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論文

Application of the spectral determination method to unified $$beta$$-, $$gamma$$- and X-ray spectra

大島 真澄*; 後藤 淳*; 早川 岳人*; 浅井 雅人; 篠原 宏文*; 鈴木 勝行*; Shen, H.*

Journal of Nuclear Science and Technology, 10 Pages, 2025/00

 被引用回数:0 パーセンタイル:0.00(Nuclear Science & Technology)

スペクトル定量法(SDM)は、$$beta$$線や$$gamma$$線のスペクトル全体の形を、標準$$beta$$線及び$$gamma$$線スペクトルを用いて最小自乗フィッティング解析することで放射能を定量する方法である。本論文では、Ge検出器と液体シンチレーション検出器で測定された2つのスペクトルを統合した統合スペクトルに対して新しくSDMを適用した。統合スペクトルを解析することで、放射能の値の不確かさを改善することができた。40核種が等しい強度で含まれる統合スペクトルを解析し、それぞれの放射能の値を正しく求めることができた。

論文

Experimental investigation on local flow structures of upward cap-bubbly flows in a vertical large-size square channel

孫 昊旻; 功刀 資彰*; 横峯 健彦*; Shen, X.*; 日引 俊*

Experimental Thermal and Fluid Science, 154, p.111171_1 - 111171_24, 2024/05

 被引用回数:3 パーセンタイル:64.78(Thermodynamics)

Taking the importance of gas-liquid two-phase flows in large square channels for advanced nuclear reactors, such as ESBWR, we experimented with upward cap-bubbly flows in a large square channel. Local void fractions, axial gas velocities, and interfacial area concentrations for two bubble-size groups were measured at three axial locations. Based on the database, cap-bubbly flow characteristics in a large square channel were understood. The existing drift-flux and interfacial area concentration correlations were validated. The void fraction covariances were obtained and used to validate their existing correlations.

論文

Chiral Dirac fermion in a collinear antiferromagnet

Zhang, A.*; Deng, K.*; Sheng, J.*; Liu, P.*; Kumar, S.*; 島田 賢也*; Jiang, Z.*; Liu, Z.*; Shen, D.*; Li, J.*; et al.

Chinese Physics Letters, 40(12), p.126101_1 - 126101_8, 2023/12

 被引用回数:11 パーセンタイル:85.96(Physics, Multidisciplinary)

In a Dirac semimetal, the massless Dirac fermion has zero chirality, leading to surface states connected adiabatically to a topologically trivial surface state as well as vanishing anomalous Hall effect. Recently, itis predicted that in the nonrelativistic limit of certain collinear antiferromagnets, there exists a type of chiral "Dirac-like" fermion, whose dispersion manifests four-fold degenerate crossing points formed by spin-degenerate linear bands, with topologically protected Fermi arcs. Here, by combining with neutron diffraction and first-principles calculations, we suggest a multidomain collinear antiferromagnetic configuration, rendering the existence of the Fermi-arc surface states induced by chiral Dirac-like fermions.

論文

Multi-dimensional characteristics of upward bubbly flows in a vertical large-size square channel

孫 昊旻; 功刀 資彰*; 横峯 健彦*; Shen, X.*; 日引 俊*

International Journal of Heat and Mass Transfer, 211, p.124214_1 - 124214_17, 2023/09

 被引用回数:4 パーセンタイル:37.98(Thermodynamics)

An experiment for upward bubbly flows was conducted in a large square channel. The local void fraction, axial gas velocity, axial liquid velocity, interfacial area concentration, and Sauter mean diameter were measured at three axial locations. Based on the measurement data, the flow characteristics through flow development were investigated. The drift-flux parameters were directly determined from the local measurement data through their definitions. It was found that the distribution parameters and the void fractions could be fairly reproduced by the existing correlations for large circular pipes. Furthermore, the interfacial area concentrations could be predicted by existing correlations with reasonable accuracy.

論文

Pressure-modulated magnetism and negative thermal expansion in the Ho$$_2$$Fe$$_{17}$$ intermetallic compound

Cao, Y.*; Zhou, H.*; Khmelevskyi, S.*; Lin, K.*; Avdeev, M.*; Wang, C.-W.*; Wang, B.*; Hu, F.*; 加藤 健一*; 服部 高典; et al.

