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論文

Residual stress measurement and lifetime evaluation of railway axles by neutron scattering technology

Hu, F.-F.*; Qin, T.-Y.*; Ao, N.*; 徐 平光; Su, Y. H.; Parker, J. D.*; 篠原 武尚; 菖蒲 敬久; Kang, G.-Z.*; Ren, M.-M.; et al.

Journal of Traffic and Transportation Engineering (English Edition), 25(2), p.75 - 93, 2025/04

To accurately predict the remaining lifetime of surface-strengthened railway axles, a damage tolerance method considering three-dimensional (3D) residual stresses was proposed. By taking the induction-hardened carbon steel S38C axle as an example, two-dimensional (2D) distribution characterization of residual strain and 3D residual stress measurement were performed through comprehensive application of the neutron Bragg-edge transmission imaging and angle-dispersive neutron diffraction experiments. A numerical method was employed to implant the 3D residual stress into the axle model, and the remaining lifetime of the full-scale axle was studied by coupling the measured load spectrum, press-fit loads, and residual stresses. Experimental results shows that, both axial and hoop directions present a compressive residual strain gradient layer of about 3 mm, with a maximum compressive residual strain of up to -4500 $$mu$$$$varepsilon$$ in the surface layer, yet a maximum tensile strain of up to 1000 $$mu$$$$varepsilon$$ in the core. The maximum axial and hoop compressive stresses of the axle are about -500 MPa and -303 MPa respectively, while radial stresses overall fluctuate in the zero mean stress range. At depths beyond 4.5 mm from the surface layer, all three components are tensile stresses. The axle surface layer is subjected to compressive residual stresses, and crack propagation does not occur if the crack depth is less than 4.5 mm. Nevertheless, cracks propagate accelerates when the crack depth is greater than 4.5 mm. Different crack propagation depth thresholds lead to a larger calculated remaining lifetime for the residual stress-free condition than for the case where 3D residual stresses are taken into account. However, the axle remaining service mileage of the axle of 227000 Km under the most conservative conditions exceeds 3.5 non-destructive inspection (NDI) cycles, with a large safety margin. The experimental results can provide a scientific reference for the development and optimization of NDI cycles for surface-strengthened railway axles.

論文

Strong low-energy rattling modes enabled liquid-like ultralow thermal conductivity in a well-ordered solid

Liu, P.-F.*; Li, X.*; Li, J.*; Zhu, J.*; Tong, Z.*; 古府 麻衣子*; 楡井 真実; Xu, J.*; Yin, W.*; Wang, F.*; et al.

National Science Review, 11(12), p.nwae216_1 - nwae216_10, 2024/12

 被引用回数:12 パーセンタイル:91.22(Multidisciplinary Sciences)

Crystalline solids exhibiting inherently low lattice thermal conductivity ($$kappa_{rm L}$$) are of great importance in applications such as thermoelectrics and thermal barrier coatings. However, $$kappa_{rm L}$$ cannot be arbitrarily low and is limited by the minimum thermal conductivity related to phonon dispersions. In this work, we report the liquid-like thermal transport in a well-ordered crystalline CsAg$$_5$$Te$$_3$$, which exhibits an extremely low $$kappa_{rm L}$$ value of $$sim$$ 0.18 Wm$$^{-1}$$K$$^{-1}$$. On the basis of first-principles calculations and inelastic neutron scattering measurements, we find that there are lots of low-lying optical phonon modes at $$sim$$ 3.1 meV hosting the avoided-crossing behavior with acoustic phonons. These strongly localized modes are accompanied by weakly bound rattling Ag atoms with thermally induced large amplitudes of vibrations. Using the two-channel model, we demonstrate that coupling of the particle-like phonon modes and the heat-carrying wave-like phonons is essential for understanding the low $$kappa_{rm L}$$, which is heavily deviated from the $$1/T$$ temperature dependence of the standard Peierls theory. In addition, our analysis indicates that the soft structural framework with liquid-like motions of the fluctuating Ag atoms is the underlying cause that leads to the suppression of the heat conduction in CsAg$$_5$$Te$$_3$$. These factors synergistically account for the ultralow $$kappa_{rm L}$$ value. Our results demonstrate that the liquid-like heat transfer could indeed exist in a well-ordered crystal.

