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Journal Articles

Angular distribution of $$gamma$$ rays from a neutron-induced $$p$$-wave resonance of $$^{132}$$Xe

Okudaira, Takuya*; Tani, Yuika*; Endo, Shunsuke; Doskow, J.*; Fujioka, Hiroyuki*; Hirota, Katsuya*; Kameda, Kento*; Kimura, Atsushi; Kitaguchi, Masaaki*; Luxnat, M.*; et al.

Physical Review C, 107(5), p.054602_1 - 054602_7, 2023/05

 Times Cited Count:1 Percentile:68.16(Physics, Nuclear)

no abstracts in English

Journal Articles

Measurement of the transverse asymmetry of $$gamma$$ rays in the $$^{117}$$Sn($$n,gamma$$)$$^{118}$$Sn reaction

Endo, Shunsuke; Okudaira, Takuya*; Abe, Ryota*; Fujioka, Hiroyuki*; Hirota, Katsuya*; Kimura, Atsushi; Kitaguchi, Masaaki*; Oku, Takayuki; Sakai, Kenji; Shima, Tatsushi*; et al.

Physical Review C, 106(6), p.064601_1 - 064601_7, 2022/12

 Times Cited Count:2 Percentile:52.69(Physics, Nuclear)

no abstracts in English

Journal Articles

Angular distribution of $$gamma$$ rays from the $$p$$-wave resonance of $$^{118}$$Sn

Koga, Jun*; Takada, Shusuke*; Endo, Shunsuke; Fujioka, Hiroyuki*; Hirota, Katsuya*; Ishizaki, Kohei*; Kimura, Atsushi; Kitaguchi, Masaaki*; Niinomi, Yudai*; Okudaira, Takuya*; et al.

Physical Review C, 105(5), p.054615_1 - 054615_5, 2022/05

 Times Cited Count:3 Percentile:66.85(Physics, Nuclear)

no abstracts in English

Journal Articles

Energy-dependent angular distribution of individual $$gamma$$ rays in the $$^{139}$$La($$n, gamma$$)$$^{140}$$La$$^{ast}$$ reaction

Okudaira, Takuya*; Endo, Shunsuke; Fujioka, Hiroyuki*; Hirota, Katsuya*; Ishizaki, Kohei*; Kimura, Atsushi; Kitaguchi, Masaaki*; Koga, Jun*; Niinomi, Yudai*; Sakai, Kenji; et al.

Physical Review C, 104(1), p.014601_1 - 014601_6, 2021/07

 Times Cited Count:4 Percentile:57.13(Physics, Nuclear)

JAEA Reports

Design and production of the valve used in Radioactive Liquid Disposal Facility

Nishimura, Arashi; Okada, Yuji; Sugaya, Naoto; Sonobe, Hiroshi; Kimura, Nobuaki; Kimura, Akihiro; Hanawa, Yoshio; Nemoto, Hiroyoshi

JAEA-Technology 2021-003, 51 Pages, 2021/05

JAEA-Technology-2021-003.pdf:5.55MB

In the Japan Materials Testing Reactor (JMTR), the leakage accidents of radioactive waste liquid were occurred from the tanks and pipes of the liquid waste disposal facility in the JMTR tank-yard building in JFY2014. In order to respond to the accident, obtain the approval of the JAEA to the design and construction method from JFY2016, the tanks and pipes were replaced from JFY2016 to 2019. In the replaced, the production of the tanks and pipes of the liquid waste disposal facility applied Japanese technical standards correspondingly. On the other hand, the valve did not fall under the category of Japanese technical standards. The manufacturing specifications when replacing the valve were decided based on the including the selecting the standards of production and inspection for valves, Fluid properties, experience in JMTR. The production proceeded while carrying out the decided inspection. The valves that passed all the inspections were installed together with the tanks and pipes of the liquid waste, and the finished inspection was performed as a systems. The construction was completed with those inspection passed. This report is summarized valve Design, production and installation.

