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Status of neutron spectrometers at J-PARC

梶本 亮一; 横尾 哲也*; 中村 充孝; 川北 至信; 松浦 直人*; 遠藤 仁*; 瀬戸 秀紀*; 伊藤 晋一*; 中島 健次; 河村 聖子

Physica B; Condensed Matter, 562, p.148 - 154, 2019/06

 被引用回数:1 パーセンタイル:70.75(Physics, Condensed Matter)

Seven time-of-flight quasielastic/inelastic neutron scattering instruments are installed on six beamlines in the Materials and Life Science Experimental Facility (MLF) at the Japan Proton Accelerator Research Complex (JPARC). Four of these instruments are chopper-type direct-geometry spectrometers, one is a near-backscattering indirect-geometry spectrometer, and the other two are spin-echo-type spectrometers. This paper reviews the characteristic features, recent scientific outcomes, and progress in development of MLF spectrometers.


Safe and rapid development of capillary electrophoresis for ultratrace uranyl ions in radioactive samples by way of fluorescent probe selection for actinide ions from a chemical library

原賀 智子; 大内 和希; 佐藤 義行; 星野 仁*; 田中 玲*; 藤原 隆司*; 黒川 秀樹*; 渋川 雅美*; 石森 健一郎; 亀尾 裕; et al.

Analytica Chimica Acta, 1032, p.188 - 196, 2018/11

 被引用回数:4 パーセンタイル:55.91(Chemistry, Analytical)



Isotope-selective microscale imaging of radioactive Cs without isobaric interferences using sputtered neutral mass spectrometry with two-step resonant ionization employing newly-developed Ti:Sapphire lasers

坂本 哲夫*; 森田 真人*; 金成 啓太*; 富田 英生*; Sonnenschein, V.*; 齊藤 洸介*; 大橋 雅也*; 加藤 弘太郎*; 井口 哲夫*; 河合 利秀*; et al.

Analytical Sciences, 34(11), p.1265 - 1270, 2018/11

 被引用回数:3 パーセンタイル:65.72(Chemistry, Analytical)

Characterization of radionuclides in Fukushima is important to determine their origins and current state in the environment. Radionuclides exist as fine particles and are mixed with other constituents. A measurement method with both micro-imaging capability and highly selective element detection is necessary to analyze these particles. We developed such an imaging technique using a time-of-flight secondary ion mass spectrometry and wavelength tunable Ti:Sapphire lasers for resonance ionization of target elements without mass interference. This is called resonant laser ionization sputtered neutral mass spectrometry. The instrument has high lateral resolution and higher ionization selectivity using two-step resonance excitation of Cs with two lasers at different wavelengths. Optimization of the wavelength for resonance ionization using a Cs compound was performed, and a real environmental particle containing radioactive Cs was analyzed. Isotope images of three kinds of Cs were successfully obtained without interfere from Ba isotopes for the first time.


第4世代原子炉の開発動向,7; ナトリウム冷却高速炉(SFR)

上出 英樹; 伊藤 隆哉*; 小竹 庄司*

日本原子力学会誌, 60(9), p.562 - 566, 2018/09

ナトリウム冷却高速炉は、ウラン資源の利用率を飛躍的に向上させるとともに、プルトニウム他の長寿命TRU核種を効率的に燃焼させ、使用済み燃料の減容化・潜在的な有害度低減を可能にする優れたポテンシャルを持ち、実証段階へと進みつつある有望な高速炉概念である。ロシアのBN-800が2016年10月より商業運転を開始したことはその実用化に向けて大きな一歩であり、ロシアはこれにより商用段階に入ったとしており、次期炉であるBN-1200ではGIFの掲げる安全性, 経済性目標の達成を目指している。中国では600MWeの実証炉の建設を開始し、インドは原型炉PFBRの運開を目前に控え、これに続き実用炉6基の建設計画を有している。ここでは各国のナトリウム冷却炉の開発の進展を概観するとともに、日本における開発状況と今後の方向性をまとめた。


Anisotropic magnetic fluctuations in ferromagnetic superconductor UGe$$_2$$; $$^{73}$$Ge-NQR study at ambient pressure

野間 雄一郎*; 小手川 恒*; 久保 徹郎*; 藤 秀樹*; 播磨 尚朝*; 芳賀 芳範; 山本 悦嗣; 大貫 惇睦*; 伊藤 公平*; Haller, E. E.*; et al.

