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Journal Articles

Computer code analysis of irradiation performance of axially heterogeneous mixed oxide fuel elements attaining high burnup in a fast reactor

Uwaba, Tomoyuki; Yokoyama, Keisuke; Nemoto, Junichi*; Ishitani, Ikuo*; Ito, Masahiro*; Pelletier, M.*

Nuclear Engineering and Design, 359, p.110448_1 - 110448_7, 2020/04

 Times Cited Count:0 Percentile:100(Nuclear Science & Technology)

Coupled computer code analyses of irradiation performance of axially heterogeneous mixed oxide (MOX) fuel elements with high burnup in a fast reactor were conducted. Post-irradiation experiments revealed local concentration of Cs near the interfaces between MOX fuel and blanket columns including the internal blanket of the fuel elements as well as an increase in their cladding diameters. The analyses indicated that the local Cs concentration occurred as a result of Cs axial migration from the MOX fuels toward the blanket pellets near the interfaces. Swelling of the blanket pellets induced by the formation of low-density Cs-U-O compound was not sufficient to cause pellet-to-cladding mechanical interaction (PCMI). The PCMI analyzed in the MOX fuel column regions was insignificant, and the cladding diameter increases were caused mainly by void swelling in cladding and irradiation creep due to fission gas pressure.

JAEA Reports

Annual report on the environmental radiation monitoring around the Tokai Reprocessing Plant FY 2018

Nakano, Masanao; Fujii, Tomoko; Nemoto, Masashi; Tobita, Keiji; Kono, Takahiko; Hosomi, Kenji; Nishimura, Shusaku; Matsubara, Natsumi; Maehara, Yushi; Narita, Ryosuke; et al.

JAEA-Review 2019-048, 165 Pages, 2020/03

JAEA-Review-2019-048.pdf:2.69MB

Environmental radiation monitoring around the Tokai Reprocessing Plant has been performed by the Nuclear Fuel Cycle Engineering Laboratories, based on "Safety Regulations for the Reprocessing Plant of Japan Atomic Energy Agency, Chapter IV - Environmental Monitoring". This annual report presents the results of the environmental monitoring and the dose estimation to the hypothetical inhabitant due to the radioactivity discharged from the plant to the atmosphere and the sea during April 2018 to March 2019. In this report, some data include the influence of the accidental release from the Fukushima Daiichi Nuclear Power Station of Tokyo Electric Power Co., Inc. (the trade name was changed to Tokyo Electric Power Company Holdings, Inc. on April 1, 2016) in March 2011. Appendices present comprehensive information, such as monitoring programs, monitoring methods, monitoring results and their trends, meteorological data and discharged radioactive wastes. In addition, the data which were influenced by the accidental release and exceeded the normal range of fluctuation in the monitoring, were evaluated.

Journal Articles

Transport and redistribution of radiocesium in Fukushima fallout through rivers

Taniguchi, Keisuke*; Onda, Yuichi*; Smith, H. G.*; Blake, W.*; Yoshimura, Kazuya; Yamashiki, Yosuke*; Kuramoto, Takayuki*; Saito, Kimiaki

Environmental Science & Technology, 53(21), p.12339 - 12347, 2019/11

 Times Cited Count:10 Percentile:10.66(Engineering, Environmental)

Journal Articles

Electronic structure of the high-$$T_C$$ ferromagnetic semiconductor (Ga,Fe)Sb; X-ray magnetic circular dichroism and resonance photoemission spectroscopy studies

Sakamoto, Shoya*; Tu, N. T.*; Takeda, Yukiharu; Fujimori, Shinichi; Hai, P. N.*; Anh, L. D.*; Wakabayashi, Yuki K.*; Shibata, Goro*; Horio, Masafumi*; Ikeda, Keisuke*; et al.

Physical Review B, 100(3), p.035204_1 - 035204_8, 2019/07

Journal Articles

Electronic structure of the high-T$$_{C}$$ ferromagnetic semiconductor (Ga,Fe)Sb; X-ray magnetic circular dichroism and resonance photoemission spectroscopy studies

Sakamoto, Shoya*; Tu, N. T.*; Takeda, Yukiharu; Fujimori, Shinichi; Hai, P. N.*; Anh, L. D.*; Wakabayashi, Yuki*; Shibata, Goro*; Horio, Masafumi*; Ikeda, Keisuke*; et al.

Physical Review B, 100(3), p.035204_1 - 035204_8, 2019/07

 Times Cited Count:4 Percentile:30.92(Materials Science, Multidisciplinary)

JAEA Reports

Annual report on the environmental radiation monitoring around the Tokai Reprocessing Plant FY 2017

Nakano, Masanao; Fujita, Hiroki; Mizutani, Tomoko; Nemoto, Masashi; Tobita, Keiji; Kono, Takahiko; Hosomi, Kenji; Hokama, Tomonori; Nishimura, Tomohiro; Matsubara, Natsumi; et al.

