Initialising ...
Initialising ...
Initialising ...
Initialising ...
Initialising ...
Initialising ...
Initialising ...
magnetic order with spatially alternating spin scalar chirality in overdoped Co
TaS
Cho, W.*; Park, P.*; Kim, C.*; An, Y.*; 飯田 一樹*; 梶本 亮一; Matin, S.*; Sibille, R.*; Crooker, S. A.*; Park, J.-G.*
Physical Review B, 113(17), p.174410_1 - 174410_14, 2026/05
被引用回数：0 パーセンタイル：0.00(Materials Science, Multidisciplinary)Co
TaS (
) exhibits a spontaneous Hall effect from spin texture in antiferromagnets, with a tetrahedral triple-Q () order and uniform spin scalar chirality. Upon Co overdoping (
), it undergoes a shift in magnetic ordering vectors from 
to 
. Interestingly, the spontaneous Hall effect disappeared in the overdoped regime, which was originally attributed to the loss of order. However, a question remains whether a new type of order can exist with alternating chirality in the overdoped regime. To address this, we investigated CoTaS using inelastic neutron scattering (INS), neutron diffraction, and optical dichroism, and found that INS data and spin-wave simulations support a order with alternating chirality. Moreover, neutron diffraction data show field-independent Bragg peaks, while linear dichroism detects no in-plane anisotropy, consistent with threefold rotation symmetry. Our data support the scenario of an alternating-chirality order in CoTaS, cancelling the spontaneous Hall effect. This study highlights a combined neutron-optical approach to identify complex spin textures.
Ahn, S. Y.*; Kim, E. S.*; Jeong, S. G.*; Harjo, S.; 川崎 卓郎; Gong, W.; Kim, H.-J.*; Hong, S.-J.*; Hong, S. I.*; Kwon, H.*; et al.
Materials Science & Engineering A, 955, p.149839_1 - 149839_18, 2026/03
被引用回数：2 パーセンタイル：93.63(Nanoscience & Nanotechnology)Additive manufacturing (AM) of particle-reinforced metal matrix composites (MMCs) enables control of both strength and deformation behavior. In this study, TiC (2 wt%) nanoparticles were added to Fe
Co
NiCr
medium-entropy alloy (MEA) using directed energy deposition (DED). Although part of the TiC decomposed during processing, the released C and Ti stabilized the 
-austenite phase and suppressed deformation-induced martensitic transformation (DIMT), shifting deformation toward slip-dominated behavior. Microstructural observations revealed dispersed TiC particles and modified grain boundary morphology that promoted distributed plastic flow. In-situ neutron diffraction during tensile testing confirmed enhanced early-stage dislocation activity. These findings demonstrate that nanoparticle-induced phase stability changes strongly influence deformation mechanisms in AM-processed MMCs.
N(
,
)
O reaction rates via the 
F(,
)
F reactionKim, S. H.*; Chae, K. Y.*; 浅井 雅人; 廣瀬 健太郎; 佐藤 哲也; 牧井 宏之; 西尾 勝久; Orlandi, R.; Smallcombe, J.; 洲嵜 ふみ; et al.
Journal of the Korean Physical Society, 6 Pages, 2026/00
被引用回数：0 パーセンタイル：0.00(Physics, Multidisciplinary)コア崩壊超新星爆発(CCSNe)の元素合成シミュレーションにおいて、N(,)O反応速度の不確実性が課題となっていた。本研究では、この反応を制約するため、JAEAタンデム加速器でF(,)F遷移反応実験を実施した。得られたトリトンスペクトルと角度分布から、関連するF共鳴の崩壊特性(部分幅)を詳細に測定し、その結果を用いて反応速度パラメータを精密化した。これにより、CCSNe核合成モデルの信頼性向上が期待できる。
Jeong, S. G.*; Kwon, J.*; Kim, E. S.*; Prasad, K.*; Harjo, S.; Gong, W.; 川崎 卓郎; Estrin, Y.*; Bouaziz, O.*; Hong, S. I.*; et al.
Materials Science & Engineering A, 942, p.148712_1 - 148712_11, 2025/10
被引用回数：2 パーセンタイル：46.97(Nanoscience & Nanotechnology)The cellular structure plays a key role in determining the mechanical properties of metal additive manufacturing (MAM) components. This study presents in situ neutron diffraction and dislocation density-based modeling for a CoCrFeMnNi high-entropy alloy (HEA) made via directed energy deposition (DED). A constitutive model based on the Kocks-Mecking-Estrin framework was used to represent the cellular structure. Parametric analysis showed lower dislocation accumulation and annihilation rates in the as-built sample (with cellular structure) than in the heat-treated one. These differences are linked to dislocation forest networks and local stacking fault energy variations. Dislocation density across cell interiors and walls was also compared with deformation-induced dislocation cells.
