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Prestwood, D.*; 吉川 貴史; 齊藤 英治; 他15名*
Physical Review B, 113(13), p.134410_1 - 134410_12, 2026/04
被引用回数：1 パーセンタイル：86.01(Materials Science, Multidisciplinary)We study a thin-film yttrium iron garnet sample that exhibits magnetic stripe domains due to a small perpendicular magnetic anisotropy. Using wide-field magneto-optic Kerr effect measurements we reveal the domain pattern evolution as a function of applied field and discuss the role of cubic anisotropy in the domain formation. Rich magnon spectra are observed in the stripe domain states, with a range of excitation conditions providing distinct spectra. The measurements are interpreted using micromagnetic simulations to provide the spatial profiles of each resonance mode. We further simulate domain patterns and resonance spectra accounting for the cubic anisotropy, with good correlation to experiment. This study highlights how noncollinear magnetic domain structures can host complex resonant behavior in a low-damping magnetic material, with potential use in future magnonic applications.
Wang, C.*; Yang, Z.*; Ren, Q.*; Mo. X.*; 吉川 貴史; 大門 俊介*; Diao, D.*; 齊藤 英治
Carbon, 246, p.120909_1 - 120909_7, 2026/01
被引用回数：0 パーセンタイル：0.00(Chemistry, Physical)Disordered carbon offers untapped potential for spin caloritronics. We report a phonon-enhanced spin-dependent Seebeck effect (SDSE) in a magnetic carbon film (MCF) with graphene nano-crystallites (10 nm), interfaced with Pt. In a longitudinal setup, the transverse thermoelectric voltage (
) peaks at (
) at 220 K, driven by a thermally induced spin current via the inverse spin Hall effect. Raman spectroscopy reveals a coincident G-band redshift peak, suggesting a phonon-spin resonance unique to MCF's hybrid structure. X-ray absorption spectra confirm stable sp
states, potentially mediating this effect. A multiple-sample study in addition reveals that smaller crystallites enhance SDSE. Unlike pristine graphene or insulators, MCF's weak ferromagnetism and phonon dynamics yield an unconventional spin-thermal regime. This finding redefines carbon's role in spin caloritronics, with tunable nano-crystallite size as a design parameter.
巻内 崇彦*; 吉川 貴史; 今井 正樹; 中堂 博之; 齊藤 英治; 他3名*
Physical Review Research (Internet), 7(3), p.033083_1 - 033083_7, 2025/09
Hybridized nuclear and electron spin excitation in a MnCO crystal, a weakly anisotropic antiferromagnet, has been investigated. In this material, the hyperfine interaction is strong enough to form a nuclear spin wave. We measure the microwave absorption induced by magnetic resonance in a bulk MnCO and observe the dispersion representing strong frequency repulsion between electron and nuclear modes due to their hybridization, the signature of nuclear spin wave. Additionally, we observe that the nuclear spin resonance enters a nonlinear regime above a certain excitation power, attributed to the excitation of finite-wavenumber nuclear spin waves.
Metzger, T. W. J.*; Fischer, P.*; 吉川 貴史; 齊藤 英治*; Kimel, A. V.*; Bossini, D.*
Physical Review Letters, 135(7), p.076702_1 - 076702_9, 2025/08
被引用回数：3 パーセンタイル：74.19(Physics, Multidisciplinary)Femtosecond laser excitation of nanometer thin heterostructures comprising a heavy metal and a magnetically ordered material is known to result in the emission of terahertz radiation. However, the nature of the emitted radiation from heavy metal/antiferromagnet heterostructures has sparked debates and controversies in the literature. Here, we unambiguously separate spin and charge contributions from Pt/NiO heterostructures by introducing an unprecedented methodology combining high external magnetic fields with a symmetry analysis of the emitted terahertz polarization. We observe two distinct mechanisms of terahertz emission, which we identify as optical difference frequency generation and ultrafast laser-induced quenching of the magnetization. We emphasize the absence of spin transport effects and signatures of coherent magnons. Overall, our Letter provides a general experimental methodology to separate spin and charge contributions to the laser-induced terahertz emission from heterostructures comprising a magnetically ordered material, thus holding great potential for advancing terahertz spintronics and establishing terahertz orbitronics.
