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Journal Articles

Chemical characterization of a volatile dubnium compound, DbOCl$$_3$$

Chiera, N. M.*; Sato, Tetsuya; Eichler, R.*; Tomitsuka, Tomohiro; Asai, Masato; Adachi, Sadia*; Dressler, R.*; Hirose, Kentaro; Inoue, Hiroki*; Ito, Yuta; et al.

Angewandte Chemie; International Edition, 60(33), p.17871 - 17874, 2021/08

 Times Cited Count:5 Percentile:20.47(Chemistry, Multidisciplinary)

The formation and the chemical characterization of single atoms of dubnium (Db, element 105), in the form of its volatile oxychloride, was investigated using the on-line gas phase chromatography technique, in the temperature range 350 - 600 $$^circ$$C. Under the exact same chemical conditions, comparative studies with the lighter homologs of group-5 in the Periodic Table clearly indicate the volatility sequence being NbOCl$$_3 > $$ TaOCl$$_3 geq$$ DbOCl$$_3$$. From the obtained experimental results, thermochemical data for DbOCl$$_3$$ were derived. The present study delivers reliable experimental information for theoretical calculations on the chemical properties of transactinides.

JAEA Reports

Annual report on the environmental radiation monitoring around the Tokai Reprocessing Plant FY2013

Watanabe, Hitoshi; Nakano, Masanao; Fujita, Hiroki; Takeyasu, Masanori; Mizutani, Tomoko; Isozaki, Tokuju; Morisawa, Masato; Nagaoka, Mika; Hokama, Tomonori; Yokoyama, Hiroya; et al.

JAEA-Review 2014-042, 175 Pages, 2015/01

JAEA-Review-2014-042.pdf:10.89MB

Environmental radiation monitoring around the Tokai Reprocessing Plant has been performed by the Nuclear Fuel Cycle Engineering Laboratories, based on "Safety Regulations for the Reprocessing Plant of Japan Atomic Energy Agency, Chapter IV - Environmental Monitoring". This annual report presents the results of the environmental monitoring and the dose estimation to the hypothetical inhabitant due to the radioactivity discharged from the plant to the atmosphere and the sea during April 2013 to March 2014. In this report, some data include the influence of the accidental release from the Fukushima Daiichi Nuclear Power Plant of Tokyo Electric Power Co. in March 2011.

JAEA Reports

Annual report on the environmental radiation monitoring around the Tokai Reprocessing Plant FY2012

Sumiya, Shuichi; Watanabe, Hitoshi; Miyagawa, Naoto; Nakano, Masanao; Nakada, Akira; Fujita, Hiroki; Takeyasu, Masanori; Isozaki, Tokuju; Morisawa, Masato; Mizutani, Tomoko; et al.

JAEA-Review 2013-056, 181 Pages, 2014/03

JAEA-Review-2013-056.pdf:6.22MB

Environmental radiation monitoring around the Tokai Reprocessing Plant has been performed by the Nuclear Fuel Cycle Engineering Laboratories, based on "Safety Regulations for the Reprocessing Plant of Japan Atomic Energy Agency, Chapter IV - Environmental Monitoring". This annual report presents the results of the environmental monitoring and the dose estimation to the hypothetical inhabitant due to the radioactivity discharged from the plant to the atmosphere and the sea during April 2012 to March 2013. In this report, some data include the influence of the accidental release from the Fukushima Daiichi Nuclear Power Plant of Tokyo Electric Power Co. in March 2011.

JAEA Reports

Annual report on the environmental radiation monitoring around the Tokai Reprocessing Plant FY2011

Sumiya, Shuichi; Watanabe, Hitoshi; Nakano, Masanao; Takeyasu, Masanori; Nakada, Akira; Fujita, Hiroki; Isozaki, Tokuju; Morisawa, Masato; Mizutani, Tomoko; Nagaoka, Mika; et al.

