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Se from combined conversion-electron and 
-ray spectroscopySmallcombe, J.; Garnsworthy, A. B.*; Korten, W.*; Singh, P.*; Muir, D.*; Pr
chniak, L.*; Ali, F. A.*; Andreoiu, C.*; Ansari, S.*; Ball, G. C.*; et al.
Physical Review C, 110(2), p.024318_1 - 024318_16, 2024/08
被引用回数：1 パーセンタイル：0.00(Physics, Nuclear)In the selenium isotopes various shape phenomena are present, in particular the emergence of a dominant oblate deformation in the most neutron-deficient isotopes has been observed. The scenario of shape coexisting oblate and prolate bands has been proposed across the isotopic chain, with the crossing point of such bands being located near Se, where no coexistence has yet been identified. To determine the presence or absence of any low-lying 
state in Se, confirm the level structure, and interpret the nuclear deformation with theoretical models. A combined internal conversion electron and -ray spectroscopy study was undertaken with the SPICE and TIGRESS spectrometers at the TRIUMF-ISAC-II facility. Nuclear models were provided by the Generalised Triaxial Rotor Model (GTRM) and the collective Generalised Bohr Hamiltonian (GBH). Despite a comprehensive search, no evidence was found for the existence of a state below 2 MeV in Se. Significant discrepancies to the previously established positive parity level scheme were found. GBH calculations using UNEDF1 mass parameters were found to reproduce the revised low-lying level structure well. Se does not have a well defined axial shape. The 2
state at 1601 keV resembles a quasi- excitation rather than a member of a shape coexisting band; the presence of such a band is all but ruled out.
Martel, I.*; Acosta, L.*; Aguado, J. L.*; Smallcombe, J.; 他68名*
Nuclear Instruments and Methods in Physics Research B, 541, p.176 - 179, 2023/08
被引用回数：3 パーセンタイル：46.61(Instruments & Instrumentation)The ISOLDE Scientific Infrastructure at CERN offers a unique range of post-accelerated radioactive beams. The scientific program can be improved with the Isolde Superconducting Recoil Separator (ISRS), an innovative spectrometer able to deliver unprecedented (A, Z) resolution. In this paper we present an overview of the physics and ongoing technical developments.
Eu; Quasiparticle configurations of excited states and structure of 
= 4
bandheads in GdYates, D.*; Kr
cken, R.*; Dillmann, I.*; Garrett, P. E.*; Smallcombe, J.; 他44名*
Physical Review C, 107(6), p.064309_1 - 064309_20, 2023/06
被引用回数：0 パーセンタイル：0.00(Physics, Nuclear)Detailed spectroscopy of neutron-rich, heavy, deformed nuclei is of broad interest for nuclear astrophysics and nuclear structure. Nuclei in the 
-process path and following freeze-out region impact the resulting -process abundance distribution, and the structure of nuclei midshell in both proton and neutron number helps to understand the evolution of subshell gaps and large deformation in these nuclei.
Sun, L. J.*; Fry, C.*; Davids, B.*; Esker, N.*; Wrede, C.*; Smallcombe, J.; 他27名*
Physics Letters B, 839, p.137801_1 - 137801_8, 2023/04
被引用回数：2 パーセンタイル：45.98(Astronomy & Astrophysics)Motivated primarily by the large uncertainties in the thermonuclear rate of the 30PS reaction that limit our understanding of classical novae, we carried out lifetime measurements of 
S excited states using the Doppler Shift Lifetimes (DSL2) facility at the TRIUMF Isotope Separator and Accelerator (ISAC-II) facility.
0 transition strength for 
Se using the SPICE spectrometerSmallcombe, J.; Garnsworthy, A. B.*; Korten, W.*; Singh, P.*; Ali, F. A.*; Andreoiu, C.*; Ansari, S.*; Ball, G. C.*; Barton, C. J.*; Bhattacharjee, S. S.*; et al.