Fe
|Pt at room temperature平田 裕也*; 吉川 貴史; 有沢 洋希*; 齊藤 英治*
Applied Physics Letters, 126(25), p.252408_1 - 252408_5, 2025/06
被引用回数：6 パーセンタイル：81.32(Physics, Applied)The nonlinear Seebeck effect, nonlinear conversion of a temperature gradient into an electric current, was observed at room temperature. Based on a second-harmonic lock-in method combined with an a.c. temperature gradient, 
, we measured a nonlinear Seebeck voltage in NiFe|Pt bilayers at 300 K, the amplitude of which increases in proportion to 
. We also observed that the nonlinear Seebeck voltage increases as the sample length along the direction decreases, showing a characteristic scaling law distinct from the conventional linear Seebeck effect. We developed a phenomenological model for the nonlinear Seebeck effect incorporating the spin-current induced modulation of the Seebeck coefficient, which well reproduces the experimental results.
GeTe
homojunctions小幡 玲二*; 齊藤 英治; 吉川 貴史; 他13名*
Advanced Materials, 37(8), p.2411459_1 - 2411459_11, 2025/02
被引用回数：13 パーセンタイル：92.74(Chemistry, Multidisciplinary)Twistronics, a novel engineering approach involving the alignment of van der Waals (vdW) integrated two-dimensional materials at specific angles, has recently attracted significant attention. Novel nontrivial phenomena have been demonstrated in twisted vdW junctions (the so-called magic angle), such as unconventional superconductivity, topological phases, and magnetism. However, there have been only few reports on integrated vdW layers with large twist angles 
, such as twisted interfacial Josephson junctions using high-temperature superconductors. Herein, vdW homojunctions of the thin-magnetic flakes, Fe
GeTe
(FGT), with large ranging from 0 to 90 deg, without inserting any tunnel barriers are assembled. Nevertheless, these vdW homojunctions exhibit tunnel-magnetoresistance (TMR) like behavior (pseudo-TMR (PTMR) effect) with the ratios highly sensitive to the values, revealing that the vdW gap at the junction interface between the twisted FGT layers behaves like a tunnel barrier and the serves a control parameter for PTMR by drastically varying magnitudes of the lattice-mismatch and the subsequent appearance of antiferromagnetic (AFM) spin alignment. First-principles calculations considering vacuum gaps indicate strong dependence of TMR on the driven by the sixfold screw rotational symmetry of bulk FGT. The present homojunctions hold promise as a platform for novel AFM spin-dependent phenomena and spintronic applications.
