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論文

$$3mathbf{Q}$$ magnetic order with spatially alternating spin scalar chirality in overdoped Co$$_{0.336}$$TaS$$_{2}$$

Cho, W.*; Park, P.*; Kim, C.*; An, Y.*; 飯田 一樹*; 梶本 亮一; Matin, S.*; Sibille, R.*; Crooker, S. A.*; Park, J.-G.*

Physical Review B, 113(17), p.174410_1 - 174410_14, 2026/05

 被引用回数:0 パーセンタイル:0.00(Materials Science, Multidisciplinary)

Co$$_{x}$$TaS$$_{2}$$ ($$x approx 1/3$$) exhibits a spontaneous Hall effect from spin texture in antiferromagnets, with a tetrahedral triple-Q ($$3mathbf{Q}$$) order and uniform spin scalar chirality. Upon Co overdoping ($$x > 1/3$$), it undergoes a shift in magnetic ordering vectors from $$mathbf{Q}_mathrm{m} = (1/2, 0, 0)$$ to $$(1/3, 0, 0)$$. Interestingly, the spontaneous Hall effect disappeared in the overdoped regime, which was originally attributed to the loss of $$3mathbf{Q}$$ order. However, a question remains whether a new type of $$3mathbf{Q}$$ order can exist with alternating chirality in the overdoped regime. To address this, we investigated Co$$_{0.336}$$TaS$$_{2}$$ using inelastic neutron scattering (INS), neutron diffraction, and optical dichroism, and found that INS data and spin-wave simulations support a $$3mathbf{Q}$$ order with alternating chirality. Moreover, neutron diffraction data show field-independent Bragg peaks, while linear dichroism detects no in-plane anisotropy, consistent with threefold rotation symmetry. Our data support the scenario of an alternating-chirality $$3mathbf{Q}$$ order in Co$$_{0.336}$$TaS$$_{2}$$, cancelling the spontaneous Hall effect. This study highlights a combined neutron-optical approach to identify complex spin textures.

論文

Cryogenic-to-ambient evolution of hetero-deformation-induced strengthening in dual-phase medium-entropy alloys

Ha, H.*; Kim, J.*; Gu, G. H.*; Harjo, S.; Gong, W.; Hong, S.-J.*; Kim, H. S.*

Materials Characterization, 234, p.116086_1 - 116086_12, 2026/04

 被引用回数:2 パーセンタイル:84.58(Materials Science, Multidisciplinary)

Dual-phase (DP) high- and medium-entropy alloys (H/MEAs), consisting of face-centered cubic (FCC) and body-centered cubic (BCC) phases, have attracted attention because of their excellent strength-ductility balance. However, the temperature dependence of hetero-deformation-induced (HDI) strengthening remains unclear. In this study, an Al$$_{7}$$(CoNiV)$$_{93}$$ DP MEA was investigated using in-situ neutron diffraction and multiscale electron microscopy. Both intrinsic strength and HDI strengthening increased at cryogenic temperature. This enhancement originated from the increased lattice friction stress of the hard BCC phase and suppressed dislocation mobility at low temperature, which promoted dislocation accumulation at heterogeneous interfaces. These findings provide insights into temperature-dependent HDI strengthening in DP H/MEAs and related alloy systems.

論文

TiC nanoparticles tune phase stability and deformation mechanisms in directed energy deposition processed Fe60Co15Ni15Cr10 medium-entropy alloy composites

Ahn, S. Y.*; Kim, E. S.*; Jeong, S. G.*; Harjo, S.; 川崎 卓郎; Gong, W.; Kim, H.-J.*; Hong, S.-J.*; Hong, S. I.*; Kwon, H.*; et al.

Materials Science & Engineering A, 955, p.149839_1 - 149839_18, 2026/03

 被引用回数:2 パーセンタイル:93.63(Nanoscience & Nanotechnology)

Additive manufacturing (AM) of particle-reinforced metal matrix composites (MMCs) enables control of both strength and deformation behavior. In this study, TiC (2 wt%) nanoparticles were added to Fe$$_{60}$$Co$$_{15}$$Ni$$_{15}$$Cr$$_{10}$$ medium-entropy alloy (MEA) using directed energy deposition (DED). Although part of the TiC decomposed during processing, the released C and Ti stabilized the $$gamma$$-austenite phase and suppressed deformation-induced martensitic transformation (DIMT), shifting deformation toward slip-dominated behavior. Microstructural observations revealed dispersed TiC particles and modified grain boundary morphology that promoted distributed plastic flow. In-situ neutron diffraction during tensile testing confirmed enhanced early-stage dislocation activity. These findings demonstrate that nanoparticle-induced phase stability changes strongly influence deformation mechanisms in AM-processed MMCs.

