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論文

Ordered graphane nanoribbons synthesized via high-pressure diels-alder polymerization of 2,2'-bipyrazine

Li, F.*; Tang, X.*; Fei, Y.*; Zhang, J.*; Liu, J.*; Lang, P.*; Che, G.*; Zhao, Z.*; Zheng, Y.*; Fang, Y.*; et al.

Journal of the American Chemical Society, 147(17), p.14054 - 14059, 2025/04

 被引用回数:1 パーセンタイル:0.00(Chemistry, Multidisciplinary)

2,2'-ビピラジン(BPZ)の圧力誘起重合により結晶性グラファンナノリボン(GANR)を合成した。中性子回折データのリートベルト精密化,核磁気共鳴スペクトル,赤外スペクトル,理論計算を行った結果、BPZは$$pi$$ $$cdots$$ $$pi$$積層した芳香環の間でディールス・アルダー重合し、並外れた長距離秩序を持つ伸びたボート型GANR構造を形成することがわかった。未反応の-C=N-基がボートの両端を橋渡ししており、さらなる機能化の余地がある。このGANRのバンドギャップは2.25eVであり、光電応答は良好である(I$$_{on}$$/I$$_{off}$$ =18.8)。われわれの研究は、高圧トポケミカル重合法が、特定の構造と望んだ特性を持つグラファンの精密な合成に有望な方法であることを強調している。

論文

Neutron reflectometry study on the interfacial layer of epoxy resin to improve adhesion strength

Liu, Y.*; 宮田 登*; 宮崎 司*; 春藤 淳臣*; 川口 大輔*; 田中 敬二*; 青木 裕之

ACS Applied Materials & Interfaces, 8 Pages, 2025/00

The performance of structural adhesives is strongly influenced by the interfacial structure between the adhesive and adherend. In this study, we developed a nanometric stable interfacial layer derived from an epoxy resin system containing excess hardener. This layer, formed on solid substrates, exhibited excellent structural stability, even after extensive solvent washing. Neutron reflectometry (NR) was employed to investigate its structure under both dry and humid conditions, revealing a robust and well-defined interface that suppressed moisture accumulation at the adherend interface. FT-IR spectroscopy confirmed an excess of unreacted amino groups in the adsorbed layer, enabling further curing reactions with freshly applied epoxy resin. Re-coating experiments demonstrated that the adsorbed layer remained intact after thermal curing, suggesting strong interfacial compatibility. Notably, the presence of the adsorbed layer led to a significant enhancement in adhesive performance. Lap shear tests showed that the adhesion strength of the epoxy resin nearly doubled when the adsorbed layer was introduced at the interface. This approach does not rely on external coupling agents or primers, but instead utilizes a homologous material system to tailor interfacial properties through molecular-level design. The strategy presented here offers a practical and scalable method for improving adhesion in epoxy systems. By directly engineering the adhesive interface using components intrinsic to the epoxy formulation, this method enables reliable and enhanced bonding performance without altering the bulk material.

論文

Soft, wearable, microfluidic system for fluorometric analysis of loss of amino acids through eccrine sweat

Cho, S. H.*; Cho, S. W.*; Lv, Z.*; 関根 由莉奈; Liu, S.*; Zhou, M.*; Nuxoll, R. F.*; Kanatzidis, E. E.*; Ghaffari, R.*; Kim, D.*; et al.

Lab on a Chip, 9 Pages, 2025/00

 被引用回数:0 パーセンタイル:0.00(Biochemical Research Methods)

アミノ酸は体内のタンパク質合成と代謝プロセスに不可欠な物質である。本研究では、運動中の汗からのアミノ酸損失について定量的に調べることを目的とした。汗中のアミノ酸含有量をリアルタイムで分析するため、測定のための技術基盤としてウェアラブルなマイクロ流体システムを構築した。定量分析を実現するため、ウェアラブルデバイスに蛍光アッセイを組み込み、さらにスマートフォンベースの画像化技術を統合させたシステムを開発した。

論文

Measurements of displacement cross sections of metals for 120-GeV proton beam irradiation

岩元 洋介; 松田 洋樹*; 明午 伸一郎; 米原 克也*; Pellemoine, F.*; Liu, Z.*; Lynch, K.*; 吉田 誠*; 藪内 敦*; 義家 敏正*; et al.