Physical Review C, 106(1), p.014312_1 - 014312_9, 2022/07
被引用回数：5 パーセンタイル：61.57(Physics, Nuclear)The selenium isotopes lie at the heart of a tumultuous region of the nuclear chart where shape coexistence effects grapple with neutron-proton pairing correlations, triaxiality, and the impending proton dripline. In this work a study of Se by internal conversion electron and -ray spectroscopy was undertaken with the SPICE and TIGRESS arrays. New measurements of the branching ratio and lifetime of the 
state were performed yielding a determination of 
milliunits. Two state mixing calculations were performed that highlighted the importance of interpretation of such 
strength values in the context of shape-coexistence.
decay of 
Te with a novel recoil-decay scintillation detectorXiao, Y.*; Go, S.*; Grzywacz, R.*; Orlandi, R.; Andreyev, A. N.; 浅井 雅人; Bentley, M. A.*; de Angelis, G.*; Gross, C. J.*; Hausladen, P.*; et al.
Physical Review C, 100(3), p.034315_1 - 034315_8, 2019/09
被引用回数：19 パーセンタイル：83.66(Physics, Nuclear)A search for super-allowed decay of N=Z nuclei Te and 
Xe was carried out using a novel recoil-decay scintillator detector at the tandem accelerator facility at Japan Atomic Energy Agency. Inorganic crystal scintillation material of YAP:Ce (Yttrium Aluminium Perovskite) coupled to position-sensitive photo-multiplier tube (PSPMT) was implemented for the first time in a radioactive decay experiment. Residues from the fusion-evaporation reaction 
Ni+
Fe
Xe
were separated by the JAEA Recoil Mass Separator (RMS) and implanted into the YAP:Ce crystal. decays of neutron-deficient tellurium isotopes were identified and proton-emission of 
I was observed. No conclusive evidence was found for the decay chain XeTe 
Sn within 3 days experiment. The cross section limit of 130 pb was obtained for production of two events of Xe, about an order of magnitude below the expectation based on earlier cross section measurements and HIVAP calculations.
廣瀬 健太郎; 西尾 勝久; 田中 翔也*; L
guillon, R.*; 牧井 宏之; 西中 一朗*; Orlandi, R.; 塚田 和明; Smallcombe, J.*; Vermeulen, M. J.; et al.
Physical Review Letters, 119(22), p.222501_1 - 222501_6, 2017/12
被引用回数：59 パーセンタイル：91.48(Physics, Multidisciplinary)JAEAタンデム加速器施設で行った
O+
U反応における多核子移行チャンネルを用いた実験により、
U, 
Np、および
Puの核分裂質量分布を励起エネルギー10
60MeVにおいて測定した。これらのうち、
U, 
Npのデータは本実験により初めて観測された。原子核の殻効果の減衰によって対称分裂すると予想されていた高励起エネルギーにおいても、質量分布が非対称を示すことがわかった。搖動散逸定理に基づく動力学モデル計算との比較から、この振る舞いはマルチチャンス核分裂によるものであることを明らかにした。
西尾 勝久; 廣瀬 健太郎; Lguillon, R.*; 牧井 宏之; Orlandi, R.; 塚田 和明; Smallcombe, J.*; 千葉 敏*; 有友 嘉浩*; 田中 翔也*; et al.
Proceedings of 6th International Conference on Fission and Properties of Neutron-rich Nuclei (ICFN-6), p.590 - 597, 2017/11
We are promoting a fission study using multi-nucleon transfer reactions, where excited states in neutron-rich actinide nuclei, which cannot be accessed by particle capture and/or fusion reactions, are populated. This allows us to study fission in the new region of chart of nuclei. Also, the excited states in the fissioning nucleus are widely populated in the reactions, thus the effects of excitation energy on fission can be investigated. Experiments were carried out at the JAEA tandem facility in Tokai, Japan. We studied reactions using the O beam (9MeV/u) and several actinide target nuclei such as 
Th, U, 
Np, 
Cm. Ejectile nuclei and thus the transfer channels were identified by a newly developed silicon 
E-E detectors. The produced nuclei in one experiment reached more than fifteen. Fission fragment mass distributions (FFMDs) were measured for each isotopes. Measured FFMDs are reproduced by a calculation based on the fluctuation-dissipation model (Langevin-type calculation), where effects of multi-chance fission were included. We also started to measure the prompt neutrons accompanied by fission.
