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JAEA Reports

Status of study of long-term assessment of transport of radioactive contaminants in the environment of Fukushima (FY2018) (Translated document)

Nagao, Fumiya; Niizato, Tadafumi; Sasaki, Yoshito; Ito, Satomi; Watanabe, Takayoshi; Dohi, Terumi; Nakanishi, Takahiro; Sakuma, Kazuyuki; Hagiwara, Hiroki; Funaki, Hironori; et al.

JAEA-Research 2020-007, 249 Pages, 2020/10

JAEA-Research-2020-007.pdf:15.83MB

The accident of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. occurred due to the Great East Japan Earthquake, Sanriku offshore earthquake, of 9.0 magnitude and the accompanying tsunami. As a result, large amount of radioactive materials was released into the environment. Under these circumstances, Japan Atomic Energy Agency (JAEA) has been conducting "Long-term Assessment of Transport of Radioactive Contaminants in the Environment of Fukushima" concerning radioactive materials released in environment, especially migration behavior of radioactive cesium since November 2012. This report is a summary of the research results that have been obtained in environmental dynamics research conducted by JAEA in Fukushima Prefecture.

Journal Articles

Controlled growth of boron-doped epitaxial graphene by thermal decomposition of a B$$_{4}$$C thin film

Norimatsu, Wataru*; Matsuda, Keita*; Terasawa, Tomoo; Takata, Nao*; Masumori, Atsushi*; Ito, Keita*; Oda, Koji*; Ito, Takahiro*; Endo, Akira*; Funahashi, Ryoji*; et al.

Nanotechnology, 31(14), p.145711_1 - 145711_7, 2020/04

 Times Cited Count:0 Percentile:100(Nanoscience & Nanotechnology)

We show that boron-doped epitaxial graphene can be successfully grown by thermal decomposition of a boron carbide thin film, which can also be epitaxially grown on a silicon carbide substrate. The interfaces of B$$_{4}$$C on SiC and graphene on B$$_{4}$$C had a fixed orientation relation, having a local stable structure with no dangling bonds. The first carbon layer on B$$_{4}$$C acts as a buffer layer, and the overlaying carbon layers are graphene. Graphene on B$$_{4}$$C was highly boron doped, and the hole concentration could be controlled over a wide range of 2$$times$$10$$^{13}$$ to 2$$times$$10$$^{15}$$ cm$$^{-2}$$. Highly boron-doped graphene exhibited a spin-glass behavior, which suggests the presence of local antiferromagnetic ordering in the spin-frustration system. Thermal decomposition of carbides holds the promise of being a technique to obtain a new class of wafer-scale functional epitaxial graphene for various applications.

Journal Articles

Measurement of the angular distribution of $$gamma$$-rays after neutron capture by $$^{139}$$La for a T-violation search

Okudaira, Takuya; Shimizu, Hirohiko*; Kitaguchi, Masaaki*; Hirota, Katsuya*; Haddock, C. C.*; Ito, Ikuya*; Yamamoto, Tomoki*; Endo, Shunsuke*; Ishizaki, Kohei*; Sato, Takumi*; et al.

EPJ Web of Conferences, 219, p.09001_1 - 09001_6, 2019/12

Parity violating effects enhanced by up to 10$$^6$$ times have been observed in several neutron induced compound nuclei. There is a theoretical prediction that time reversal (T) violating effects can also be enhanced in these nuclei implying that T-violation can be searched for by making very sensitive measurements. However, the enhancement factor has not yet been measured in all nuclei. The angular distribution of the (n,$$gamma$$) reaction was measured with $$^{139}$$La by using a germanium detector assembly at J-PARC, and the enhancement factor was obtained. From the result, the measurement time to achieve the most sensitive T-violation search was estimated as 1.4 days, and a 40% polarized $$^{139}$$La target and a 70% polarized $$^3$$He spin filter whose thickness is 70 atm$$cdot$$cm are needed. Therefore high quality $$^3$$He spin filter is developed in JAEA. The measurement result of the (n,$$gamma$$) reaction at J-PARC and the development status of the $$^3$$He spin filter will be presented.

