Microbially formed Mn(IV) oxide as a novel adsorbent for removal of Radium

Tanaka, Kazuya; Yamaji, Keiko*; Masuya, Hayato*; Tomita, Jumpei; Ozawa, Mayumi*; Yamasaki, Shinya*; Tokunaga, Kohei; Fukuyama, Kenjin*; Ohara, Yoshiyuki*; Maamoun, I.*; et al.

Chemosphere, 355, p.141837_1 - 141837_11, 2024/05

https://doi.org/10.1016/j.chemosphere.2024.141837

In this study, biogenic Mn(IV) oxide was applied to remove Ra from mine water collected from a U mill tailings pond in the Ningyo-toge center. Just 7.6 mg of biogenic Mn(IV) oxide removed more than 98% of the Ra from 3 L of mine water, corresponding to a distribution coefficient of 10 mL/g for Ra at pH 7. The obtained value was convincingly high for practical application of biogenic Mn(IV) oxide in water treatment.

An Examination of rapid analysis of Ra in natural water samples by ICP-MS

Tomita, Jumpei; Ozawa, Mayumi; Ohara, Yoshiyuki; Miyamoto, Yutaka

KEK Proceedings 2021-2, p.130 - 134, 2021/12

https://lib-extopc.kek.jp/preprints/PDF/2021/2125/2125002.pdf

no abstracts in English

Development of spin-contrast-variation neutron powder diffractometry for extracting the structure factor of hydrogen atoms

Miura, Daisuke*; Kumada, Takayuki; Sekine, Yurina; Motokawa, Ryuhei; Nakagawa, Hiroshi; Oba, Yojiro; Ohara, Takashi; Takata, Shinichi; Hiroi, Kosuke; Morikawa, Toshiaki*; et al.

Journal of Applied Crystallography, 54(2), p.454 - 460, 2021/04

AA2020-0724.pdf:2.05MB

https://doi.org/10.1107/S1600576721000303

We developed a spin-contrast-variation neutron powder diffractometry technique that extracts the structure factor of hydrogen atoms, namely, the contribution of hydrogen atoms to a crystal structure factor. Crystals of L-glutamic acid were dispersed in a dpolystyrene matrix containing 4-methacryloyloxy-2,2,6,6,-tetramethyl-1-piperidinyloxy (TEMPO methacrylate) to polarize their proton spins dynamically. The intensities of the diffraction peaks of the sample changed according to the proton polarization, and the structure factor of the hydrogen atoms was extracted from the proton-polarization dependent intensities. This technique is expected to enable analyses of the structures of hydrogen-containing materials that are difficult to determine with conventional powder diffractometry.

Generation of He clusters via neutron-He absorption reaction toward visualization of full velocity field in quantum turbulence

Matsushita, Taku*; Sonnenschein, V.*; Guo, W.*; Hayashida, Hirotoshi*; Hiroi, Kosuke; Hirota, Katsuya*; Iguchi, Tetsuo*; Ito, Daisuke*; Kitaguchi, Masaaki*; Kiyanagi, Yoshiaki*; et al.

Journal of Low Temperature Physics, 196(1-2), p.275 - 282, 2019/07

https://doi.org/10.1007/s10909-018-02112-3

Changes in groundwater flow after remediation with capping for the Upstream of Mill Tailings Pond at Ningyo-toge Environmental Engineering Center

Nishida, Nobuho; Ohara, Yoshiyuki; Kawamoto, Tsutomu

Heisei-28-Nendo Zenkoku Kozan, Seirenjo Gemba Tantosha Kaigi Shigen/Shinzozai Koenshu, p.69 - 74, 2016/06

Japan Atomic Energy Agency Ningyo-toge Environmental Engineering Center, has been conducting environmental remediation of the Ningyo-toge mine and Togo mine, after decades of mine-related activities including uranium exploration, mining and test milling were terminated, with doing safety measure, under Mining Safety law. As the one, culvert installation and multi-layered capping were performed at Upstream of Yotsugi Mill Tailings Pond to inspect about stability of multi-layered capping with checking rainwater infiltration restraint and radon dissipation inhibiting effect, from FY 2011 to FY 2012. And it was presumed possibility of amount of underground water is increased, as result of fluctuation numerical analysis for Upstream of Yotsugi Mill Tailings Pond before and after the multi-layered capping, and the water level of bowling holes around the Pond and spring water which flows from lower place of the Pond. But a culvert possesses enough drainage function and groundwater does not rise to the multi-layered capping part. Therefore, it is considered that there isn't problem to the stability of the current state of the multi-layered capping, but we will continue the monitoring of the water level of the bowling hole around the Pond, and the spring water which flows from lower place of the Pond.

