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Journal Articles

Level structures of $$^{56,58}$$Ca cast doubt on a doubly magic $$^{60}$$Ca

Chen, S.*; Browne, F.*; Doornenbal, P.*; Lee, J.*; Obertelli, A.*; Tsunoda, Yusuke*; Otsuka, Takaharu*; Chazono, Yoshiki*; Hagen, G.*; Holt, J. D.*; et al.

Physics Letters B, 843, p.138025_1 - 138025_7, 2023/08

Gamma decays were observed in $$^{56}$$Ca and $$^{58}$$Ca following quasi-free one-proton knockout reactions from $$^{57,59}$$Sc. For $$^{56}$$Ca, a $$gamma$$ ray transition was measured to be 1456(12) keV, while for $$^{58}$$Ca an indication for a transition was observed at 1115(34) keV. Both transitions were tentatively assigned as the $$2^{+}_{1} rightarrow 0^{+}_{gs}$$ decays. A shell-model calculation in a wide model space with a marginally modified effective nucleon-nucleon interaction depicts excellent agreement with experiment for $$2^{+}_{1}$$ level energies, two-neutron separation energies, and reaction cross sections, corroborating the formation of a new nuclear shell above the N = 34 shell. Its constituents, the $$0_{f5/2}$$ and $$0_{g9/2}$$ orbitals, are almost degenerate. This degeneracy precludes the possibility for a doubly magic $$^{60}$$Ca and potentially drives the dripline of Ca isotopes to $$^{70}$$Ca or even beyond.

Journal Articles

"Southwestern" boundary of the $$N = 40$$ island of inversion; First study of low-lying bound excited states in $$^{59}$$V and $$^{61}$$V

Elekes, Z.*; Juh$'a$sz, M. M.*; Sohler, D.*; Sieja, K.*; Yoshida, Kazuki; Ogata, Kazuyuki*; Doornenbal, P.*; Obertelli, A.*; Achouri, N. L.*; Baba, Hidetada*; et al.

Physical Review C, 106(6), p.064321_1 - 064321_10, 2022/12

 Times Cited Count:0 Percentile:0.02(Physics, Nuclear)

The low-lying level structure of $$^{59}$$V and $$^{61}$$V was investigated for the first time. The neutron knockout reaction and inelastic proton scattering were applied for $$^{61}$$V while the neutron knock-out reaction provided the data for $$^{59}$$V. Four and five new transitions were determined for $$^{59}$$V and $$^{61}$$V, respectively. Based on the comparison to our shell-model calculations using the Lenzi-Nowacki-Poves-Sieja (LNPS) interaction, three of the observed $$gamma$$ rays for each isotope could be placed in the level scheme and assigned to the decay of the first 11/2$$^{-}$$ and 9/2$$^{-}$$ levels. The ($$p$$,$$p'$$) excitation cross sections for $$^{61}$$V were analyzed by the coupled-channels formalism assuming quadrupole plus hexadecapole deformations. Due to the role of the hexadecapole deformation, $$^{61}$$V could not be unambiguously placed on the island of inversion.

Journal Articles

A First glimpse at the shell structure beyond $$^{54}$$Ca; Spectroscopy of $$^{55}$$K, $$^{55}$$Ca, and $$^{57}$$Ca

Koiwai, Takuma*; Wimmer, K.*; Doornenbal, P.*; Obertelli, A.*; Barbieri, C.*; Duguet, T.*; Holt, J. D.*; Miyagi, Takayuki*; Navr$'a$til, P.*; Ogata, Kazuyuki*; et al.

Physics Letters B, 827, p.136953_1 - 136953_7, 2022/04

 Times Cited Count:2 Percentile:54.36(Astronomy & Astrophysics)

no abstracts in English

JAEA Reports

Radiation monitoring using manned helicopter around the Nuclear Power Station in the fiscal year 2020 (Contract research)

Futemma, Akira; Sanada, Yukihisa; Ishizaki, Azusa; Kawasaki, Yoshiharu*; Iwai, Takeyuki*; Hiraga, Shogo*; Sato, Kazuhiko*; Haginoya, Masashi*; Matsunaga, Yuki*; Kikuchi, Hikaru*; et al.