論文

Brightening triplet excitons enable high-performance white-light emission in organic small molecules via integrating n-$$pi^*/pi$$-$$pi^*$$ transitions

Yang, Q.*; Yang, X.*; Wang, Y.*; Fei, Y.*; Li, F.*; Zheng, H.*; Li, K.*; Han, Y.*; 服部 高典; Zhu, P.*; et al.

Nature Communications (Internet), 15, p.7778_1 - 7778_9, 2024/09

 被引用回数:9 パーセンタイル:88.46(Multidisciplinary Sciences)

明るい一重項励起子と三重項励起子を同時に発現する発光材料は、オプトエレクトロニクス、サイネージ、情報暗号化において大きな可能性を秘めている。しかしながら、高性能の白色発光を実現するためには、蛍光と燐光の寄与が不均衡であることが大きな障害となっている。ここでは、水素結合の協同効果による圧力処理エンジニアリングによって、n-$$pi^*/pi$$-$$pi^*$$遷移の混合を実現し、イソフタル酸(IPA)中で三重項状態の発光を7%から40%に高めることで、この課題に対処した。加圧処理したIPAでは、蛍光と燐光のハイブリッドに基づく優れた白色発光が得られ、フォトルミネッセンス量子収率は当初の19%(青色発光)から75%に増加した。その場での高圧IRスペクトル、X線回折、中性子回折から、圧力の上昇に伴い水素結合が連続的に強化されることが明らかになった。さらに、この強化された水素結合は、圧力処理後も常圧条件下まで保持され、バランスの取れた一重項/三重項励起子集団のための効率的な系間交差を目的としたIPAに与え、効率的な白色発光をもたらした。この研究は、有機低分子の三重項状態を明るくするルートを提案するだけでなく、一重項励起子と三重項励起子の比率を調節して、高性能の白色発光を構築するものである。

論文

Gradient residual strain determination of surface impacted railway S38C axles by neutron Bragg-edge transmission imaging

Hu, F. F.*; Qin, T. Y.*; Ao, N.*; Su, Y. H.; Zhou, L.*; 徐 平光; Parker, J. D.*; 篠原 武尚; Chen, J.*; Wu, S. C.*

Engineering Fracture Mechanics, 306, p.110267_1 - 110267_18, 2024/08

 被引用回数:2 パーセンタイル:60.53(Mechanics)

Non-destructive and quantitative mapping of gradient residual strain distribution in surface-hardened railway S38C axles could provide a positive reference for determining service lifetime and maintenance strategy. To tackle this concern, time-of-flight neutron Bragg-edge transmission imaging was employed by real axle samples with and without impacted crater. A novel and simple procedure to formulate the residual strain field was also developed in this work, with the transmission batch code in Appendix A. By mapping the global two- dimensional residual strains, it can be verified that the residual strains into the axle are uniformly distributed in the hoop direction. Subsequently, it was revealed that the axial and hoop residual strains, respectively in the cylinder and the long strip samples prepared from a real S38C hollow axle, indicated a gradient evolution distribution with a depth of $$sim$$ 8 mm, covering a range of -5500 $$sim$$ 1000 $$mu$$$$varepsilon$$ for axial strains and -6500 $$sim$$ 1000 $$mu$$$$varepsilon$$ for hoop strains. More importantly, the maximum compressive lattice strain of the cylinder sample was increased by 15.61%, and 22.35% at the impacting speeds of 100, and 125 m/s, respectively; and that of the long strip sample increased by 29.17%, and 43.70%, respectively. It can thus be concluded that lattice strains have redistributed around the impact crater, demonstrating the local alteration of the residual strain field. These new findings suggest the localized variation in residual strains should be taken into account while evaluating the service damage evolution of railway axles, especially those affected by high-speed impacts during operation.