Chemistry of Materials, 35(8), p.3249 - 3255, 2023/04

 被引用回数:4 パーセンタイル:20.33(Chemistry, Physical)

静水圧や化学圧力は、結晶構造を変化させる効率的な刺激であり、材料科学において電気的、磁気的特性のチューニングによく利用されている。しかし、化学圧力は定量化が困難であり、これら両者の定量的な対応関係はまだよくわかっていない。本研究では、負の熱膨張(NTE)を持つ永久磁石の候補である金属間化合物を調べた。放射光X線その場観察により、AlをドープしたHo$$_2$$Fe$$_{17}$$に負の化学圧力があることを明らかにし、単位セル体積の温度・圧力依存性を用いそれを定量的に評価した。また、磁化測定と中性子回折測定を組み合わせることで、磁気秩序に対する化学圧力と静水圧の違いを比較した。興味深いことに、圧力はNTEの抑制と増強を制御するために使用することができた。電子状態計算から、圧力がFermiレベル(EF)に対する主要バンドの上部に影響を与えたことを示しており、これは磁気安定性に影響を与え、それが磁気とNTEを調節する上で重要な役割を果たしていることがわかった。本研究は、圧力の影響を理解し、それを利用して機能性材料の特性を制御する良い例を示している。

論文

New $$K$$ isomers in $$^{248}$$Cf

Orlandi, R.; 牧井 宏之; 西尾 勝久; 廣瀬 健太郎; 浅井 雅人; 塚田 和明; 佐藤 哲也; 伊藤 由太; 洲嵜 ふみ; 永目 諭一郎*; et al.

Physical Review C, 106(6), p.064301_1 - 064301_11, 2022/12

 被引用回数:4 パーセンタイル:52.14(Physics, Nuclear)

The nuclear structure of $$^{248}$$Cf produced by the $$^{18}$$O+$$^{249}$$Cf multinucleon transfer reaction was investigated using $$gamma$$-ray spectroscopy. Analysis of the $$gamma$$-ray spectrum of $$^{248}$$Cf revealed the presence of multiple long-lived (isomeric) excited states at low excitation energies. The energies and half-lives of the isomers contain information on the proton and neutron orbits in the heavy-element region and the deformation of atomic nuclei, and are important data to predict the properties of nuclei in the "island of stability".

論文

Evidence for strong correlations at finite temperatures in the dimerized magnet Na$$_{2}$$Cu$$_{2}$$TeO$$_{6}$$

Shangguan, Y.*; Bao, S.*; Dong, Z.-Y.*; Cai, Z.*; Wang, W.*; Huang, Z.*; Ma, Z.*; Liao, J.*; Zhao, X.*; 梶本 亮一; et al.

Physical Review B, 104(22), p.224430_1 - 224430_8, 2021/12

 被引用回数:2 パーセンタイル:10.46(Materials Science, Multidisciplinary)

Dimerized magnets forming alternating Heisenberg chains exhibit quantum coherence and entanglement and thus can find potential applications in quantum information and computation. However, magnetic systems typically undergo thermal decoherence at finite temperatures. Here, we show inelastic neutron scattering results on an alternating antiferromagnetic-ferromagnetic chain compound Na$$_{2}$$Cu$$_{2}$$TeO$$_{6}$$ that the excited quasiparticles can counter thermal decoherence and maintain strong correlations at elevated temperatures. At low temperatures, we observe clear dispersive singlet-triplet excitations arising from the dimers formed along the crystalline $$b$$-axis. The excitation gap is of $$sim$$18 meV and the bandwidth is about half of the gap. The band top energy has a weak modulation along the [100] direction, indicative of a small interchain coupling. The gap increases while the bandwidth decreases with increasing temperature, leading to a strong reduction in the available phase space for the triplons. As a result, the Lorentzian-type energy broadening becomes highly asymmetric as the temperature is raised. These results are associated with a strongly correlated state resulting from hard-core constraint and quasiparticle interactions. We consider these results to be not only evidence for strong correlations at finite temperatures in Na$$_{2}$$Cu$$_{2}$$TeO$$_{6}$$, but also for the universality of the strongly correlated state in a broad range of quantum magnetic systems.

