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論文

Measurement of 107-MeV proton-induced double-differential neutron yields for iron for research and development of accelerator-driven systems

岩元 大樹; 中野 敬太; 明午 伸一郎; 佐藤 大樹; 岩元 洋介; 石 禎浩*; 上杉 智教*; 栗山 靖敏*; 八島 浩*; 西尾 勝久; et al.

JAEA-Conf 2022-001, p.129 - 133, 2022/11

https://doi.org/10.11484/jaea-conf-2022-001

加速器駆動システム(ADS)の核特性予測精度の向上と京都大学臨界集合体実験装置(KUCA)におけるADS炉物理実験で用いる中性子源情報の取得を目的として、京都大学の固定磁場強集束(FFAG)加速器を用いた核データ測定実験プログラムを開始した。このプログラムの一環として、鉄に対する陽子入射二重微分中性子収量(TTNY)及び断面積(DDX)を測定した。測定では、真空チェンバ内に設置された鉄標的に107MeVの陽子ビームを照射し、核反応によって標的から発生した粒子の信号を、小型の中性子検出器を用いて検出した。検出信号とFFAGキッカー電磁石の信号の時間差から飛行時間(TOF)を求め、ガンマ線の事象を波形弁別法によって除去して中性子事象をカウントすることで中性子のTOFスペクトルを求めた。得られた中性子のTOFスペクトルから、相対論的運動学により鉄標的に対するTTNY及びDDXを求めた。

論文

Angular momentum transfer in multinucleon transfer channels of $$^{18}$$O + $$^{237}$$Np

田中 翔也*; 廣瀬 健太郎; 西尾 勝久; Kean, K. R.*; 牧井 宏之; Orlandi, R.; 塚田 和明; 有友 嘉浩*

Physical Review C, 105(2), p.L021602_1 - L021602_5, 2022/02

https://doi.org/10.1103/PhysRevC.105.L021602
 被引用回数：0 パーセンタイル：0.03(Physics, Nuclear)

The angular momentum of a primary excited compound nucleus produced in multinucleon transfer reaction is an important quantity to evaluate cross sections to synthesize neutron-rich heavy element nuclei as well as for surrogate reaction studies. The mechanism is, however, not enough understood due to the lack of detailed experimental data. In the present study, we determined the angular momentum of primary excited nuclei, $$^{237,238,239}$$Np, $$^{238,239,240}$$Pu, and $$^{239,240,241}$$Am, produced in the multi-nucleon transfer channels of the $$^{18}$$O + $$^{237}$$Np reaction. With this aim, angular distributions of fission fragments with respect to the axis perpendicular to the reaction plane were measured for each compound nucleus. The distributions show an anisotropy exhibiting an enhanced yield on the reaction plane. They are well reproduced by a saddle point model, from which the average angular momentum is derived in the model framework. The angular momentum increases with the compound-nucleus mass, thus the number of nucleons exchanged, but shows a saturating trend toward heavier compound nuclei. These results are the first ones to point to the dependence of the angular momentum on the transfer channels.

論文

Measurement of 107-MeV proton-induced double-differential thick target neutron yields for Fe, Pb, and Bi using a fixed-field alternating gradient accelerator at Kyoto University

岩元 大樹; 中野 敬太; 明午 伸一郎; 佐藤 大樹; 岩元 洋介; 杉原 健太; 西尾 勝久; 石 禎浩*; 上杉 智教*; 栗山 靖敏*; et al.