論文

Spin excitation continuum from degenerate states in the mixed ferro-antiferromagnetic exchange system CeMgAl$$_{11}$$O$$_{19}$$

Gao, B.*; Chen, T.*; Liu, C.*; Klemm, M. L.*; Zhang, S.*; Ma, Z.*; Xu, X.*; Won, C.*; McCandless, G. T.*; Rao, K.*; et al.

Science Advances (Internet), 12(10), p.eaed7778_1 - eaed7778_7, 2026/03

In the search for unconventional magnetism, exotic quantum states are characterized by a lack of order and a broad spin excitation continuum approaching zero temperature. We study the two-dimensional triangular-lattice effective spin-system CeMgAl$$_{11}$$O$$_{19}$$, which shows slight disorder but no magnetic ordering down to 100 millikelvin. Spin-wave analysis in the magnetic-field-polarized state determines the spin Hamiltonian featuring a mixed ferromagnetic-antiferromagnetic nearest-neighbor exchange interaction. This places the system near an exactly solvable point of the spin-triangular-lattice XXZ model with extensive ground-state degeneracy. In zero field, neutron spectroscopy reveals a prominent continuum; we show that this arises from an ensemble average of spin-wave spectra across the degenerate ground-state manifold. This demonstrates that the role of weak quenched disorder can be quantitatively constrained: It inhibits unique ground-state selection and stabilizes a local distribution within the degenerate manifold, yielding continuum-like spectra that necessitate a critical reevaluation of the experimental signatures of exotic quantum states.

論文

Surface severe plastic deformation-enabled deformation behavior control and mechanical property enhancement in metastable ferrous medium-entropy alloys

Gu, G. H.*; Jeong, S. G.*; Lee, J. H.*; Harjo, S.; Gong, W.; Amanov, A.*; Bae, J. W.*; Kwon, H.*; Kim, H. S.*

International Journal of Plasticity, 197, p.104581_1 - 104581_21, 2026/02

 被引用回数:6 パーセンタイル:80.21(Engineering, Mechanical)

Stacking fault energy (SFE) controls key deformation mechanisms in metals. This study demonstrates that apparent SFE and deformation behavior can be tuned by modifying only the near-surface microstructure ($$sim$$100 um) through surface severe plastic deformation. The resulting gradient microstructure reduces apparent SFE, promoting martensitic transformation via preferential nucleation and stress partitioning. Consequently, mechanical properties are enhanced, achieving higher strength with minimal ductility loss, highlighting the effectiveness of localized microstructural engineering.

論文

Microdosimetric analysis of proton boron capture therapy using microdosimetric kinetic model

Rahim, A.*; 佐藤 達彦; 福田 寛*; Beni, M. S.*; 渡部 浩司*

Biomedical Physics & Engineering Express (Internet), 12(1), p.015056_1 - 015056_13, 2026/01

Proton boron fusion therapy (PBFT) aims to enhance proton therapy through $$alpha$$ particles generated by the $$p + ^{11}mathrm{B} rightarrow 3alpha$$ reaction. While early reports suggested large dose gains near the Bragg peak, later studies questioned its feasibility due to the low cross section and the need for unrealistically high boron concentrations. In this study, Monte Carlo microdosimetric analysis showed that protons dominate total dose delivery, with $$alpha$$ particles contributing only locally to high-LET deposition. The resulting RBE enhancement factors were negligible at 100-1000 ppm boron and modest ($$approx 1.13$$) only at 10,000 ppm. These findings indicate that, under clinically realistic conditions, the therapeutic benefit of PBFT is minimal.