O medium岡田 敬志*; 斉藤 淳一; 浪江 将成; 西村 文宏*
Materials Today Communications (Internet), 42, p.111244_1 - 111244_6, 2025/01
被引用回数：1 パーセンタイル：7.27(Materials Science, Multidisciplinary)Ca(OH)存在下、500
Cの溶融KOH-BO媒体中で希酸可溶性白金化合物を合成した。酸可溶性白金化合物は、熱処理中に生成したCaCOの表面に形成された。白金化合物は白金-O結合、二ホウ酸基、AlO
からなり、これらの成分のネットワーク構造はKイオンとCaイオンを取り込むことができる。化合物は1M塩酸(aq)で抽出され、Pt抽出効率は83%であった。白金化合物の形態は、反応容器の表面条件によって変化した。液体ナトリウムで表面を改質したアルミナプレート上で化合物を合成した場合、繊維状の白金化合物が生成し、その結晶化度は未処理のアルミナプレート上で得られたものより高かった。
涌井 隆; 斎藤 滋; 二川 正敏
実験力学, 24(4), p.212 - 218, 2024/12
J-PARCの核破砕中性子源水銀ターゲット容器の寿命を決定する主要な要因の一つは照射損傷である。使用済み容器の材料劣化を把握するため、使用済み容器の構造材料に対する押込み試験と数値実験による逆解析を用いた評価を行う予定である。照射量の異なる2種類のイオン照射材料に対して、この評価手法を適用した。照射量の増加に伴い、引張強度が増加し、全伸びが減少することが確認された。これらの傾向は、ばらつきを考慮した微小試験片の引張試験によって報告されている材料劣化挙動と同等である。さらに、容器は繰り返し熱負荷を受け、定格最大ビーム出力では容器の温度が140Cを超えると推定されるため、温度上昇に伴う全伸びと照射材料の疲労強度の低下について検討した。
涌井 隆; 斎藤 滋; 二川 正敏
Materials, 17(23), p.5925_1 - 5925_14, 2024/12
被引用回数：0 パーセンタイル：0.00(Chemistry, Physical)照射された材料の延性特性は、その構造的完全性に関連する重要な指標の1つである。これらの特性は、通常、照射環境下で照射された材料に引張試験を実施することによって決定される。押込み試験は、延性特性を簡単かつ迅速に評価するために使用され、Swift型の材料構成方程式の定数は、カルマンフィルターを使用した逆解析によって同定された。胴体された定数を用いて数値引張実験を実施し、公称応力およびひずみ曲線を取得した。さらに、全伸びを評価するための2つの方法を提案した。2つの方法で評価された最小全伸びはともに10%となった。イオン照射された材料の評価結果は、照射された材料の引張試験結果と同様の結果が得られた。
小杉 美央子*; 吉川 貴史; 齊藤 英治; 他10名*
ACS Applied Materials & Interfaces, 16(46), p.64190 - 64196, 2024/11
被引用回数：4 パーセンタイル：34.77(Nanoscience & Nanotechnology)Atom-vacancy-defects present in various materials yield numerous interesting physical phenomena, even obstructing high performance in some cases. On the other hand, their valuable applications to novel devices, such as nitrogen vacancy centers in diamond for quantum bits, have gathered significant attention. In particular, these tendencies become more substantial in two-dimensional (2D) (atomically) thin van der Waals layers. However, correlations with various kinds of atom defects are still under exploration. Herein, we find the stochastic behaviors of large hysteresis loops with strong photoresponse in the static electrical properties in few-atom layer semiconductors, molybdenum disulfide (MoS). The temperature dependence and transmission electron microscopy reveal that they arise from pairs of two neighboring in-plane S-vacancy defects, which predominantly present only around the interface at the MoS flake/substrate, with activation energies similar to 0.35 eV. The low-frequency (
) (LF) noise measurements clarify a high f shift in the two 1/ 2-dependent regimes, implying stochastic behaviors of electric charges through the S-vacancy pairs with high-speed charge(spin) transitions across low kinetic energy barriers between narrow discrete states. The shallow energy sates are formed from the highly uniform S-vacancy pairs interacting with Mo atoms, which act like quantum dots. The observed stochastic operation holds promise for various application, particularly for probabilistic neuromorphic computation in artificial intelligence.
GeTe nanomeshes小幡 玲二*; 吉川 貴史*; 齊藤 英治; 他7名*
Nanotechnology, 35(47), p.475601_1 - 475601_9, 2024/11
被引用回数：3 パーセンタイル：33.64(Nanoscience & Nanotechnology)The growth of two-dimensional van der Waals magnetic materials presents attractive opportunities for exploring new physical phenomena and valuable applications. Among these materials, FeGeTe (FGT) exhibits a variety of remarkable properties and has garnered significant attention. Herein, we have for the first time created a nanomesh structure-a honeycomb-like array of hexagonal nanopores-with the zigzag pore-edge atomic structure on thin FGT flakes with and without oxidation of the pore edges. It is revealed that the magnitude of ferromagnetism (FM) significantly increases in both samples compared with bulk flakes without nanomeshes. Critical temperature annealing results in the formation of zigzag pore edges and interpore zigzag-edge nanoribbons. We unveil that the non-oxide (O) termination of the Fe dangling bonds on these zigzag edges enhances FM behavior, while O-termination suppresses this FM by introducing antiferromagnetic behavior through edge O-Fe coupling. FGT nanomeshes hold promise for the creation of strong FM and their effective application in magnetic and spintronic systems.