Journal Articles

Spin-polarized Weyl cones and giant anomalous Nernst effect in ferromagnetic Heusler films

Sumida, Kazuki; Sakuraba, Yuya*; Masuda, Keisuke*; Kono, Takashi*; Kakoki, Masaaki*; Goto, Kazuki*; Zhou, W.*; Miyamoto, Koji*; Miura, Yoshio*; Okuda, Taichi*; et al.

Communications Materials (Internet), 1, p.89_1 - 89_9, 2020/11

JAEA Reports

Validation of repairing method for concrete wall of the JMTR tank-yard building

Sugaya, Naoto; Okada, Yuji; Nishimura, Arashi; Sonobe, Hiroshi; Kimura, Nobuaki; Kimura, Akihiro; Hanawa, Yoshio; Nemoto, Hiroyoshi

JAEA-Testing 2020-004, 67 Pages, 2020/08

JAEA-Testing-2020-004.pdf:8.17MB

In the Japan Materials Testing Reactor (JMTR), the leakage accidents of radioactive waste liquid were occurred from the tanks and pipes of the liquid waste disposal facility in the JMTR tank-yard building in JFY2014. In order to respond to the accident, the tanks and pipes were replaced from JFY2016 to 2019. On the other hand, a lot of cracks were occurred on the concreate wall of the tank-yard building when the frame structure supports were fixed to the concrete wall in the replacement work. Thus, it is necessary to repair the concreate wall of the tank-yard building. Especially, some cracks with swelling (cone-shaped fracture) were raised around some anchor bolts (the post-installed chemical anchor bolts) fixed the frame structure supports. The repairing method for the cone-shaped fracture of the concrete wall is standardized, but there was no reference value of tensile strength for the validation of the post-installed chemical anchor bolts after the repairing method. In this report, the repairing method was selected for the cone-shaped fracture on the concreate wall and the reference value of tensile strength for the validation of the post-installed chemical anchor bolts by this repairing method. The mock-ups for repairing cone-shaped fracture were fabricated by the selected repairing method and the tensile tests of the post-installed chemical anchor bolts were performed. From the results, the validation of the repairing method was obtained in this test and it was obvious the repairing of cone-shaped fracture is preferable method for the concreate wall of the JMTR tank-yard building.

Journal Articles

Transverse asymmetry of $$gamma$$ rays from neutron-induced compound states of $$^{140}$$La

Yamamoto, Tomoki*; Okudaira, Takuya; Endo, Shunsuke; Fujioka, Hiroyuki*; Hirota, Katsuya*; Ino, Takashi*; Ishizaki, Kohei*; Kimura, Atsushi; Kitaguchi, Masaaki*; Koga, Jun*; et al.

Physical Review C, 101(6), p.064624_1 - 064624_8, 2020/06

 Times Cited Count:9 Percentile:73.66(Physics, Nuclear)

Journal Articles

Measurement of the angular distribution of $$gamma$$-rays after neutron capture by $$^{139}$$La for a T-violation search

Okudaira, Takuya; Shimizu, Hirohiko*; Kitaguchi, Masaaki*; Hirota, Katsuya*; Haddock, C. C.*; Ito, Ikuya*; Yamamoto, Tomoki*; Endo, Shunsuke*; Ishizaki, Kohei*; Sato, Takumi*; et al.

EPJ Web of Conferences, 219, p.09001_1 - 09001_6, 2019/12

Parity violating effects enhanced by up to 10$$^6$$ times have been observed in several neutron induced compound nuclei. There is a theoretical prediction that time reversal (T) violating effects can also be enhanced in these nuclei implying that T-violation can be searched for by making very sensitive measurements. However, the enhancement factor has not yet been measured in all nuclei. The angular distribution of the (n,$$gamma$$) reaction was measured with $$^{139}$$La by using a germanium detector assembly at J-PARC, and the enhancement factor was obtained. From the result, the measurement time to achieve the most sensitive T-violation search was estimated as 1.4 days, and a 40% polarized $$^{139}$$La target and a 70% polarized $$^3$$He spin filter whose thickness is 70 atm$$cdot$$cm are needed. Therefore high quality $$^3$$He spin filter is developed in JAEA. The measurement result of the (n,$$gamma$$) reaction at J-PARC and the development status of the $$^3$$He spin filter will be presented.

