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論文

Mechanical multiplexer of nuclear spin states

中堂 博之; 横井 直人*; 松尾 衛; 針井 一哉*; 鈴木 淳*; 今井 正樹; 佐藤 正寛*; 前川 禎通*; 齊藤 英治*

Physical Review Letters, 134(13), p.130603_1 - 130603_5, 2025/04

A spin 1/2 is the simplest system that has been believed to support a single two-level quantum system, represented by a single resonance. We experimentally demonstrate that a spin-1/2 nucleus of $$^{19}$$F in C$$_{6}$$F$$_{6}$$ exhibits an extra resonance corresponding to the emergence of the states, by mechanically rotating a sample and a coil in nuclear magnetic resonance (NMR) measurements. On the basis of the Floquet formalism, we identify the emergence of the extra two-level state due to the temporal periodicity generated by the mechanical rotation (mechanical spin multiplexing) and derive an operator algebra analogous to the planar rotor algebra in an effective description of the system. The observed multiplexing allows a single spin 1/2 to carry more than two states and potentially enabling the processing of multiple quantum bits on a single spin.

論文

Gyro-spintronic material science using vorticity gradient in solids

能崎 幸雄*; 介川 裕章*; 渡邉 紳一*; 柚木 清司*; 洞口 泰輔*; 中山 颯人*; 山野井 一人*; Wen, Z.*; He, C.*; Song, J.*; et al.

Science and Technology of Advanced Materials, 26(1), p.2428153_1 - 2428153_39, 2025/02

 被引用回数:0

We present a novel method for generating spin currents using the gyromagnetic effect, a phenomenon discovered over a century ago. This effect, crucial for understanding the origins of magnetism, enables the coupling between various macroscopic rotational motions and electron spins. While higher rotational speeds intensify the effect, conventional mechanical rotations, typically, below 10,000 RPM, produce negligible results comparable to geomagnetic fluctuations, limiting applied research. Our studies demonstrate that spin current generation comparable to that of rare metals can be achieved through atomic rotations induced by GHz- range surface acoustic waves and the rotational motion of conduction electrons in metallic thin films with nanoscale gradient modulation of electrical conductivity. These effects, termed the acoustic gyromagnetic effect and the current-vorticity gyromagnetic effect, are significant in different contexts.

論文

Observation of nonreciprocal diffraction of surface acoustic wave

新居 陽一*; 山本 慧; 菅野 将誠*; 前川 禎通*; 小野瀬 佳文*

Physical Review Letters, 134(2), p.027001_1 - 027001_5, 2025/01

 被引用回数:1 パーセンタイル:94.79(Physics, Multidisciplinary)

While the rectification phenomenon caused by the simultaneous breaking of time reversal and spatial inversion symmetries has been extended to a wide range of (quasi)particles and waves, the nonreciprocal diffraction, which is the imbalance of upward and downward deflections, was previously observed only for photons and remained to be extended to other (quasi)particles. Here, we present evidence of the nonreciprocal diffraction of surface acoustic wave (SAW) utilizing a magnetoelastic grating on a SAW device. Asymmetric diffraction intensities were observed when the ferromagnetic resonance was acoustically excited. Based on a theoretical model, we ascribe the microscopic origin of this phenomenon to the resonant scattering involving ferromagnetic resonance excitations. The novel property may pave an avenue to further development of SAW devices for various purposes including microwave communications and quantum engineering applications.

論文

Magnetostatic field induced by mechanical deformations

山本 慧; 前川 禎通*

Annalen der Physik, 536(5), p.2300395_1 - 2300395_11, 2024/05

 被引用回数:0 パーセンタイル:0.00(Physics, Multidisciplinary)

We derive a general expression for the magnetostatic field generated by mechanical deformations to a ferromagnetic material in the continuum description. Linearization with respect to the displacement vector is shown to be well defined. To demonstrate the use of the formulation, we discuss two examples. Firstly, a complete derivation of the magneto-rotation coupling for a uniformly magnetized film is given. Secondly, the lowest asymmetric mode of Lamb waves propagating through a magnetic vortex is shown to induce in-plane magnetostatic field localized around the vortex core.