二宮 和彦*; 久保 謙哉*; 稲垣 誠*; 吉田 剛*; 竹下 聡史*; 反保 元伸*; 下村 浩一郎*; 河村 成肇*; Strasser, P.*; 三宅 康博*; et al.
Journal of Radioanalytical and Nuclear Chemistry, 333(7), p.3445 - 3450, 2024/07
被引用回数：1 パーセンタイル：20.46(Chemistry, Analytical)A novel nondestructive light element analysis method for bulk materials using muon beams was demonstrated. This method is based on the lifetime measurement of muons in a material and performed by measuring muon-decay electrons and identifying elements using the atomic number based on muon lifetimes. Muon irradiation on pure iron and two steel samples with known carbon contents was conducted to prepare a calibration curve for the quantitative analysis. We also performed a muon lifetime measurement for a Japanese sword and successfully determined its carbon content as 0.51 wt% using the calibration curve, without sample destruction.
根本 隆弘; 藤原 佑輔; 荒川 了紀; 長山 侑矢; 長住 達; 長谷川 俊成; 横山 佳祐; 渡部 雅; 大西 貴士; 川本 大樹; et al.
JAEA-Technology 2024-003, 17 Pages, 2024/06
JAEA-Technology-2024-003.pdf:1.91MB
RS-14サイクルに発生した1次ヘリウム循環機フィルタの差圧上昇の原因を調査するため、フィルタ付着物を調査した。調査の結果、フィルタエレメント表面にシリコンオイルに起因する付着物を確認した。この結果から、フィルタ差圧上昇の原因は、1次ヘリウム純化設備ガス循環機のチャコールフィルタの性能劣化により、1次系内にシリコンオイルが混入したためであることが明らかとなった。また、この再発防止対策として、従来の1次ヘリウム純化設備ガス循環機の運転時間による管理に加え、チャコールフィルタの交換頻度を3年毎とする定期交換計画を新たに策定した。
substrate小幡 玲二*; 齊藤 英治; 吉川 貴史; 他7名*
Advanced Materials, 36(19), p.2311339_1 - 2311339_8, 2024/05
被引用回数：3 パーセンタイル：21.99(Chemistry, Multidisciplinary)SrTiO (STO) substrate, a perovskite oxide material known for its high dielectric constant (epsilon), facilitates the observation of various (high-temperature) quantum phenomena. A quantum Hall topological insulating (QHTI) state, comprising two copies of QH states with antiparallel two ferromagnetic edge-spin overlap protected by the U(1) axial rotation symmetry of spin polarization, has recently been achieved in low magnetic field (B) even as high as approximate to 100 K in a monolayer graphene/thin hexagonal boron nitride (hBN) spacer placed on an STO substrate, thanks to the high epsilon of STO. Despite the use of the heavy STO substrate, however, proximity-induced quantum spin Hall (QSH) states in 2D TI phases, featuring a topologically protected helical edge spin phase within time-reversal-symmetry, is not confirmed. Here, with the use of a monolayer hBN spacer, it is revealed the coexistence of QSH (at B = 0T) and QHTI (at B not equal 0) states in the same single graphene sample placed on an STO, with a crossover regime between the two at low B. It is also classified that the different symmetries of the two nontrivial helical edge spin phases in the two states lead to different interaction with electron-puddle quantum dots, caused by a local surface pocket of the STO, in the crossover regime, resulting in a spin dephasing only for the QHTI state. The results obtained using STO substrates open the doors to investigations of novel QH spin states with different symmetries and their correlations with quantum phenomena. This exploration holds value for potential applications in spintronic devices.