Journal of Nuclear Science and Technology, 15 Pages, 2022/00

https://doi.org/10.1080/00223131.2022.2115423
 被引用回数：0

加速器駆動核変換システム(ADS)の研究開発及び京都大学臨界実験装置(KUCA)におけるADS未臨界炉物理の基礎研究を目的として、固定磁場強収束(FFAG)加速器を用いて107MeV陽子による鉄、鉛及びビスマス標的に対する二重微分中性子収量(TTNY)を測定した。TTNYは8個の中性子検出器(各検出器は小型のNE213液体有機シンチレータと光電子増倍管より構成される)からなる中性子検出器システムを用いて飛行時間法により得られたものである。測定で得られたTTNYを、粒子・重イオン輸送コードシステム(PHITS)に組み込まれたモンテカルロ法に基づく核破砕反応モデル(INCL4.6/GEM, Bertini/GEM, JQMD/GEM, JQMD/SMM/GEM)及び評価済み高エネルギー核データライブラリ(JENDL-4.0/HE)による計算結果と比較した。JENDL-4.0/HEを含む比較対象のモデルは、検出器角度5度における高エネルギーピークを再現しないなどの特徴的な不一致が見られた。測定で得られたTTNYとPHITSによって評価した20MeV以下のエネルギー及び角度積分中性子収率を比較した結果、INCL4.6/GEMがKUCAにおけるADS炉物理実験のモンテカルロ輸送シミュレーションに適していることが示された。

論文

The $$^{59}$$Fe(n,$$gamma$$)$$^{60}$$Fe cross section from the surrogate ratio method and its effect on the $$^{60}$$Fe nucleosynthesis

Yan, S. Q.*; Li, X. Y.*; 西尾 勝久; Lugaro, M.*; Li, Z. H.*; 牧井 宏之; Pignatari, M.*; Wang, Y. B.*; Orlandi, R.; 廣瀬 健太郎; et al.

Astrophysical Journal, 919(2), p.84_1 - 84_7, 2021/10

https://doi.org/10.3847/1538-4357/ac12ce
 被引用回数：1 パーセンタイル：22.62(Astronomy & Astrophysics)

The long-lived $$^{60}$$Fe (with a half-life of 2.62 Myr) is a crucial diagnostic of active nucleosynthesis in the Milky Way galaxy and in supernovae near the solar system. The neutron-capture reaction $$^{59}$$Fe(n,$$gamma$$)$$^{60}$$Fe on $$^{59}$$Fe (half-life=44.5 days) is the key reaction for the production of $$^{60}$$Fe in massive stars. This reaction cross section has been previously constrained by the Coulomb dissociation experiment, which offered partial constraint on the E1 $$gamma$$-ray strength function but a negligible constraint on the M1 and E2 components. In this work, for the first time, we use the surrogate ratio method to experimentally determine the $$^{59}$$Fe(n,$$gamma$$)$$^{60}$$Fe cross sections in which all the components are included. We derived a Maxwellian-averaged cross section of 27.5$$pm$$3.5 mb at $$kT$$ = 30 keV and 13.4$$pm$$1.7 mb at $$kT$$ = 90 keV, roughly 10%-20% higher than previous estimates. We analyzed the impact of our new reaction rates in nucleosynthesis models of massive stars and found that uncertainties in the production of $$^{60}$$Fe from the $$^{59}$$Fe(n,$$gamma$$)$$^{60}$$Fe rate are at most 25$$%$$. We conclude that stellar physics uncertainties now play a major role in the accurate evaluation of the stellar production of $$^{60}$$Fe.

論文

Chemical characterization of a volatile dubnium compound, DbOCl$$_3$$

Chiera, N. M.*; 佐藤 哲也; Eichler, R.*; 富塚 知博; 浅井 雅人; 安達 サディア*; Dressler, R.*; 廣瀬 健太郎; 井上 浩樹*; 伊藤 由太; et al.