Gu, G. H.*; Jeong, S. G.*; Heo, Y.-U.*; Harjo, S.; Gong, W.; Cho, J.*; Kim, H. S.*; 他4名*
Journal of Materials Science & Technology, 223, p.308 - 324, 2025/07
被引用回数：9 パーセンタイル：88.88(Materials Science, Multidisciplinary)Face-centered cubic (FCC) equi-atomic multi-principal element alloys (MPEAs) exhibit excellent mechanical properties from cryogenic to room temperatures. At room temperature, deformation is dominated by dislocation slip, while at cryogenic temperatures (CTs), reduced stacking fault energy enhances strain hardening with twinning. This study uses in-situ neutron diffraction to analyze the temperature-dependent deformation behavior of Al
(CoNiV)
, a dual-phase (FCC/BCC) medium-entropy alloy (MEA). At liquid nitrogen temperature (LNT), deformation twinning in the FCC matrix leads to additional strain hardening through the dynamic Hall-Petch effect, giving the appearance of improved strengthening at LNT. In contrast, BCC precipitates show dislocation slip at both 77 K and 298 K, with temperature-dependent lattice friction stress playing a significant role in strengthening. The study enhances understanding of deformation behaviors and provides insights for future alloy design.
magnetic orderings in a triangular lattice; Implications for multi- orderings in general two-dimensional latticesPark, P.*; Cho, W.*; Kim, C.*; An, Y.*; 飯田 一樹*; 梶本 亮一; Matin, S.*; Zhang, S.-S.*; Batista, C. D.*; Park, J.-G.*
Physical Review X, 15(3), p.031032_1 - 031032_29, 2025/07
被引用回数：5 パーセンタイル：84.08(Physics, Multidisciplinary)Multi- magnetic structures on two-dimensional (2D) lattices provide a key route to realizing topological physics in 2D magnetism. A major experimental challenge is to unambiguously confirm their formation by excluding the possibility of topologically trivial multi-domain single- or double- magnetic orders, which cannot be distinguished using conventional diffraction techniques. Here, we propose that long-wavelength spin dynamics offers a universal diagnostic for triangular lattices: triple- orders that preserve rotational symmetry and single- or double- orders that break it exhibit qualitatively distinct anisotropies in their Goldstone mode velocities, stemming from fundamental differences in their underlying spin configurations. We validate this concept using the metallic triangular-lattice antiferromagnet Co
TaS, which hosts both a stripe-type single- state and a triple- tetrahedral ordering at different temperatures. Using inelastic neutron-scattering and spin dynamics simulations, we first refine the spin Hamiltonian by fitting the paramagnetic excitation spectra, allowing us to develop an unbiased model independent of magnetic ordering. We then show that the observed velocity profiles of the Goldstone modes agree with the high-temperature model's predictions: markedly anisotropic for the single- phase and near isotropic for the triple- phase. Importantly, this contrast persists across various exchange parameters, highlighting its model-independent nature and suggesting potential applicability to other 2D lattice systems. Beyond the long-wavelength regime, we present a substantial discrepancy between the measured and simulated magnon spectra exclusively in the triple- phase. We attribute this discrepancy to magnon energy renormalization arising from order-of-magnitude-enhanced magnon-magnon interactions in the triple- phase, due to its noncollinear configuration. This work provides universal insight into the dynamical properties of topological multi- magnetic orderings in 2D lattice structures, offering a broadly applicable diagnostic to distinguishing them from topologically trivial single- or double- counterparts. The unequivocal confirmation of the triple- structure in CoTaS further establishes it as a prominent material platform for exploring topological spin textures in the genuine 2D limit.
Kim, Y. S.*; Kang, T.*; Hong, S.-K.*; Brechtl, J.*; Lebyodkin, M.*; Cheng, Y.-H.*; Huang, E.-W.*; Liaw, P. K.*; Harjo, S.; Gong, W.; et al.