JAEA-Review 2013-009, 195 Pages, 2013/06

JAEA-Review-2013-009.pdf:3.35MB

Environmental radiation monitoring around the Tokai Reprocessing Plant has been performed by the Nuclear Fuel Cycle Engineering Laboratories, based on "Safety Regulations for the Reprocessing Plant of Japan Atomic Energy Agency, Chapter IV - Environmental Monitoring". This annual report presents the results of the environmental monitoring and the dose estimation to the hypothetical inhabitant due to the radioactivity discharged from the plant to the atmosphere and the sea during April 2011 to March 2012. In this report, some data include the influence of the accidental release from the Fukushima Daiichi Nuclear Power Plant on Tokyo Electric Power Co. in March 2011.

JAEA Reports

Annual report on the environmental radiation monitoring around the Tokai Reprocessing Plant FY2010

Sumiya, Shuichi; Watanabe, Hitoshi; Nakano, Masanao; Takeyasu, Masanori; Nakada, Akira; Fujita, Hiroki; Isozaki, Tokuju; Morisawa, Masato; Mizutani, Tomoko; Kokubun, Yuji; et al.

JAEA-Review 2012-015, 166 Pages, 2012/05

JAEA-Review-2012-015.pdf:3.53MB

Environmental radiation monitoring around the Tokai Reprocessing Plant has been performed by the Nuclear Fuel Cycle Engineering Laboratories, based on "Safety Regulations for the Reprocessing Plant of Japan Atomic Energy Agency, Chapter IV - Environmental Monitoring". This annual report presents the results of the environmental monitoring and the dose estimation to the hypothetical inhabitant due to the radioactivity discharged from the plant to the atmosphere and the sea during April 2010 to March 2011. In this report, some data include the influence of the accidental release from the Fukushima Daiichi Nuclear Power Plant on Tokyo Electric Power Co. in 2011 March. Appendices present comprehensive information, such as monitoring program, monitoring methods, monitoring results and their trends, meteorological data and discharged radioactive wastes. In addition, the data exceeded the normal range of fluctuation by the accidental release was evaluated in the appendices.

Journal Articles

Progress in development and design of the neutral beam injector for JT-60SA

Hanada, Masaya; Kojima, Atsushi; Tanaka, Yutaka; Inoue, Takashi; Watanabe, Kazuhiro; Taniguchi, Masaki; Kashiwagi, Mieko; Tobari, Hiroyuki; Umeda, Naotaka; Akino, Noboru; et al.

Fusion Engineering and Design, 86(6-8), p.835 - 838, 2011/10

 Times Cited Count:16 Percentile:72.13(Nuclear Science & Technology)

Neutral beam (NB) injectors for JT-60 Super Advanced (JT-60SA) have been designed and developed. Twelve positive-ion-based and one negative-ion-based NB injectors are allocated to inject 30 MW D$$^{0}$$ beams in total for 100 s. Each of the positive-ion-based NB injector is designed to inject 1.7 MW for 100s at 85 keV. A part of the power supplies and magnetic shield utilized on JT-60U are upgraded and reused on JT-60SA. To realize the negative-ion-based NB injector for JT-60SA where the injection of 500 keV, 10 MW D$$^{0}$$ beams for 100s is required, R&Ds of the negative ion source have been carried out. High-energy negative ion beams of 490-500 keV have been successfully produced at a beam current of 1-2.8 A through 20% of the total ion extraction area, by improving voltage holding capability of the ion source. This is the first demonstration of a high-current negative ion acceleration of $$>$$1 A to 500 keV. The design of the power supplies and the beamline is also in progress. The procurement of the acceleration power supply starts in 2010.

Journal Articles

Development of the JT-60SA Neutral Beam Injectors

Hanada, Masaya; Kojima, Atsushi; Inoue, Takashi; Watanabe, Kazuhiro; Taniguchi, Masaki; Kashiwagi, Mieko; Tobari, Hiroyuki; Umeda, Naotaka; Akino, Noboru; Kazawa, Minoru; et al.