Journal Articles

Angular distribution of $$gamma$$ rays from neutron-induced compound states of $$^{140}$$La

Okudaira, Takuya*; Takada, Shusuke*; Hirota, Katsuya*; Kimura, Atsushi; Kitaguchi, Masaaki*; Koga, Jun*; Nagamoto, Kosuke*; Nakao, Taro*; Okada, Anju*; Sakai, Kenji; et al.

Physical Review C, 97(3), p.034622_1 - 034622_15, 2018/03

 Times Cited Count:12 Percentile:71.12(Physics, Nuclear)

Journal Articles

Characterization of germanium detectors for the measurement of the angular distribution of prompt $$gamma$$-rays at the ANNRI in the MLF of the J-PARC

Takada, Shusuke*; Okudaira, Takuya*; Goto, Fumiya*; Hirota, Katsuya*; Kimura, Atsushi; Kitaguchi, Masaaki*; Koga, Jun*; Nakao, Taro*; Sakai, Kenji; Shimizu, Hirohiko*; et al.

Journal of Instrumentation (Internet), 13(2), p.P02018_1 - P02018_21, 2018/02

 Times Cited Count:6 Percentile:31.02(Instruments & Instrumentation)

Journal Articles

Development of prototype national nuclear forensics library at Japan Atomic Energy Agency

Kimura, Yoshiki; Shinohara, Nobuo; Funatake, Yoshio

Proceedings of INMM 56th Annual Meeting (Internet), 8 Pages, 2015/07

JAEA Reports

Report on research and development of nuclear forensics technologies

Okubo, Ayako; Kimura, Yoshiki; Shinohara, Nobuo; Toda, Nobufumi; Funatake, Yoshio; Watahiki, Masaru; Sakurai, Satoshi; Kuno, Yusuke

JAEA-Technology 2015-001, 185 Pages, 2015/03

JAEA-Technology-2015-001.pdf:56.65MB

Nuclear forensics is the analysis of intercepted illicit nuclear or radioactive material and any associated material to provide evidence for nuclear attribution by determining origin, history, transit routes and purpose involving such material. Nuclear forensics activity includes sampling of the illicit material, analysis of the samples and evaluation of the attribution by comparing the analyzed data with database or numerical simulation. Because the nuclear forensics technologies specify the origin of the nuclear materials used illegal dealings or nuclear terrorism, it becomes possible to identify and indict offenders, hence to enhance deterrent effect against such terrorism. Worldwide network on nuclear forensics can contribute to strengthen global nuclear security regime. In this paper, the results of research and development of fundamental nuclear forensics technologies performed in Japan Atomic Energy Agency during the fiscal term of 2011-2013 were reported.

Journal Articles

Progress and future prospects of nuclear forensics technology development project at JAEA

Kimura, Yoshiki; Shinohara, Nobuo; Sato, Kaneaki; Toda, Nobufumi; Shinoda, Yoshiharu; Funatake, Yoshio; Watahiki, Masaru; Kuno, Yusuke

Proceedings of INMM 55th Annual Meeting (Internet), 7 Pages, 2014/07

In 2010, the Japan Government issued the national statement at Nuclear Security Summit (Washington D.C., USA) to develop technologies related to measurement and detection of nuclear materials for nuclear forensics within three-year timeframe, and to share the products with the international community in order to contribute to strengthening the nuclear security system. In response to this statement, JAEA that possesses sufficient technical capabilities to fulfil this nuclear forensics mission has started a nuclear forensics technology development project since JFY 2011. This paper will present the progress of the development project during JFY 2011 to 2013. This project includes the developments of analytical technologies such as isotope and impurity measurements, morphology analysis, age determination technique, and the prototype of national nuclear forensics library (NNFL). Some future prospects of this project will be also presented in this paper.