Acta Materialia, 292, p.120970_1 - 120970_16, 2025/06
被引用回数：15 パーセンタイル：96.30(Materials Science, Multidisciplinary)Metallic materials can exhibit low-temperature serrated deformation (LTSD) at cryogenic temperatures, potentially causing sudden failures. Understanding LTSD is thus crucial for ensuring material reliability in such environments. LTSD has been explained by two main mechanisms: (i) dislocation-based mechanical instability and (ii) thermomechanical instability, but each has limitations when considered alone. To address this, we propose a new LTSD mechanism, a thermally induced dislocation dynamics model, based on cryogenic experimental evidence. This model accounts for dislocation avalanches and localized heating, leading to hierarchical dislocation networks and transitions in deformation modes. A modified deformation-mechanism map for SS316L is also presented. Our findings highlight the rate-dependent nature of LTSD and negative strain-rate sensitivity, including the first observation of links between small stress fluctuations and large serrations.
杉田 裕; 大野 宏和; Beese, S.*; Pan, P.*; Kim, M.*; Lee, C.*; Jove-Colon, C.*; Lopez, C. M.*; Liang, S.-Y.*
Geomechanics for Energy and the Environment, 42, p.100668_1 - 100668_21, 2025/06
被引用回数：6 パーセンタイル：87.84(Energy & Fuels)国際共同プロジェクトDECOVALEX-2023は、数値解析を使用してベントナイト系人工バリアの熱-水-応力(または熱-水)相互作用を研究するためのタスクDとして、幌延人工バリア性能確認試験を対象とした。このタスクは、モデル化のために、1つの実物大の原位置試験と、補完的な4つの室内試験が選択された。幌延人工バリア性能確認試験は、人工的な地下水注入と組み合わせた温度制御非等温の試験であり、加熱フェーズと冷却フェーズで構成されている。6つの研究チームが、さまざまなコンピューターコード、定式化、構成法則を使用して、熱-水-応力または熱-水(研究チームのアプローチによって異なる)数値解析を実行した。
Go, G.*; Goli, D. P.*; 江崎 蘭世; Tserkovnyak, Y.*; Kim, S. K.*
Physical Review Research (Internet), 7(2), p.L022066_1 - L022066_7, 2025/06
It remains an open question whether or not the scalar spin chirality itself can exhibit a Hall-type transport. In this work, we show that the answer is yes: The scalar spin chirality is Hall-transported in Kagome ferromagnets and antiferromagnets under an external bias, engendering a phenomenon which we dub the scalar spin chirality Nernst effect. Our findings call for the need to lift the conventional assumption that the scalar spin chirality is a static quantity in order to discover the active roles of the scalar spin chirality in transport properties.
Cho, S. H.*; Cho, S. W.*; Lv, Z.*; 関根 由莉奈; Liu, S.*; Zhou, M.*; Nuxoll, R. F.*; Kanatzidis, E. E.*; Ghaffari, R.*; Kim, D.*; et al.
Lab on a Chip, 25(7), p.1647 - 1655, 2025/04
被引用回数：16 パーセンタイル：98.61(Biochemical Research Methods)アミノ酸は体内のタンパク質合成と代謝プロセスに不可欠な物質である。本研究では、運動中の汗からのアミノ酸損失について定量的に調べることを目的とした。汗中のアミノ酸含有量をリアルタイムで分析するため、測定のための技術基盤としてウェアラブルなマイクロ流体システムを構築した。定量分析を実現するため、ウェアラブルデバイスに蛍光アッセイを組み込み、さらにスマートフォンベースの画像化技術を統合させたシステムを開発した。
川崎 卓郎; 福田 竜生; 山中 暁*; 村山 一郎*; 加藤 孝典*; 馬場 将亮*; 橋本 英樹*; Harjo, S.; 相澤 一也; 田中 裕久*; et al.
Journal of Applied Physics, 137(9), p.094101_1 - 094101_7, 2025/03
被引用回数：1 パーセンタイル：28.15(Physics, Applied)Energy harvesting from waste heat can improve energy efficiency in society. This research investigated the structural behaviors of lead zirconate titanate-based ferroelectric ceramics using operando neutron diffraction measurements under the conditions of two energy-harvesting cycles that involve consideration of the temperature changes of automobile exhaust gas for achieving good harvesting efficiencies. Input and output electrical energies and neutron diffraction data were simultaneously collected. The obtained time-resolved neutron-diffraction intensity data indicate that the applied electric fields and temperature changes induced 90
domain rotation and lattice strain. These structural changes and their variations depending on cycle conditions, such as temperature changes, applied electric fields, and circuit switching, provide insight into the origins of the differences in the behaviors of electrical input/output energies in the cycles.
signatures in two-dimensional cone beam interferometrySarenac, D.*; Gorbet, G.*; Clark, C. W.*; Cory, D. G.*; Ekinci, H.*; Henderson, M. E.*; Huber, M. G.*; Hussey, D. S.*; Kapahi, C.*; Kienzle, P. A.*; et al.