Angewandte Chemie; International Edition, 60(33), p.17871 - 17874, 2021/08

https://doi.org/10.1002/anie.202102808
 被引用回数：2 パーセンタイル：41.05(Chemistry, Multidisciplinary)

等温ガスクロマトグラフ法を用いて、105番元素ドブニウム(Db)の単一原子を対象として、揮発性オキシ塩化物を合成し、化学的性質を調べた。同一条件下で同族元素ニオブおよびタンタルの揮発性と比較したところ、NbOCl$$_3 > $$ TaOCl$$_3 geq$$ DbOCl$$_3$$の関係が得られた。これはDb分子中の共有結合性が周期表からの予想よりも強くなっているためと考えられる。本成果により、超アクチノイド元素の化学的性質に関する理論計算に対する信頼できる実験データを与えることができた。

論文

Experimental study of the $$Gamma_{p1}/Gamma_{p0}$$ ratios of resonance states in $$^{8}$$Be for deducing the $$^{7}$$Be($$n$$,$$p_{1}$$)$$^{7}$$Li$$^{*}$$ reaction rate relevant to the cosmological lithium problem

岩佐 直仁*; 石川 竣喜*; 久保野 茂*; 榊原 昂浩*; 小湊 和也*; 西尾 勝久; 松田 誠; 廣瀬 健太郎; 牧井 宏之; Orlandi, R.; et al.

Physical Review C, 103(1), p.015801_1 - 015801_5, 2021/01

https://doi.org/10.1103/PhysRevC.103.015801
 被引用回数：0 パーセンタイル：0.02(Physics, Nuclear)

The $$^{9}$$Be($$^{3}$$He,$$alpha$$)$$^{8}$$Be($$p$$)$$^{7}$$Li reaction was studied at $$E_{rm lab}$$($$^{3}$$He)=30 MeV to deduce the branching ratios of $$Gamma_{p1}/Gamma_{p0}$$ of resonant state at 18.91 - 20.1 MeV in $$^{8}$$Be, which are necessary to extract the $$^{7}$$Be($$n$$, $$p_{1}$$)$$^{7}$$Li$$^{*}$$ reaction rate relevant to the $$^{7}$$Be destruction in the big bang nucleosynthesis, from the $$^{7}$$Li($$p$$,$$n_{0}$$)$$^{7}$$Be reaction cross section. The decay protons from $$^{8}$$Be$$^{*}$$ to the ground and first excited states in $$^{7}$$Li were well-separately measured. The $$Gamma_{p1}/Gamma_{p0}$$ ratio of the 19.235-MeV state was deduced to be 3.4$$pm$$1.9%. The 19.86- and 20.1-MeV states were found to decay dominantly into the first excited and ground states of $$^{7}$$Li, respectively.

論文

Measurement of fission-fragment mass distributions in the multinucleon transfer channels of the $$^{18}$$O+$$^{237}$$Np reaction

Vermeulen, M. J.; 西尾 勝久; 廣瀬 健太郎; Kean, K. R.; 牧井 宏之; Orlandi, R.; 塚田 和明; Tsekhanovich, I.*; Andreyev, A. N.; 石崎 翔馬*; et al.

Physical Review C, 102(5), p.054610_1 - 054610_11, 2020/11

https://doi.org/10.1103/PhysRevC.102.054610
 被引用回数：3 パーセンタイル：50.86(Physics, Nuclear)

Fission fragment mass distributions for 23 nuclei ($$^{234-237}$$U, $$^{236-239}$$Np, $$^{238-241}$$Pu, $$^{240-243}$$Am, $$^{242-245}$$Cm, and $$^{244-246}$$Bk) were measured using the multi-nucleon transfer approach in the reaction of $$^{18}$$O+$$^{237}$$Np, and their excitation-energy dependence was obtained up to a maximum of 70 MeV. Among them, the low energy fission of $$^{236}$$Np, $$^{238}$$Pu, and $$^{245}$$Cm is reported for the first time. The experimental data for all the studied nuclei were compared to the Langevin calculations. The calculation which takes into account the effects of multi-chance fission well reproduced the peak-to-valley ratio and mass-asymmetric peak positions of the distributions. The angular momenta given to the fissioning nucleus is also discussed.