論文

Production of doubly heavy baryons with the quark-diquark description

Shim, S.-I.*; 保坂 淳

Proceedings of Science (Internet), 500, p.010_1 - 010_6, 2026/01

$$p + K^- to Xi^{*-} + K^+$$反応によって$$Xi^-$$粒子の励起状態の生成を調べた結果を報告する。

論文

Investigating the $$^{13}$$N($$alpha$$,$$p$$)$$^{16}$$O reaction rates via the $$^{19}$$F($$p$$,$$t$$)$$^{17}$$F reaction

Kim, S. H.*; Chae, K. Y.*; 浅井 雅人; 廣瀬 健太郎; 佐藤 哲也; 牧井 宏之; 西尾 勝久; Orlandi, R.; Smallcombe, J.; 洲嵜 ふみ; et al.

Journal of the Korean Physical Society, 6 Pages, 2026/00

 被引用回数:0 パーセンタイル:0.00(Physics, Multidisciplinary)

コア崩壊超新星爆発(CCSNe)の元素合成シミュレーションにおいて、$$^{13}$$N($$alpha$$,$$p$$)$$^{16}$$O反応速度の不確実性が課題となっていた。本研究では、この反応を制約するため、JAEAタンデム加速器で$$^{19}$$F($$p$$,$$t$$)$$^{17}$$F遷移反応実験を実施した。得られたトリトンスペクトルと角度分布から、関連する$$^{17}$$F共鳴の崩壊特性(部分幅)を詳細に測定し、その結果を用いて反応速度パラメータを精密化した。これにより、CCSNe核合成モデルの信頼性向上が期待できる。

論文

Mechanistic insights into deformation, load redistribution, and stress partitioning in high-strength dual-phase medium-entropy alloys

Gu, G. H.*; Ha, H.*; Harjo, S.; Gong, W.; Louzguine-Luzgin, D. V.*; Kim, H. S.*

Materials Science & Engineering A, 943, p.148818_1 - 148818_10, 2025/10

 被引用回数:4 パーセンタイル:60.79(Nanoscience & Nanotechnology)

High-strength structural alloys are essential for advanced engineering. This study explores the mechanical behavior of a dual-phase AlCoNiV medium-entropy alloy (MEA) with FCC and BCC phases. The alloy shows excellent performance, with a yield strength of 1148 MPa, tensile strength of 1556 MPa, and 40% uniform elongation. In-situ neutron diffraction and EBSD analyses reveal that strength originates from the intrinsic responses of both phases. The BCC phase carries more load, while dislocation buildup at phase boundaries enhances strength via hetero-deformation-induced (HDI) strengthening. Synergistic effects, including stress partitioning and load redistribution, further improve mechanical performance. These findings highlight the role of phase-specific properties and interphase interactions in alloy robustness and offer insights for microstructural optimization.

論文

Neutron diffraction-assisted constitutive modeling of directed energy deposited CoCrFeMnNi high entropy alloy

Jeong, S. G.*; Kwon, J.*; Kim, E. S.*; Prasad, K.*; Harjo, S.; Gong, W.; 川崎 卓郎; Estrin, Y.*; Bouaziz, O.*; Hong, S. I.*; et al.

Materials Science & Engineering A, 942, p.148712_1 - 148712_11, 2025/10

 被引用回数:2 パーセンタイル:46.97(Nanoscience & Nanotechnology)

The cellular structure plays a key role in determining the mechanical properties of metal additive manufacturing (MAM) components. This study presents in situ neutron diffraction and dislocation density-based modeling for a CoCrFeMnNi high-entropy alloy (HEA) made via directed energy deposition (DED). A constitutive model based on the Kocks-Mecking-Estrin framework was used to represent the cellular structure. Parametric analysis showed lower dislocation accumulation and annihilation rates in the as-built sample (with cellular structure) than in the heat-treated one. These differences are linked to dislocation forest networks and local stacking fault energy variations. Dislocation density across cell interiors and walls was also compared with deformation-induced dislocation cells.

論文

Magnon-induced scalar spin chirality in kagome and honeycomb ferromagnets

江崎 蘭世; Go, G.*; Kim, S. K.*

Physical Review B, 112(10), p.104440_1 - 104440_10, 2025/09

 被引用回数:0 パーセンタイル:0.00(Materials Science, Multidisciplinary)

In this study, we theoretically demonstrate that thermally excited magnons can induce scalar spin chirality (SSC) even in collinear spin systems. We show both numerically and analytically that the SSC increases with the magnitude of DMI and temperature and reveal that the magnon-induced SSC can achieve a magnitude comparable to those observed in non-coplanar spin configurations. These findings suggest that SSC plays a significant role even in collinear spin systems, providing new insights into the chiral physics of magnetic materials.