JAEA-Technology 2021-029, 132 Pages, 2022/02

JAEA-Technology-2021-029.pdf:24.58MB

By the nuclear disaster of Fukushima Daiichi Nuclear Power Station (FDNPS), Tokyo Electric Power Company (TEPCO), caused by the Great East Japan Earthquake and the following tsunami on March 11, 2011, a large amount of radioactive material was released from the FDNPS. After the nuclear disaster, airborne radiation monitoring using manned helicopter has been conducted around FDNPS. The results of the airborne radiation monitoring and the evaluation for temporal change of dose rate in the fiscal 2020 were summarized in this report. Analysis considering topographical effects was applied to the result of the airborne monitoring to improve the accuracy of conventional method. In addition, technique for discriminating gamma rays from the ground and those from the airborne Rn-progenies was also utilized to evaluate their effect on airborne radiation monitoring.

Journal Articles

Investigation of the ground-state spin inversion in the neutron-rich $$^{47,49}$$Cl isotopes

Linh, B. D.*; Corsi, A.*; Gillibert, A.*; Obertelli, A.*; Doornenbal, P.*; Barbieri, C.*; Chen, S.*; Chung, L. X.*; Duguet, T.*; G$'o$mez-Ramos, M.*; et al.

Physical Review C, 104(4), p.044331_1 - 044331_16, 2021/10

AA2021-0468.pdf:1.29MB

 Times Cited Count:3 Percentile:48.27(Physics, Nuclear)

no abstracts in English

Journal Articles

Pairing forces govern population of doubly magic $$^{54}$$Ca from direct reactions

Browne, F.*; Chen, S.*; Doornenbal, P.*; Obertelli, A.*; Ogata, Kazuyuki*; Utsuno, Yutaka; Yoshida, Kazuki; Achouri, N. L.*; Baba, Hidetada*; Calvet, D.*; et al.

Physical Review Letters, 126(25), p.252501_1 - 252501_7, 2021/06

 Times Cited Count:8 Percentile:70.49(Physics, Multidisciplinary)

Direct proton-knockout reactions of $$^{55}$$Sc were studied at the RIKEN Radioactive Isotope Beam Factory. Populated states of $$^{54}$$Ca were investigated through $$gamma$$-ray and invariant-mass spectroscopy. Level energies were calculated from the nuclear shell model employing a phenomenological inter-nucleon interaction. Theoretical cross sections to states were calculated from distorted-wave impulse approximation estimates multiplied by the shell model spectroscopic factors. Despite the calculations showing a significant amplitude of excited neutron configurations in the ground-state of $$^{55}$$Sc, valence proton removals populated predominantly the ground-state of $$^{54}$$Ca. This counter-intuitive result is attributed to pairing effects leading to a dominance of the ground-state spectroscopic factor. Owing to the ubiquity of the pairing interaction, this argument should be generally applicable to direct knockout reactions from odd-even to even-even nuclei.

Journal Articles

First spectroscopic study of $$^{51}$$Ar by the ($$p$$,2$$p$$) reaction

Juh$'a$sz, M. M.*; Elekes, Z.*; Sohler, D.*; Utsuno, Yutaka; Yoshida, Kazuki; Otsuka, Takaharu*; Ogata, Kazuyuki*; Doornenbal, P.*; Obertelli, A.*; Baba, Hidetada*; et al.

Physics Letters B, 814, p.136108_1 - 136108_8, 2021/03

AA2020-0747.pdf:0.83MB

 Times Cited Count:3 Percentile:48.27(Astronomy & Astrophysics)

The nuclear structure of $$^{51}$$Ar was studied by the ($$p$$,2$$p$$) reaction using $$gamma$$-ray spectroscopy for the bound and unbound states. Comparing the results to our shell-model calculations, two bound and six unbound states were established. The low cross sections populating the two bound states of $$^{51}$$Ar could be interpreted as a clear signature for the presence of significant sub-shell closures at neutron numbers 32 and 34 in argon isotopes.

JAEA Reports

Robot operation manual for reconnaissance

Chiba, Yusuke; Nishiyama, Yutaka; Tsubaki, Hirohiko; Iwai, Masaki; Furukawahara, Ryo; Ono, Hayato*; Hayasaka, Toshiro*

JAEA-Testing 2020-007, 42 Pages, 2021/02

JAEA-Testing-2020-007.pdf:4.38MB

Maintenance and Operation Section for Remote Control Equipment in Naraha Center for Remote Control Technology Development was the main part of the nuclear emergency response team of JAEA in full-scale operation starts on the 1st of April, 2020. In this section, we need to develop equipment for a JAEA nuclear emergency. To support full-scale operation, we have created a work robot for opening and closing doors, a work robot for opening and closing valves, and a reconnaissance robot for measuring radiation dose. This report describes how to operate a Reconnaissance robot.

