぼ縮退しており、これは
Caが二重魔法核である可能性を排除し、Ca同位体のドリップラインを
Caあるいはそれ以上にまで広げる可能性がある。
Lind, T.*; Kalilainen, J.*; Marchetto, C.*; Beck, S.*; 中村 康一*; 木野 千晶*; 丸山 結; 城戸 健太朗; Kim, S. I.*; Lee, Y.*; et al.
Proceedings of 20th International Topical Meeting on Nuclear Reactor Thermal Hydraulics (NURETH-20) (Internet), p.4796 - 4809, 2023/08
The OECD/NEA ARC-F project was established to investigate the accidents at Fukushima Daiichi nuclear power station with the aim of consolidating the observations for deeper understanding of the severe accident progression and the status of reactors and containment vessels. Additionally, the project formed an information sharing framework in reactor safety between Japan and international experts. In order to achieve these objectives, the project focused on three tasks: i) to refine analysis for accident scenarios and associated fission-product transport and dispersion, ii) to compile and manage data on the Fukushima Daiichi NPS accident, and iii) to discuss future long-term projects relevant to the Fukushima Daiichi NPS accident. The work was carried out by 22 partners from 12 countries. In the fission product group, ten organizations worked on five topics which were ranked with a high significance as open issues based on the BSAF project and were thereby selected for further investigations. The five fission product related topics were: i) fission product speciation, ii) iodine chemistry, iii) pool scrubbing, iv) fission product transport and behavior in the buildings, and v) uncertainty analysis and variant calculations. In this paper, the work carried out to investigate these five fission product release and transport topics of special interest in the ARC-F project will be described and summarized.
Kwon, H.*; Sathiyamoorthi, P.*; Gangaraju, M. K.*; Zargaran, A.*; Wang, J.*; Heo, Y.-U.*; Harjo, S.; Gong, W.; Lee, B.-J.*; Kim, H. S.*
Acta Materialia, 248, p.118810_1 - 118810_12, 2023/04
被引用回数:48 パーセンタイル:99.21(Materials Science, Multidisciplinary)Maraging steels, known for ultrahigh strength and good fracture toughness, derive their superior properties from lath martensite structure with high-density nanoprecipitates. In this work, we designed a novel Fe-based medium-entropy alloy with a chemical composition of FeCo
Ni
Mo
in atomic% by utilizing the characteristics of the maraging steels. By a single-step aging of only 10 min at 650
C, the alloy showed microstructures consisting of a very high number density of (Fe, Co, Ni)
Mo
-type nanoprecipitates in lath martensite structure and reverted FCC phase, which led to ultrahigh yield strength higher than 2 GPa. This work demonstrates a novel direction to produce strong and ductile materials by expanding the horizons of material design with the aid of high-entropy concept and overcoming the limits of conventional materials.
Pohl, T.*; Sun, Y. L.*; Obertelli, A.*; Lee, J.*; Gmez-Ramos, M.*; 緒方 一介*; 吉田 数貴; Cai, B. S.*; Yuan, C. X.*; Brown, B. A.*; et al.
Physical Review Letters, 130(17), p.172501_1 - 172501_8, 2023/04
被引用回数:12 パーセンタイル:88.25(Physics, Multidisciplinary)大きなフェルミ面非対称性を持つ陽子過剰なO原子核からの100MeV/nucleonでの陽子による陽子・中性子除去反応について報告した。この結果は、quasi-freeノックアウト反応、非弾性散乱、核子移行反応を含む複数の反応機構の定量的寄与を初めて示すものである。このようなエネルギー領域では通常無視される非弾性散乱と核子移行の寄与が、弱束縛陽子と強束縛中性子の除去反応断面積にそれぞれ約50%と30%寄与していることが示された。
Woo, W.*; Kim, Y. S.*; Chae, H. B.*; Lee, S. Y.*; Jeong, J. S.*; Lee, C. M.*; Won, J. W.*; Na, Y. S.*; 川崎 卓郎; Harjo, S.; et al.