論文

L$"u$ders band-assisted high uniform ductility in ultrastrong ferrous medium-entropy alloy via hierarchical microstructure

Kwon, H.*; Lee, J. H.*; Zargaran, A.*; Harjo, S.; Gong, W.; Wang, J.*; Gu, G. H.*; Lee, B.-J.*; Bae, J. W.*; Kim, H. S.*

International Journal of Plasticity, 190, p.104378_1 - 104378_18, 2025/07

 被引用回数:15 パーセンタイル:94.66(Engineering, Mechanical)

In this work, we harness a hierarchical microstructure to simultaneously tailor strengthening and deformation mechanisms in a Co$$_{21}$$Cr$$_{12.5}$$Fe$$_{55}$$Ni$$_{4}$$Mo$$_{7.5}$$ (at%) ferrous medium-entropy alloy (MEA). A simple thermomechanical process (cold rolling and 90 s annealing) produces ultrafine recrystallized grains, non-recrystallized grains with substructures, and intragranular nanoprecipitates. This structure, with high dislocation density and fine grains, yields a high strength of $$sim$$1.60 GPa but can risk premature fracture. To overcome this, L$"u$ders deformation, enabled by ultrafine grain boundaries and stress-induced martensitic transformation at pre-existing nucleation sites, is employed. Stable L$"u$ders band propagation delays strain hardening and enables large uniform ductility. As a result, a tensile strength of $$sim$$1.84 GPa and uniform elongation of $$sim$$20% are achieved, matching the best tensile properties among reported multi-principal element alloys.

論文

Temperature-dependent deformation behavior of dual-phase medium-entropy alloy; In-situ neutron diffraction study

Gu, G. H.*; Jeong, S. G.*; Heo, Y.-U.*; Harjo, S.; Gong, W.; Cho, J.*; Kim, H. S.*; 他4名*

Journal of Materials Science & Technology, 223, p.308 - 324, 2025/07

 被引用回数:9 パーセンタイル:88.88(Materials Science, Multidisciplinary)

Face-centered cubic (FCC) equi-atomic multi-principal element alloys (MPEAs) exhibit excellent mechanical properties from cryogenic to room temperatures. At room temperature, deformation is dominated by dislocation slip, while at cryogenic temperatures (CTs), reduced stacking fault energy enhances strain hardening with twinning. This study uses in-situ neutron diffraction to analyze the temperature-dependent deformation behavior of Al$$_{7}$$(CoNiV)$$_{93}$$, a dual-phase (FCC/BCC) medium-entropy alloy (MEA). At liquid nitrogen temperature (LNT), deformation twinning in the FCC matrix leads to additional strain hardening through the dynamic Hall-Petch effect, giving the appearance of improved strengthening at LNT. In contrast, BCC precipitates show dislocation slip at both 77 K and 298 K, with temperature-dependent lattice friction stress playing a significant role in strengthening. The study enhances understanding of deformation behaviors and provides insights for future alloy design.

論文

Spin dynamics of triple-$$mathbf{Q}$$ magnetic orderings in a triangular lattice; Implications for multi-$$mathbf{Q}$$ orderings in general two-dimensional lattices

Park, P.*; Cho, W.*; Kim, C.*; An, Y.*; 飯田 一樹*; 梶本 亮一; Matin, S.*; Zhang, S.-S.*; Batista, C. D.*; Park, J.-G.*

Physical Review X, 15(3), p.031032_1 - 031032_29, 2025/07

 被引用回数:5 パーセンタイル:84.08(Physics, Multidisciplinary)