論文

Gradient residual stress and fatigue life prediction of induction hardened carbon steel S38C axles; Experiment and simulation

Qin, T. Y.*; Hu, F. F.*; 徐 平光; Zhang, H.*; Zhou, L.*; Ao, N.*; Su, Y. H.; 菖蒲 敬久; Wu, S. C.*

International Journal of Fatigue, 185, p.108336_1 - 108336_13, 2024/08

 被引用回数:8 パーセンタイル:94.71(Engineering, Mechanical)

Gradient distribution of triaxial residual stresses to a depth of several millimeters is retained in middle carbon steel S38C axles after high-frequency induction hardening, which has become a critical concern for fatigue structural integrity. To address this, the axial, hoop, and radial gradient residual strains inside the axles were measured for the first time by advanced neutron diffraction. The SIGINI Fortran subroutine was then adopted to reconstruct the global initial residual stress field from the measured data. Experimental and simulation results show that residual stresses of about -520 MPa (axial), -710 MPa (hoop), and -40 MPa (radial) residual stress were retained below the axle surface. Subsequently, the fatigue crack propagation behavior of S38C axles was numerically investigated in the framework of fracture mechanics. The calculated results clearly show that the compressive residual stresses at a depth of 0?3 mm from the axle surface lead to a low crack growth driving force, and that fatigue cracks do not propagate as long as the crack depth is less than 3.7 mm for hollow S38C axles. These results further indicate that the maximum defect size allowed in routine inspections is acceptable from a safety and economic point of view. Accurate measurement and characterization of the global gradient residual stress field through experiments and simulations can provide an important reference for optimizing the mileage intervals of nondestructive testing (NDT) of surface defects in these surface-strengthened railway axles.

論文

Gradient residual strain measurement procedure in surface impacted railway steel axles by using neutron scattering

Zhou, L.*; Zhang, H.*; Qin, T. Y.*; Hu, F. F.*; 徐 平光; Ao, N.*; Su, Y. H.; He, L. H.*; Li, X. H.*; Zhang, J. R.*; et al.

Metallurgical and Materials Transactions A, 55(7), p.2175 - 2185, 2024/07

 被引用回数:3 パーセンタイル:75.40(Materials Science, Multidisciplinary)

High-speed railway S38C axles undergo surface induction hardening for durability, but are susceptible to fatigue cracks from foreign object impact. The neutron diffraction method was employed to measure the residual strain in S38C axles, obtaining microscopic lattice distortion data, for the gradient layer at a depth of 8 mm under the surface. The results showed that after induction-hardening, the microscopic lattice distortion had a gradient distribution, decreasing with the distance from the surface. However, in the case of impacting speed of 600 km/m, the average microscopic lattice distortion increased with the distance from the surface, reaching a maximum augmentation of 55 pct. These findings indicate a strong experimental basis, and improve our understanding of the relationship between macroscopic residual stress and decision-making, in regard to operation and maintenance.

論文

Microscopic insights of the extraordinary work-hardening due to phase transformation

Ma, Y.*; Naeem, M.*; Zhu, L.*; He, H.*; Sun, X.*; Yang, Z.*; He, F.*; Harjo, S.; 川崎 卓郎; Wang, X.-L.*

Acta Materialia, 270, p.119822_1 - 119822_13, 2024/05

 被引用回数:9 パーセンタイル:95.42(Materials Science, Multidisciplinary)

We report an in situ neutron diffraction study of 316 L that reveals an extraordinary work-hardening rate (WHR) of $$sim$$7 GPa at 15 K. Detailed analyses show that the major contribution to the excellent strength and ductility comes from the transformation-induced plasticity (TRIP) effect, introduced by the austenite-to-martensite ($$gamma$$-to-$$alpha$$') phase transition. A dramatic increase in the WHR is observed along with the transformation; the WHR declined when the austenite phase is exhausted. During plastic deformation, the volume-fraction weighted phase stress and stress contribution from the $$alpha$$'-martensite increase significantly. The neutron diffraction data further suggest that the $$gamma$$-to-$$alpha$$' phase transformation was mediated by the $$varepsilon$$-martensite, as evidenced by the concurrent decline of the $$varepsilon$$ phase with the $$gamma$$ phase.