JAEA Reports

Status of study of long-term assessment of transport of radioactive contaminants in the environment of Fukushima (FY2018)

Nagao, Fumiya; Niizato, Tadafumi; Sasaki, Yoshito; Ito, Satomi; Watanabe, Takayoshi; Dohi, Terumi; Nakanishi, Takahiro; Sakuma, Kazuyuki; Hagiwara, Hiroki; Funaki, Hironori; et al.

JAEA-Research 2019-002, 235 Pages, 2019/08

JAEA-Research-2019-002.pdf:21.04MB

The accident of the Fukushima Daiichi Nuclear Power Station (hereinafter referred to 1F), Tokyo Electric Power Company Holdings, Inc. occurred due to the Great East Japan Earthquake, Sanriku offshore earthquake, of 9.0 magnitude and the accompanying tsunami. As a result, large amount of radioactive materials was released into the environment. Under these circumstances, JAEA has been conducting Long-term Environmental Dynamics Research concerning radioactive materials released in environment, especially migration behavior of radioactive cesium since November 2012. This report is a summary of the research results that have been obtained in environmental dynamics research conducted by JAEA in Fukushima Prefecture.

Journal Articles

Longitudinal strain of epitaxial graphene monolayers on SiC substrates evaluated by $$z$$-polarization Raman microscopy

Saito, Yuika*; Tokiwa, Kenshiro*; Kondo, Takahiro*; Bao, J.*; Terasawa, Tomoo; Norimatsu, Wataru*; Kusunoki, Michiko*

AIP Advances (Internet), 9(6), p.065314_1 - 065314_6, 2019/06

 Times Cited Count:0 Percentile:100(Nanoscience & Nanotechnology)

JAEA Reports

Measurement and analysis of in-vessel component activation and gamma dose rate distribution in Joyo, 2

Yamamoto, Takahiro; Ito, Chikara; Maeda, Shigetaka; Ito, Hideaki; Sekine, Takashi

JAEA-Technology 2017-036, 41 Pages, 2018/02

JAEA-Technology-2017-036.pdf:7.86MB

In the experimental fast reactor Joyo, the damaged upper core structure (UCS) was retrieved into the cask in May 2014 The dose rate on UCS surface was quite high due to the activation for over 30 years operation. In order to attain the optimum safety design, manufacture and operation of equipment for UCS replacement, the method to evaluate UCS surface dose rate was developed on the basis of C/E obtained by the in-vessel dose rate measurement in Joyo. In order to verify the evaluation method, the axial gamma-ray distribution measurement on the surface of the cask, which contained UCS, was conducted using a plastic scintillating optical fiber (PSF) detector. This paper describes the comparison results between calculation and measurement as follows. (1) The measured axial gamma-ray distribution on the cask surface had a peak on proper location with considering the cask shielding structure and agree well with the calculated distribution. (2) The C/E of axial gamma-ray distribution on the cask surface was ranged from 1.1 to 1.7. It was confirmed that the calculation for UCS replacement equipment design had a margin conservatively. Then, the results showed that the developed evaluation method for UCS replacement equipment design was sufficiently reliable.

JAEA Reports

Status of study of long-term assessment of transport of radioactive contaminants in the environment of Fukushima; As a part of dissemination of evidence-based information

Tsuruta, Tadahiko; Niizato, Tadafumi; Nakanishi, Takahiro; Dohi, Terumi; Nakama, Shigeo; Funaki, Hironori; Misono, Toshiharu; Oyama, Takuya; Kurikami, Hiroshi; Hayashi, Seiji*; et al.