JAEA-Review 2018-025, 171 Pages, 2019/02

JAEA-Review-2018-025.pdf:3.81MB

Environmental radiation monitoring around the Tokai Reprocessing Plant has been performed by the Nuclear Fuel Cycle Engineering Laboratories, based on "Safety Regulations for the Reprocessing Plant of Japan Atomic Energy Agency, Chapter IV - Environmental Monitoring". This annual report presents the results of the environmental monitoring and the dose estimation to the hypothetical inhabitant due to the radioactivity discharged from the plant to the atmosphere and the sea during April 2016 to March 2017. In this report, some data include the influence of the accidental release from the Fukushima Daiichi Nuclear Power Station of Electric Power Company Holdings, Inc. in March 2011. Appendices present comprehensive information, such as monitoring programs, monitoring methods, monitoring results and their trends, meteorological data and discharged radioactive wastes. In addition, the data which were influenced by the accidental release and were exceeded the normal range of fluctuation in the monitoring, were evaluated.

Journal Articles

Development of remote sensing technique using radiation resistant optical fibers under high-radiation environment

Ito, Chikara; Naito, Hiroyuki; Ishikawa, Takashi; Ito, Keisuke; Wakaida, Ikuo

JPS Conference Proceedings (Internet), 24, p.011038_1 - 011038_6, 2019/01

A high-radiation resistant optical fiber has been developed in order to investigate the interiors of the reactor pressure vessels and the primary containment vessels at the Fukushima Daiichi Nuclear Power Station. The tentative dose rate in the reactor pressure vessels is assumed to be up to 1 kGy/h. We developed a radiation resistant optical fiber consisting of a 1000 ppm hydroxyl doped pure silica core and 4 % fluorine doped pure silica cladding. We attempted to apply the optical fiber to remote imaging technique by means of fiberscope. The number of core image fibers was increased from 2000 to 22000 for practical use. The transmissive rate of infrared images was not affected after irradiation of 1 MGy. No change in the spatial resolution of the view scope by means of image fiber was noted between pre- and post-irradiation. We confirmed the applicability of the probing system, which consists of a view scope using radiation-resistant optical fibers.

Journal Articles

Quantum paramagnet near spin-state transition

Tomiyasu, Keisuke*; Ito, Naoko*; Okazaki, Ryuji*; Takahashi, Yuki*; Onodera, Mitsugi*; Iwasa, Kazuaki*; Nojima, Tsutomu*; Aoyama, Takuya*; Ogushi, Kenya*; Ishikawa, Yoshihisa*; et al.

Advanced Quantum Technologies (Internet), 1(3), p.1800057_1 - 1800057_7, 2018/12

Spin-state transition, also known as spin crossover, plays a key role in diverse systems. In theory, the boundary range between the low- and high-spin states is expected to enrich the transition and give rise to unusual physical states. However, no compound that realizes a nearly degenerate critical range as the ground state without requiring special external conditions has yet been experimentally identified. This study reports that the Sc substitution in LaCoO3 destabilizes its nonmagnetic low-spin state and generates an anomalous paramagnetic state accompanied by the enhancement of transport gap and magneto-lattice-expansion as well as the contraction of Co-O distance with the increase of electron site transfer. These phenomena are not well described by the mixture of conventional low- and high-spin states, but by their quantum superposition occurring on the verge of a spin-state transition.

Journal Articles

Local magnetic states of the weakly ferromagnetic iron-based superconductor Sr$$_{2}$$VFeAsO$$_{3-delta}$$ studied by X-ray magnetic circular dichroism

Horio, Masafumi*; Takeda, Yukiharu; Namiki, Hiromasa*; Katagiri, Takao*; Wakabayashi, Yuki*; Sakamoto, Shoya*; Nonaka, Yosuke*; Shibata, Goro*; Ikeda, Keisuke*; Saito, Yuji; et al.

Journal of the Physical Society of Japan, 87(10), p.105001_1 - 105001_2, 2018/10

 Times Cited Count:1 Percentile:76.74(Physics, Multidisciplinary)

Journal Articles

Cation distribution and magnetic properties in ultrathin (Ni$$_{1-x}$$Co$$_{x}$$)Fe$$_{2}$$O$$_{4}$$ (x=0-1) layers on Si(111) studied by soft X-ray magnetic circular dichroism

Wakabayashi, Yuki*; Nonaka, Yosuke*; Takeda, Yukiharu; Sakamoto, Shoya*; Ikeda, Keisuke*; Chi, Z.*; Shibata, Goro*; Tanaka, Arata*; Saito, Yuji; Yamagami, Hiroshi; et al.