Nuclear Instruments and Methods in Physics Research B, 557, p.165543_1 - 165543_8, 2024/12

 被引用回数:0 パーセンタイル:0.00(Instruments & Instrumentation)

陽子加速器施設における材料の照射損傷の指標として、原子1個当たりの変位数(dpa)が広く用いられている。金属材料のdpaを検証するために、3GeV以下の陽子に対する実験が行われてきた。しかし、3GeV以上の高エネルギー陽子に対する弾き出し断面積の測定は行われておらず、計算による検証も行われていない。そこで、高エネルギー領域における金属の弾き出し断面積を検証するため、温度8Kにおけるアルミニウム、銅、タングステンのワイヤーの電気抵抗率変化を、エネルギー120GeVの陽子を用いて測定した。その結果、粒子・重イオン輸送計算コードPHITSの従来の照射損傷モデルは実験データを過大評価することがわかった。一方、熱再結合補正モデルを用いた新たな計算結果は、測定された弾き出し断面積と一致した。この結果は、1GeV以上の陽子エネルギー領域では、弾き出し断面積はほぼ一定であり、1GeV陽子照射下での材料の損傷エネルギーは120GeV陽子照射下とほぼ同じであることに起因すると推定される。

論文

Study on heat transfer behavior of a cylindrical particle bed with volumetric heating

Wen, J.*; 鎌田 悠斗*; 横山 貢成*; 松元 達也*; Liu, W.*; 守田 幸路*; 今泉 悠也; 田上 浩孝; 松場 賢一; 神山 健司

Proceedings of 13th Korea-Japan Symposium on Nuclear Thermal Hydraulics and Safety (NTHAS13) (Internet), 8 Pages, 2024/11

The influence of water pool height, particles diameter and wall cooling on particle bed-water pool heat transfer was evaluated by assessing the time variation of average temperatures of the particle bed and water pool, and their difference. The concept of macroscopic heat transfer coefficient of the particle bed-water pool system was introduced to elucidate the intensity of natural convection. The results show that the time variation of temperature difference initially increases, peaks, and then decreases. Based on this phenomenon, the process of heat transfer of the particles bed-water pool system was explained. According to the result, the water pool height and particle diameter will affect the heat transfer, but the current cooling conditions have little influence on the heat transfer of the particle bed.

論文

Study on heat transfer behavior of a rectangular particle bed with volumetric heating

Wen, J.*; 鎌田 悠斗*; 横山 貢成*; 松元 達也*; Liu, W.*; 守田 幸路*; 今泉 悠也; 田上 浩孝; 松場 賢一; 神山 健司

Proceedings of 31st International Conference on Nuclear Engineering (ICONE31) (Internet), 8 Pages, 2024/11

To investigate the coolability of fuel debris bed immersed in molten steel, a rectangular experimental system was built in which the particle bed was volumetrically heated via direct current heating. The experimental apparatus consists of a particle bed immersed in water and a water pool above it, which simulate disrupted solid fuel and molten steel, respectively. Computer code simulations with reactor safety analysis code SIMMER-IV were performed to help understanding the heat transfer characteristics and to validate the applicability of the newly embedded momentum exchange function (MXF) models. Under the current experimental conditions, some key parameters like the particle bed average temperature, water pool average temperature, and temperature difference between the bed and the pool were evaluated to compare with the simulation results. The comparison results showed the most applicable MXF model under the current experimental conditions, and the analysis with it well reproduced the phenomena which was observed in the experiments.