論文

Strongly coupled spin waves and surface acoustic waves at room temperature

Hwang, Y.*; Puebla, J.*; 近藤 浩太*; Gonzalez-Ballestero, C.*; 一色 弘成*; S$'a$nchez Mu$~n$oz, C.*; Liao, L.*; Chen, F.*; Luo, W.*; 前川 禎通*; et al.

Physical Review Letters, 132(5), p.056704_1 - 056704_7, 2024/01

 被引用回数:9 パーセンタイル:96.33(Physics, Multidisciplinary)

Here, we report the observation of strong coupling between magnons and surface acoustic wave (SAW) phonons in a thin CoFeB film constructed in an on-chip SAW resonator by analyzing SAW phonon dispersion anticrossings. We employ a nanostructured SAW resonator design that, in contrast to conventional SAW resonators, allows us to enhance shear-horizontal strain. Crucially, this type of strain couples strongly to magnons. Our device design provides the tunability of the film thickness with a fixed phonon wavelength, which is a departure from the conventional approach in strong magnon-phonon coupling research. We detect a monotonic increase in the coupling strength by expanding the film thickness, which agrees with our theoretical model. Our work offers a significant way to advance fundamental research and the development of devices based on magnon-phonon hybrid quasiparticles.

論文

Acoustically driven magnon-phonon coupling in a layered antiferromagnet

Lyons, T. P.*; Puebla, J.*; 山本 慧; Deacon, R. S.*; Hwang, Y.*; 石橋 幸治*; 前川 禎通*; 大谷 義近*

Physical Review Letters, 131(19), p.196701_1 - 196701_6, 2023/11

 被引用回数:10 パーセンタイル:85.64(Physics, Multidisciplinary)

Harnessing the causal relationships between mechanical and magnetic properties of van der Waals materials presents a wealth of untapped opportunity for scientific and technological advancement, from precision sensing to novel memories. This can, however, only be exploited if the means exist to efficiently interface with the magnetoelastic interaction. Here, we demonstrate acoustically-driven spin-wave resonance in a crystalline antiferromagnet, chromium trichloride, via surface acoustic wave irradiation. The resulting magnon-phonon coupling is found to depend strongly on sample temperature and external magnetic field orientation, and displays a high sensitivity to extremely weak magnetic anisotropy fields in the few mT range. Our work demonstrates a natural pairing between power-efficient strain-wave technology and the excellent mechanical properties of van der Waals materials, representing a foothold towards widespread future adoption of dynamic magneto-acoustics.

論文

Valley-selective phonon-magnon scattering in magnetoelastic superlattices

Liao, L.*; Puebla, J.*; 山本 慧; Kim, J.*; 前川 禎通*; Hwang, Y.*; Ba, Y.*; 大谷 義近*

Physical Review Letters, 131(17), p.176701_1 - 176701_6, 2023/10

 被引用回数:8 パーセンタイル:83.30(Physics, Multidisciplinary)

Phonons and magnons are engineered by periodic potential landscapes in phononic and magnonic crystals, and their combined studies may enable valley phonon transport tunable by the magnetic field. Through nonreciprocal surface acoustic wave transmission, we demonstrate valley-selective phonon-magnon scattering in magnetoelastic superlattices. The lattice symmetry and the out-of-plane magnetization component control the sign of nonreciprocity. The phonons in the valleys play a crucial role in generating nonreciprocal transmission by inducing helical strains that couple with the magnons. The transmission spectra show a nonreciprocity peak near a transmission gap, matching the phononic band structure. Our results open the way for manipulating valley phonon transport through periodically varying magnon-phonon coupling.

論文

Hybridized propagation of spin waves and surface acoustic waves in a multiferroic-ferromagnetic heterostructure

Chen, J.*; 山本 慧; Zhang, J.*; Ma, J.*; Wang, H.*; Sun, Y.*; Chen, M.*; Liu, S.*; Gao, P.*; Yu, D.*; et al.