JAEA-Review 2017-018, 86 Pages, 2017/10

JAEA-Review-2017-018.pdf:17.58MB

Since the accidents at Fukushima Daiichi Nuclear Power Plant following the Tohoku Region Pacific Coast Earthquake on March 11th, 2011, Fukushima Environmental Safety Center has carried out research on natural mobilization of radionuclide (especially radiocesium) and future forecast from forest to water system and surrounding residential areas. The report summarizes the latest results that have been accumulated from each study field, of our agency together with the other related research organizations. The contents of the report is to be used as evidence-based information for the QA-styled pages in the website of JAEA Sector of Fukushima Research and Development at the time of next renewal.

JAEA Reports

Horonobe Underground Research Laboratory Project; Synthesis of Phase II (Construction Phase) investigations to a depth of 350m

Sato, Toshinori; Sasamoto, Hiroshi; Ishii, Eiichi; Matsuoka, Toshiyuki; Hayano, Akira; Miyakawa, Kazuya; Fujita, Tomoo*; Tanai, Kenji; Nakayama, Masashi; Takeda, Masaki; et al.

JAEA-Research 2016-025, 313 Pages, 2017/03

JAEA-Research-2016-025.pdf:45.1MB

The Horonobe Underground Research Laboratory (URL) Project is being pursued by the Japan Atomic Energy Agency (JAEA) to enhance the reliability of relevant disposal technologies through investigations of the deep geological environment within the host sedimentary formations at Horonobe, northern Hokkaido. This report summarizes the results of the Phase II investigations carried out from April 2005 to June 2014 to a depth of 350m. Integration of work from different disciplines into a "geosynthesis" ensures that the Phase II goals have been successfully achieved and identifies key issues that need to made to be addressed in the Phase II investigations Efforts are made to summarize as many lessons learnt from the Phase II investigations and other technical achievements as possible to form a "knowledge base" that will reinforce the technical basis for both implementation and the formulation of safety regulations.

Journal Articles

Comprehensive study on initial thermal oxidation of GaN(0001) surface and subsequent oxide growth in dry oxygen ambient

Yamada, Takahiro*; Ito, Joyo*; Asahara, Ryohei*; Watanabe, Kenta*; Nozaki, Mikito*; Nakazawa, Satoshi*; Anda, Yoshiharu*; Ishida, Masahiro*; Ueda, Tetsuzo*; Yoshigoe, Akitaka; et al.

Journal of Applied Physics, 121(3), p.035303_1 - 035303_9, 2017/01

 Times Cited Count:33 Percentile:7.32(Physics, Applied)

Initial oxidation of GaN(0001) epilayers and subsequent growth of thermal oxides in dry oxygen ambient were investigated by means of X-ray photoelectron spectroscopy, spectroscopic ellipsometry, atomic force microscopy and X-ray diffraction measurements. It was found that, whereas initial oxide formation tends to saturate at temperatures below 800$$^{circ}$$C, selective growth of small oxide grains proceeds at dislocations in the epilayers, followed by noticeable grain growth leading to rough surface morphology at higher oxidation temperatures. This indicates that oxide growth and its morphology are crucially dependent on the defect density in the GaN epilayers. Structural characterizations also revealed that polycrystalline $$alpha$$- and $$beta$$-phase Ga$$_{2}$$O$$_{3}$$ grains in an epitaxial relation with the GaN substrate are formed from the initial stage of the oxide growth. On the basis of these experimental findings, we also developed a comprehensive model for GaN oxidation mediated by nitrogen removal and mass transport.

Journal Articles

Beam commissioning of the linac for iBNCT

Naito, Fujio*; Anami, Shozo*; Ikegami, Kiyoshi*; Uota, Masahiko*; Ouchi, Toshikatsu*; Onishi, Takahiro*; Oba, Toshiyuki*; Obina, Takashi*; Kawamura, Masato*; Kumada, Hiroaki*; et al.