論文

Enhancing mechanical properties of medium Mn steel by warm rolling based on laminated elemental segregation

Chen, H. F.*; Liu, B. X.*; 徐 平光; Fang, W.*; Tong, H. C.*; Yin, F. X.*

Journal of Materials Research and Technology, 32, p.3060 - 3069, 2024/09

 被引用回数:1 パーセンタイル:0.00(Materials Science, Multidisciplinary)

The hot-rolled microstructure of medium Mn steel has coarse grains and severe elemental segregation, resulting in low strength and plasticity. Constructing a multiphase structure, refining the microstructure, and regulating elemental segregation enhance the mechanical properties. In this study, liquid nitrogen treatment created a layered distribution of austenite and martensite. Warm rolling was then used to reduce layer thickness and refine grain structure. After liquid nitrogen and warm rolling treatments, the strength and plasticity of medium Mn steel increased to 1270 MPa and 23.3%, respectively, far exceeding the hot-rolled state (724 MPa, 12.8%). Warm rolling also triggers austenite reverted transformation (ART) and introduces high-density dislocations, further improving austenite stability. This strengthening effect is higher than that from intercritical annealing alone. Improved austenite stability delays the transformation induced plasticity (TRIP) effect, preventing brittle fracture and enhancing deformation coordination between layers, significantly increasing the plastic deformation capacity of medium Mn steel.

論文

Influence of interstitial carbon on bulk texture evolution of carbide-free high-entropy alloys during cold rolling using neutron diffraction

Fang, W.*; Liu, C.*; Zhang, J.*; 徐 平光; Peng, T.*; Liu, B.*; 諸岡 聡; Yin, F.*

Scripta Materialia, 249, p.116046_1 - 116046_6, 2024/08

 被引用回数:2 パーセンタイル:57.76(Nanoscience & Nanotechnology)

The influence of interstitial carbon on the texture evolution of high-entropy alloys during cold rolling was investigated. To prevent carbide formation, elements with weak carbon affinity were carefully selected in the (FeMnCoNi)$$_{96.5}$$C$$_{3.5}$$ alloy. Neutron diffraction, electron channeling contrast imaging, and electron backscatter diffraction were used to analyze the texture and microstructure evolution in alloys with and without carbon addition. Though their texture components are similar at the early stage of deformation, the Brass and Goss textures in the carbon-containing alloy at 50% cold rolling reduction are obviously higher than those in the carbon-free alloy, while Copper and S textures are lower. A large number of deformation twins induced in the carbon containing alloy is attributed as the significant reason for the texture differences. This work helps to understand the impact of interstitial carbon on the texture evolution of high-entropy alloys, providing valuable insights for microstructure and performance optimization.

論文

Stability enhancement by hydrophobic anchoring and a cross-linked structure of a phospholipid copolymer film for medical devices

内田 和杜*; 増田 造*; 原 伸太郎*; 松尾 陽一*; Liu, Y.*; 青木 裕之; 浅野 吉彦*; 宮田 一輝*; 福間 剛士*; 小野 俊哉*; et al.

ACS Applied Materials & Interfaces, 16(30), p.39104 - 39116, 2024/07

 被引用回数:1 パーセンタイル:30.18(Nanoscience & Nanotechnology)

Zwitterionic MPC polymer coatings effectively deter blood coagulation and protein buildup on medical devices. Researchers synthesized MPC copolymers containing a cross-linking unit (MPTMSi) plus one of four hydrophobic anchoring groups (MPTSSi, BMA, EHMA, LMA) and applied them to PDMS, PP, and PMP. These treatments yielded uniformly hydrophilic, electrically neutral surfaces. Protein adsorption tests showed that PMBSi (BMA) best resisted fluorescently labeled BSA, while PMLSi (LMA) was comparatively weaker, although all four coatings minimized platelet adhesion. Further analyses linked these differences in protein adsorption to varying swelling behaviors in water. Indeed, PMLSi absorbed more water, allowing some protein infiltration yet still repelling platelets. When tested under circulating flow to mimic shear stress, PMMMSi (MPTSSi) and PMLSi coatings on PP and PMP demonstrated excellent durability and platelet repellency. Overall, this study highlights how hydrophobic moieties can boost both hemocompatibility and stability of MPC-based coatings, promising improved performance in medical devices requiring low protein fouling, reduced platelet adhesion, and long-term reliability.