AIP Conference Proceedings 1390, p.536 - 544, 2011/09

 Times Cited Count:7 Percentile:83.71(Physics, Atomic, Molecular & Chemical)

no abstracts in English

Journal Articles

Achievement of 500 keV negative ion beam acceleration on JT-60U negative-ion-based neutral beam injector

Kojima, Atsushi; Hanada, Masaya; Tanaka, Yutaka*; Kawai, Mikito*; Akino, Noboru; Kazawa, Minoru; Komata, Masao; Mogaki, Kazuhiko; Usui, Katsutomi; Sasaki, Shunichi; et al.

Nuclear Fusion, 51(8), p.083049_1 - 083049_8, 2011/08

 Times Cited Count:53 Percentile:87.84(Physics, Fluids & Plasmas)

Hydrogen negative ion beams of 490 keV, 3 A and 510 keV, 1 A have been successfully produced in the JT-60 negative ion source with three acceleration stages. These successful productions of the high-energy beams at high current have been achieved by overcoming the most critical issue, i.e., a poor voltage holding of the large negative ion sources with the grids of 2 m$$^{2}$$ for JT-60SA and ITER. To improve voltage holding capability, the breakdown voltages for the large grids was examined for the first time. It was found that a vacuum insulation distance for the large grids was 6-7 times longer than that for the small-area grid (0.02 m$$^{2}$$). From this result, the gap lengths between the grids were tuned in the JT-60 negative ion source. The modification of the ion source also realized a significant stabilization of voltage holding and a short conditioning time. These results suggest a practical use of the large negative ion sources in JT-60SA and ITER.

JAEA Reports

Annual report on the environmental radiation monitoring around the Tokai Reprocessing Plant FY2009

Sumiya, Shuichi; Matsuura, Kenichi; Watanabe, Hitoshi; Nakano, Masanao; Takeyasu, Masanori; Fujita, Hiroki; Isozaki, Tokuju; Morisawa, Masato; Mizutani, Tomoko; Kokubun, Yuji; et al.

JAEA-Review 2011-004, 161 Pages, 2011/03

JAEA-Review-2011-004.pdf:4.09MB

Environmental radiation monitoring around the Tokai Reprocessing Plant has been performed by the Nuclear Fuel Cycle Engineering Laboratories, based on "Safety Regulations for the Reprocessing Plant of Japan Atomic Energy Agency, Chapter IV - Environmental Monitoring". This annual report presents the results of the environmental monitoring and the dose estimation to the hypothetical inhabitant due to the radioactivity discharged from the plant to the atmosphere and the sea during April 2009 to March 2010. Appendices present comprehensive information, such as monitoring program, monitoring methods, monitoring results and their trends, meteorological data and discharged radioactive wastes.

Journal Articles

Demonstration of 500 keV beam acceleration on JT-60 negative-ion-based neutral beam injector

Kojima, Atsushi; Hanada, Masaya; Tanaka, Yutaka*; Kawai, Mikito*; Akino, Noboru; Kazawa, Minoru; Komata, Masao; Mogaki, Kazuhiko; Usui, Katsutomi; Sasaki, Shunichi; et al.

Proceedings of 23rd IAEA Fusion Energy Conference (FEC 2010) (CD-ROM), 8 Pages, 2011/03

Hydrogen negative ion beams of 490keV, 3A and 510 keV, 1A have been successfully produced in the JT-60 negative ion source with three acceleration stages. These successful productions of the high-energy beams at high current have been achieved by overcoming the most critical issue, i.e., a poor voltage holding of the large negative ion sources with the grids of $$sim$$ 2 m$$^{2}$$ for JT-60SA and ITER. To improve voltage holding capability, the breakdown voltages for the large grids was examined for the first time. It was found that a vacuum insulation distance for the large grids was 6-7 times longer than that for the small-area grid (0.02 m$$^{2}$$). From this result, the gap lengths between the grids were tuned in the JT-60 negative ion source. The modification of the ion source also realized a significant stabilization of voltage holding and a short conditioning time. These results suggest a practical use of the large negative ion sources in JT-60 SA and ITER.