Physical Review Research (Internet), 6(3), p.L032054_1 - L032054_8, 2024/09
Neutron interferometry has played a distinctive role in fundamental science and characterization of materials. Moir neutron interferometers are candidate next-generation instruments: they offer microscopy-like magnification of the signal, enabling direct camera recording of interference patterns across the full neutron wavelength spectrum. Here we demonstrate the extension of phase-grating moir interferometry to two-dimensional geometries. Our measurements of phase topologies and gravitationally induced phase shifts are in good agreement with theory.
Nguyen, T.-D.*; Singh, C.*; Kim, Y. S.*; Han, J. H.*; Lee, D.-H.*; Lee, K.*; Harjo, S.; Lee, S. Y.*
Journal of Materials Research and Technology, 31, p.1547 - 1556, 2024/07
被引用回数：9 パーセンタイル：68.96(Materials Science, Multidisciplinary)This study investigates the mechanical properties of a friction-stir-welded (FSW) AA6061-T6 aluminum alloy at ultra-low temperature (ULT) of 20 K. In-situ neutron diffraction and orientation imaging microscopy were employed to compare the tensile deformation behavior of the base metal (BM) and heat-affected zone (HAZ) in the FSW aluminum plate. The results demonstrate that compared to room-temperature (RT), ULT induces a significant improvement in tensile strength and ductility in both the BM and HAZ. The enhanced mechanical properties in BM at ULT result from a more homogeneous deformation than occurs at RT. On the other hand, HAZ at ULT exhibits an even lower yield strength than at RT, but the strain hardening rate (SHR) is the most significant among the alloys, leading to a tensile strength of 346 MPa and the highest ductility of 46.8%. The lowest yield strength corresponds to the lowest-hardness zones in HAZ, caused by dissolved/coarsened precipitates during the FSW process.
久保田 真彦*; Kim, S.-Y.*; Wu, H.*; 渡部 創; 佐野 雄一; 竹内 正行; 新井 剛*
Journal of Radioanalytical and Nuclear Chemistry, 333(5), p.2413 - 2420, 2024/05
被引用回数：4 パーセンタイル：64.33(Chemistry, Analytical)To minimize the use of organic solvents and achieve a selective adsorption separation of minor actinides (MA(III)) and Ln(III), adsorbents consisting of SiO-P particles impregnated with hexaoctylnitrilotriacetamide (HONTA) were prepared. Batch experiments were performed to evaluate the adsorption properties of the HONTA/SiO-P adsorbent for MA(III) and simulated fission products in HNO
solution. The uniform distribution of Eu(III) on the adsorbent was confirmed via particle induced X-ray emission analysis, and X-ray photoelectron spectroscopy revealed that EuNO was the adsorbed species. This study provides a simplified process for the separation of MA(III) using a HONTA/SiO-P packed column.
Kim, Y. S.*; Chae, H.*; Lee, D.-Y.*; Han, J. H.*; Hong, S.-K.*; Na, Y. S.*; Harjo, S.; 川崎 卓郎; Woo, W.*; Lee, S.-Y.*
Materials Science & Engineering A, 899, p.146453_1 - 146453_7, 2024/05
被引用回数：12 パーセンタイル：78.71(Nanoscience & Nanotechnology)This work focused on the mechanical properties and serration-involved deformation behavior of advanced alloys at 15 K. Evolution of stacking faults and 
-martensite improved the mechanical performance of CoCrNi alloys, and significant strain-induced martensite transformation of DED-SS316L led to superior strength and strain hardening. A magnitude in stress drop was governed by dislocation density, phase type, and lattice defects, irrespective of processing method. FCC {200} notably was influenced recovery behavior after stress drop, and the contribution of strain energy density by serration on tensile toughness was the greatest for HR-CoCrNi.
大沢 直樹*; Kim, S.-Y.*; 久保田 真彦*; Wu, H.*; 渡部 創; 伊藤 辰也; 永石 隆二
Nuclear Engineering and Technology, 56(3), p.812 - 818, 2024/03
被引用回数：5 パーセンタイル：64.33(Nuclear Science & Technology)An impregnated silica-based adsorbent was prepared by combining HONTA extractant, Crea extractant, and macroporous silica polymer composite particles (SiO-P). The performance of platinum-group metals adsorption and separation on prepared (HONTA + Crea)/SiO-P adsorbent was assessed by batch-adsorption and chromatographic separation studies. (HONTA + Crea)/SiO-P adsorbent showed high adsorption performance of Pd(II) owing to an affinity between Pd(II) and Crea extractant based on the Hard and Soft Acids and Bases theory. The chromatographic experiment showed that Pd(II) was recovered entirely from the feed solution using 0.2 M thiourea in 0.1 M HNO. Possibility of recovery of Zr(IV), Mo(VI), and Re(VII) was also observed using the (HONTA + Crea)/SiO-P adsorbent.