論文

In-plane movement of isolated poly(methacrylate) chains on a hydrophilic solid surface

Kawano, Masayuki*; 盛満 裕真*; Liu, Y.*; 宮田 登*; 宮崎 司*; 青木 裕之; 川口 大輔*; 山本 悟*; 田中 敬二*

Macromolecules, 57(14), p.6625 - 6633, 2024/07

 被引用回数:0 パーセンタイル:0.00(Polymer Science)

A better understanding of the dynamic behavior of polymer chains on solid surfaces is indispensable for the design and construction of high-performance polymer composites. We herein visualized the in-plane movement of isolated poly(methyl methacrylate) (PMMA) and poly(tert-butyl methacrylate) (PtBMA) single chains on hydrophilic silicon wafers under ambient conditions by atomic force microscopy. Isolated PMMA chains adsorbed to the substrate, whereas PtBMA chains diffused, the degree of which was dependent on the humidity. Neutron reflectivity revealed the formation of a layer of condensed water on the substrate. All-atomistic molecular dynamics simulations implied that the diffusivity difference of the two polymers was based on the submerged depth in which a part of a chain existed. That is, the interaction of a polymer with the surface of the hydrophilic substrate primarily governs its lateral movement, or adsorption behavior, facilitated by the presence of water.

論文

Dual nanoprecipitation and nanoscale chemical heterogeneity in a secondary hardening steel for ultrahigh strength and large uniform elongation

Wang, S.*; Wang, J.*; Zhang, S.*; Wei, D.*; Chen, Y.*; Rong, X.*; Gong, W.; Harjo, S.; Liu, X.*; Jiao, Z.*; et al.

Journal of Materials Science & Technology, 185, p.245 - 258, 2024/06

 被引用回数:17 パーセンタイル:98.00(Materials Science, Multidisciplinary)

Nanoprecipitates and nanoscale retained austenite (RA) with suitable stability play crucial roles in determining the yield strength (YS) and ductility of ultrahigh strength steels (UHSSs). However, owing to the kinetics incompatibility between nanoprecipitation and austenite reversion, it is highly challenging to simultaneously introduce high-density nanoprecipitates and optimized RA in UHSSs. In this work, through the combination of austenite reversion treatment (ART) and subsequent flash austenitizing (FA), nanoscale chemical heterogeneity was successfully introduced into a low-cost UHSS prior to the aging process. This chemical heterogeneity involved the enrichment of Mn and Ni in the austenite phase. The resulting UHSS exhibited dual-nanoprecipitation of Ni(Al,Mn) and (Mo,Cr)$$_{2}$$ C and nanoscale austenite stabilized via Mn and Ni enrichment. The hard martensitic matrix strengthened by high-density dual-nanoprecipitates constrains the plastic deformation of soft RA with a relatively low fraction, and the presence of relatively stable nanoscale RA with adequate Mn and Ni enrichment leads to a marginal loss in YS but keeps a persistent transformation-induced plasticity (TRIP) effect. As a result, the newly-developed UHSS exhibits an ultrahigh YS of 1.7 GPa, an ultimate tensile strength (UTS) of 1.8 GPa, a large uniform elongation (UE) of 8.5 percent, and a total elongation (TE) of 13 percent. The strategy of presetting chemical heterogeneity to introduce proper metastable phases before aging can be extended to other UHSSs and precipitation-hardened alloys.

論文

A Systematic approach for the adequacy analysis of a set of experimental databases; Application in the framework of the ATRIUM activity

Baccou, J.*; Glantz, T.*; Ghione, A.*; Sargentini, L.*; Fillion, P.*; Damblin, G.*; Sueur, R.*; Iooss, B.*; Fang, J.*; Liu, J.*; et al.

Nuclear Engineering and Design, 421, p.113035_1 - 113035_16, 2024/05

 被引用回数:6 パーセンタイル:96.49(Nuclear Science & Technology)