Physical Review Applied (Internet), 19(2), p.024046_1 - 024046_9, 2023/02

 被引用回数:6 パーセンタイル:69.27(Physics, Applied)

Coherent coupling in magnon based hybrid system has many potential applications in quantum information processing. Magnons can propagate in magnetically ordered materials without any motion of electrons, offering a unique method to build low-power-consumption devices and information channels free of heat dissipation. In this article, we demonstrate the coherent propagation of hybridized modes between spin waves and Love surface acoustic waves in a multiferroic BiFeO$$_{3}$$ and ferromagnetic La$$_{0.67}$$Sr$$_{0.33}$$MnO$$_{3}$$ based heterostructure. The magneto-elastic coupling enables a giant enhancement of strength of the hybridized mode by a factor of 26 compared to that of the pure spin waves. A short wavelength down to 250 nm is demonstrated for the hybridized mode, which is desirable for nanoscale acousto-magnonic applications. Our combined experimental and theoretical analyses represent an important step towards the coherent control in hybrid magnonics, which may inspire the study of magnon-phonon hybrid systems for coherent information processing and manipulation.

論文

Shapiro steps in charge-density-wave states driven by ultrasound

森 道康; 前川 禎通

Applied Physics Letters, 122(4), p.042202_1 - 042202_5, 2023/01

 被引用回数:4 パーセンタイル:54.88(Physics, Applied)

We show that ultrasound can induce the Shapiro steps (SS) in the charge-density-wave (CDW) state. When ultrasound with frequency $$omega$$ and a dc voltage are applied, the SS occur at the current $$Ipropto nomega$$ with integer $$n$$. Even and odd multiples of SS are represented by two couplings between the CDW and ultrasound. Although an ac voltage bias with frequency $$omega$$ induces the SS at $$Ipropto nomega$$, the ultrasound bias enhances the odd multiples more strongly than the even ones. This is the difference between the ultrasound and the ac voltage. Since the SS cause abrupt peaks in the $$dV/dI$$, the extreme changes in the $$I-V$$ curve will be applied to a very sensitive ultrasound detector.

論文

Spin and spin current; From fundamentals to recent progress

前川 禎通; 吉川 貴史*; 中堂 博之; 家田 淳一; 齊藤 英治

Journal of Applied Physics, 133(2), p.020902_1 - 020902_24, 2023/01

 被引用回数:21 パーセンタイル:93.58(Physics, Applied)

Along with the progress of spin science and spintronics research, the flow of electron spins, i.e., spin current, has attracted interest. New phenomena and electronic states were explained in succession using the concept of spin current. Moreover, as many of the conventionally known spintronics phenomena became well organized based on spin current, it has rapidly been recognized as an essential concept in a wide range of condensed matter physics. In this article, we focus on recent developments in the physics of spin, spin current, and their related phenomena, where the conversion between spin angular momentum and different forms of angular momentum plays an essential role. Starting with an introduction to spin current, we first discuss the recent progress in spintronic phenomena driven by spin-exchange coupling: spin pumping, topological Hall torque, and emergent inductor. We, then, extend our discussion to the interaction/interconversion of spins with heat, lattice vibrations, and charge current and address recent progress and perspectives on the spin Seebeck and Peltier effects. Next, we review the interaction between mechanical motion and electron/nuclear spins and argue the difference between the Barnett field and rotational Doppler effect. We show that the Barnett effect reveals the angular momentum compensation temperature, at which the net angular momentum is quenched in ferrimagnets.