Multi-$$mathbf{Q}$$ magnetic structures on two-dimensional (2D) lattices provide a key route to realizing topological physics in 2D magnetism. A major experimental challenge is to unambiguously confirm their formation by excluding the possibility of topologically trivial multi-domain single- or double-$$mathbf{Q}$$ magnetic orders, which cannot be distinguished using conventional diffraction techniques. Here, we propose that long-wavelength spin dynamics offers a universal diagnostic for triangular lattices: triple-$$mathbf{Q}$$ orders that preserve rotational symmetry and single- or double-$$mathbf{Q}$$ orders that break it exhibit qualitatively distinct anisotropies in their Goldstone mode velocities, stemming from fundamental differences in their underlying spin configurations. We validate this concept using the metallic triangular-lattice antiferromagnet Co$$_{0.325}$$TaS$$_{2}$$, which hosts both a stripe-type single-$$mathbf{Q}$$ state and a triple-$$mathbf{Q}$$ tetrahedral ordering at different temperatures. Using inelastic neutron-scattering and spin dynamics simulations, we first refine the spin Hamiltonian by fitting the paramagnetic excitation spectra, allowing us to develop an unbiased model independent of magnetic ordering. We then show that the observed velocity profiles of the Goldstone modes agree with the high-temperature model's predictions: markedly anisotropic for the single-$$mathbf{Q}$$ phase and near isotropic for the triple-$$mathbf{Q}$$ phase. Importantly, this contrast persists across various exchange parameters, highlighting its model-independent nature and suggesting potential applicability to other 2D lattice systems. Beyond the long-wavelength regime, we present a substantial discrepancy between the measured and simulated magnon spectra exclusively in the triple-$$mathbf{Q}$$ phase. We attribute this discrepancy to magnon energy renormalization arising from order-of-magnitude-enhanced magnon-magnon interactions in the triple-$$mathbf{Q}$$ phase, due to its noncollinear configuration. This work provides universal insight into the dynamical properties of topological multi-$$mathbf{Q}$$ magnetic orderings in 2D lattice structures, offering a broadly applicable diagnostic to distinguishing them from topologically trivial single- or double-$$mathbf{Q}$$ counterparts. The unequivocal confirmation of the triple-$$mathbf{Q}$$ structure in Co$$_{0.325}$$TaS$$_{2}$$ further establishes it as a prominent material platform for exploring topological spin textures in the genuine 2D limit.

論文

Fundamental mechanisms of discontinuous deformation in metals for cryogenic-environment applications

Kim, Y. S.*; Kang, T.*; Hong, S.-K.*; Brechtl, J.*; Lebyodkin, M.*; Cheng, Y.-H.*; Huang, E.-W.*; Liaw, P. K.*; Harjo, S.; Gong, W.; et al.

Acta Materialia, 292, p.120970_1 - 120970_16, 2025/06

 被引用回数:15 パーセンタイル:96.30(Materials Science, Multidisciplinary)

Metallic materials can exhibit low-temperature serrated deformation (LTSD) at cryogenic temperatures, potentially causing sudden failures. Understanding LTSD is thus crucial for ensuring material reliability in such environments. LTSD has been explained by two main mechanisms: (i) dislocation-based mechanical instability and (ii) thermomechanical instability, but each has limitations when considered alone. To address this, we propose a new LTSD mechanism, a thermally induced dislocation dynamics model, based on cryogenic experimental evidence. This model accounts for dislocation avalanches and localized heating, leading to hierarchical dislocation networks and transitions in deformation modes. A modified deformation-mechanism map for SS316L is also presented. Our findings highlight the rate-dependent nature of LTSD and negative strain-rate sensitivity, including the first observation of links between small stress fluctuations and large serrations.

論文

Numerical simulation of coupled THM behaviour of full-scale EBS in backfilled experimental gallery in the Horonobe URL

杉田 裕; 大野 宏和; Beese, S.*; Pan, P.*; Kim, M.*; Lee, C.*; Jove-Colon, C.*; Lopez, C. M.*; Liang, S.-Y.*

Geomechanics for Energy and the Environment, 42, p.100668_1 - 100668_21, 2025/06

 被引用回数:6 パーセンタイル:87.84(Energy & Fuels)

国際共同プロジェクトDECOVALEX-2023は、数値解析を使用してベントナイト系人工バリアの熱-水-応力(または熱-水)相互作用を研究するためのタスクDとして、幌延人工バリア性能確認試験を対象とした。このタスクは、モデル化のために、1つの実物大の原位置試験と、補完的な4つの室内試験が選択された。幌延人工バリア性能確認試験は、人工的な地下水注入と組み合わせた温度制御非等温の試験であり、加熱フェーズと冷却フェーズで構成されている。6つの研究チームが、さまざまなコンピューターコード、定式化、構成法則を使用して、熱-水-応力または熱-水(研究チームのアプローチによって異なる)数値解析を実行した。