Linh, B. D.*; Corsi, A.*; Gillibert, A.*; Obertelli, A.*; Doornenbal, P.*; Barbieri, C.*; Duguet, T.*; G
mez-Ramos, M.*; Holt, J. D.*; Hu, B. S.*; et al.
Physical Review C, 109(3), p.034312_1 - 034312_15, 2024/03
被引用回数：6 パーセンタイル：78.06(Physics, Nuclear)理化学研究所RIビームファクトリーにて中性子過剰核
Arビームからの1中性子ノックアウト反応実験を行い、
Arのエネルギー準位および分光学的因子を導出した。特に、第一励起状態の
への分光学的因子が大きいことから、始状態のArの基底状態において中性子が
軌道を多く占めていることがわかった。これは、中性子数32がよい魔法数として知られる
Caとは異なった性質であり、カルシウムからアルゴンへと陽子が2個減ることで閉殻構造が大きく崩れることが明らかになった。
TaSPark, P.*; Cho, W.*; Kim, C.*; An, Y.*; Kang, Y.-G.*; Avdeev, M.*; Sibille, R.*; 飯田 一樹*; 梶本 亮一; Lee, K. H.*; et al.
Nature Communications (Internet), 14, p.8346_1 - 8346_9, 2023/12
被引用回数：70 パーセンタイル：94.42(Multidisciplinary Sciences)The triangular lattice antiferromagnet (TLAF) has been the standard paradigm of frustrated magnetism for several decades. The most common magnetic ordering in insulating TLAFs is the 120 structure. However, a new triple- chiral ordering can emerge in metallic TLAFs, representing the short wavelength limit of magnetic skyrmion crystals. We report the metallic TLAF CoTaS as the first example of tetrahedral triple- magnetic ordering with the associated topological Hall effect (non-zero 
). We also present a theoretical framework that describes the emergence of this magnetic ground state, which is further supported by the electronic structure measured by angle-resolved photoemission spectroscopy. Additionally, our measurements of the inelastic neutron scattering cross section are consistent with the calculated dynamical structure factor of the tetrahedral triple- state.
Yang, D. S.*; Wu, Y.*; Kanatzidis, E. E.*; Avila, R.*; Zhou, M.*; Bai, Y.*; Chen, S.*; 関根 由莉奈; Kim, J.*; Deng, Y.*; et al.
Materials Horizons, 10(11), p.4992 - 5003, 2023/09
被引用回数：31 パーセンタイル：86.05(Chemistry, Multidisciplinary)本論文では、ハード及びソフトハイブリッド材料システムでの3Dプリントによって形成されたマイクロ流体ネットワーク、統合バルブ、およびマイクロスケール光学キュベットにより、汗成分に対してその場で分光および蛍光分析した成果を紹介する。一連の試験により、これらのマイクロキュベットシステムが汗中の銅、塩化物、グルコースの濃度と汗のpHを実験室レベルの精度と感度で評価できることが実証された。
Ca cast doubt on a doubly magic 
CaChen, S.*; Browne, F.*; Doornenbal, P.*; Lee, J.*; Obertelli, A.*; 角田 佑介*; 大塚 孝治*; 茶園 亮樹*; Hagen, G.*; Holt, J. D.*; et al.
Physics Letters B, 843, p.138025_1 - 138025_7, 2023/08
被引用回数：21 パーセンタイル：93.22(Astronomy & Astrophysics)
Scからの1陽子ノックアウト反応を用いて、
Caと
Caのガンマ崩壊を観測した。Caでは1456(12)keVの線遷移が、Caでは1115(34)keVの遷移が観測された。どちらの遷移も暫定的に
と割り当てられた。有効核子間相互作用をわずかに修正した広い模型空間での殻模型計算では、
準位エネルギー、2中性子分離エネルギー、反応断面積が実験とよく一致し、N=34閉殻の上に新しい殻が形成されていることを裏付けた。その構成要素である
と
軌道はほぼ縮退しており、これはCaが二重魔法核である可能性を排除し、Ca同位体のドリップラインを
Caあるいはそれ以上にまで広げる可能性がある。