Journal Articles

Development and design of the negative-ion-based NBI for JT-60 Super Advanced

Hanada, Masaya; Akino, Noboru; Endo, Yasuei; Inoue, Takashi; Kawai, Mikito; Kazawa, Minoru; Kikuchi, Katsumi; Komata, Masao; Kojima, Atsushi; Mogaki, Kazuhiko; et al.

Journal of Plasma and Fusion Research SERIES, Vol.9, p.208 - 213, 2010/08

A large negative ion source with an ion extraction area of 110 cm $$times$$ 45 cm has been developed to produce 500 keV, 22 A D$$^{-}$$ ion beams required for JT-60 Super Advanced. To realize the JT-60SA negative ion source, the JT-60 negative ion source has been modified and tested on the negative-ion-based neutral beam injector on JT-60U. A 500 keV H$$^{-}$$ ion beam has been produced at 3 A without a significant degradation of beam optics. This is the first demonstration of a high energy negative ion acceleration of more than one-ampere to 500 keV in the world. The beam current density of 90 A/m$$^{2}$$ is being increased to meet 130 A/m$$^{2}$$ of the design value for JT-60SA by tuning the operation parameters. A long pulse injection of 30 s has been achieved at a injection D$$^{0}$$ power of 3 MW. The injection energy, defined as the product of the injection time and power, reaches 80 MJ by neutralizing a 340 keV, 27 A D$$^{-}$$ ion beam produced with two negative ion sources.

JAEA Reports

Annual report on the environmental radiation monitoring around the Tokai Reprocessing Plant FY2008

Takeishi, Minoru; Sumiya, Shuichi; Matsuura, Kenichi; Watanabe, Hitoshi; Nakano, Masanao; Takeyasu, Masanori; Isozaki, Hisaaki*; Isozaki, Tokuju; Morisawa, Masato; Fujita, Hiroki; et al.

JAEA-Review 2009-048, 177 Pages, 2009/12

JAEA-Review-2009-048.pdf:19.3MB
JAEA-Review-2009-048(errata).pdf:0.12MB

Environmental radiation monitoring around the Tokai Reprocessing Plant has been performed by the Nuclear Fuel Cycle Engineering Laboratories, based on "Safety Regulations for the Reprocessing Plant of Japan Atomic Energy Agency, Chapter IV; Environmental Monitoring". This annual report presents the results of the environmental monitoring and the dose estimation to the hypothetical inhabitant due to the radioactivity discharged from the plant to the atmosphere and the sea during April 2008 to March 2009. Appendices present comprehensive information, such as monitoring program, monitoring methods, monitoring results and their trends, meteorological data and discharged radioactive wastes.

JAEA Reports

Annual report on the environmental radiation monitoring around the Tokai Reprocessing Plant FY2007

Takeishi, Minoru; Matsuura, Kenichi; Watanabe, Hitoshi; Nakano, Masanao; Takeyasu, Masanori; Isozaki, Hisaaki; Isozaki, Tokuju; Morisawa, Masato; Fujita, Hiroki; Kokubun, Yuji; et al.

JAEA-Review 2008-057, 155 Pages, 2008/11

JAEA-Review-2008-057.pdf:2.15MB

Environmental radiation monitoring around the Tokai Reprocessing Plant has been performed by the Nuclear Fuel Cycle Engineering Laboratories, based on "Safety Regulations for the Reprocessing Plant of JAEA, Chapter IV; Environmental Monitoring". This annual report presents the results of the environmental monitoring and the dose estimation to the hypothetical inhabitant due to the radioactivity discharged to the atmosphere and the sea during April 2007 to March 2008. Appendices present comprehensive information, such as monitoring program, monitoring methods, monitoring results and its trends, meteorological data and discharged radioactive wastes.

Journal Articles

Recent R&D activities of negative-ion-based ion source for JT-60SA

Ikeda, Yoshitaka; Hanada, Masaya; Kamada, Masaki; Kobayashi, Kaoru; Umeda, Naotaka; Akino, Noboru; Ebisawa, Noboru; Inoue, Takashi; Honda, Atsushi; Kawai, Mikito; et al.