論文

The $$^{59}$$Fe(n,$$gamma$$)$$^{60}$$Fe cross section from the surrogate ratio method and its effect on the $$^{60}$$Fe nucleosynthesis

Yan, S. Q.*; Li, X. Y.*; 西尾 勝久; Lugaro, M.*; Li, Z. H.*; 牧井 宏之; Pignatari, M.*; Wang, Y. B.*; Orlandi, R.; 廣瀬 健太郎; et al.

Astrophysical Journal, 919(2), p.84_1 - 84_7, 2021/10

 被引用回数:5 パーセンタイル:33.27(Astronomy & Astrophysics)

The long-lived $$^{60}$$Fe (with a half-life of 2.62 Myr) is a crucial diagnostic of active nucleosynthesis in the Milky Way galaxy and in supernovae near the solar system. The neutron-capture reaction $$^{59}$$Fe(n,$$gamma$$)$$^{60}$$Fe on $$^{59}$$Fe (half-life=44.5 days) is the key reaction for the production of $$^{60}$$Fe in massive stars. This reaction cross section has been previously constrained by the Coulomb dissociation experiment, which offered partial constraint on the E1 $$gamma$$-ray strength function but a negligible constraint on the M1 and E2 components. In this work, for the first time, we use the surrogate ratio method to experimentally determine the $$^{59}$$Fe(n,$$gamma$$)$$^{60}$$Fe cross sections in which all the components are included. We derived a Maxwellian-averaged cross section of 27.5$$pm$$3.5 mb at $$kT$$ = 30 keV and 13.4$$pm$$1.7 mb at $$kT$$ = 90 keV, roughly 10%-20% higher than previous estimates. We analyzed the impact of our new reaction rates in nucleosynthesis models of massive stars and found that uncertainties in the production of $$^{60}$$Fe from the $$^{59}$$Fe(n,$$gamma$$)$$^{60}$$Fe rate are at most 25$$%$$. We conclude that stellar physics uncertainties now play a major role in the accurate evaluation of the stellar production of $$^{60}$$Fe.

論文

Flow regime and void fraction predictions in vertical rod bundle flow channels

Han, X.*; Shen, X.*; 山本 俊弘*; 中島 健*; 孫 昊旻; 日引 俊*

International Journal of Heat and Mass Transfer, 178, p.121637_1 - 121637_24, 2021/10

 被引用回数:20 パーセンタイル:76.84(Thermodynamics)

This paper studies the flow regimes, their transitions and the drift-flux correlations in upward gas-liquid two-phase flows in vertical rod bundle flow channels. The flows are classified into 5 flow regimes, namely, bubbly, finely dispersed bubbly, cap-bubbly, churn and annular flows according to their different flow characteristics. Transition criteria between the flow regimes are proposed mechanistically. Those criteria can correctly predict 83% of the existing experimental observation of the flow regime. The drift-flux correlations for the distribution parameter and the drift velocity are also improved. The void fractions predicted by those correlations are compared with the existing experimental data, showing satisfactory agreement with mean relative error of 8%.

論文

Systematic study on the quark-hadron mixed phase in compact stars

Xia, C.-J.*; 丸山 敏毅; 安武 伸俊*; 巽 敏隆*; Shen, H.*; 富樫 甫*

Physical Review D, 102(2), p.023031_1 - 023031_18, 2020/07

 被引用回数:29 パーセンタイル:81.87(Astronomy & Astrophysics)

高密度星を構成する物質のクォーク-ハドロン混合相について調べる。クォーク相とハドロン相はそれぞれいくつかのモデルにより計算し、混合相の形状と状態方程式については、Ravenhallらによる連続的な幾何学的次元による計算法を踏襲する。その際表面張力は固定した値のものの他、多重反射展開法によるものと、equivparticle法によるものとを使う。これによって天体の全体的構造や質量,半径などが得られる。天体の半径と潮汐変形性の相関はハイブリッド星でも中性子星のときと同様であった。重い天体になると中心付近にクォーク物質が現れ、クォーク-ハドロンの境界の表面張力が全体の構造に対して重要になる。0.8fm$$^{-3}$$以下の密度では観測量により状態方程式に対する制限が良く得られるが、高密度では不定性が大きかった。

論文

Multiple magnetic bilayers and unconventional criticality without frustration in BaCuSi$$_2$$O$$_6$$

Allenspach, S.*; Biffin, A.*; Stuhr, U.*; Tucker, G. S.*; 河村 聖子; 古府 麻衣子; Voneshen, D. J.*; Boehm, M.*; Normand, B.*; Laflorencie, N.*; et al.