論文

Nonresonant $$p$$-wave direct capture and interference effect observed in the $$^{16}$$O$$(n,gamma)^{17}$$O reaction

永井 泰樹*; 木下 充隆*; 井頭 政之*; 延原 由利子*; 牧井 宏之; 三島 賢二*; 嶋 達志*; Mengoni, A.*

Physical Review C, 102(4), p.044616_1 - 044616_8, 2020/10

https://doi.org/10.1103/PhysRevC.102.044616
 被引用回数：0 パーセンタイル：0.02(Physics, Nuclear)

We measured the total capture cross section of the $$^{16}$$O$$(n,gamma)^{17}$$O reaction, as well as partial cross sections leading to the ground ($$J^{pi} = 5/2^{+})$$ and first excited ($$J^{pi} = 1/2^{+})$$ states in $$^{17}$$O. The measurement was carried out at average neutron energies of 157, 349, 398, 427, 468, 498, and 556 keV by using pulsed neutrons produced via the $$^{7}$$Li$$(p,n)^{7}$$Be reaction and a $$gamma$$-ray detection system based on an anti-Compton NaI(Tl) spectrometer. We observed the interference effect between the $$3/2^{-}$$ resonance state at 4554 keV of $$^{17}$$O, corresponding to a neutron energy of 411 keV in the center-of-mass system, and a non-resonant contribution in the capture process. The measured partial cross sections are in good agreement with theoretical calculations obtained taking into account the interference between the $$3/2^{-}$$ resonance and a non-resonant p-wave direct radiative capture contribution. Using the present results, together with our previous measurement, we derived the Maxwellian-averaged capture cross sections (MACS) for thermal energies between kT = 5 and 100 keV, key quantities for ${it s}$ process nucleosynthesis studies in massive stars.

論文

New excited 2$$^+$$ and 3$$^-$$ two-proton states in $$_{84}^{210}$$Po$$_{126}$$ populated by two-proton transfer

Dupont, E.*; Astier, A.*; Petrache, C. M.*; Lv, B. F.*; Deloncle, I.*; Kiener, J.*; Orlandi, R.; 牧井 宏之; 西尾 勝久; 廣瀬 健太郎; et al.

Physical Review C, 101(1), p.014309_1 - 014309_6, 2020/01

https://doi.org/10.1103/PhysRevC.101.014309
 被引用回数：1 パーセンタイル：20.31(Physics, Nuclear)

Five new 2$$^+$$ levels and one new 3$$^-$$ level were established in $$^{210}$$Po. The states were populated via the $$^{208}$$Pb($$^{12}$$C, $$^{10}$$Be) two-proton reaction experiment, performed at the JAEA Tandem in Tokai. A setup combining Ge, LaBr$$_3$$, and Si telescopes was used to detect in-beam $$gamma$$-rays and ejectile residues. Two-proton configurations were assigned to all new states. All assignments are strongly supported by shell-model calculations.

論文

Effects of the nuclear structure of fission fragments on the high-energy prompt fission $$gamma$$-ray spectrum in $$^{235}$$U($$n_{rm th},f$$)

牧井 宏之; 西尾 勝久; 廣瀬 健太郎; Orlandi, R.; L$'e$guillon, R.; 小川 達彦; Soldner, T.*; K$"o$ster, U.*; Pollitt, A.*; Hambsch, F.-J.*; et al.

Physical Review C, 100(4), p.044610_1 - 044610_7, 2019/10

https://doi.org/10.1103/PhysRevC.100.044610
 被引用回数：9 パーセンタイル：78(Physics, Nuclear)

The prompt fission $$gamma$$-ray energy spectrum for cold-neutron induced fission of $$^{235}$$U was measured in the energy range $$E_{rm gamma}$$ = 0.8 - 20,MeV, by gaining a factor of about 10$$^{5}$$ in statistics compared to the measurements performed so far. The spectrum exhibits local bump structures at $$E_{rm gamma}approx$$4,MeV and $$approx$$6,MeV, and also a broad one at $$approx$$15,MeV. In order to understand the origins of these bumps, the $$gamma$$-ray spectra were calculated using a statistical Hauser-Feshbach model, taking into account the de-excitation of all the possible primary fission fragments. It is shown that the bump at $$approx$$4,MeV is created by the transitions between the discrete levels in the fragments around $$^{132}$$Sn, and the bump at $$approx$$6,MeV mostly comes from the complementary light fragments. It is also indicated that a limited number of nuclides, which have high-spin states at low excitation energies, can contribute to the bump structure around $$E_{rm gamma}approx$$15,MeV, induced by the transition feeding into the low-lying high-spin states.