論文

Skyrmion creation and annihilation by electric current vorticity

藤本 純治*; 船木 博志*; 小椎八重 航*; 松尾 衛; 前川 禎通*

IEEE Transactions on Magnetics, 58(8), p.1500407_1 - 1500407_7, 2022/08

 被引用回数:2 パーセンタイル:21.37(Engineering, Electrical & Electronic)

Motivated by the recent experiment done by Yu et al. [X. Z. Yu, et. al., Sci. Adv., 6, 25, eaaz9744 (2020)] on magnetic skyrmion creation and annihilation by electric currents in FeGe devices with a notch structure, we examine the interaction between the electric current vorticity near the notch and localized spins, and obtain three effects of the current vorticity on the localized spins. The first one is an effective Zeeman field induced by the current vorticity. This effective Zeeman field is responsible for skyrmion creation. The second effect is a vorticity-induced Dzyaloshinskii-Moriya (DM) interaction with the direction of the DM vector being parallel to the vorticity direction and is different from the vector of the intrinsic DM interaction. This vorticity-induced DM interaction makes the skyrmions distorted. The third effect is a spin current due to the gradient of the vorticity and the spin current drives the magnetic skyrmions far from the notch. Our theory opens a new path to design the magnetic textures by using structural settings.

論文

Magnetic properties and electronic configurations of Mn ions in the diluted magnetic semiconductor Ba$$_{1-x}$$K$$_x$$(Zn$$_{1-y}$$Mn$$_y$$)$$_2$$As$$_2$$ studied by X-ray magnetic circular dichroism and resonant inelastic X-ray scattering

鈴木 博人*; Zhao, G.*; 岡本 淳*; 坂本 祥哉*; Chen, Z.-Y.*; 野中 洋亮*; 芝田 悟朗; Zhao, K.*; Chen, B.*; Wu, W.-B.*; et al.

Journal of the Physical Society of Japan, 91(6), p.064710_1 - 064710_5, 2022/06

 被引用回数:0 パーセンタイル:0.00(Physics, Multidisciplinary)

The magnetic properties and the electronic excitations of the new diluted magnetic semiconductor Ba$$_{1-x}$$K$$_x$$(Zn$$_{1-y}$$Mn$$_y$$)$$_2$$As$$_2$$ have been studied by X-ray magnetic circular dichroism (XMCD) and resonant inelastic X-ray scattering (RIXS). The sum rule analysis of the XMCD spectra indicates that the Mn atoms are in the high-spin configurations of $$d^5$$, whereas the presence of competing ferromagnetic and antiferromagnetic interactions between the Mn ions reduces the net spin moment. Based on a comparison of the RIXS line shapes with those of Ga$$_{1-x}$$Mn$$_x$$As, it is concluded that the ground state of Mn in Ba$$_{1-x}$$K$$_x$$(Zn$$_{1-y}$$Mn$$_y$$)$$_2$$As$$_2$$ consists of both the $$3d^5 underline{L}$$ and $$3d^5$$ electron configurations.

論文

Perspectives on spintronics with surface acoustic waves

Puebla, J.*; Hwang, Y.*; 前川 禎通*; 大谷 義近*

Applied Physics Letters, 120(22), p.220502_1 - 220502_9, 2022/05

 被引用回数:34 パーセンタイル:93.71(Physics, Applied)

Surface acoustic waves (SAWs) are elastic waves propagating on the surface of solids with the amplitude decaying into the solid. The well- established fabrication of compact SAW devices, together with well-defined resonance frequencies, places SAWs as an attractive route to manipulate the magnetization states in spintronics, all of which is made possible by the magnetostriction and magnetoelastic effects. Here, we review the basic characteristics of SAW devices and their interaction out-of-resonance and in-resonance with the magnetization in thin films. We describe our own recent results in this research field and closely related works and provide our perspectives moving forward.