JAEA Reports

Work robot (for valves opening/closing) operation manual

Chiba, Yusuke; Nishiyama, Yutaka; Tsubaki, Hirohiko; Iwai, Masaki; Ono, Hayato*; Hayasaka, Toshiro*

JAEA-Testing 2020-006, 24 Pages, 2021/02

JAEA-Testing-2020-006.pdf:3.35MB

Maintenance and Operation Section for Remote Control Equipment in Naraha Center for Remote Control Technology Development was the main part of the nuclear emergency response team of JAEA in full-scale operation starts on the 1st of April, 2020. In this section, we need to develop equipment for a JAEA nuclear emergency. To support full- scale operation, we have created a work robot for opening and closing doors, a work robot for opening and closing valves, and a reconnaissance robot for measuring radiation dose. This report describes how to operate a work robot (opening and closing valves).

JAEA Reports

Work robot (for opening and closing the door) operation manual

Chiba, Yusuke; Nishiyama, Yutaka; Tsubaki, Hirohiko; Iwai, Masaki; Furukawahara, Ryo; Ono, Hayato*; Hayasaka, Toshiro*

JAEA-Testing 2020-005, 29 Pages, 2021/02

JAEA-Testing-2020-005.pdf:3.07MB

Maintenance and Operation Section for Remote Control Equipment in Naraha Center for Remote Control Technology Development was the main part of the nuclear emergency response team of JAEA in full-scale operation starts on the 1st of April, 2020. In this section, we need to develop equipment for a JAEA nuclear emergency. To support full-scale operation, we have created a work robot for opening and closing doors, a work robot for opening and closing valves, and a reconnaissance robot for measuring radiation dose. This report describes how to operate the work robot (for opening and closing the door).

Journal Articles

$$N$$ = 32 shell closure below calcium; Low-lying structure of $$^{50}$$Ar

Cort$'e$s, M. L.*; Rodriguez, W.*; Doornenbal, P.*; Obertelli, A.*; Holt, J. D.*; Men$'e$ndez, J.*; Ogata, Kazuyuki*; Schwenk, A.*; Shimizu, Noritaka*; Simonis, J.*; et al.

Physical Review C, 102(6), p.064320_1 - 064320_9, 2020/12

AA2020-0748.pdf:0.75MB

 Times Cited Count:9 Percentile:74.44(Physics, Nuclear)

Low-lying excited states in the $$N$$ = 32 isotope $$^{50}$$Ar were investigated by in-beam $$gamma$$-ray spectroscopy following proton- and neutron-knockout, multinucleon removal, and proton inelastic scattering at the RIKEN Radioactive Isotope Beam Factory. The energies of the two previously reported transitions have been confirmed, and five additional states are presented for the first time, including a candidate for a 3$$^{-}$$ state. The level scheme built using $$gamma$$ $$gamma$$ coincidences was compared to shell-model calculations in the $$sd-pf$$ model space and to ${it ab initio}$ predictions based on chiral two- and three-nucleon interactions. Theoretical proton- and neutron-knockout cross sections suggest that two of the new transitions correspond to 2$$^{+}$$ states, while the previously proposed 4$$^{+}_{1}$$ state could also correspond to a 2$$^{+}$$ state.

JAEA Reports

Design and produce two sets of multi-joint manipulator (for opening a door) against nuclear disaster and a crawler robot for opening and closing manual valves

Nishiyama, Yutaka; Iwai, Masaki; Chiba, Yusuke; Tsubaki, Hirohiko; Ono, Hayato*; Hayasaka, Toshiro*; Hanyu, Toshinori*

JAEA-Technology 2020-007, 18 Pages, 2020/09

JAEA-Technology-2020-007.pdf:2.33MB

Maintenance and Operation Section for Remote Control Equipment in Naraha Center for Remote Control Technology Development is the main part of the nuclear emergency response team of Japan Atomic Energy Agency (JAEA) in full-scale operation starts on the 1st of April, 2020. The section needs to develop equipment for JAEA nuclear emergency. Because of dealing the full-scale operation, the section designed and produced two sets of Multi-joint Manipulator or (for Opening Doors) against Nuclear Disaster in order to put them on two crawler robots in 2018 fiscal year. And the section also designed and produced a Crawler Robot for Opening and Closing Manual Valves in 2019 fiscal year. This report shows two sets of Multi-Joint Manipulator (for Opening Doors) and a Crawler Robot for Opening and Closing Manual Valves designed and produced by Maintenance and Operation Section for Remote Control Equipment in 2018 and 2019 fiscal year.