Physical Review Materials (Internet), 2(10), p.104416_1 - 104416_12, 2018/10

 Times Cited Count:3 Percentile:69.7(Materials Science, Multidisciplinary)

Journal Articles

Reduction and resource recycling of high-level radioactive wastes through nuclear transmutation; Isolation techniques of Pd, Zr, Se and Cs in simulated high level radioactive waste using solvent extraction

Sasaki, Yuji; Morita, Keisuke; Ito, Keisuke; Suzuki, Shinichi; Shiwaku, Hideaki; Takahashi, Yuya*; Kaneko, Masaaki*; Omori, Takashi*; Asano, Kazuhito*

Proceedings of International Nuclear Fuel Cycle Conference (GLOBAL 2017) (USB Flash Drive), 4 Pages, 2017/09

no abstracts in English

Journal Articles

Extraction and separation of Se, Zr, Pd, and Cs including long-lived radionuclides

Sasaki, Yuji; Morita, Keisuke; Suzuki, Shinichi; Shiwaku, Hideaki; Ito, Keisuke; Takahashi, Yuya*; Kaneko, Masaaki*

Solvent Extraction Research and Development, Japan, 24(2), p.113 - 122, 2017/06

The solvent extraction of Se, Zr, Pd, and Cs from nitric acid into 1-octanol (OC) and dodecane has been performed. These elements include long-lived radionuclides in spent nuclear fuels, so a simple separation method is indispensable for the development of the treatment of high-level liquid radioactive waste. It was found that Se can be extracted using phenylenediamine, Zr can be extracted using tetraoctyl diglycolamide and di-2-ethylhexyl phosphoric acid, and Pd can be extracted using (methylimino)bis(dioctylacetamide) and hexaoctylnitrilotriacetamide. These elements can be recovered in over 90% yield by these extractants from nitric acid into OC. A distribution ratio of Cs of greater than 1 can be obtained using di-t-butyldibenzo-18-crown-6. It is clear that 90% recovery of Cs can be achieved using an extraction solvent with ten times the volume of the aqueous phase.

Journal Articles

Uniaxial pressure effect on the magnetic ordered moment and transition temperatures in BaFe$$_{2-x}$$T$$_{x}$$As$$_{2}$$ ($$T$$ = Co,Ni)

Tam, D. M.*; Song, Y.*; Man, H.*; Cheung, S. C.*; Yin, Z.*; Lu, X.*; Wang, W.*; Frandsen, B. A.*; Liu, L.*; Gong, Z.*; et al.

Physical Review B, 95(6), p.060505_1 - 060505_6, 2017/02

 Times Cited Count:14 Percentile:23.13(Materials Science, Multidisciplinary)

Journal Articles

Electronic structure of EuAl$$_4$$ studied by photoelectron spectroscopy

Kobata, Masaaki; Fujimori, Shinichi; Takeda, Yukiharu; Okane, Tetsuo; Saito, Yuji; Kobayashi, Keisuke*; Yamagami, Hiroshi; Nakamura, Ai*; Hedo, Masato*; Nakama, Takao*; et al.

Journal of the Physical Society of Japan, 85(9), p.094703_1 - 094703_6, 2016/09

 Times Cited Count:5 Percentile:53.75(Physics, Multidisciplinary)

Journal Articles

Room-temperature local ferromagnetism and its nanoscale expansion in the ferromagnetic semiconductor Ge$$_{1-x}$$Fe$$_{x}$$

Wakabayashi, Yuki*; Sakamoto, Shoya*; Takeda, Yukiharu; Ishigami, Keisuke*; Takahashi, Yukio*; Saito, Yuji; Yamagami, Hiroshi; Fujimori, Atsushi*; Tanaka, Masaaki*; Oya, Shinobu*

Scientific Reports (Internet), 6, p.23295_1 - 23295_9, 2016/03

AA2016-0503.pdf:1.66MB

 Times Cited Count:11 Percentile:36.41(Multidisciplinary Sciences)

Journal Articles

Thickness-dependent magnetic properties and strain-induced orbital magnetic moment in SrRuO$$_{3}$$ thin films

Ishigami, Keisuke*; Yoshimatsu, Kohei*; Toyota, Daisuke*; Takizawa, Masaru*; Yoshida, Teppei*; Shibata, Goro*; Harano, Takayuki*; Takahashi, Yukio*; Kadono, Toshiharu*; Verma, V. K.*; et al.