IEEE Transactions on Plasma Science, 36(4), p.1519 - 1529, 2008/08

 Times Cited Count:13 Percentile:45.21(Physics, Fluids & Plasmas)

The JT-60SA N-NBI system is required to inject 10 MW for 100 s at 500 keV. Three key issues should be solved for the JT-60SA N-NBI ion source. One is to improve the voltage holding capability. Recent R&D tests suggested that the accelerator with a large area of grids may need a high margin in the design of electric field and a long time for conditioning. The second issue is to reduce the grid power loading. It was found that some beamlets were strongly deflected due to beamlet-beamlet interaction and strike on the grounded grid. The grids are to be designed by taking account of beamlet-beamlet interaction in three-dimensional simulation. Third is to maintain the D- production for 100 s. A simple cooling structure is proposed for the active cooled plasma grid, where a key is the temperature gradient on the plasma grid for uniform D- production. The modified N-NBI ion source will start on JT-60SA in 2015.

JAEA Reports

Annual report on the environmental radiation monitoring around the Tokai Reprocessing Plant FY2006

Takeishi, Minoru; Miyagawa, Naoto; Nakano, Masanao; Takeyasu, Masanori; Isozaki, Hisaaki; Isozaki, Tokuju; Morisawa, Masato; Fujita, Hiroki; Kokubun, Yuji; Kato, Chiaki; et al.

JAEA-Review 2007-044, 155 Pages, 2008/02

JAEA-Review-2007-044.pdf:2.58MB
JAEA-Review-2007-044(errata).pdf:0.13MB

Environmental radiation monitoring around the Tokai Reprocessing Plant has been performed by the Nuclear Fuel Cycle Engineering Laboratories, based on "Safety Regulations for the Reprocessing Plant of JAEA, Chapter 4; Environmental Monitoring". This annual report presents the results of the environmental monitoring and the dose estimation to the hypothetical inhabitant due to the radioactivity discharged to the atmosphere and the sea during April 2006 to March 2007. Appendices present comprehensive information, such as monitoring program, monitoring methods, monitoring results and its trends, meteorological data and discharged radioactive wastes.

Journal Articles

Technical design of NBI system for JT-60SA

Ikeda, Yoshitaka; Akino, Noboru; Ebisawa, Noboru; Hanada, Masaya; Inoue, Takashi; Honda, Atsushi; Kamada, Masaki; Kawai, Mikito; Kazawa, Minoru; Kikuchi, Katsumi; et al.

Fusion Engineering and Design, 82(5-14), p.791 - 797, 2007/10

 Times Cited Count:25 Percentile:81.85(Nuclear Science & Technology)

Modification of JT-60U to a superconducting device (so called JT-60SA) has been planned to contribute to ITER and DEMO. The NBI system is required to inject 34 MW for 100 s. The upgraded NBI system consists of twelve positive ion based NBI (P-NBI) units and one negative ion based NBI (N-NBI) unit. The injection power of the P-NBI units are 2 MW each at 85 keV, and the N-NBI unit will be 10 MW at 500 keV, respectively. On JT-60U, the long pulse operation of 30 s at 2 MW (85 keV) and 20 s at 3.2 MW (320 keV) have been achieved on P-NBI and N-NBI units, respectively. Since the temperature increase of the cooling water in both ion sources is saturated within 20 s, further pulse extension up to 100 s is expected to mainly modify the power supply systems in addition to modification of the N-NBI ion source for high acceleration voltage. The detailed technical design of the NBI system for JT-60SA is presented.

JAEA Reports

Annual report on the environmental radiation monitoring around Tokai Reprocessing Plant FY2005

Takeishi, Minoru; Miyagawa, Naoto; Nakano, Masanao; Takeyasu, Masanori; Isozaki, Hisaaki; Isozaki, Tokuju; Morisawa, Masato; Fujita, Hiroki; Kokubun, Yuji; Kato, Chiaki; et al.