Fe
O
川本 陽*; 吉川 貴史; 齊藤 英治; 他9名*
Applied Physics Letters, 124(13), p.132406_1 - 132406_7, 2024/03
被引用回数：8 パーセンタイル：68.36(Physics, Applied)Magnon spin currents in the ferrimagnetic garnet TbFe
O with 4 electrons were examined through the spin-Seebeck effect and neutron scattering measurements. The compound shows a magnetic compensation, where the spin-Seebeck signal reverses above and below 
= 249.5(4) K. Unpolarized neutron scattering unveils two major magnon branches with finite energy gaps, which are well explained in the framework of spin-wave theory. Their temperature dependencies and the direction of the precession motion of magnetic moments, i.e., magnon polarization, defined using polarized neutrons, explain the reversal at and decay of the spin-Seebeck signals at low temperatures. We illustrate an example that momentum- and energy-resolved microscopic information is a prerequisite to understand the magnon spin current.
池田 一貴*; 佐次田 頌*; 大友 季哉*; 大下 英敏*; 本田 孝志*; 羽合 孝文*; 齋藤 開*; 伊藤 晋一*; 横尾 哲也*; 榊 浩司*; et al.
International Journal of Hydrogen Energy, 51(Part A), p.79 - 87, 2024/01
被引用回数：10 パーセンタイル：37.60(Chemistry, Physical)Low-vanadium-concentration alloys have low durability, and their hydrogen absorption and desorption amounts decrease by 20% after 100 cycles. In this study, we conducted reverse Monte Carlo modeling on X-ray diffraction patterns and neutron pair distribution functions of the hydrogen-absorbed and desorbed samples of a V
Ti
Cr
alloy to analyze the variations in the local structure. The local structure surrounding the hydrogen atom in the hydrogen-absorbed phase exhibited minimal changes. In contrast, hydrogen occupied both tetrahedral and octahedral sites of the hydrogen-desorbed phase almost equally during the early cycles; however, the amount of hydrogen occupying the tetrahedral sites increased with the number of cycles.
二宮 和彦*; 久保 謙哉*; 稲垣 誠*; 吉田 剛*; Chiu, I.-H.; 工藤 拓人*; 浅利 駿介*; 千徳 佐和子*; 竹下 聡史*; 下村 浩一郎*; et al.
Scientific Reports (Internet), 14, p.1797_1 - 1797_8, 2024/01
被引用回数：1 パーセンタイル：18.83(Multidisciplinary Sciences)鋼の特性を決める上で重要な鋼中のC量は、鋼の生産技術に大きく左右される。このため、ミュオンを使って鋼のC含有量を非破壊で測定する新しい方法を提案する。この方法は、生産中の鋼の品質管理だけでなく、貴重な鋼製考古学的遺物の分析にも使えるかもしれない。負の電荷を持つミュオンは原子系を形成し、最終的には核に吸収されるか電子に崩壊する。ミュオンの寿命は、Fe原子かC原子に捕らわれるかによってかなり違い、ミュオン停止位置での元素含有量をミュオン寿命測定で特定できる。C/Feのミュオン捕獲確率とCの元素含有量の関係は直線的で、ミュオン寿命測定で鋼のC含有量を定量的に決められる。さらに、ミュオンの入射エネルギーを調整して、0.5mm厚の3種類の鋼板からなる積層サンプルの各層でミュオンを停止させ、0.20-1.03wt%の範囲でC含有量を深さ選択的に、サンプルを壊さずに決定することに成功した。
Ga K-edge XANES study of Ga-exchanged zeolites at high temperatures under different atmospheres including vacuum, CO, and pressurized HHuang, M.*; 金城 哲弥*; 安村 駿作*; 鳥屋尾 隆*; 松村 大樹; 齋藤 寛之*; 清水 研一*; 並木 則和*; 前野 禅*
Catalysis Science & Technology, 13(23), p.6832 - 6838, 2023/12
被引用回数：3 パーセンタイル：11.91(Chemistry, Physical)Ga-exchanged zeolites are promising catalysts for dehydrogenative alkane transformations. Reduced Ga species, such as Ga hydrides and Ga