In the Best-Estimate Plus Uncertainty (BEPU) framework, the use of best-estimate code requires to go through a Verification, Validation and Uncertainty Quantification process (VVUQ). The relevance of the experimental data in relation to the physical phenomena of interest in the VVUQ process is crucial. Adequacy analysis of selected experimental databases addresses this problem. The outcomes of the analysis can be used to select a subset of relevant experimental data, to encourage designing new experiments or to drop some experiments from a database because of their substantial lack of adequacy. The development of a specific transparent and reproducible approach to analyze the relevance of experimental data for VVUQ still remains open and is the topic of this contribution. In this paper, the concept of adequacy initially introduced in the OECD/NEA SAPIUM (Systematic APproach for model Input Uncertainty quantification Methodology) activity is formalized. It is defined through two key properties, called representativeness and completeness, that allows considering the multifactorial dimension of the adequacy problem. A new systematic approach is then proposed to analyze the adequacy of a set of experimental databases. It relies on the introduction of two sets of criteria to characterize representativeness and completeness and on the use of multi-criteria decision analysis method to perform the analysis. Finally, the approach is applied in the framework of the new OECD/NEA ATRIUM activity which includes a set of practical IUQ exercises in thermal-hydraulics to test the SAPIUM guideline in determining input uncertainties and forward propagating them on an application case. It allows evaluating the adequacy of eight experimental databases coming from the Super Moby-dick, Sozzi-Sutherland and Marviken experiments and identifying the most adequate ones.

論文

Phase transformation and equation of state in Ti-45Al alloy under high pressure

Li, X.*; Zhu, R.*; Xin, J.*; Luo, M.*; Shang, S.-L.*; Liu, Z.-K.*; Yin, C.*; 舟越 賢一*; Dippenaar, R. J.*; 肥後 祐司*; et al.

CALPHAD; Computer Coupling of Phase Diagrams and Thermochemistry, 84, p.102641_1 - 102641_6, 2024/03

 被引用回数:0 パーセンタイル:0.00(Thermodynamics)

The phase transformations and pressure-volume dependencies of the Ti-45Al alloy with respect to pressure have been investigated by means of in-situ observation using multi anvil-type high-pressure devices and synchrotron radiation. Under hydrostatic compression from 0 to 10.1 GPa, about 2.3 vol. % of $$gamma$$ transforms continuously to $$alpha$$2. Lattice parameters as well as volume fractions of these two phases have been determined as a function of pressure. Bulk moduli estimated using Birch-Murnaghan's equation of state are 148 GPa for the $$gamma$$ phase, 138 GPa for the $$alpha$$2 phase, and 149 GPa for their two-phase mixture of Ti-45Al alloy. First-principles have also applied to investigate bulk moduli of two single phases, and the deviation between calculations and measurements is discussed and attributed to mainly phase transformation. The presently study provides useful insights into thermodynamics of $$alpha$$2 and $$gamma$$ phases under high pressure.

論文

Onset of collectivity for argon isotopes close to $$N=32$$

Linh, B. D.*; Corsi, A.*; Gillibert, A.*; Obertelli, A.*; Doornenbal, P.*; Barbieri, C.*; Duguet, T.*; G$'o$mez-Ramos, M.*; Holt, J. D.*; Hu, B. S.*; et al.

Physical Review C, 109(3), p.034312_1 - 034312_15, 2024/03

 被引用回数:2 パーセンタイル:74.11(Physics, Nuclear)

理化学研究所RIビームファクトリーにて中性子過剰核$$^{50}$$Arビームからの1中性子ノックアウト反応実験を行い、$$^{49}$$Arのエネルギー準位および分光学的因子を導出した。特に、第一励起状態の$$1/2^-$$への分光学的因子が大きいことから、始状態の$$^{50}$$Arの基底状態において中性子が$$p_{1/2}$$軌道を多く占めていることがわかった。これは、中性子数32がよい魔法数として知られる$$^{52}$$Caとは異なった性質であり、カルシウムからアルゴンへと陽子が2個減ることで閉殻構造が大きく崩れることが明らかになった。

論文

The BCC $$rightarrow$$ FCC hierarchical martensite transformation under dynamic impact in FeMnAlNiTi alloy

Li, C.*; Fang, W.*; Yu, H. Y.*; Peng, T.*; Yao, Z. T.*; Liu, W. G.*; Zhang, X.*; 徐 平光; Yin, F.*

Materials Science & Engineering A, 892, p.146096_1 - 146096_11, 2024/02

 被引用回数:6 パーセンタイル:79.11(Nanoscience & Nanotechnology)