Proceedings of 13th Annual Meeting of Particle Accelerator Society of Japan (Internet), p.1244 - 1246, 2016/11

The proton linac installed in the Ibaraki Neutron Medical Research Center is used for production of the intense neutron flux for the Boron Neutron Capture Therapy (BNCT). The linac consists of the 3-MeV RFQ and the 8-MeV DTL. Design average beam current is 10mA. Target is made of Beryllium. First neutron production from the Beryllium target was observed at the end of 2015 with the low intensity beam as a demonstration. After the observation of neutron production, a lot of improvement s was carried out in order to increase the proton beam intensity for the real beam commissioning. The beam commissioning has been started on May 2016. The status of the commissioning is summarized in this report.

Journal Articles

Effect of nitrogen incorporation into Al-based gate insulators in AlON/AlGaN/GaN metal-oxide-semiconductor structures

Asahara, Ryohei*; Nozaki, Mikito*; Yamada, Takahiro*; Ito, Joyo*; Nakazawa, Satoshi*; Ishida, Masahiro*; Ueda, Tetsuzo*; Yoshigoe, Akitaka; Hosoi, Takuji*; Shimura, Takayoshi*; et al.

Applied Physics Express, 9(10), p.101002_1 - 101002_4, 2016/10

 Times Cited Count:28 Percentile:12.38(Physics, Applied)

The superior physical and electrical properties of AlON gate dielectrics on AlGaN/GaN substrates in terms of thermal stability, reliability, and interface quality were demonstrated by direct AlON deposition and subsequent annealing. Nitrogen incorporation into alumina was proven to be beneficial both for suppressing intermixing at the insulator/AlGaN interface and reducing the number of electrical defects in Al$$_{2}$$O$$_{3}$$ films. Consequently, we achieved high-quality AlON/AlGaN/GaN metal-oxide-semiconductor capacitors with improved stability against charge injection and a reduced interface state density as low as 1.2$$times$$10$$^{11}$$ cm$$^{-2}$$eV$$^{-1}$$. The impact of nitrogen incorporation into the insulator was discussed on the basis of experimental findings.

JAEA Reports

Development of active control technology for impurities in coolant helium using High Temperature Engineering Test Reactor (HTTR)

Hamamoto, Shimpei; Nemoto, Takahiro; Sekita, Kenji; Saito, Kenji

JAEA-Technology 2015-048, 62 Pages, 2016/03

JAEA-Technology-2015-048.pdf:2.58MB

The decarburization may take place depending on the chemical impurity composition in helium gas used as the primary coolant in High-Temperature Gas-cooled Reactors, and will significantly reduce the strength of the alloy. The ability to remove impurities by a helium purification system was designed according to the predicted generation rate of impurities so as to make the coolant become the carburizing atmosphere. It has been confirmed that the coolant becomes the carburizing atmosphere during the operation period of the High Temperature engineering Test Reactor (HTTR). However, it is necessary to consider changes of generation rates of impurities since lifetime of commercial reactor is longer than the life of the HTTR. To avoid the influence of the change of generation rate, the control of removal efficiency of impurity in the helium purification system was considered in this study. To reform the decarburizing into the carburizing atmosphere, it is effective to increase the H$$_{2}$$ and CO concentration in the coolant helium. By controlling the efficiency of the Cooper Oxide Trap (CuOT), it is possible to increase the H$$_{2}$$ and CO concentrations. Therefore, an experiment was carried out by injecting the gas mixture of H$$_{2}$$ and CO into the existing purification system of HTTR to investigate the dependencies of temperature and impurity concentration on the removal efficiency of CuOT. The experimental results are described as the following, (1) By adjusting the temperature of helium at the CuOT within a range from 110$$^{circ}$$C to 50$$^{circ}$$C, it is possible to reduce the removal efficiency of H$$_{2}$$ sufficiently. (2) Temperature change of helium gas in the CuOT is sufficiently reduced by the cooler located at the downstream of the CuOT, which does not affect the primary cooling system of HTTR. As the results, the applicability of removal efficiency control of CuOT was verified to improve the decarburizing atmosphere for the actual HTGR system.