Application of support vector machine to rapid classification of uranium waste drums using low-resolution -ray spectra

Hata, Haruhi; Yokoyama, Kaoru; Ishimori, Yuu; Ohara, Yoshiyuki; Tanaka, Yoshio; Sugitsue, Noritake

Applied Radiation and Isotopes, 104, p.143 - 146, 2015/10

https://doi.org/10.1016/j.apradiso.2015.06.030

We investigated the feasibility of using support vector machine (SVM), a computer learning method, to classify uranium waste drums as natural uranium or reprocessed uranium based on their origins. The method was trained using 12 training datasets were used and tested on 955 datasets of -ray spectra obtained with NaI(Tl) scintillation detectors. The results showed that only 4 out of 955 test datasets were different from the original labels-one of them was mislabeled and the other three were misclassified by SVM. These findings suggest that SVM is an effective method to classify a large quantity of data within a short period of time. Consequently, SVM is a feasible method for supporting the scaling factor method and as a supplemental tool to check original labels.

Verification of uranium 238 quantity calculated using waste assay systems

Yokoyama, Kaoru; Hata, Haruhi; Ohara, Yoshiyuki; Naganuma, Masaki; Sugitsue, Noritake

Radioisotopes, 63(12), p.559 - 566, 2014/12

https://doi.org/10.3769/radioisotopes.63.559

The amount of U in uranium-contaminated waste drums generated in the decommissioning of nuclear facilities is evaluated using ray measurement. We used the -ray measurement system made from CANBERRA: Qualitative and Quantitative (Q) Low Level Waste Assay Systems and measured the waste drum. This equipment assumes uniform distribution of the uranium radiation source. But, homogeneity is not checked with a real waste drum. Authors developed the new analysis technique which calculates the amount of uranium by correcting the influence of uneven distribution of the uranium radiation source. As a result of evaluating using the new analysis technique, the error which the radiation source uneven distribution in a drum gives to U quantitative value of this equipment has been evaluated.

Further study of measurement of performance of the NDA using Q2 system for uranium waste drum

Naganuma, Masaki; Ohara, Yoshiyuki; Miyamoto, Yasunori*; Murashita, Tatsuya*; Makita, Akinori*; Nohiro, Tetsuya*

JAEA-Technology 2014-012, 11 Pages, 2014/06

JAEA-Technology-2014-012.pdf:1.06MB

In Japan Atomic Energy Agency Ningyo-toge environmental engineering center, exploration for uranium and technical development of uranium refining, conversion and enrichment which are the front end of a nuclear fuel cycle have been performed since 1955. In 2002, we introduced Q2 low-level-waste drum measuring system which is a bulk measuring method of the passive ray. In 2007, OS2 analyzing operation system which was used in Q2, was replaced with windows system. This replacement improved the performance of the analysis of Q2. But quantified values of uranium obtained from win system did not correspond exactly to OS2 system. We considered whether the drum which was measured by OS2 system, was measured again by windows system. But it was difficult to measure these drum by win system. So in this study, we studied a calculation method for adjusting quantified values of uranium obtained by each system.

Measurement performance of the NDA using Q2 system for uranium waste drum

Ohara, Yoshiyuki; Naganuma, Masaki; Nohiro, Tetsuya*; Yoshida, Kimikazu*; Makita, Akinori*; Sakate, Mitsuo*; Irisawa, Takumi*; Murashita, Tatsuya*

JAEA-Technology 2012-048, 39 Pages, 2013/03

JAEA-Technology-2012-048.pdf:5.1MB

In Japan Atomic Energy Agency Ningyo-Toge Environmental Engineering Center, exploration for uranium and technical development of uranium refining, conversion and enrichment which are the front end of a nuclear fuel cycle have been performed since 1955. By these research and development, about 15000 radioactive waste (200 liter drum) has occurred by now. The analytical and measurement technique of the amount of uranium which are included in radioactive waste drum were very an inexperienced in those days. Therefore, measurement strict till 2002 was not able to be started. Such a situation as this, we introduced "Q2 low-level-waste drum measuring system" which is a bulk measuring method of the passive ray using a NaI scintillation detector in 2002. As a result, the total amount of uranium in a waste drum was estimated as about 20 tons.

The H-Invitational Database (H-InvDB); A Comprehensive annotation resource for human genes and transcripts

Yamasaki, Chisato*; Murakami, Katsuhiko*; Fujii, Yasuyuki*; Sato, Yoshiharu*; Harada, Erimi*; Takeda, Junichi*; Taniya, Takayuki*; Sakate, Ryuichi*; Kikugawa, Shingo*; Shimada, Makoto*; et al.

Nucleic Acids Research, 36(Database), p.D793 - D799, 2008/01

https://doi.org/10.1093/nar/gkm999

Here we report the new features and improvements in our latest release of the H-Invitational Database, a comprehensive annotation resource for human genes and transcripts. H-InvDB, originally developed as an integrated database of the human transcriptome based on extensive annotation of large sets of fulllength cDNA (FLcDNA) clones, now provides annotation for 120 558 human mRNAs extracted from the International Nucleotide Sequence Databases (INSD), in addition to 54 978 human FLcDNAs, in the latest release H-InvDB. We mapped those human transcripts onto the human genome sequences (NCBI build 36.1) and determined 34 699 human gene clusters, which could define 34 057 protein-coding and 642 non-protein-coding loci; 858 transcribed loci overlapped with predicted pseudogenes.