The quasi-static superelastic responses and hierarchical martensite transformation from body-centered cubic (BCC) to face-centered cubic (FCC) under dynamic impact in Fe$$_{42}$$Mn$$_{34}$$Al$$_{15}$$Ni$$_{7.5}$$Ti$$_{1.5}$$ alloys were investigated. Polycrystalline and oligocrystalline alloys were produced through solution heat treatment and cyclic heat treatment processes, respectively. The results show the volume fraction of residual martensite for oligocrystalline alloys is lower, which exhibits better superelastic responses compared with polycrystalline alloys. Dynamic impact tests indicate that, despite the weakening of the grain boundary strengthening effect, the ultimate strength of the oligocrystalline alloys closely matches that of the polycrystalline alloys under dynamic impact. The martensite transformation of the FeMnAlNiTi alloy is characterized as hierarchical under dynamic impact, and increasing strain rates and grain sizes can enhance the BCC $$rightarrow$$ FCC martensite transformation, resulting in higher martensite phase fractions for oligocrystalline alloys. The increase in ultimate strength is attributed to the dynamic Hall-Petch effect introduced by more martensite phase interfaces under dynamic impact.

論文

J-PARC Linac and RCS; Operational status and upgrade plan to 2 MW

山本 風海; 守屋 克洋; 沖田 英史; 山田 逸平; 地村 幹; Saha, P. K.; 菖蒲田 義博; 田村 文彦; 山本 昌亘; 森下 卓俊; et al.

Journal of Neutron Research, 26(2-3), p.59 - 67, 2024/01

J-PARC Linacおよび3GeVシンクロトロン(RCS)は、1MWの大強度ビームを中性子実験施設および主リングシンクロトロンに供給するために運転している。これまで進めてきたビーム調整および機器改良により、当初想定よりもはるかに低いビームロス量で1MWのビーム運転を行うことが出来ている。現在のビーム出力はビームロスではなくRCSの高周波加速空胴の電源容量によって制限されている。近年、RCSグループではより少ない消費電力でビームを加速することのできる新しい構造の加速空胴の開発に成功した。この空胴によって、利用運転中に加速空胴で消費される電力を大幅に削減することが出来、さらに1MW以上の大出力での運転も可能となる。これまでの試験結果から、RCSの加速空胴を全て新しい物へ更新すれば、1.5MW以上の大出力も可能となる事が判っている。今後、中性子利用および主リングシンクロトロンの更なる成果創出のため、2MWを目標にRCSで必要な改良について検討を行った。その結果、高周波空胴の更新以外にも、高周波増幅器の増強やビームモニタの増強が必要であることが判ったため、今後順次更新を進める。

論文

Chiral Dirac fermion in a collinear antiferromagnet

Zhang, A.*; Deng, K.*; Sheng, J.*; Liu, P.*; Kumar, S.*; 島田 賢也*; Jiang, Z.*; Liu, Z.*; Shen, D.*; Li, J.*; et al.

Chinese Physics Letters, 40(12), p.126101_1 - 126101_8, 2023/12

 被引用回数:11 パーセンタイル:85.96(Physics, Multidisciplinary)

In a Dirac semimetal, the massless Dirac fermion has zero chirality, leading to surface states connected adiabatically to a topologically trivial surface state as well as vanishing anomalous Hall effect. Recently, itis predicted that in the nonrelativistic limit of certain collinear antiferromagnets, there exists a type of chiral "Dirac-like" fermion, whose dispersion manifests four-fold degenerate crossing points formed by spin-degenerate linear bands, with topologically protected Fermi arcs. Here, by combining with neutron diffraction and first-principles calculations, we suggest a multidomain collinear antiferromagnetic configuration, rendering the existence of the Fermi-arc surface states induced by chiral Dirac-like fermions.