Physical Review Letters, 124(17), p.177205_1 - 177205_7, 2020/05

 被引用回数:11 パーセンタイル:59.90(Physics, Multidisciplinary)

The dimerized quantum magnet BaCuSi$$_2$$O$$_6$$ was proposed as an example of "dimensional reduction" arising near the magnetic-field-induced quantum critical point (QCP) due to perfect geometrical frustration of its interbilayer interactions. We demonstrate by high-resolution neutron spectroscopy experiments that the effective intrabilayer interactions are ferromagnetic, thereby excluding frustration. We explain the apparent dimensional reduction by establishing the presence of three magnetically inequivalent bilayers, with ratios $$3 colon 2 colon 1$$, whose differing interaction parameters create an extra field-temperature scaling regime near the QCP with a nontrivial but nonuniversal exponent. We demonstrate by detailed quantum Monte Carlo simulations that the magnetic interaction parameters we deduce can account for all the measured properties of BaCuSi$$_2$$O$$_6$$, opening the way to a quantitative understanding of nonuniversal scaling in any modulated layered system.

論文

Experimental study on local interfacial parameters in upward air-water bubbly flow in a vertical 6$$times$$6 rod bundle

Han, X.*; Shen, X.*; 山本 俊弘*; 中島 健*; 孫 昊旻; 日引 俊*

International Journal of Heat and Mass Transfer, 144, p.118696_1 - 118696_19, 2019/12

 被引用回数:24 パーセンタイル:73.38(Thermodynamics)

This paper presents a database of local flow parameters for upward adiabatic air-water two-phase flows in a vertical 6$$times$$6 rod bundle flow channel. The local void fraction, interfacial area concentration (IAC), bubble diameter and bubble velocity vector were measured by using a four-sensor optical probe. Based on an existing state-of-the-art four-sensor probe methodology with the characteristic to count small bubbles, IAC in this study was derived more reliably than those in the existing studies. In addition, bubble velocity vector could be measured by the methodology. Based on this database, flow characteristics were investigated. The area-averaged void fraction and IAC were compared with the predictions from the drift-flux model and the IAC correlations, respectively. The applicability of those to the rod bundle flow channel was evaluated.

論文

Pre- and post-accident $$^{14}$$C activities in tree rings near the Fukushima Dai-ichi Nuclear Power Plant

松中 哲也*; 笹 公和*; 高橋 努*; 松村 万寿美*; 佐藤 志彦; Shen, H.*; 末木 啓介*; 松崎 浩之*

Radiocarbon, 61(6), p.1633 - 1642, 2019/12

 被引用回数:2 パーセンタイル:9.19(Geochemistry & Geophysics)

Areas affected by routine radiocarbon ($$^{14}$$C) discharges from the Fukushima Dai-ichi Nuclear Power Plant (FDNPP) and accidental releases in March 2011 were investigated by analysis of cores from Japanese cypress and cedar trees growing at sites 9 and 24 km northwest of the plant. $$^{14}$$C concentrations in tree rings from 2008-2014 (before and after the accident) were determined by accelerator mass spectrometry, with $$^{14}$$C activities in the range 231-256 Bq kg$$^{-1}$$ C. Activities during the period 2012-2014, after FDNPP shutdown, represent background levels, while the significantly higher levels recorded during 2008-2010, before the accident, indicate uptake of $$^{14}$$C from routine FDNPP operations. The mean excess $$^{14}$$C activity for the pre-accident period at the sites 9 and 24 km northwest of the plant were 21 and 12 Bq kg$$^{-1}$$ C, respectively, indicating that the area of influence during routine FDNPP operations extended at least 24 km northwest. The mean excess tree-ring $$^{14}$$C activities in 2011 were 10 and 5.8 Bq kg$$^{-1}$$ C at 9 and 24 km northwest, respectively, documenting possible impact of the FDNPP accident on $$^{14}$$C levels in trees.