Journal of the Physical Society of Japan, 87(3), p.033704_1 - 033704_5, 2018/03

 被引用回数:3 パーセンタイル:46.46(Physics, Multidisciplinary)

$$^{73}$$Ge nuclear quadrupole resonance study of ferromagnetic superconductor UGe$$_2$$ is reported. Detailed analyses successfully assigned crystallographic sites of Ge atoms. The measurement of the nuclear spin-lattice relaxation rate revealed highly anisotropic magnetic fluctuations.


Materials and Life Science Experimental Facility (MLF) at the Japan Proton Accelerator Research Complex, 2; Neutron scattering instruments

中島 健次; 川北 至信; 伊藤 晋一*; 阿部 淳*; 相澤 一也; 青木 裕之; 遠藤 仁*; 藤田 全基*; 舟越 賢一*; Gong, W.*; et al.

Quantum Beam Science (Internet), 1(3), p.9_1 - 9_59, 2017/12



Evaluation of bending strain in Nb$$_{3}$$Sn strands of CIC conductor using neutron diffraction

辺見 努*; Harjo, S.; 梶谷 秀樹*; 諏訪 友音*; 齊藤 徹*; 相澤 一也; 長村 光造*; 小泉 徳潔*

IEEE Transactions on Applied Superconductivity, 27(4), p.4200905_1 - 4200905_5, 2017/06

The superconducting property of Nb$$_{3}$$Sn strands is very sensitive to strain. The transverse electromagnetic loading has been considered as a major origin of the degradation of Nb$$_{3}$$Sn cable-in-conduit conductors (CICCs) due to the local bending. Since the bending pitch is around 5 mm due to contacting of strands compacted by the electromagnetic transverse loading, there is a possibility of a large bending strain with small deflection of strands. The bending strain of the strands cannot be evaluated from only the small deflection obtained visually. Measuring bending strain of Nb$$_{3}$$Sn strand in CICCs is important for evaluating the conductor performance. Neutrons, which have a large penetration depth, are a powerful tool to evaluate the internal strain of Nb$$_{3}$$Sn in the CICC. This paper shows that the bending strain in Nb$$_{3}$$Sn strands of CICCs can be determined by the neutron diffraction profile nondestructively and quantitatively.


Study on reactor vessel coolability of sodium-cooled fast reactor under severe accident condition; Water experiments using a scale model

小野 綾子; 栗原 成計; 田中 正暁; 大島 宏之; 上出 英樹; 三宅 康洋*; 伊藤 真美*; 中根 茂*

Proceedings of 2017 International Congress on Advances in Nuclear Power Plants (ICAPP 2017) (CD-ROM), 10 Pages, 2017/04



Study on the deterioration mechanism of layered rock-salt electrodes using epitaxial thin films; Li(Ni, Co, Mn)O$$_{2}$$ and their Zr-O surface modified electrodes

阿部 真知子*; 射場 英紀*; 鈴木 耕太*; 南嶋 宏映*; 平山 雅章*; 田村 和久; 水木 純一郎*; 齋藤 智浩*; 幾原 雄一*; 菅野 了次*

Journal of Power Sources, 345, p.108 - 119, 2017/03

 被引用回数:7 パーセンタイル:51.59(Chemistry, Physical)

Ni, Co, Mn三元系リチウムイオン電池正極材料について、その劣化機構について、電気化学測定、X線・中性子線測定により調べた。実験の結果、Ni, Co, Mn三元系正極は、層状岩塩型構造とスピネル構造で構成されており、充放電を繰り返すと、充放電に関与しないスピネル構造が表面を覆っていくことが分かった。一方で、Zr-Oで表面をコートした材料は劣化しないことが知られており、その原因を調べた結果、層状岩塩型構造が安定に存在し続けていることが分かった。さらに、電極/溶液界面のLi濃度を上昇していることも分かった。


Inelastic and quasi-elastic neutron scattering spectrometers in J-PARC

瀬戸 秀紀; 伊藤 晋一; 横尾 哲也*; 遠藤 仁*; 中島 健次; 柴田 薫; 梶本 亮一; 河村 聖子; 中村 充孝; 川北 至信; et al.