論文

Petrophysical properties of representative geological rocks encountered in carbon storage and utilization

Hu, Q.*; Wang, Q. M.*; Zhang, T.*; Zhao, C.*; Iltaf, K. H.*; Liu, S. Q.*; 深津 勇太

Energy Reports (Internet), 9, p.3661 - 3682, 2023/12

 被引用回数:11 パーセンタイル:64.37(Energy & Fuels)

This study evaluates petrophysical properties of representative geological rocks in the context of injectivity, storage space, and caprock integrity for effective utilization and long-term storage of carbon dioxide. A total of 10 geological rocks were selected as representative storage media for consideration as saline aquifers & depleted oil and gas reservoirs, basalts, and cap rocks, as well as utilization in organic-rich shale and coal seams. An integrated suite of laboratory tests, including liquid immersion porosimetry, gas expansion porosimetry, grain size distribution, mercury intrusion porosimetry, and gas diffusion, were performed on these various rock samples. The results exhibit a disparity of petrophysical properties among two broad groups of rocks: rocks selected for possible storage of CO$$_{2}$$ have porosities of $$sim$$10-25%, permeabilities of $$sim$$10$$^{-16}$$-10$$^{-13}$$ m$$^{2}$$, $$mu$$m-sized pore-throat size distribution, and mostly good pore connectivity; in contrast, the potential caprocks have porosities of $$sim$$0.5-5%, permeabilities of $$sim$$10$$^{-20}$$-10$$^{-18}$$ m$$^{2}$$, pore throat sizes of $$<$$50 nm, and probably poorly connected pore networks. An understanding of the measured facets of pore structure and contribution of fractures is also critical in the context of different testing principles and data interpretation of petrophysical analyses, as well as observational scales in the laboratory and field, and therefore reliable confidence of CO$$_{2}$$ storage and utilization performance. Our work further illustrates the controlling influence of grain size distribution and geological processes on pore size distribution and pore connectivity for a wide range of rock types and lithologies, and particularly presents the extent and behavior of CO$$_{2}$$ gas diffusion with a custom-designed apparatus for a holistic understanding of various petrophysical attributes of widely different geological rocks.

論文

Validation of the $$^{10}$$Be ground-state molecular structure using $$^{10}$$Be($$p,palpha$$)$$^{6}$$He triple differential reaction cross-section measurements

Li, P. J.*; Beaumel, D.*; Lee, J.*; Assi$'e$, M.*; Chen, S.*; Franchoo, S.*; Gibelin, J.*; Hammache, F.*; Harada, T.*; 延与 佳子*; et al.

Physical Review Letters, 131(21), p.212501_1 - 212501_7, 2023/11

 被引用回数:21 パーセンタイル:94.59(Physics, Multidisciplinary)

$$^{10}$$Beのクラスター構造を($$p,palpha$$)反応を用いて調査した。三重微分断面積が実験的に測定され、Tohsaki-Horiuchi-Schuck-R$"o$pke波動関数の方法や反対称化分子動力学を用いた歪曲波インパルス近似計算と比較した。実験データと理論計算の顕著な一致が確認され、$$^{10}$$Beの比較的コンパクトな分子状態を確認した。

論文

Level structures of $$^{56,58}$$Ca cast doubt on a doubly magic $$^{60}$$Ca

Chen, S.*; Browne, F.*; Doornenbal, P.*; Lee, J.*; Obertelli, A.*; 角田 佑介*; 大塚 孝治*; 茶園 亮樹*; Hagen, G.*; Holt, J. D.*; et al.

Physics Letters B, 843, p.138025_1 - 138025_7, 2023/08

 被引用回数:9 パーセンタイル:89.00(Astronomy & Astrophysics)

$$^{57,59}$$Scからの1陽子ノックアウト反応を用いて、$$^{56}$$Caと$$^{58}$$Caのガンマ崩壊を観測した。$$^{56}$$Caでは1456(12)keVの$$gamma$$線遷移が、$$^{58}$$Caでは1115(34)keVの遷移が観測された。どちらの遷移も暫定的に$$2^{+}_{1} rightarrow 0^{+}_{gs}$$と割り当てられた。有効核子間相互作用をわずかに修正した広い模型空間での殻模型計算では、$$2^{+}_{1}$$準位エネルギー、2中性子分離エネルギー、反応断面積が実験とよく一致し、N=34閉殻の上に新しい殻が形成されていることを裏付けた。その構成要素である$$0_{f5/2}$$$$0_{g9/2}$$軌道はほぼ縮退しており、これは$$^{60}$$Caが二重魔法核である可能性を排除し、Ca同位体のドリップラインを$$^{70}$$Caあるいはそれ以上にまで広げる可能性がある。

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