JAEA Reports

Design and mounting advanced wireless communication equipment on the crawler-type robots for tasks and on the crawler-type scouting robot

Nishiyama, Yutaka; Iwai, Masaki; Tsubaki, Hirohiko; Chiba, Yusuke; Hayasaka, Toshiro*; Ono, Hayato*; Hanyu, Toshinori*

JAEA-Technology 2020-006, 26 Pages, 2020/08

JAEA-Technology-2020-006.pdf:2.43MB

Maintenance and Operation Section for Remote Control Equipment in Naraha Center for Remote Control Technology Development is the main part of the nuclear emergency response team of JAEA deal with Act on Special Measures Concerning Nuclear Emergency Preparedness. The section needs to remodel crawler-type robots for tasks, crawler-type scouting robots, and so on. About two crawler-type robots for tasks, the section designed and mounted advanced wireless communication equipment on manipulators mounted on the two robots. The crawler part of the robot has been able to be controlled by way of the new equipment, and when it is broken down, it can be changed by way of an original equipment. And the new equipment makes a single relay robot controllable both the crawler part and the manipulator part of the robot, in case of wireless relay robots being needed. And after checking the ability and characteristic about 5 wireless communication equipment, the section chose and mounted the best equipment on one crawler-type scouting robot. This report shows design and mounting advanced wireless communication equipment on the two crawler-type robots for tasks and on the one crawler-type scouting robot.

JAEA Reports

Development of the vertically moveable dose rate meter for a nuclear emergency response robot

Iwai, Masaki

JAEA-Technology 2020-004, 14 Pages, 2020/06

JAEA-Technology-2020-004.pdf:2.88MB

Maintenance and Operation Section for Remote Control Equipment in Naraha Center for Remote Control Technology Development needs to develop equipment for JAEA nuclear emergency, and because of reasonably and effectively developing machines, the section members examined plants in JAEA must deal with the new low. Then, radiation rates detectors with an elevator on a crawler robot were found as a very useful system, and the system was designed and produced. This report shows radiation rates detectors with an elevator for a crawler robot designed and produced by Maintenance and Operation Section for Remote Control Equipment in 2018 fiscal year.

Journal Articles

Shell evolution of $$N$$ = 40 isotones towards $$^{60}$$Ca; First spectroscopy of $$^{62}$$Ti

Cort$'e$s, M. L.*; Rodriguez, W.*; Doornenbal, P.*; Obertelli, A.*; Holt, J. D.*; Lenzi, S. M.*; Men$'e$ndez, J.*; Nowacki, F.*; Ogata, Kazuyuki*; Poves, A.*; et al.

Physics Letters B, 800, p.135071_1 - 135071_7, 2020/01

 Times Cited Count:28 Percentile:96.38(Astronomy & Astrophysics)

Excited states in the $$N$$ = 40 isotone $$^{62}$$Ti were populated via the $$^{63}$$V($$p$$,$$2p$$)$$^{62}$$Ti reaction at $$sim$$200 MeV/nucleon at the Radioactive Isotope Beam Factory and studied using $$gamma$$-ray spectroscopy. The energies of the $$2_1^+ rightarrow 0_{rm gs}^+$$ and $$4_1^+ rightarrow 2_1^+$$ transitions, observed here for the first time, indicate a deformed Ti ground state. These energies are increased compared to the neighboring $$^{64}$$Cr and $$^{66}$$Fe isotones, suggesting a small decrease of quadrupole collectivity. The present measurement is well reproduced by large-scale shell-model calculations based on effective interactions, while ab initio and beyond mean-field calculations do not yet reproduce our findings.

Journal Articles

Quasifree neutron knockout from $$^{54}$$Ca corroborates arising $$N=34$$ neutron magic number

Chen, S.*; Lee, J.*; Doornenbal, P.*; Obertelli, A.*; Barbieri, C.*; Chazono, Yoshiki*; Navr$'a$til, P.*; Ogata, Kazuyuki*; Otsuka, Takaharu*; Raimondi, F.*; et al.