西尾 勝久; 廣瀬 健太郎; Lguillon, R.*; 牧井 宏之; Orlandi, R.; 塚田 和明; Smallcombe, J.*; 千葉 敏*; 有友 嘉浩*; 田中 翔也*; et al.
EPJ Web of Conferences, 146, p.04009_1 - 04009_6, 2017/09
被引用回数：3 パーセンタイル：83.66(Nuclear Science & Technology)The objective of this work is to extend fission data for actinide nuclei not investigated so far in order to understand the fission mechanism, especially for neutron-rich nuclei. Multi-nucleon transfer reactions were used to populate the compound nuclei which cannot be accessed by particle capture or fusion reactions. The experiment was carried out at the tandem facility of Japan Atomic Energy Agency. In the multi-nucleon transfer reactions using O beam, a wide variety of nuclei around a target nucleus was produced. By identifying transfer channels, fission data of nuclei more than fifteen compound nuclei were generated in one experiment. Another feature of transfer reaction is that the excitation energies of a compound nucleus can be populated continuously from the ground state up to several tens MeV, allowing us to study the excitation energy dependence of fission properties. From the excitation function of fission probabilities, fission-barrier heights of neutron-rich actinide nuclei were obtained. Experiments were carried out in the reactions of O + U, Th, Cm, Np. The obtained fission fragment mass distributions were reproduced by a model calculation based on a fluctuation dissipation model.
O + Th reactionLguillon, R.; 西尾 勝久; 廣瀬 健太郎; 牧井 宏之; 西中 一朗*; Orlandi, R.; 塚田 和明; Smallcombe, J.*; 千葉 敏*; 有友 嘉浩*; et al.
Physics Letters B, 761, p.125 - 130, 2016/10
被引用回数：45 パーセンタイル：92.51(Astronomy & Astrophysics)It is shown that the multinucleon transfer reactions is a powerful tool to study fission of exotic neutron-rich actinide nuclei, which cannot be accessed by particle-capture or heavy-ion fusion reactions. In this work, multinucleon transfer channels of the O + Th reaction are used to study fission of fourteen nuclei 
Th, 
Pa, and 
U. Identification of fissioning nuclei and of their excitation energy is performed on an event-by-event basis, through the measurement of outgoing ejectile particle in coincidence with fission fragments. Fission fragment mass distributions are measured for each transfer channel, in selected bins of excitation energy. In particular, the mass distributions of 
Th and 
Pa are measured for the first time. Predominantly asymmetric fission is observed at low excitation energies for all studied cases, with a gradual increase of the symmetric mode towards higher excitation energy. The experimental distributions are found to be in general agreement with predictions of the fluctuation-dissipation model.
廣瀬 健太郎; 西尾 勝久; 田中 翔也*; Leguillon, R.*; 牧井 宏之; 西中 一朗*; Orlandi, R.; 塚田 和明; Smallcombe, J.*; Vermeulen, M. J.*; et al.
no journal, ,
The multi-nucleon transfer reaction is very useful way to populate a multitude of nuclides in a wide excitation energy range. We have developed a measurement system at the JAEA tandem accelerator facility to obtain fission observables such as fission-fragment mass distributions (FFMD), prompt fission neutron multiplicities and so on. By identifying the ejectile, the initial compound nucleus is also identified. At high excitation energies, fission of nuclides produced via neutron emission from the initial compound nucleus also contribute to FFMD. In the present study, effects of the multi-chance fission on FFMDs were successfully separated by a combination of a systematic data set obtained from experiments using O beams and actinide targets and a dynamical fission calculation based on the fluctuation-dissipation model.