論文

Low spin spectroscopy of neutron-rich $$^{43,44,45}$$Cl via $$beta^-$$ and $$beta n$$ decay

Tripathi, V.*; Bhattacharya, S.*; Rubino, E.*; Benetti, C.*; Perello, J. F.*; Tabor, S. L.*; Liddick, S. N.*; Bender, P. C.*; Carpenter, M. P.*; Carroll, J. J.*; et al.

Physical Review C, 109(4), p.044320_1 - 044320_15, 2024/04

 被引用回数:0 パーセンタイル:0.00(Physics, Nuclear)

ミシガン州立大学の国立超伝導サイクロトロン研究所において$$^{48}$$Caのフラグメンテーション反応によって中性子過剰核$$^{43,45}$$Sを生成し、そこからのベータ崩壊および遅発中性子放出ベータ崩壊によって$$^{43,44,45}$$Clの励起状態を得た。得られた実験データをSDPFSDG-MU相互作用を用いた大規模殻模型計算と比較し、よい一致を得た。

論文

Crystal-liquid duality driven ultralow two-channel thermal conductivity in $$alpha$$-MgAgSb

Li, J.*; Li, X.*; Zhang, Y.*; Zhu, J.*; Zhao, E.*; 古府 麻衣子; 中島 健次; Avdeev, M.*; Liu, P.-F.*; Sui, J.*; et al.

Applied Physics Reviews (Internet), 11(1), p.011406_1 - 011406_8, 2024/03

 被引用回数:7 パーセンタイル:91.57(Physics, Applied)

The desire for intrinsically low lattice thermal conductivity ($$kappa_L$$) in thermoelectrics motivates numerous efforts on understanding the microscopic mechanisms of heat transport in solids. Here, based on theoretical calculations, we demonstrate that $$alpha$$-MgAgSb hosts low-energy localized phonon bands and avoided crossing of the rattler modes, which coincides with the inelastic neutron scattering result. Using the two-channel lattice dynamical approach, we find, besides the conventional contribution ($$sim$$70% at 300 K) from particlelike phonons propagating, the coherence contribution dominated by the wavelike tunneling of phonons accounts for $$sim$$30% of total $$kappa_L$$ at 300 K. By considering dual contributions, our calculated room-temperature $$kappa_L$$ of 0.64 Wm$$^{-1}$$K$$^{-1}$$ well agrees with the experimental value of 0.63 Wm$$^{-1}$$K$$^{-1}$$. More importantly, our computations give a nonstandard $$kappa_L propto T^{-0.61}$$ dependence, perfectly explaining the abnormal temperature-trend of $$sim T^{-0.57}$$ in experiment for $$alpha$$-MgAgSb. By molecular dynamics simulation, we reveal that the structure simultaneously has soft crystalline sublattices with the metavalent bonding and fluctuating liquid-like sublattices with thermally induced large amplitude vibrations. These diverse forms of chemical bonding arouse mixed part-crystal part-liquid state, scatter strongly heat-carrying phonons, and finally produce extremely low $$kappa_L$$. The fundamental research from this study will accelerate the design of ultralow-$$kappa_L$$ materials for energy-conversion applications.

論文

Onset of collectivity for argon isotopes close to $$N=32$$

Linh, B. D.*; Corsi, A.*; Gillibert, A.*; Obertelli, A.*; Doornenbal, P.*; Barbieri, C.*; Duguet, T.*; G$'o$mez-Ramos, M.*; Holt, J. D.*; Hu, B. S.*; et al.