Physical Review Letters, 123(14), p.142501_1 - 142501_7, 2019/10

AA2019-0306.pdf:0.57MB

 Times Cited Count:41 Percentile:92.88(Physics, Multidisciplinary)

no abstracts in English

JAEA Reports

Training programs of emergency response robots operation for operators in each site of JAEA beginner class / intermediate class

Chiba, Yusuke; Nishiyama, Yutaka; Tsubaki, Hirohiko; Iwai, Masaki

JAEA-Technology 2019-002, 29 Pages, 2019/03

JAEA-Technology-2019-002.pdf:2.43MB

Act on Special Measures Concerning Nuclear Emergency Preparedness was amended on the 30th of October in 2017. As the JAEA Emergency Assistance Organization, Maintenance and Operation Section for Remote Control Equipment in Naraha Center for Remote Control Technology Development started training for emergency response robots operation for operators in each site of JAEA in response to the new amendment. The training consists of three operations: small crawler-type mobile scouting robots, big crawler-type mobile robots with a manipulator or a long tong and small radio-controlled helicopters. The training has three classes (beginner, intermediate and advanced classes) depending on skills and experiences. This paper reports the training programs of emergency response robots operation of the beginner and intermediate classes which were used in the first half of fiscal 2018.

Journal Articles

Pyrochemical treatment of spent nitride fuels for MA transmutation

Hayashi, Hirokazu; Sato, Takumi; Shibata, Hiroki; Kurata, Masaki; Iwai, Takashi; Arai, Yasuo

Science China; Chemistry, 57(11), p.1427 - 1431, 2014/11

 Times Cited Count:5 Percentile:5.9(Chemistry, Multidisciplinary)

Nitride fuels have several advantages, such as high thermal conductivity and high metal density like metallic fuels, and high melting point and isotropic crystal structure like oxide fuels. Since the late 1990s, the partitioning and transmutation of minor actinides (MA) has been studied to decrease the long term radio-toxicity of high level waste and mitigate the burden on the final disposal. Japan Atomic Energy Agency (JAEA) has been proposing dedicated transmutation cycle using the Accelerator-Driven System (ADS) with the nitride fuels containing MA. We have been developing the nitride fuel cycle including pyrochemical process. Our focus is on electrolysis of nitride fuels and refabrication of nitride fuel from the recovered actinides because other processes are similar to the technology for the metal fuel treatment and have been studied elsewhere. In this paper, we summarized our activity on developments of the pyrochemical treatment of the spent nitride fuels.

Journal Articles

Preparation of TRU alloys by electrochemical or lithium reduction method

Nakajima, Kunihisa; Iwai, Takashi; Arai, Yasuo; Kurata, Masaki*; Nakamura, Kinya*; Arita, Yuji*

Proceedings of 10th OECD/NEA Information Exchange Meeting on Actinide and Fission Product Partitioning and Transmutation (CD-ROM), 9 Pages, 2010/00

Information on phase diagram and thermodynamic data of transuranium (TRU) alloys are required for the development of metallic fuel fabrication technology and fuel design for TRU transmutation. In the present study, TRU alloys were prepared from their mixed oxides to establish these informations. A few grams of mother alloys containing TRU elements were prepared from their mixed oxides in the electrochemical reduction method. However, it was found in the electrochemical reduction of PuO$$_{2}$$ that only the sample surfaces were reduced to metal. It is anticipated that the electrochemical conversion of mixed oxides with high Np and Pu contents into metals are difficult owing to production of low-melting metals. Thus, the Li reduction method was applied to the reduction of mixed oxides with high TRU contents and the alloys with high Np and Pu contents were prepared.

Journal Articles

Simultaneous recovery of all actinides from spent nuclear fuel by carbamoylmethylphosphine oxide in fluorinated diluents

Ozawa, Masaki; Iwai, Takehiko*; Babain, V.*; Shadrin, A.*

Proceedings of International Solvent Extraction Conference "Solvent Extraction-Fundamentals to Industrial Applications" (ISEC 2008), p.623 - 628, 2008/09

Bifunctional organophosphorus extractants dissolved in polar fluorinated diluents were studied aiming at directly recovering all f-elements from the dissolver solution of spent nuclear fuel. Distribution ratios of U, Np and Pu were sufficiently high for 0.4$$sim$$0.8MCMPO in this solvent system, and combination of salt-free, methylamine carbonate (MAC), etc, were evaluated to obtain fractional stripping of f-elements. Static multi-stage extraction using artificial FBR dissolver solution supported the process feasibility.

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