cations, are possible active sites for alkane dehydrogenation based on in situ spectroscopic studies. However, most of the reported studies were conducted at lower temperatures compared with those encountered in actual operating conditions. In this study, the in situ Ga K-edge XANES analysis of Ga-exchanged MFI zeolite was performed under actual operating temperatures and different atmospheres (H, He, CO, vacuum, and CH). The absorption edge appeared at similarly lower energy values than that of GaO in all atmospheres, whereas the main absorption peak intensity differed depending on the presence or absence of a hydride source in the gas phase. Higher intensities were observed under H and CH atmospheres than under CO and vacuum atmospheres.
layers on SrTiO substrates小杉 美央子*; 齊藤 英治; 吉川 貴史*; 他11名*
APL Materials (Internet), 11(8), p.081106_1 - 081106_6, 2023/08
被引用回数：3 パーセンタイル：22.29(Nanoscience & Nanotechnology)Strontium titanate [SrTiO (STO)], a perovskite oxide with an extremely high gate-tunable dielectric constant (
) due to quantum paraelectric phases, is attracting considerable attention for yielding various physical phenomena when two-dimensional (2D) layers are integrated. Superconductivity is such a typical phenomenon. However, the influence of the STO substrates on enhancing transition temperatures (
) for (atomically) thin 2D flakes attached to them has been rarely investigated. Here, we report gate-tunable and gradual four-terminal resistance drops with critical onset (
) and scanning tunneling spectroscopy (STS) spectra in devices comprising thin TaS flakes attached on monolayer hexagonal boron nitride (hBN) spacer/STO substrates. Observation of STS spectra confirms the presence of local superconducting gaps. (similar to 1.5 meV) with transition (
three-times higher than previous reports of under absent pressure and strong position dependence of 
. Depending on 
on back gate voltages (
) and magnetic fields, there is a strong correlation between and the onset of superconductivity, implying an enhancement of approximately five times compared with the previous highest-onset values without pressure as the applied increases. The high onset and. are discussed based on screening of the long-range Coulomb interaction (CI) due to the high- of SrTiO, while the short-ranged CI remains strong in the 2D limit, causing the superconductivity. Using a monolayer hBN/SrTiO substrate with opens doors to enhancement in thin superconducting layers integrated on it and wide application due to the solid-state high- substrates.
O近藤 洋介*; Achouri, N. L.*; Al Falou, H.*; Atar, L.*; Aumann, T.*; 馬場 秀忠*; Boretzky, K.*; Caesar, C.*; Calvet, D.*; Chae, H.*; et al.
Nature, 620(7976), p.965 - 970, 2023/08
被引用回数：53 パーセンタイル：95.82(Multidisciplinary Sciences)非常に中性子が過剰な原子核Oは、陽子、中性子ともに魔法数であることから古くからその性質に興味が持たれていたが、酸素の最後の束縛核
Oよりも中性子が4個も多いため、これまで観測されてこなかった。この論文では、理化学研究所RIBFにて
Fからの1陽子ノックアウト反応によってOを生成し、そこから放出される中性子を測定することによって初めてその観測に成功した。核構造の観点からは、Oでは二重閉殻が保たれているか興味が持たれていたが、実験で得られた分光学的因子が殻模型計算で予言されて程度の大きいことから、閉殻構造をもたない可能性が高いことがわかった。