Physical Review B, 92(6), p.064402_1 - 064402_5, 2015/08

 Times Cited Count:21 Percentile:22.87(Materials Science, Multidisciplinary)

Journal Articles

Evaluation of the cryogenic tensile properties for aramid fiber rod

Saito, Toru; Okubo, Toshikazu*; Izumi, Keisuke*; Okawa, Yoshinao*; Kobayashi, Norihiro*; Yamazaki, Toru; Kawano, Katsumi; Isono, Takaaki

Teion Kogaku, 50(8), p.400 - 408, 2015/08

Aramid fiber-reinforced plastic (AFRP) has been developed as a structural material that has the advantages of light weight and high strength. In this study, tensile tests were carried out to measure the tensile properties of AFRP rod on the market for reinforcement of concrete at room temperature, 77 K and 4.2 K. Especially at cryogenic temperatures, it is difficult to perform a tensile test of the bar because the specimen slips through the jig grip. To prevent the rod from slipping, tensile tests were carried out with some filling conditions. The applicable and appropriate tensile test conditions were established by modifying the jig grip, treating the surface of the rod and using cryogenic epoxy infill to grip the rod. They were more than 1100 MPa. Additionally, the AFRP rod included a temperature dependence in which the Young's modulus increased as the test temperature decreased. It was confirmed that the Young's modulus increased because aramid fiber was more dominant than epoxy.

Journal Articles

Characterization and storage of radioactive zeolite waste

Yamagishi, Isao; Nagaishi, Ryuji; Kato, Chiaki; Morita, Keisuke; Terada, Atsuhiko; Kamiji, Yu; Hino, Ryutaro; Sato, Hiroyuki; Nishihara, Kenji; Tsubata, Yasuhiro; et al.

Journal of Nuclear Science and Technology, 51(7-8), p.1044 - 1053, 2014/07

 Times Cited Count:7 Percentile:39.01(Nuclear Science & Technology)

For safe storage of zeolite wastes generated by treatment of radioactive saline water at the Fukushima Daiichi Nuclear Power Station, properties of the Herschelite adsorbent were studied and its adsorption vessel was evaluated for hydrogen production and corrosion. Hydrogen production depends on its water level and dissolved species because hydrogen is oxidized by radicals in water. It is possible to evaluate hydrogen production rate in Herschelite submerged in seawater or pure water by taking into account of the depth effect of the water. The reference vessel of decay heat 504 W with or without residual pure water was evaluated for the hydrogen concentration by thermal hydraulic analysis using obtained fundamental properties. Maximum hydrogen concentration was below the lower explosive limit (4 %). The steady-state corrosion potential of a stainless steel 316L increased with absorbed dose rate but its increase was repressed by the presence of Herschelite. At 750 Gy/h and $$<$$60$$^{circ}$$C which were values evaluated at the bottom of the vessel of 504 W, the localized corrosion of SUS316L contacted with Herschelite would not immediately occur under 20,000 ppm of Cl$$^{-}$$ concentration.

Journal Articles

Orbital magnetic moment and coercivity of SiO$$_2$$-coated FePt nanoparticles studied by X-ray magnetic circular dichroism

Takahashi, Yukio*; Kadono, Toshiharu*; Yamamoto, Shimpei*; Singh, V. R.*; Verma, V.*; Ishigami, Keisuke*; Shibata, Goro*; Harano, Takayuki*; Takeda, Yukiharu; Okane, Tetsuo; et al.

Physical Review B, 90(2), p.024423_1 - 024423_5, 2014/07

AA2015-0417.pdf:0.45MB

 Times Cited Count:3 Percentile:80.67(Materials Science, Multidisciplinary)

Journal Articles

In-vessel inspection probing technique using optical fibers under high radiation dose

Ito, Chikara; Naito, Hiroyuki; Oba, Hironori; Saeki, Morihisa; Ito, Keisuke; Ishikawa, Takashi; Nishimura, Akihiko; Wakaida, Ikuo; Sekine, Takashi

Proceedings of 22nd International Conference on Nuclear Engineering (ICONE-22) (DVD-ROM), 7 Pages, 2014/07

A high-radiation resistant optical fiber has been developed in order to investigate the interiors of the reactor pressure vessels and the primary containment vessels of the Fukushima Daiichi Nuclear Power Station. The radiation resistance of an optical fiber was improved by increasing the amount of hydroxyl up to 1000 ppm in pure silica fiber. The improved image fiber consists of common cladding and a large number of fiber cores made from pure silica that contains 1000 ppm hydroxyl. The transmissive rate of an infrared image was not affected after the irradiation of 1 MGy. We have developed the fiber-coupled LIBS system to detect plasma emission efficiently in near-infrared region. In addition, we have performed a $$gamma$$ ray dose rate measurement using an optical fiber of which scintillator is attached to the tip. As a result, the concept of applicability of a probing system using the high-radiation resistant optical fibers has been confirmed.

312 (Records 1-20 displayed on this page)