Physical Review C, 109(3), p.034312_1 - 034312_15, 2024/03

 被引用回数:2 パーセンタイル:58.81(Physics, Nuclear)

理化学研究所RIビームファクトリーにて中性子過剰核$$^{50}$$Arビームからの1中性子ノックアウト反応実験を行い、$$^{49}$$Arのエネルギー準位および分光学的因子を導出した。特に、第一励起状態の$$1/2^-$$への分光学的因子が大きいことから、始状態の$$^{50}$$Arの基底状態において中性子が$$p_{1/2}$$軌道を多く占めていることがわかった。これは、中性子数32がよい魔法数として知られる$$^{52}$$Caとは異なった性質であり、カルシウムからアルゴンへと陽子が2個減ることで閉殻構造が大きく崩れることが明らかになった。

論文

Extreme phonon anharmonicity underpins superionic diffusion and ultralow thermal conductivity in argyrodite Ag$$_{8}$$SnSe$$_{6}$$

Ren, Q.*; Gupta, M. K.*; Jin, M.*; Ding, J.*; Wu, J.*; Chen, Z.*; Lin, S.*; Fabelo, O.*; Rodriguez-Velamazan, J. A.*; 古府 麻衣子; et al.

Nature Materials, 22(8), p.999 - 1006, 2023/08

 被引用回数:76 パーセンタイル:99.20(Chemistry, Physical)

Ultralow thermal conductivity and fast ionic diffusion endow superionic materials with excellent performance both as thermoelectric converters and as solid-state electrolytes. Yet the correlation and interdependence between these two features remain unclear owing to a limited understanding of their complex atomic dynamics. Here we investigate ionic diffusion and lattice dynamics in argyrodite Ag$$_{8}$$SnSe$$_{6}$$ using synchrotron X-ray and neutron scattering techniques along with machine-learned molecular dynamics. We identify a critical interplay of the vibrational dynamics of mobile Ag and a host framework that controls the overdamping of low-energy Ag-dominated phonons into a quasi-elastic response, enabling superionicity. Concomitantly, the persistence of long-wavelength transverse acoustic phonons across the superionic transition challenges a proposed 'liquid-like thermal conduction' picture. Rather, a striking thermal broadening of low-energy phonons, starting even below 50 K, reveals extreme phonon anharmonicity and weak bonding as underlying features of the potential energy surface responsible for the ultralow thermal conductivity ($$<$$ 0.5 Wm$$^{-1}$$K$$^{-1}$$) and fast diffusion. Our results provide fundamental insights into the complex atomic dynamics in superionic materials for energy conversion and storage.

論文

Pressure-modulated magnetism and negative thermal expansion in the Ho$$_2$$Fe$$_{17}$$ intermetallic compound

Cao, Y.*; Zhou, H.*; Khmelevskyi, S.*; Lin, K.*; Avdeev, M.*; Wang, C.-W.*; Wang, B.*; Hu, F.*; 加藤 健一*; 服部 高典; et al.

Chemistry of Materials, 35(8), p.3249 - 3255, 2023/04

 被引用回数:2 パーセンタイル:21.90(Chemistry, Physical)

静水圧や化学圧力は、結晶構造を変化させる効率的な刺激であり、材料科学において電気的、磁気的特性のチューニングによく利用されている。しかし、化学圧力は定量化が困難であり、これら両者の定量的な対応関係はまだよくわかっていない。本研究では、負の熱膨張(NTE)を持つ永久磁石の候補である金属間化合物を調べた。放射光X線その場観察により、AlをドープしたHo$$_2$$Fe$$_{17}$$に負の化学圧力があることを明らかにし、単位セル体積の温度・圧力依存性を用いそれを定量的に評価した。また、磁化測定と中性子回折測定を組み合わせることで、磁気秩序に対する化学圧力と静水圧の違いを比較した。興味深いことに、圧力はNTEの抑制と増強を制御するために使用することができた。電子状態計算から、圧力がFermiレベル(EF)に対する主要バンドの上部に影響を与えたことを示しており、これは磁気安定性に影響を与え、それが磁気とNTEを調節する上で重要な役割を果たしていることがわかった。本研究は、圧力の影響を理解し、それを利用して機能性材料の特性を制御する良い例を示している。

論文

Nested antiferromagnetic spin fluctuations and non-Fermi-liquid behavior in electron-doped CeCo$$_{1-x}$$Ni$$_{x}$$In$$_5$$

酒井 宏典; 徳永 陽; 神戸 振作; Zhu, J.-X.*; Ronning, F.*; Thompson, J. D.*; 小手川 恒*; 藤 秀樹*; 鈴木 康平*; 大島 佳樹*; et al.