Journal Articles

Development of inspection and repair techniques for reactor vessel of experimental fast reactor "Joyo"; Replacement of upper core structure

Takamatsu, Misao; Kawahara, Hirotaka; Ito, Hiromichi; Ushiki, Hiroshi; Suzuki, Nobuhiro; Sasaki, Jun; Ota, Katsu; Okuda, Eiji; Kobayashi, Tetsuhiko; Nagai, Akinori; et al.

Nippon Genshiryoku Gakkai Wabun Rombunshi, 15(1), p.32 - 42, 2016/03

In the experimental fast reactor Joyo, it was confirmed that the top of the irradiation test sub-assembly of "MARICO-2" (material testing rig with temperature control) had been broken and bent onto the in-vessel storage rack as an obstacle and had damaged the upper core structure (UCS). This paper describes the results of the in-vessel repair techniques for UCS replacement, which are developed in Joyo. UCS replacement was successfully completed in 2014. In-vessel repair techniques for sodium cooled fast reactors (SFRs) are important in confirming its safety and integrity. In order to secure the reliability of these techniques, it was necessary to demonstrate the performance under the actual reactor environment with high temperature, high radiation dose and remained sodium. The experience and knowledge gained in UCS replacement provides valuable insights into further improvements for In-vessel repair techniques in SFRs.

Journal Articles

Replacement of upper core structure in experimental fast reactor Joyo, 1; Existing damaged upper core structure jack-up test

Ito, Hiromichi; Suzuki, Nobuhiro; Kobayashi, Tetsuhiko; Kawahara, Hirotaka; Nagai, Akinori; Sakao, Ryuta*; Murata, Chotaro*; Tanaka, Junya*; Matsusaka, Yasunori*; Tatsuno, Takahiro*

Proceedings of 2015 International Congress on Advances in Nuclear Power Plants (ICAPP 2015) (CD-ROM), p.1058 - 1067, 2015/05

In the experimental fast reactor Joyo (Sodium-cooled Fast Reactor (SFR)), it was confirmed that the top of the irradiation test sub-assembly had bent onto the in-vessel storage rack as an obstacle and had damaged the upper core structure (UCS). There is a risk of deformation of the UCS and guide sleeve (GS) caused by interference between them unless inclination is controlled precisely. To mitigate the risk, special jack-up equipment for applying three-point suspension was developed. The existing damaged UCS (ed-UCS) jack-up test using the jack-up equipment was conducted on May 7, 2014. As a result of this test, it was confirmed that the ed-UCS could be successfully jacked-up to 1000 mm without consequent overload. The experience and knowledge gained in the ed-UCS jack-up test provides valuable insights and prospects not only for UCS replacement but also for further improving and verifying repair techniques in SFRs.

Journal Articles

Application of natural linear polysaccharide to green resist polymers for electron beam and extreme-ultraviolet lithography

Takei, Satoshi*; Oshima, Akihiro*; Oyama, Tomoko; Ito, Kenta*; Sugahara, Kigen*; Kashiwakura, Miki*; Kozawa, Takahiro*; Tagawa, Seiichi*; Hanabata, Makoto*

Japanese Journal of Applied Physics, 53(11), p.116505_1 - 116505_7, 2014/11

 Times Cited Count:5 Percentile:70.05(Physics, Applied)

The application of natural linear polysaccharide to green resists was demonstrated for electron beam (EB) and extreme-ultraviolet (EUV) lithography. Because of the water solubility of natural polysaccharides, the water spin-coating and water-developable processes realize an environmentally friendly manufacturing process for next-generation electronic devices. The developed green resist with a weight-average molecular weight of 83,000 and 70 mol % hydroxyl groups was found to have acceptable properties such as spin-coat ability on 200 mm wafers, pillar patterns of 100-400 nm with a high EB sensitivity of 10 $$mu$$ C/cm$$^{2}$$, etch selectivity with a silicon-based middle layer in CF$$_{4}$$ plasma treatment, and high prediction sensitivity to EUV region.