Biochimica et Biophysica Acta; General Subjects, 1861(1), p.3651 - 3660, 2017/01

 被引用回数:17 パーセンタイル:16.28(Biochemistry & Molecular Biology)




江連 俊樹; 伊藤 啓; 亀山 祐理*; 上出 英樹; 功刀 資彰*

日本原子力学会和文論文誌, 15(3), p.151 - 158, 2016/09



Study on behavior of vortex cavitation around suction pipes in sodium-cooled fast reactor geometry

江連 俊樹; 伊藤 啓; 上出 英樹; 功刀 資彰*

Thermal Science and Engineering, 24(3), p.31 - 38, 2016/07

Vortex cavitation behavior is studied using a 1/22 scaled upper plenum water model of advanced loop-type sodium-cooled fast reactor. Vortex cavitation occurrences are quantitatively grasped through visualization measurements including its transient behavior under various conditions of inlet velocity of suction pipe, water temperature and system pressure. In addition, the relation between local velocity around vortex and vortex cavitation occurrences are investigated based on results from visualization and Particle Image Velocimetry measurements. Experimental results show the difficulty of evaluation of vortex cavitation occurrences simply based on cavitation factor. And also, vortex evaluation with local circulation shows the effectiveness to organize the vortex cavitation occurrences via the evaluation of pressure decrease using vortex model.


Science from the initial operation of HRC

伊藤 晋一*; 横尾 哲也*; 益田 隆嗣*; 吉澤 英樹*; 左右田 稔*; 池田 陽一*; 井深 壮史*; 川名 大地*; 佐藤 卓*; 南部 雄亮*; et al.

JPS Conference Proceedings (Internet), 8, p.034001_1 - 034001_6, 2015/09

Since the installation of the High Resolution Chopper Spectrometer, HRC, experiments using the HRC are being conducted to observe the dynamics in wide range of physics. Scientific results during the period since the initial construction are summarized.


Accuracy of prediction method of cryogenic tensile strength for austenitic stainless steels in ITER toroidal field coil structure

櫻井 武尊; 井口 将秀; 中平 昌隆; 斎藤 徹*; 森本 将明*; 稲垣 隆*; Hong, Y.-S.*; 松井 邦浩; 辺見 努; 梶谷 秀樹; et al.

Physics Procedia, 67, p.536 - 542, 2015/07

 被引用回数:1 パーセンタイル:44.56

原子力機構はこれまで、極低温で使用されるITER超伝導コイルに適用するオーステナイト系ステンレス鋼の合理的な品質管理手法の開発確立を目的に、室温で測定された引張強さと、炭素と窒素の含有量の関数として二次曲線を用いた4Kでの引張強度予測手法を開発してきた。核融合発電の技術的成立の実証を目指して建設が進んでいるITERでは、超伝導コイルが使用される。超伝導コイルシステムの一つであるTFコイルの容器構造物には巨大な電磁力に耐えるため、構造材料として高マンガンステンレス鋼JJ1及び高窒素添加型316LNが使用される。原子力機構はITER TFコイル構造物の調達責任を負っており、2012年から実機構造材料調達を開始し、矩形材,丸棒材,異形鍛造材などの製造を進めている。原子力機構は、構造材料の高マンガンステンレス鋼JJ1及び高窒素添加型316LNの機械特性を多数取得しており、本研究ではこれらの試験データを用いて、原子力機構が開発してきた4K強度予測手法の実機TFコイル構造物用材料に対する予測精度について評価を実施したので報告する。


JSFR design progress related to development of safety design criteria for generation IV sodium-cooled fast reactors, 1; Overview

上出 英樹; 安藤 将人*; 伊藤 隆哉*

Proceedings of 23rd International Conference on Nuclear Engineering (ICONE-23) (DVD-ROM), 7 Pages, 2015/05

原子力機構, 日本原子力発電, 三菱FBRシステムズは、将来の持続可能な基幹電源の候補として、ナトリウム冷却高速増殖炉の実用化概念であるJSFRの設計研究を実施してきている。2011年以降は、東京電力福島第一原子力発電所事故の教訓を踏まえたGIFにおけるナトリウム冷却高速炉の安全設計クライテリア及び安全設計ガイドライン構築の活動に貢献するために、地震・津波等の厳しい外的事象に対する安全対策を取り入れるとともに、より実現性の高いものとするため、より細部の成立性や保守補修性に配慮して、設計概念の具体化を進めた。本報では、75万kWeのJSFR実証施設を対象として、2011年以降の設計進捗を取り入れた設計概念を概括する。


Numerical study on influence of Ohnesorge number and Reynolds number on the jet breakup behavior using the lattice Boltzmann method

岩澤 譲*; 阿部 豊*; 金子 暁子*; 金川 哲也*; 齋藤 慎平*; 松尾 英治*; 海老原 健一; 坂場 弘*; 小山 和也*; 成合 英樹*

Proceedings of 23rd International Conference on Nuclear Engineering (ICONE-23) (DVD-ROM), 7 Pages, 2015/05