論文

Coexistence of ferromagnetic and stripe-type antiferromagnetic spin fluctuations in YFe$$_{2}$$Ge$$_{2}$$

Wo, H.*; Wang, Q.*; Shen, Y.*; Zhang, X.*; Hao, Y.*; Feng, Y.*; Shen, S.*; He, Z.*; Pan, B.*; Wang, W.*; et al.

Physical Review Letters, 122(21), p.217003_1 - 217003_5, 2019/05

 被引用回数:7 パーセンタイル:46.81(Physics, Multidisciplinary)

We report neutron scattering measurements of single-crystalline YFe$$_{2}$$Ge$$_{2}$$ in the normal state, which has the same crystal structure as the 122 family of iron pnictide superconductors. YFe$$_{2}$$Ge$$_{2}$$ does not exhibit long-range magnetic order but exhibits strong spin fluctuations. Like the iron pnictides, YFe$$_{2}$$Ge$$_{2}$$ displays anisotropic stripe-type antiferromagnetic spin fluctuations at ($$pi, 0, pi$$). More interesting, however, is the observation of strong spin fluctuations at the in-plane ferromagnetic wave vector ($$0, 0, pi$$). These ferromagnetic spin fluctuations are isotropic in the ($$H, K$$) plane, whose intensity exceeds that of stripe spin fluctuations. Both the ferromagnetic and stripe spin fluctuations remain gapless down to the lowest measured energies. Our results naturally explain the absence of magnetic order in YFe$$_{2}$$Ge$$_{2}$$ and also imply that the ferromagnetic correlations may be a key ingredient for iron-based materials.

論文

Radiocarbon variations in tree rings since 1960 near the Tokai nuclear facility, Japan

松中 哲也*; 笹 公和*; 高橋 努*; 細谷 青児*; 松村 万寿美*; 佐藤 志彦; Shen, H.*; 末木 啓介*

Nuclear Instruments and Methods in Physics Research B, 439, p.64 - 69, 2019/01

 被引用回数:2 パーセンタイル:19.99(Instruments & Instrumentation)

炭素14による環境影響を評価するため、東海原子力発電所周辺で採取した松の切り株から加速器質量分析を使用して炭素14の量を測定した。1959年から2013年までの間において232-403Bq/kgCが確認され、1959-1965年および2011-2013年はバックグラウンドレベルだった。1966-2010年の間は東海原子力発電所および東海再処理工場の公開されている運転履歴にマッチした。一方、これらの炭素14から受ける放射線量は1年あたり3.9$$mu$$Sv以下であり、影響は十分無視できるレベルである。

論文

Local gas-liquid two-phase flow characteristics in rod bundle geometry

Xiao, Y.*; Shen, X.*; 三輪 修一郎*; 孫 昊旻; 日引 俊*

混相流シンポジウム2018講演論文集(インターネット), 2 Pages, 2018/08

ロッドバンドル体系における二流体モデルの構成式の高度化を図るために、6$$times$$6ロッドバンドル体系における上昇気液二相流実験を実施した。ボイド率や界面積濃度等の局所流動パラメータを2針式光プローブで計測した。計測した断面平均ボイド率と界面積濃度の結果と、既存ドリフトフラックスモデルや界面積濃度相関式から予測した結果と比較した。

論文

Some characteristics of gas-liquid two-phase flow in vertical large-diameter channels

Shen, X.*; Schlegel, J. P.*; 日引 俊*; 中村 秀夫

Nuclear Engineering and Design, 333, p.87 - 98, 2018/07

 被引用回数:12 パーセンタイル:30.29(Nuclear Science & Technology)

Two phase flows in large-diameter channels are important to efficiently and safely transfer mass and energy in a wide variety of applications including nuclear power plants. Two-phase flows in vertical large-diameter channels, however, show much more complex multi-dimensional nature than those in small diameter channels. Various constitutive equations are required to mathematically close the model to predict two-phase flows with two-fluid model. Validations of the constitutive equations require extensive experiment effort. This paper summarizes the recent experimental studies on two-phase flows in vertical large-diameter channels, which includes measuring technique and available databases. Then, a comprehensive review of constitutive equations is provided covering flow regime transition criteria, drift-flux correlations, interfacial area concentration correlations and one- and two-group interfacial area transport equation(s), with discussions on typical characteristics of large-diameter channel flows. Recent 1D numerical simulations of large-diameter channel flows is reviewed too. Finally, future research directions are suggested.