Physical Review B, 106(23), p.235152_1 - 235152_8, 2022/12

 被引用回数:1 パーセンタイル:7.32(Materials Science, Multidisciplinary)

Ni置換系CeCo$$_{1-x}$$Ni$$_x$$In$$_5$$について、核四重極共鳴と核磁気共鳴(NQR/NMR)を用いて調べた。$$T_{rm c}$$=2.3Kの超伝導転移gは、Ni置換によって徐々に下がってゆき、$$x$$=0.25の時にゼロとなる。超格子を用いた密度関数計算によってNQRスペクトルの帰属を行い、スピン格子緩和率$$1/T_1$$が一様に抑えられ、反強磁性スピン揺らぎがNi置換によって弱められることを明らかにした。$$x$$=0.25のとき、$$(T_1T)^{-1}$$が、$$T_{rm g}$$=2Kで極大を示すことがわかった。このことは、遍歴電子の反強磁性スピン揺らぎがネスティングによって打ち消し合っているとして理解できる。

論文

$$beta^-$$ decay of exotic P and S isotopes with neutron number near 28

Tripathi, V.*; Bhattacharya, S.*; Rubino, E.*; Benetti, C.*; Perello, J. F.*; Tabor, S. L.*; Liddick, S. N.*; Bender, P. C.*; Carpenter, M. P.*; Carroll, J. J.*; et al.

Physical Review C, 106(6), p.064314_1 - 064314_14, 2022/12

 被引用回数:4 パーセンタイル:53.47(Physics, Nuclear)

ミシガン州立大学の国立超伝導サイクロトロン研究所にて、中性子過剰なリン、硫黄同位体を生成し、そこからのベータ崩壊半減期および娘核の励起準位を測定した。$$^{42}$$Pの崩壊によって得られるエネルギー準位から、この原子核の基底状態は$$2^-$$あるいは$$3^-$$であることが示唆された。中性子数が偶数の硫黄同位体からの崩壊様式を系統的に調べた結果、中性子数が増えるにつれてガモフテラー遷移強度の大きな準位の励起エネルギーが高くなることがわかった。これは、大規模殻模型計算によって予言されている現象に一致する。

論文

Structure of an aqueous RbCl solution in the gigapascal pressure range by neutron diffraction combined with empirical potential structure refinement modeling

Zhang, W. Q.*; 山口 敏男*; Fang, C. H.*; 吉田 亨次*; Zhou, Y. Q.*; Zhu, F. Y.*; 町田 真一*; 服部 高典; Li, W.*

Journal of Molecular Liquids, 348, p.118080_1 - 118080_11, 2022/02

 被引用回数:3 パーセンタイル:15.57(Chemistry, Physical)

3mol/kgのRbCl水溶液におけるイオンの水和・会合と水素結合した水の構造を、298K/0.1MPa, 298K/1GPa, 523K/1GPa, 523K/4GPaにおける中性子回折と経験的ポテンシャル構造精密化モデリングにより調べた。その結果、構造パラメータは温度と圧力に依存していることがわかった。高圧・高温条件では、Rb$$^+$$とCl$$^-$$の第二水和層がより明確になる。第一水和層におけるRb$$^+$$の平均酸素配位数は、配位距離を0.290nmから0.288nmに縮めながら、常圧では6.3だったのが、4GPaでは8.9に増加した。第一水和シェルのCl$$^-$$の平均酸素配位数は、常圧で5.9、4GPaで9.1と圧力により増加し、対応する配位距離は0.322nmから0.314nmへと減少した。Rb$$^+$$と中心の水分子の第一溶媒和シェルにおける水双極子の配向は圧力に敏感であるが、Cl$$^-$$の第一溶媒和シェルにおける水双極子の配向は温度圧力によらずあまり変化しなかった。Rb$$^+$$-Cl$$^-$$の隣接イオンペアの数は、温度が高くなると減少し、圧力が高くなると増加する。水分子は密に詰まっており、極限状態では水分子の四面体水素結合ネットワークはもはや存在しない。