Journal Articles

Lessons learned from the international tabletop exercise of national nuclear forensics library at JAEA

Kimura, Yoshiki; Shinohara, Nobuo; Funatake, Yoshio

Journal of Nuclear Materials Management, 42(4), p.40 - 45, 2014/00

Japan Atomic Energy Agency (JAEA) has initiated an R&D project on nuclear forensics technology from 2011. This project includes development of prototype national nuclear forensics library (NNFL), and the JAEA attended to the first international table top exercise of NNFL "Galaxy Serpent" held by ITWG as a part of our NNFL development project. In this paper, outline and experiences of the JAEA investigation in the table top exercise are described and the lessons learned from the experiences were discussed. Brief current status of the NNFL development project at JAEA was also introduced in the present paper. The lessons from the experiences in the exercise will be effectively applied to the development of NNFL at JAEA.

JAEA Reports

Preliminary test for Mo recycling system in $$^{99}$$Mo manufacturing process, 1; Reusability evaluation of Mo absorbent (Joint research)

Kimura, Akihiro; Niizeki, Tomotake*; Kakei, Sadanori*; Chakrova, Y.*; Nishikata, Kaori; Hasegawa, Yoshio*; Yoshinaga, Hideo*; Chakrov, P.*; Tsuchiya, Kunihiko

JAEA-Technology 2013-025, 40 Pages, 2013/10

JAEA-Technology-2013-025.pdf:2.62MB

Neutron Irradiation and Testing Reactor Center has developed the production of a medical isotope of $$^{99}$$Mo, the parent nuclide of $$^{99m}$$Tc by the (n,$$gamma$$) method using JMTR. The (n,$$gamma$$) method has an advantage of easy manufacturing process and low radioactive wastes generation. However, the low radioactivity concentration of $$^{99m}$$Tc is remaining as an issue. Therefore, PZC and PTC have been developed as adsorbent of molybdenum. Meanwhile, it is necessary to recycle the absorbent and Mo for the reduction of the radioactive waste of used-adsorbent and the effective use of limited resources, respectively. This report summarizes results of the synthesis of Mo adsorbents such as PZC and PTC, and the performance tests.

Journal Articles

Present status and future plan of development on National Nuclear Forensics Library at JAEA

Kimura, Yoshiki; Shinohara, Nobuo; Funatake, Yoshio; Sato, Kaneaki; Toda, Nobufumi; Shinoda, Yoshiharu; Watahiki, Masaru; Kuno, Yusuke

Kaku Busshitsu Kanri Gakkai (INMM) Nihon Shibu Dai-34-Kai Nenji Taikai Rombunshu (Internet), 9 Pages, 2013/10

Japan Atomic Energy Agency (JAEA) has initiated R&D project on nuclear forensics technology such as analytical technologies towards the establishment of nuclear forensics capabilities in Japan. National Nuclear Forensics Library (NNFL) is one of the fundamental nuclear forensics capabilities and a prototype NNFL has been developed as one R&D topic of the project at JAEA. Main objective of a NNFL is to determine whether a seized nuclear or other radioactive material from nuclear security event (e.g. illicit trafficking) is originated from a country or not. Analytical data of the seized material are compared with the existing materials populated in a NNFL, and its attributions such as origin and history will be identified. This paper describes the current status and future plan on the development of prototype NNFL. The outline and the results of the participation in an international table top exercise on NNFL named "Galaxy Serpent" were also reported in the present paper.