論文

Scalar spin chirality Nernst effect

Go, G.*; Goli, D. P.*; 江崎 蘭世; Tserkovnyak, Y.*; Kim, S. K.*

Physical Review Research (Internet), 7(2), p.L022066_1 - L022066_7, 2025/06

It remains an open question whether or not the scalar spin chirality itself can exhibit a Hall-type transport. In this work, we show that the answer is yes: The scalar spin chirality is Hall-transported in Kagome ferromagnets and antiferromagnets under an external bias, engendering a phenomenon which we dub the scalar spin chirality Nernst effect. Our findings call for the need to lift the conventional assumption that the scalar spin chirality is a static quantity in order to discover the active roles of the scalar spin chirality in transport properties.

論文

Soft, wearable, microfluidic system for fluorometric analysis of loss of amino acids through eccrine sweat

Cho, S. H.*; Cho, S. W.*; Lv, Z.*; 関根 由莉奈; Liu, S.*; Zhou, M.*; Nuxoll, R. F.*; Kanatzidis, E. E.*; Ghaffari, R.*; Kim, D.*; et al.

Lab on a Chip, 25(7), p.1647 - 1655, 2025/04

 被引用回数:16 パーセンタイル:98.61(Biochemical Research Methods)

アミノ酸は体内のタンパク質合成と代謝プロセスに不可欠な物質である。本研究では、運動中の汗からのアミノ酸損失について定量的に調べることを目的とした。汗中のアミノ酸含有量をリアルタイムで分析するため、測定のための技術基盤としてウェアラブルなマイクロ流体システムを構築した。定量分析を実現するため、ウェアラブルデバイスに蛍光アッセイを組み込み、さらにスマートフォンベースの画像化技術を統合させたシステムを開発した。

論文

Comparative analysis of primary variables selection in modeling non-isothermal two-phase flow; Insights from EBS experiment at Horonobe URL

Kim, M.*; Lee, C.*; 杉田 裕; Kim, J.-S.*; Jeon, M.-K.*

Geomechanics for Energy and the Environment, 41, p.100628_1 - 100628_9, 2025/03

 被引用回数:2 パーセンタイル:53.68(Energy & Fuels)

この研究では、DECOVALEX-2023プロジェクトの一環として幌延の地下研究施設で実施された実規模大の人工バリア試験の数値解析を使用して、非等温二相流のモデリングに対する主要変数の選択の影響を調査した。検証済みの数値モデルを使用して、人工バリアシステム内の不均質多孔質媒体の熱-水連成挙動を解析した。支配方程式を離散化する際の2つの異なる主要変数スキームを比較したところ、結果に大きな違いがあることが明らかになった。

論文

Structural behaviors of lead zirconate titanate-based ferroelectric ceramics during pyroelectric-power generation cycles

川崎 卓郎; 福田 竜生; 山中 暁*; 村山 一郎*; 加藤 孝典*; 馬場 将亮*; 橋本 英樹*; Harjo, S.; 相澤 一也; 田中 裕久*; et al.

Journal of Applied Physics, 137(9), p.094101_1 - 094101_7, 2025/03

 被引用回数:1 パーセンタイル:28.15(Physics, Applied)

Energy harvesting from waste heat can improve energy efficiency in society. This research investigated the structural behaviors of lead zirconate titanate-based ferroelectric ceramics using operando neutron diffraction measurements under the conditions of two energy-harvesting cycles that involve consideration of the temperature changes of automobile exhaust gas for achieving good harvesting efficiencies. Input and output electrical energies and neutron diffraction data were simultaneously collected. The obtained time-resolved neutron-diffraction intensity data indicate that the applied electric fields and temperature changes induced 90$$^{circ}$$ domain rotation and lattice strain. These structural changes and their variations depending on cycle conditions, such as temperature changes, applied electric fields, and circuit switching, provide insight into the origins of the differences in the behaviors of electrical input/output energies in the cycles.

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