JAEA-Review 2006-031, 155 Pages, 2006/10

JAEA-Review-2006-031.pdf:7.76MB
JAEA-Review-2006-031(errata).pdf:0.13MB

Environmental radiation monitoring around the Tokai Reprocessing Plant has been performed by the Nuclear Fuel Cycle Engineering Laboratories, based on "Safety Regulations for the Reprocessing Plant of JAEA, Chapter IV - Environmental Monitoring". This annual report presents the results of the environmental monitoring and the dose estimation to the hypothetical inhabitant due to the radioactivity discharged to the atmosphere and the sea during April 2005 to March 2006. Appendices present comprehensive information, such as monitoring program, monitoring methods, monitoring results and its trends, meteorological data and discharged radioactive wastes.

Journal Articles

Present status of the negative ion based NBI system for long pulse operation on JT-60U

Ikeda, Yoshitaka; Umeda, Naotaka; Akino, Noboru; Ebisawa, Noboru; Grisham, L. R.*; Hanada, Masaya; Honda, Atsushi; Inoue, Takashi; Kawai, Mikito; Kazawa, Minoru; et al.

Nuclear Fusion, 46(6), p.S211 - S219, 2006/06

 Times Cited Count:62 Percentile:87.04(Physics, Fluids & Plasmas)

Recently, the extension of the pulse duration up to 30 sec has been intended to study quasi-steady state plasma on JT-60U N-NBI system. The most serious issue is to reduce the heat load on the grids for long pulse operation. Two modifications have been proposed to reduce the heat load. One is to suppress the beam spread which may be caused by beamlet-beamlet interaction in the multi-aperture grid due to the space charge force. Thin plates were attached on the extraction grid to modify the local electric field. The plate thickness was optimized to steer the beamlet deflection. The other is to reduce the stripping loss, where the electron of the negative ion beam is stripped and accelerated in the ion source and then collides with the grids. The ion source was modified to reduce the pressure in the accelerator column to suppress the beam-ion stripping loss. Up to now, long pulse injection of 17 sec for 1.6 MW and 25 sec for $$sim$$1 MW has been obtained by one ion source with these modifications.

Journal Articles

Beam deflection by plasma grid filter current in the negative-ion source for JT-60U neutral beam injection system

Umeda, Naotaka; Ikeda, Yoshitaka; Hanada, Masaya; Inoue, Takashi; Kawai, Mikito; Kazawa, Minoru; Komata, Masao; Mogaki, Kazuhiko; Oga, Tokumichi

Review of Scientific Instruments, 77(3), p.03A529_1 - 03A529_3, 2006/03

 Times Cited Count:6 Percentile:33.21(Instruments & Instrumentation)

no abstracts in English

Journal Articles

Recent progress of negative ion based neutral beam injector for JT-60U

Umeda, Naotaka; Yamamoto, Takumi; Hanada, Masaya; Grisham, L. R.*; Kawai, Mikito; Oga, Tokumichi; Akino, Noboru; Inoue, Takashi; Kazawa, Minoru; Kikuchi, Katsumi*; et al.

Fusion Engineering and Design, 74(1-4), p.385 - 390, 2005/11

 Times Cited Count:9 Percentile:51.95(Nuclear Science & Technology)

In negative ion based neutral beam injector (N-NBI) for JT-60U, some modifications for extent pulse duration from 10 second, which is design value, to 30 second was conducted. Main limit to prevent pulse extension was heat loads onto grounded grid in an ion source and onto beam limiter placed at 22 m from the ion source. To reduce these heat loads, beam extraction area was optimized and the limiter was changed to one which had about twice thermal capacity. As a result of these modifications, the temperature rise of the water which was cooling grounded grid could be suppressed under 40 degree, which can operate in steady state condition. The temperature rise of the limiter could be restricted to 60%. Untill now the beam pulse extended to 17 second of 1.6MW power at 366keV energy, and injection of 30 seconds will be achieved in next experiment.

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