論文

Solving the puzzles of the decay of the heaviest known proton-emitting nucleus $$^{185}$$Bi

Doherty, D. T.*; Andreyev, A. N.; Seweryniak, D.*; Woods, P. J.*; Carpenter, M. P.*; Auranen, K.*; Ayangeakaa, A. D.*; Back, B. B.*; Bottoni, S.*; Canete, L.*; et al.

Physical Review Letters, 127(20), p.202501_1 - 202501_6, 2021/11

 被引用回数:10 パーセンタイル:64.86(Physics, Multidisciplinary)

$$^{185}$$Bi is the heaviest known proton emitting isotope. Its decay had been observed, but the assumed ground-state lifetime ($$sim$$$$60~mu$$s) was incorrect, leading to unexplained hindrance. With two new experiments at Argonne National Laboratory, two states were clearly identified. One is the proton-emitting ground-state (spin 1/2$$^+$$, half-life: 2.8$$^{+2.3}_{-1.0}$$ $$mu$$s), the second is a 58(2) $$mu$$s $$gamma$$-decaying isomer. The new data show the inversion of the ground and isomeric states compared to neighboring Bi isotopes. This is the only known example of a ground-state proton decay to a daughter nucleus ($$^{184}$$Pb) with a major shell closure.

論文

The $$^{59}$$Fe(n,$$gamma$$)$$^{60}$$Fe cross section from the surrogate ratio method and its effect on the $$^{60}$$Fe nucleosynthesis

Yan, S. Q.*; Li, X. Y.*; 西尾 勝久; Lugaro, M.*; Li, Z. H.*; 牧井 宏之; Pignatari, M.*; Wang, Y. B.*; Orlandi, R.; 廣瀬 健太郎; et al.

Astrophysical Journal, 919(2), p.84_1 - 84_7, 2021/10

 被引用回数:6 パーセンタイル:33.92(Astronomy & Astrophysics)

The long-lived $$^{60}$$Fe (with a half-life of 2.62 Myr) is a crucial diagnostic of active nucleosynthesis in the Milky Way galaxy and in supernovae near the solar system. The neutron-capture reaction $$^{59}$$Fe(n,$$gamma$$)$$^{60}$$Fe on $$^{59}$$Fe (half-life=44.5 days) is the key reaction for the production of $$^{60}$$Fe in massive stars. This reaction cross section has been previously constrained by the Coulomb dissociation experiment, which offered partial constraint on the E1 $$gamma$$-ray strength function but a negligible constraint on the M1 and E2 components. In this work, for the first time, we use the surrogate ratio method to experimentally determine the $$^{59}$$Fe(n,$$gamma$$)$$^{60}$$Fe cross sections in which all the components are included. We derived a Maxwellian-averaged cross section of 27.5$$pm$$3.5 mb at $$kT$$ = 30 keV and 13.4$$pm$$1.7 mb at $$kT$$ = 90 keV, roughly 10%-20% higher than previous estimates. We analyzed the impact of our new reaction rates in nucleosynthesis models of massive stars and found that uncertainties in the production of $$^{60}$$Fe from the $$^{59}$$Fe(n,$$gamma$$)$$^{60}$$Fe rate are at most 25$$%$$. We conclude that stellar physics uncertainties now play a major role in the accurate evaluation of the stellar production of $$^{60}$$Fe.