Journal Articles

Development of timing system for RF ion source & RFQ III test stand

Sawabe, Yuki; Ito, Yuichi; Kawase, Masato; Fukuta, Shimpei; Suzuki, Takahiro*; Kikuzawa, Nobuhiro; Ouchi, Nobuo

Proceedings of 11th Annual Meeting of Particle Accelerator Society of Japan (Internet), p.748 - 751, 2014/10

no abstracts in English

Journal Articles

Present status of J-PARC linac

Oguri, Hidetomo; Hasegawa, Kazuo; Ito, Takashi; Chishiro, Etsuji; Hirano, Koichiro; Morishita, Takatoshi; Shinozaki, Shinichi; Ao, Hiroyuki; Okoshi, Kiyonori; Kondo, Yasuhiro; et al.

Proceedings of 11th Annual Meeting of Particle Accelerator Society of Japan (Internet), p.389 - 393, 2014/10

no abstracts in English

Journal Articles

Organic solvent-free water-developable sugar resist material derived from biomass in green lithography

Takei, Satoshi*; Oshima, Akihiro*; Ichikawa, Takumi*; Sekiguchi, Atsushi*; Kashiwakura, Miki*; Kozawa, Takahiro*; Tagawa, Seiichi*; Oyama, Tomoko; Ito, Shoji*; Miyasaka, Hiroshi*

Microelectronic Engineering, 122, p.70 - 76, 2014/06

 Times Cited Count:21 Percentile:17.73(Engineering, Electrical & Electronic)

Biomass-derived branched sugar resist material was developed for environmentally-friendly electron beam lithography (EBL). The developed resist enables organic solvent-free water-developable process. The resist performance was evaluated using 75 keV EBL system. Lines of 50-200 nm were fabricated with high sensitivity of 7 $$mu$$C/cm$$^{2}$$. The resist is developable in pure water at 23 $$^{circ}$$C for 60 s, and it has acceptable CF$$_{4}$$ etch selectivity.

Journal Articles

Construction of control system for J-PARC RF ion source & RFQ III test stand

Fukuta, Shimpei; Sawabe, Yuki; Suzuki, Takahiro*; Ishiyama, Tatsuya*; Kawase, Masato*; Ito, Yuichi; Kato, Yuko; Yoshii, Akinobu; Kikuzawa, Nobuhiro; Ouchi, Nobuo

Proceedings of 10th Annual Meeting of Particle Accelerator Society of Japan (Internet), p.1122 - 1125, 2014/06

The installation of Cs-seeded RF-driven H$$^{-}$$ ion source (RF ion source) to J-PARC LINAC is scheduled in 2014. Similarly the replacement of RFQ III from RFQ is scheduled in 2014. The test stand of the cooperation of RF ion source & RFQ III is being made in the J-PARC LINAC building for the beam acceleration examination now. The J-PARC control group designed test stand control system by thinking that test stand control system had to be equal to J-PARC accelerator control system. Specifically, Introduction of MPS for protect an apparatus. Implementation of EPICS environment for remotely controlling the equipment. It is construction of the timing system for sending a timing signal to each accelerator component device. This report describes construction of the control system in a test stand.

Journal Articles

Upgrade of power supply system for RF-chopper at J-PARC Linac

Futatsukawa, Kenta*; Ikegami, Masanori*; Ito, Yuichi; Kikuzawa, Nobuhiro; Sato, Fumiaki; Shinozaki, Shinichi; Suzuki, Takahiro*; Chishiro, Etsuji; Hirano, Koichiro; Fang, Z.*; et al.

Proceedings of 10th Annual Meeting of Particle Accelerator Society of Japan (Internet), p.1149 - 1153, 2014/06

no abstracts in English

244 (Records 1-20 displayed on this page)