論文

Search for $$alpha$$ decay of $$^{104}$$Te with a novel recoil-decay scintillation detector

Xiao, Y.*; Go, S.*; Grzywacz, R.*; Orlandi, R.; Andreyev, A. N.; 浅井 雅人; Bentley, M. A.*; de Angelis, G.*; Gross, C. J.*; Hausladen, P.*; et al.

Physical Review C, 100(3), p.034315_1 - 034315_8, 2019/09

https://doi.org/10.1103/PhysRevC.100.034315
 被引用回数：13 パーセンタイル：87.08(Physics, Nuclear)

A search for super-allowed $$alpha$$ decay of N=Z nuclei $$^{104}$$Te and $$^{108}$$Xe was carried out using a novel recoil-decay scintillator detector at the tandem accelerator facility at Japan Atomic Energy Agency. Inorganic crystal scintillation material of YAP:Ce (Yttrium Aluminium Perovskite) coupled to position-sensitive photo-multiplier tube (PSPMT) was implemented for the first time in a radioactive decay experiment. Residues from the fusion-evaporation reaction $$^{58}$$Ni+$$^{54}$$Fe$$rightarrow$$ $$^{112}$$Xe$$^*$$ were separated by the JAEA Recoil Mass Separator (RMS) and implanted into the YAP:Ce crystal. $$alpha$$ decays of neutron-deficient tellurium isotopes were identified and proton-emission of $$^{109}$$I was observed. No conclusive evidence was found for the decay chain $$^{108}$$Xe$$rightarrow$$$$^{104}$$Te$$rightarrow$$ $$^{100}$$Sn within 3 days experiment. The cross section limit of 130 pb was obtained for production of two events of $$^{108}$$Xe, about an order of magnitude below the expectation based on earlier cross section measurements and HIVAP calculations.

論文

Validation of the multinucleon transfer method for the determination of the fission barrier height

Kean, K. R.; 西尾 勝久; 廣瀬 健太郎; Vermeulen, M. J.; 牧井 宏之; Orlandi, R.; 塚田 和明; Andreyev, A. N.; Tsekhanovich, I.*; 千葉 敏*

Physical Review C, 100(1), p.014611_1 - 014611_6, 2019/07

https://doi.org/10.1103/PhysRevC.100.014611
 被引用回数：2 パーセンタイル：29.91(Physics, Nuclear)

The validity of the multinucleon transfer (MNT) approach for deduction of fission barrier heights was investigated in an experiment carried out at the JAEA tandem accelerator facility. By using the $$^{18}$$O+$$^{237}$$Np reaction, fission barrier heights were inferred from fission probabilities of the nuclei $$^{239}$$Np and $$^{239,240}$$Pu produced in the $$2n$$ and $$pn/p2n$$ transfer channels, respectively. The deduced values of fission barriers agree well with the literature data, thus demonstrating the potential of the MNT reactions for obtaining fission-barrier data for nuclei not accessible for fission studies via neutron- or light charged particle-induced reactions.

論文

Observation of the competing fission modes in $$^{178}$$Pt

Tsekhanovich, I.*; Andreyev, A. N.; 西尾 勝久; Denis-Petit, D.*; 廣瀬 健太郎; 牧井 宏之; Matheson, Z.*; 森本 幸司*; 森田 浩介*; Nazarewicz, W.*; et al.