Acta Materialia, 246, p.118699_1 - 118699_13, 2023/03
被引用回数:47 パーセンタイル:99.25(Materials Science, Multidisciplinary)In situ neutron diffraction experiments have been performed under loading in cast-wrought (CW) and additively manufactured (AM) equiatomic CoCrNi medium-entropy alloys. The diffraction line profile analysis correlated the faulting-embedded crystal structure to the dislocation density, stacking/twin fault probability, and stacking fault energy as a function of strain. The results showed the initial dislocation density of 1.810
m
in CW and 1.3
10
m
in AM. It significantly increased up to 1.3
10
m-
in CW and 1.7
10
m
in AM near fracture. The dislocation density contributed to the flow stress of 470 MPa in CW and 600 MPa in AM, respectively. Meanwhile, the twin fault probability of CW (2.7%) was about two times higher than AM (1.3%) and the stacking fault probability showed the similar tendency. The twinning provided strengthening of 360 MPa in CW and 180 MPa in AM. Such a favorable strengthening via deformation twinning in CW and dislocation slip in AM was attributed to the stacking fault energy. It was estimated as 18.6 mJ/m
in CW and 37.5 mJ/m
in AM by the strain field of dislocations incorporated model. Dense dislocations, deformation twinning, and atomic-scale stacking structure were examined by using electron backscatter diffraction (EBSD) and transmission electron microscopy (TEM).
芝田 悟朗; Won, C.*; Kim, J.*; 野中 洋亮*; 池田 啓祐*; Wan, Y.*; 鈴木 雅弘*; 小出 常晴*; 田中 新*; Cheong, S.-W.*; et al.
Photon Factory Activity Report 2022 (インターネット), 2 Pages, 2023/00
Feをインターカレートした遷移金属ダイカルコゲナイド化合物FeTiS
およびFe
TaS
は、巨大な保磁力および垂直磁気異方性を示す強磁性体になることが知られている。我々は以前、Fe
TiS
についてのX線磁気円二色性(XMCD)実験の結果から、Fe
の凍結していない軌道磁気モーメントが結晶場の1次摂動によって直接磁気異方性エネルギーを生むことを明らかにした。今回、Fe
TiS
よりもさらに強い磁気異方性を示す遷移金属ダイカルコゲナイドFe
TaS
について同様にXMCD実験を行い、磁気異方性の強さが何によって左右されているかを探ることを試みた。
阿久澤 禎*; Kim, S.-Y.*; 久保田 真彦*; Wu, H.*; 渡部 創; 佐野 雄一; 竹内 正行; 新井 剛*
Journal of Radioanalytical and Nuclear Chemistry, 331(12), p.5851 - 5858, 2022/12
被引用回数:5 パーセンタイル:61.74(Chemistry, Analytical)In this work, we have examined Ln(III) and MA(III) separation conditions by the extraction chromatography using HONTA adsorbent to decide the Ln(III)/MA(III) separation process fow. From the research results, we found the simulated element of Am(III) for HONTA adsorbent and the conditions to use it. In addition, Ln(III) and Am(III) (simulated element) separation experiments were carried out using the HONTA adsorbent packed column, we have determined the column separation conditions for Am(III) such as order of fow solution and fow rate.
Elekes, Z.*; Juhsz, M. M.*; Sohler, D.*; Sieja, K.*; 吉田 数貴; 緒方 一介*; Doornenbal, P.*; Obertelli, A.*; Achouri, N. L.*; 馬場 秀忠*; et al.
Physical Review C, 106(6), p.064321_1 - 064321_10, 2022/12
被引用回数:3 パーセンタイル:32.42(Physics, Nuclear)Vと
Vの低励起準位構造を初めて探索した。
Vについては中性子ノックアウト反応と陽子非弾性散乱が、
Vについては中性子ノックアウト反応データが得られた。
Vについては4つ、
Vについては5つの新たな遷移が確認された。Lenzi-Nowacki-Poves-Sieja (LNPS)相互作用に基づく殻模型計算との比較によって、それぞれの同位体について確認されたガンマ線のうち3つが、first 11/2
状態とfirst 9/2
状態からの崩壊と決定された。
Vについては、(
,
)非弾性散乱断面積は四重極変形と十六重極変形を想定したチャネル結合法により解析されたが、十六重極変形の影響により、明確に反転の島に属するとは決定できなかった。