Journal Articles

Mo recycling property from generator materials with irradiated molybdenum

Kakei, Sadanori*; Kimura, Akihiro; Niizeki, Tomotake*; Ishida, Takuya; Nishikata, Kaori; Kurosawa, Makoto; Yoshinaga, Hideo*; Hasegawa, Yoshio*; Tsuchiya, Kunihiko

Proceedings of 6th International Symposium on Material Testing Reactors (ISMTR-6) (Internet), 7 Pages, 2013/10

The Japan Materials Testing Reactor (JMTR) is expected to contribute to the expansion of industrial utilization, such as the domestic production of $$^{99}$$Mo for the medical diagnosis medicine $$^{rm 99m}$$Tc. Production by the (n, $$gamma$$) method is proposed as domestic $$^{99}$$Mo production in JMTR because of the low amount of radioactive wastes and the easy $$^{99}$$Mo/$$^{rm 99m}$$Tc production process. Molybdenum oxide (MoO$$_{3}$$) pellets, poly zirconium compounds (PZC) and poly titanium compounds (PTC) are used as the irradiation target and generator for the production of $$^{99}$$Mo/$$^{rm 99m}$$Tc by the (n, $$gamma$$) method. However, it is necessary to use the enriched $$^{98}$$MoO$$_{3}$$, which is very expensive, to increase the specific activity of $$^{99}$$Mo. Additionally, a large amount of used PZC and PTC is generated after the decay of $$^{99}$$Mo. Therefore, this recycling technology of used PZC/PTC has been developed to recover molybdenum (Mo) as an effective use of resources and a reduction of radioactive wastes. The total Mo recovery rate of this process was 95.8%. From the results of the hot experiments, we could demonstrate that the recovery of MoO$$_{3}$$ and the recycling of PZC are possible. In the future, the equipment of recovering Mo will be installed in JMTR-Hot Cell, and this recycling process will be able to contribute to the reduction of production costs of $$^{rm 99m}$$Tc and the reduction of radioactive wastes.

JAEA Reports

Development of new molybdenum adsorbent

Kimura, Akihiro; Tanimoto, Masataka; Ishida, Takuya; Tsuchiya, Kunihiko; Hasegawa, Yoshio*; Hishinuma, Yukio*; Suzuki, Masashi*

JAEA-Technology 2011-012, 17 Pages, 2011/06

JAEA-Technology-2011-012.pdf:1.72MBJP, 2010-263801   Patent publication (In Japanese)

PZC (Poly-Zirconium Compound) was developed as adsorbent of molybdenum for $$^{99}$$Mo-$$^{rm 99m}$$Tc generator. However, PZC has some faults. So, new adsorbent based on titanium (PTC), was developed for getting rid of faults. This time, $$^{99}$$Mo adsorption and $$^{rm 99m}$$Tc elution tests with PZC and PTC were carried out. As a result, the $$^{99}$$Mo adsorption performance of the PTC was lower than PZC, on the other hand, $$^{rm 99m}$$Tc elution performance of the PTC was higher than PZC.

Journal Articles

Crystal growth procedure of HIV-1 protease-inhibitor KNI-272 complex for neutron structural analysis at 1.9 ${AA}$ resolution

Shimizu, Noriko*; Sugiyama, Shigeru*; Maruyama, Mihoko*; Takahashi, Yoshinori*; Adachi, Motoyasu; Tamada, Taro; Hidaka, Koshi*; Hayashi, Yoshio*; Kimura, Toru*; Kiso, Yoshiaki*; et al.

Crystal Growth & Design, 10(7), p.2990 - 2994, 2010/06

 Times Cited Count:11 Percentile:72.02(Chemistry, Multidisciplinary)

We report crystal growth of human immunodeficiency virus 1 protease (HIV PR) in a complex with its inhibitor KNI-272 by six different methods. Comparative analysis indicates that top-seeded solution growth (TSSG) and TSSG combined with the floating and stirring technique (TSSG-FAST) are efficient strategies for rapidly obtaining large single crystals and effectively preventing polycrystallization of the seed crystal. Neutron diffraction analysis confirmed that the crystalobtained by TSSG is a high-quality single crystal. Furthermore, crystal shape was observed to be influenced by solution flow, suggesting that the degree of supersaturation significantly affects the crystal growth direction of HIV PR complex. This finding implies that the shape of the HIV PR complex crystal might be controlled by the solution flow rate.

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