Physics Letters B, 790, p.583 - 588, 2019/03

https://doi.org/10.1016/j.physletb.2019.02.006
 被引用回数：23 パーセンタイル：94.96(Astronomy & Astrophysics)

Fragment mass distributions from fission of the excited compound nucleus $$^{178}$$Pt have been deduced from the measured fragment velocities. The $$^{178}$$Pt nucleus was created at the JAEA tandem facility in a complete fusion reaction $$^{36}$$Ar+$$^{142}$$Nd, at beam energies of 155, 170 and 180 MeV. The data are indicative of a mixture of the mass-asymmetric and mass-symmetric fission modes associated with higher and lower total kinetic energies of the fragments, respectively. The measured fragment yields are dominated by asymmetric mass splits, with the symmetric mode contributing at the level of $$approx$$ 1/3. This constitutes the first observation of a multimodal fission in the sub-lead region. Most probable experimental fragment-mass split of the asymmetric mode, $$A_{rm L}$$/$$A_{rm H}$$ $$approx$$ 79/99, is well reproduced by nuclear density functional theory using the UNEDF1-HFB and D1S potentials. The symmetric mode is associated by theory with very elongated fission fragments, which is consistent with the observed total kinetic energy/fragment mass correlation.

論文

First ionization potentials of Fm, Md, No, and Lr; Verification of filling-up of 5f electrons and confirmation of the actinide series

佐藤 哲也; 浅井 雅人; Borschevsky, A.*; Beerwerth, R.*; 金谷 佑亮*; 牧井 宏之; 水飼 秋菜*; 永目 諭一郎; 長 明彦; 豊嶋 厚史; et al.

Journal of the American Chemical Society, 140(44), p.14609 - 14613, 2018/11

https://doi.org/10.1021/jacs.8b09068
 被引用回数：25 パーセンタイル：75(Chemistry, Multidisciplinary)

第一イオン化エネルギー(IP$$_1$$)は、原子の価電子軌道に関する情報を与える。99番元素アインスタイニウムよりも重いアクチノイドのIP$$_1$$は、一度に一つの原子しか扱うことのできない実験の難しさから、これまでに実験的に測定された例はなかった。我々は表面電離法を応用した新しい測定手法により、103番元素ローレンシウム(Lr)のIP$$_1$$測定に成功し、Lrが弱く束縛された最外殻電子をもつことを強く示唆する結果を得た。一方、Lrとは対象的に、102番元素ノーベリウムは充填された5f軌道および7s軌道をもつために、アクチノイド中最高のIP$$_1$$をもつと考えられている。表面電離法によるIP$$_1$$決定法をNoおよび100番元素フェルミウム, 101番元素メンデレビウムに適用することにより求められた各IP$$_1$$から、5f軌道への電子の充填に伴ってIP$$_1$$が単調に増加し、Noで最も大きくなることを確かめることができた。このことから、f軌道に電子が充填され、アクチノイド系列がLrで終わることを実験的に確かめた。

論文

A New detector system for the measurement of high-energy prompt $$gamma$$-rays for low-energy neutron induced fission

牧井 宏之; 西尾 勝久; 廣瀬 健太郎; Orlandi, R.; L$'e$guillon, R.*; 小川 達彦; Soldner, T.*; Hambsch, F.-J.*; A$"i$che, M.*; Astier, A.*; et al.

Nuclear Instruments and Methods in Physics Research A, 906, p.88 - 96, 2018/10

https://doi.org/10.1016/j.nima.2018.07.055
 被引用回数：3 パーセンタイル：37.65(Instruments & Instrumentation)

中性子誘起核分裂における即発高エネルギー$$gamma$$線を観測するための新しい測定システムの開発を行った。測定システムは核分裂片を観測するための多芯線比例計数管と$$gamma$$線測定用のLaBr$$_{3}$$(Ce)シンチレータから構成される。開発したシステムを仏国ラウエ・ランジュバン研究所にある高中性子束炉のPF1Bコースに設置して、$$^{235}$$U中性子誘起核分裂における即発$$gamma$$線を行った。測定ではエネルギー最大20MeVまでの$$gamma$$線スペクトルの観測に成功し、$$^{235}$$U中性子誘起核分裂において非常に高いエネルギーの$$gamma$$線が放出されていることを確認した。