論文

Nanoscale heterogeneity induced by nonmagnetic Zn dopants in the quantum critical metal CeCoIn$$_5$$; $$^{115}$$In NQR/NMR and $$^{59}$$Co NMR study

酒井 宏典; 徳永 陽; 神戸 振作; Zhu, J.-X.*; Ronning, F.*; Thompson, J. D.*; Ramakrishna, S. K.*; Reyes, A. P.*; 鈴木 康平*; 大島 佳樹*; et al.

Physical Review B, 104(8), p.085106_1 - 085106_12, 2021/08

 被引用回数:5 パーセンタイル:30.79(Materials Science, Multidisciplinary)

典型的な量子臨界金属であるCeCoIn$$_5$$は、In元素をZn元素で少量置換することで、反強磁性を誘起できることが知られており、7%Zn置換系では、超伝導も共存する。NQRおよびNMRを用いて、微視的に電子状態を調べた結果、反強磁性はZn置換子周辺で起こり、超伝導は置換子から離れた電子状態が核となって起こり、近接効果により、バルク全体に超伝導が拡がる、という不均一性を見出した。Zn置換子周辺にある局所不均一性は、磁場をかけても残存することも見出した。

論文

Thermally altered subsurface material of asteroid (162173) Ryugu

北里 宏平*; Milliken, R. E.*; 岩田 隆浩*; 安部 正真*; 大竹 真紀子*; 松浦 周二*; 高木 靖彦*; 中村 智樹*; 廣井 孝弘*; 松岡 萌*; et al.

Nature Astronomy (Internet), 5(3), p.246 - 250, 2021/03

 被引用回数:58 パーセンタイル:96.23(Astronomy & Astrophysics)

2019年4月「はやぶさ2」ミッションは、地球に近い炭素質の小惑星(162173)リュウグウの人工衝撃実験を成功させた。これは露出した地下物質を調査し、放射加熱の潜在的な影響をテストする機会を提供した。はやぶさ2の近赤外線分光器(NIRS3)によるリュウグウの地下物質の観測結果を報告する。発掘された材料の反射スペクトルは、表面で観測されたものと比較して、わずかに強くピークがシフトした水酸基(OH)の吸収を示す。これは、宇宙風化や放射加熱が最上部の表面で微妙なスペクトル変化を引き起こしたことを示している。ただし、このOH吸収の強度と形状は、表面と同様に、地下物質が300$$^{circ}$$Cを超える加熱を経験したことを示している。一方、熱物理モデリングでは、軌道長半径が0.344AUに減少しても、推定される掘削深度1mでは放射加熱によって温度が200$$^{circ}$$Cを超えて上昇しないことが示されている。これは、リュウグウ母天体が放射加熱と衝撃加熱のいずれか、もしくは両方により熱変化が発生したという仮説を裏付けている。

論文

Suppressed lattice disorder for large emission enhancement and structural robustness in hybrid lead iodide perovskite discovered by high-pressure isotope effect

Kong, L.*; Gong, J.*; Hu, Q.*; Capitani, F.*; Celeste, A.*; 服部 高典; 佐野 亜沙美; Li, N.*; Yang, W.*; Liu, G.*; et al.

Advanced Functional Materials, 31(9), p.2009131_1 - 2009131_12, 2021/02

 被引用回数:32 パーセンタイル:82.55(Chemistry, Multidisciplinary)

有機-無機ハロゲン化物ペロブスカイトは非常に柔らかいために、圧力などの外部刺激により格子定数を容易に変化させることができ、有用な光電特性を引き出すのに有効である。一方でこの特性は、多少の加圧でも、格子を歪ませてしまい、光と物質の相互作用を弱め、それによる性能の低下を引き起こす。そこで本研究では、代表的な物質であるヨウ化メチルアンモニウム鉛に対して圧力効果および同位体効果を調べ、それらが格子歪を抑制することが分かった。このことは、それらが、これまで得られなかったような光学的,機械的特性を持つ物質を得る手段として有効であることを示している。

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