論文

Interaction between surface acoustic waves and spin waves in a ferromagnetic thin film

山本 慧; Xu, M.*; Puebla, J.*; 大谷 義近*; 前川 禎通*

Journal of Magnetism and Magnetic Materials, 545, p.168672_1 - 168672_10, 2022/03

 被引用回数:15 パーセンタイル:65.38(Materials Science, Multidisciplinary)

We present a theoretical description of magnon-phonon interactions in a multi-layer structure containing a ferromagnetic thin film. The formalism is applicable to an arbitrary direction of external magnetic field and various types of acoustic waves including Rayleigh and Love surface modes. A particular attention is paid to the spatial profile of the acoustic wave modes and analytical expressions for the effective coupling coefficients are derived taking into account the degree of mode profile overlap between spin waves and acoustic waves. The results are applied to reproduce a strongly anisotropic and non-reciprocal linewidth of acoustic ferromagnetic resonance reported in a recent experiment.

論文

Long decay length of magnon-polarons in BiFeO$$_{3}$$/La$$_{0.67}$$Sr$$_{0.33}$$MnO$$_{3}$$ heterostructures

Zhang, J.*; Chen, M.*; Chen, J.*; 山本 慧; Wang, H.*; Hamdi, M.*; Sun, Y.*; Wagner, K.*; He, W.*; Zhang, Y.*; et al.

Nature Communications (Internet), 12, p.7258_1 - 7258_8, 2021/12

 被引用回数:19 パーセンタイル:77.91(Multidisciplinary Sciences)

Magnons can transfer information in metals and insulators without Joule heating, and therefore are promising for low-power computation. The on-chip magnonics however suffers from high losses due to limited magnon decay length. In metallic thin films, it is typically on the tens of micrometre length scale. Here, we demonstrate an ultra-long magnon decay length of up to one millimetre in multiferroic/ferromagnetic BiFeO$$_{3}$$(BFO)/La$$_{0.67}$$Sr$$_{0.33}$$MnO$$_{3}$$ (LSMO) heterostructures at room temperature. This decay length is attributed to a magnon-phonon hybridization and is more than two orders of magnitude longer than that of bare metallic LSMO. The long-distance modes have high group velocities of 2.5 km$$^{-1}$$ as detected by time-resolved Brillouin light scattering. Numerical simulations suggest that magnetoelastic coupling via the BFO/LSMO interface hybridizes phonons in BFO with magnons in LSMO. Our results provide a solution to the long-standing issue on magnon decay lengths in metallic magnets and advance the bourgeoning field of hybrid magnonics.

論文

Half-integer Shapiro-steps in superconducting qubit with a $$pi$$-Josephson junction

森 道康; 前川 禎通

Applied Physics Express, 14(10), p.103001_1 - 103001_4, 2021/10

 被引用回数:1 パーセンタイル:4.92(Physics, Applied)

A superconducting quantum interference device (SQUID) comprising 0- and $$pi$$-Josephson junctions (JJs), called $$pi$$-SQUID, is studied by the resistively shunted junction model. The $$pi$$-SQUID shows half-integer Shapiro-steps (SS) under microwave irradiation at the voltage $$V$$ = $$(hbar/2e)Omega (n/2)$$, with angular frequency $$Omega$$ and half-integer $$n$$/2 in addition to integer $$n$$. We show that the $$pi$$-SQUID can be a $$pi$$-qubit with spontaneous loop currents by which the half-integer SS are induced. Making the 0- and $$pi$$-JJs equivalent is a key for the half-integer SS and realizing the $$pi$$-qubit.

論文

Half-integer Shapiro steps in strong ferromagnetic Josephson junctions

Yao, Y.*; Cai, R.*; Yang, S.-H.*; Xing, W.*; Ma, Y.*; 森 道康; Ji, Y.*; 前川 禎通; Xie, X.-C.*; Han, W.*

Physical Review B, 104(10), p.104414_1 - 104414_6, 2021/09

 被引用回数:7 パーセンタイル:43.89(Materials Science, Multidisciplinary)

We report the experimental observation of half-integer Shapiro steps in the strong ferromagnetic Josephson junction (Nb-NiFe-Nb) by investigating the current-phase relation under radio-frequency microwave excitation. The half-integer Shapiro steps are robust in a wide temperature range from T = 4 to 7 K. The half-integer Shapiro steps could be attributed to co-existence of 0- and $$pi$$-states in the strong ferromagnetic NiFe Josephson junctions with the spatial variation of the NiFe thickness. This scenario is also supported by the high-resolution transmission electron microscopy characterization of the Nb/NiFe/Nb junction.