論文

Production of iodine radionuclides using $$^{7}$$Li ion beams

西中 一朗*; 横山 明彦*; 鷲山 幸信*; 牧井 宏之; 橋本 和幸*

Journal of Radioanalytical and Nuclear Chemistry, 314(3), p.1947 - 1965, 2017/12

https://doi.org/10.1007/s10967-017-5525-2
 被引用回数：2 パーセンタイル：24.09(Chemistry, Analytical)

$$^{7}$$Li + $$^{nat}$$Sn反応により生成されるI, Te, Sn同位体の生成断面積を入射エネルギー24-59MeVの領域で測定した。得られた生成断面積のエネルギー依存性を統計模型計算の結果と比較することにより、各同位体の生成機構と崩壊様式の観点から完全・不完全融合反応の生成断面積への寄与を議論した。また、医学的に有用な$$^{123,124}$$Iの生成という観点から、様々なSn同位体と$$^{7}$$Liビームの組み合わせにより、$$^{123,124,125,126}$$I同位体がどの程度生成されるかを計算し、$$^{7}$$Li以外をビームとして用いた場合との比較を行った。

論文

Role of multichance fission in the description of fission-fragment mass distributions at high energies

廣瀬 健太郎; 西尾 勝久; 田中 翔也*; L$'e$guillon, R.*; 牧井 宏之; 西中 一朗*; Orlandi, R.; 塚田 和明; Smallcombe, J.*; Vermeulen, M. J.; et al.

Physical Review Letters, 119(22), p.222501_1 - 222501_6, 2017/12

https://doi.org/10.1103/PhysRevLett.119.222501
 被引用回数：37 パーセンタイル：90.07(Physics, Multidisciplinary)

JAEAタンデム加速器施設で行った$$^{18}$$O+$$^{238}$$U反応における多核子移行チャンネルを用いた実験により、$$^{237-240}$$U, $$^{239-242}$$Np、および$$^{241-244}$$Puの核分裂質量分布を励起エネルギー10$$sim$$60MeVにおいて測定した。これらのうち、$$^{240}$$U, $$^{240,241,242}$$Npのデータは本実験により初めて観測された。原子核の殻効果の減衰によって対称分裂すると予想されていた高励起エネルギーにおいても、質量分布が非対称を示すことがわかった。搖動散逸定理に基づく動力学モデル計算との比較から、この振る舞いはマルチチャンス核分裂によるものであることを明らかにした。

論文

Study of fission using multi-nucleon transfer reactions

西尾 勝久; 廣瀬 健太郎; Vermeulen, M. J.; 牧井 宏之; Orlandi, R.; 塚田 和明; 浅井 雅人; 豊嶋 厚史; 佐藤 哲也; 永目 諭一郎; et al.

EPJ Web of Conferences, 163, p.00041_1 - 00041_6, 2017/11

https://doi.org/10.1051/epjconf/201716300041
 被引用回数：1 パーセンタイル：64.38

We are promoting a study of fission using multi-nucleon transfer (MNT) reactions, where excited states in neutron-rich actinide nuclei, which cannot be accessed by particle capture and/or fusion reactions, are populated. Also, the excited states in the fissioning nucleus are widely populated by the MNT reactions, from which effects of excitation energy on fission properties can be investigated. Experiments were carried out at the JAEA tandem facility in Tokai, Japan. We studied reactions using the $$^{18}$$O beam and several actinide target nuclei such as $$^{232}$$Th, $$^{238}$$U, $$^{237}$$Np, $$^{248}$$Cm. Ejectile nucleus was identified by a silicon $$Delta$$E-E telescope to identify transfer channel and hence the compound nucleus. Fission fragments were detected by multi-wire proportional counters, and fission fragment mass distributions (FFMDs) were measured for each isotope. Measured FFMDs are reproduced by a calculation based on the fluctuation-dissipation model, and importance of multi-chance fission concept is investigated. Fission fragment angular distribution relative to the recoil direction suggested the increase of the spin of the fissioning nucleus with the number of transferred nucleons.