論文

The $$^{95}$$Zr($$n, gamma$$)$$^{96}$$Zr cross section from the surrogate ratio method and its effect on $$s$$-process nucleosynthesis

Yan, S. Q.*; Li, Z. H.*; Wang, Y. B.*; 西尾 勝久; Lugaro, M.*; Karakas, A. I.*; 牧井 宏之; Mohr, P.*; Su, J.*; Li, Y. J.*; et al.

Astrophysical Journal, 848(2), p.98_1 - 98_8, 2017/10

 被引用回数:8 パーセンタイル:28.75(Astronomy & Astrophysics)

The $$^{95}$$Zr($$n, gamma$$)$$^{96}$$Zr reaction cross section is crucial in the modelling of $$s$$-process nucleosynthesis in asymptotic giant branch stars because it controls the operation of the branching point at the unstable $$^{95}$$Zr and the subsequent production of $$^{96}$$Zr. We have carried out the measurement of the $$^{90}$$Zr($$^{18}$$O,$$^{16}$$O) and $$^{94}$$Zr($$^{18}$$O,$$^{16}$$O) reactions and obtained the $$gamma$$-decay probability ratio of $$^{92}$$Zr$$^{*}$$ and $$^{96}$$Zr$$^{*}$$ to determine the $$^{95}$$Zr($$n, gamma$$)$$^{96}$$Zr reaction cross sections with the surrogate ratio method. We tested our deduced maxwellian-averaged cross section in stellar models with masses between 2 and 6 $$M_{odot}$$ and metallicities 0.014 and 0.03. The largest changes - up 80 % variations in $$^{96}$$Zr - are seen in the models of 3-4 $$M_{odot}$$, where the $$^{22}$$Ne neutron source is mildly activated. The new rate can still provide a match to data from meteoritic stardust silicon carbide grains, provided the maximum mass of the parent stars is below 4 $$M_{odot}$$, for a metallicity of 0.03.

論文

Experimental study on interfacial area transport of two-phase bubbly flow in a vertical large-diameter square duct

Shen, X.*; 孫 昊旻; Deng, B.*; 日引 俊*; 中村 秀夫

International Journal of Heat and Fluid Flow, 67(Part A), p.168 - 184, 2017/10

 被引用回数:17 パーセンタイル:58.92(Thermodynamics)

主に4センサープローブを用いて、鉛直大口径正方形管内における上昇気泡流に関する実験的研究を実施した。流れ方向3断面における、局所界面積濃度、ボイド率、3次元気泡速度、気泡径を計測した。界面積輸送方程式やその中の気泡合体分裂モデルは、二相流における界面積濃度の予測に多用されてきたものの、主に円管や小口径管の二相流実験から構築されており、大口径正方形管に対する適応性の検証がされていない。そこで本研究では、大口径正方形管で取得したデータベースを用いて、既存の1次元1グループ界面積輸送方程式の気泡合体分裂モデルの大口径正方形管への適応性を評価した。最良のモデルに基づく予測と実験結果との誤差は25%であることを示した。

論文

Self-learning Monte Carlo method; Continuous-time algorithm

永井 佑紀; Shen, H.*; Qi, Y.*; Liu, J.*; Fu, L.*

Physical Review B, 96(16), p.161102_1 - 161102_6, 2017/10

 被引用回数:55 パーセンタイル:87.64(Materials Science, Multidisciplinary)

モンテカルロ法は原子力分野以外にも様々な分野で利用される極めて汎用的な手法である。近年、機械学習の手法を取り込むことで、高速なモンテカルロ法が開発されている。本論文では、銅酸化物高温超伝導体をはじめとする様々な物質のシミュレーションにおいて汎用的に用いられている連続時間量子モンテカルロ法に対して機械学習の手法を適用した結果を報告する。なお、上記課題の解決にあたり、モンテカルロ法でネックの一つとなる次の配置をどう決めるか、という問題に対して、機械学習によって自動的に決めるという手法を提案した。この手法の開発により、より高精度な超伝導体シミュレーションや、ウランなどの重い元素を含む第一原理計算の高速化が期待できる。これらの結果は、広く原子力分野のためのシミュレーション技術開発に資する成果である。

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