Study on vortex cavitation in scaled upper plenum model of Japan Sodium-cooled Fast Reactor, 2; Investigation of effective cavitation suppressor

萩原 裕之*; 江連 俊樹; 伊藤 啓; 上出 英樹

Proceedings of 9th Korea-Japan Symposium on Nuclear Thermal Hydraulics and Safety (NTHAS-9) (CD-ROM), 7 Pages, 2014/11

A water test visualizing vortex cavitation inception have been carried out using 1/11 scale upper plenum model of Japan Sodium-cooled Fast Reactor. The influence of the splitter on the vortex cavitation has been examined. In addition to that, a measurement test for flow velocity distribution around the vortex has been performed by means of the particle imaging velocimetry (PIV). In the visualization test, the vortex cavitation inception occurs much more easily in the case without the flow splitter than that with the flow splitter. Besides, it has been observed that the influence of kinematic viscosity coefficient on the vortex cavitation inception decreases by installing flow splitter. As a result of the measurement test, the correlation has been found between the magnitude of circulation and the vortex cavitation inception.


Experimental study on vortex cavitation in scaled upper plenum model of Japan Sodium-cooled Fast Reactor, 1; Evaluation of circulation and vortex cavitation occurrences using vortex model

江連 俊樹; 伊藤 啓; 亀山 祐理*; 萩原 裕之*; 上出 英樹

Proceedings of 9th Korea-Japan Symposium on Nuclear Thermal Hydraulics and Safety (NTHAS-9) (CD-ROM), 7 Pages, 2014/11

A water experiment in the 1/22 scaled upper plenum model of JSFR was performed to clarify behavior of vortex cavitation occurrences. Velocity distributions between H/L intakes and R/V wall were obtained under various H/L inlet velocity and temperature conditions. Pressure drop at vortex center was evaluated from obtained velocity distributions based on the Burgers vortex model. Evaluated value of pressure drop in time series was also compared with temporal behavior of vortex cavitation occurrences. As the results, circulation around vortex was quantified and time-averaged normalized circulation was observed to be nearly constant independent on the variation of Reynolds number at H/L pipe intakes. The evaluated value of pressure drop showed qualitatively consistent behavior to occurrences of vortex cavitation in time series. Consequently, it is confirmed that occurrences of vortex cavitation can be predicted by means of the evaluation method based on Burgers vortex model.


A High-precision calculation method for interface normal and curvature on an unstructured grid

伊藤 啓; 功刀 資彰*; 大野 修司; 上出 英樹; 大島 宏之

Journal of Computational Physics, 273, p.38 - 53, 2014/09

 被引用回数:11 パーセンタイル:30.29(Computer Science, Interdisciplinary Applications)

In the volume-of-fluid algorithm, the calculations of the interface normal and curvature are crucially important for accurately simulating interfacial flows. In this paper, the authors develop a height function method that works appropriately on an unstructured grid. In the process, the definition of the height function is discussed, and the high-precision calculation method of the interface normal is developed to meet the necessary condition for a second-order method. The curvature calculation method is also discussed and the approximated quadric curve of an interface is employed to calculate the curvature. Following a basic verification, the developed height function method is shown to successfully provide superior calculation accuracy and highly reduced computational cost compared with conventional calculation methods in terms of the interface normal and curvature.


Effect of physical properties on gas entrainment rate from free surface by vortex, 2

小泉 安郎*; 大手 直介*; 上出 英樹; 大野 修司; 伊藤 啓

Proceedings of 22nd International Conference on Nuclear Engineering (ICONE-22) (DVD-ROM), 7 Pages, 2014/07

A sodium-cooled fast breeder reactor is now at the developing stage in Japan. One concern for safety is cover gas entrainment into the sodium coolant. The gas entrainment rate into liquid by the vortex formed on the free surface was examined experimentally. Four kinds of test fluid were used; water at 25$$^{circ}$$C, water at 60 $$^{circ}$$C, 20 cSt silicone oil and kerosene. The gas entrainment rate into liquid was measured. The relation between gas entrainment rate and liquid velocity was mainly affected by the viscosity of liquid. As viscosity became large, higher exit velocity was required to get the same gas entrainment rate. No systematic trend by the surface tension was noticed in the gas entrainment rate. A flow state at the outlet piping has significant effect on the gas entrainment rate. The dimension of the outlet piping may become important to consider the gas entrainment rate in the vortex type region.

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