論文

Study of fission using multi-nucleon transfer reactions

西尾 勝久; 廣瀬 健太郎; L$'e$guillon, R.*; 牧井 宏之; Orlandi, R.; 塚田 和明; Smallcombe, J.*; 千葉 敏*; 有友 嘉浩*; 田中 翔也*; et al.

Proceedings of 6th International Conference on Fission and Properties of Neutron-rich Nuclei (ICFN-6), p.590 - 597, 2017/11

https://doi.org/10.1142/9789813229426_0101

We are promoting a fission study using multi-nucleon transfer reactions, where excited states in neutron-rich actinide nuclei, which cannot be accessed by particle capture and/or fusion reactions, are populated. This allows us to study fission in the new region of chart of nuclei. Also, the excited states in the fissioning nucleus are widely populated in the reactions, thus the effects of excitation energy on fission can be investigated. Experiments were carried out at the JAEA tandem facility in Tokai, Japan. We studied reactions using the $$^{18}$$O beam ($$sim$$9MeV/u) and several actinide target nuclei such as $$^{232}$$Th, $$^{238}$$U, $$^{237}$$Np, $$^{248}$$Cm. Ejectile nuclei and thus the transfer channels were identified by a newly developed silicon $$Delta$$E-E detectors. The produced nuclei in one experiment reached more than fifteen. Fission fragment mass distributions (FFMDs) were measured for each isotopes. Measured FFMDs are reproduced by a calculation based on the fluctuation-dissipation model (Langevin-type calculation), where effects of multi-chance fission were included. We also started to measure the prompt neutrons accompanied by fission.

論文

The $$^{95}$$Zr($$n, gamma$$)$$^{96}$$Zr cross section from the surrogate ratio method and its effect on $$s$$-process nucleosynthesis

Yan, S. Q.*; Li, Z. H.*; Wang, Y. B.*; 西尾 勝久; Lugaro, M.*; Karakas, A. I.*; 牧井 宏之; Mohr, P.*; Su, J.*; Li, Y. J.*; et al.

Astrophysical Journal, 848(2), p.98_1 - 98_8, 2017/10

https://doi.org/10.3847/1538-4357/aa8c74
 被引用回数：4 パーセンタイル：20.68(Astronomy & Astrophysics)

The $$^{95}$$Zr($$n, gamma$$)$$^{96}$$Zr reaction cross section is crucial in the modelling of $$s$$-process nucleosynthesis in asymptotic giant branch stars because it controls the operation of the branching point at the unstable $$^{95}$$Zr and the subsequent production of $$^{96}$$Zr. We have carried out the measurement of the $$^{90}$$Zr($$^{18}$$O,$$^{16}$$O) and $$^{94}$$Zr($$^{18}$$O,$$^{16}$$O) reactions and obtained the $$gamma$$-decay probability ratio of $$^{92}$$Zr$$^{*}$$ and $$^{96}$$Zr$$^{*}$$ to determine the $$^{95}$$Zr($$n, gamma$$)$$^{96}$$Zr reaction cross sections with the surrogate ratio method. We tested our deduced maxwellian-averaged cross section in stellar models with masses between 2 and 6 $$M_{odot}$$ and metallicities 0.014 and 0.03. The largest changes - up 80 % variations in $$^{96}$$Zr - are seen in the models of 3-4 $$M_{odot}$$, where the $$^{22}$$Ne neutron source is mildly activated. The new rate can still provide a match to data from meteoritic stardust silicon carbide grains, provided the maximum mass of the parent stars is below 4 $$M_{odot}$$, for a metallicity of 0.03.

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