論文

Observation of the angular momentum compensation by Barnett effect and NMR

中堂 博之; 今井 正樹; 松尾 衛; 前川 禎通; 齊藤 英治

Journal of the Physical Society of Japan, 90(8), p.081003_1 - 081003_11, 2021/08

 被引用回数:4 パーセンタイル:39.84(Physics, Multidisciplinary)

We demonstrate observation of the angular momentum compensation temperature $$T_{rm A}$$, at which the net angular momentum is quenched in ferrimagnets. Using the Barnett effect, in which an object is magnetized by mechanical rotation owing to spin-rotation coupling, we measure $$T_{rm A}$$ in the Ho$$_{3-x}$$Dy$$_{x}$$Fe$$_{5}$$O$$_{12}$$ system. We determine $$T_{rm A}$$ to be 240 K in Ho$$_{3}$$Fe$$_{5}$$O$$_{12}$$ (HoIG). We find that $$T_{rm A}$$ increases with Dy content and show that $$T_{rm A}$$ of Ho$$_{1.5}$$Dy$$_{1.5}$$Fe$$_{5}$$O$$_{12}$$ corresponds with room temperature. We also demonstrate that $$^{57}$$Fe-NMR measurements can be applied to explore domain wall dynamics in HoIG. We find that the NMR intensity exhibits a maximum at $$T_{rm A}$$ in the multi-domain state. We provide a simple model for describing this NMR signal enhancement caused by enhancement of domain-wall mobility at $$T_{rm A}$$.

論文

Zeeman coupling and Dzyaloshinskii-Moriya interaction driven by electric current vorticity

藤本 純治*; 小椎八重 航*; 松尾 衛; 前川 禎通

Physical Review B, 103(22), p.L220402_1 - L220402_5, 2021/06

 被引用回数:8 パーセンタイル:43.89(Materials Science, Multidisciplinary)

The Dzyaloshinskii-Moriya interaction, i.e., antisymmetric exchange interaction, combined with a Zeeman magnetic field gives rise to various magnetic states such as chiral, helical, and skyrmionic states. This interaction conventionally originates from spin-orbit coupling and thus needs somewhat heavy elements. In contrast, we here show a Dzyaloshinskii-Moriya interaction which is driven by electric current vorticity. We also find that the vorticity acts on localized spins as a Zeeman field, which may explain a recent experiment on current-driven magnetic skyrmion creation and annihilation without an external magnetic field in a device with a notch structure in FeGe. The theory explains the control of skyrmion creation and annihilation by current direction and opens different possibilities for studies of magnetic textures by using structural settings.

論文

Barnett field, rotational Doppler effect, and Berry phase studied by nuclear quadrupole resonance with rotation

中堂 博之; 松尾 衛*; 前川 禎通*; 齊藤 英治

Physical Review B, 103(17), p.174308_1 - 174308_10, 2021/05

 被引用回数:7 パーセンタイル:43.89(Materials Science, Multidisciplinary)

We report the observation of the Barnett field, rotational Doppler effect, and Berry phase using the rotating nuclear quadrupole resonance (NQR) methods. We have developed coil-spinning techniques that enable us to systematically study the effects of rotation in setups involving rotation of the signal detector, rotation of the sample, and simultaneous rotation of both the signal detector and sample. Applying these setups to NQR measurements, we observe NQR line splittings in which the spectral structures are clearly distinct among the setups. By analyzing these structures, we clarify the origin of the NQR line splittings and discuss the relationship between the rotational Doppler effect, Barnett field effect, and Berry phase in terms of the rotational degrees of freedom, such as the relative rotation and the sample rotation itself, and the observation frame of reference. We also provide clear evidence of the difference between the rotational Doppler effect and the Barnett field, and the equivalence of the Barnett field and the Berry phase.

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