洲嵜 ふみ; 西尾 勝久; Andreyev, A. N.*; 廣瀬 健太郎; Orlandi, R.; 牧井 宏之; Smallcombe, J.; 伊藤 由太
no journal, ,
天体における元素合成や超重元素の合成の分野において、中性子の多い原子核を生成する反応として多核子移行反応が注目されている。これら中性子過剰核の生成断面積は、多核子移行反応で複合核を生成する断面積と、複合核が核分裂することなく脱励起して生き残る確率の積で表される。この生き残り確率は、複合核の励起エネルギー分布とスピン分布に依存するが、核分裂が競合する領域での詳細なデータはほとんどない。本研究では、蒸発残留核断面積を測定することでこれらを明らかにすることを目標とする。実験は、JAEA反跳生成核分離装置(JAEA-RMS)を用いて行った。JAEA-RMSを回転させることで、断面積の角度依存性を調べることができる。実験手法を確立するため、まず
Si+
Bi反応を調べた。JAEA-RMSの焦点において蒸発残留核の崩壊を測定し、核種を同定した。その上で、核種ごとに断面積の角度依存性を決定したので報告する。
洲嵜 ふみ; 西尾 勝久; Andreyev, A. N.*; 廣瀬 健太郎; Orlandi, R.; 牧井 宏之; Smallcombe, J.; 伊藤 由太
no journal, ,
多核子移行反応は天体での元素合成や超重元素合成の分野において、中性子の多い原子核を蒸発残留核として生成する反応として注目されているが、目的核を生成する最適な反応と実験条件を決めるためには、詳細な実験データの取得と理論の構築が必要である。多核子移行反応の蒸発残留核は、反応の直後にできる複合核がいくつかの中性子を放出して生成されるものであるが、複合核の生成断面積や中性子の蒸発確率など反応についての詳細はわかっていない。JAEAでは反跳生成核分離装置(RMS)を用いた蒸発残留核の測定により反応機構の解明を進めている。まずビスマス標的を用いた実験を行った。蒸発残留核はRMSを用いてビームから分離され、焦点検出器であるシリコンストリップ検出器にインプラントされる。インプラントされた核のアルファ崩壊を測定することで、核種をオンライン同定した。RMSを標的まわりに0度から40度まで回転することで、放出角度に対する生成断面積のデータを得た。本講演では、Si Bi反応を用いて実験について、新たに実施した実験の取得データを含めた最新結果を報告する。
U熱中性子核分裂における即発線スペクトルの測定牧井 宏之; 西尾 勝久; 西中 一朗; 廣瀬 健太郎; Orlandi, R.; Smallcombe, J.; Lguillon, R.; 関本 俊*; 高宮 幸一*; 大槻 勤*
no journal, ,
福島第一原子力発電所では廃止措置に向け、溶解しデブリとなった核燃料の取り出しが計画されている。その際、体系が未臨界であることを保証しながら作業を進める必要があるが、そのためには核分裂事象の頻度を観測する必要がある。しかしながら、使用済核燃料から放出されるバックグラウンド線等により、核分裂事象に伴い発生する即発中性子を観測することは容易ではない。一方、
Cfの自発核分裂事象においては、核分裂生成物の
崩壊等で生じる線(最大数MeV)を超える高エネルギー線が発生することが知られている。我々はこの高エネルギー線に感度を有する未臨界監視線検出器の開発を提案している。しかしながら、Uの熱核分裂事象においては最大7MeVまでの線しか測定されていない。そこで我々は未臨界監視線検出器の開発に資するため、Uの熱核分裂事象において発生する、最大20MeVまでの高エネルギー線の収率を確認することを目的とした測定を開始した。本発表ではバックグラウンドの発生量等を確認した試験測定の結果を報告する。
線の測定西尾 勝久; 牧井 宏之; 廣瀬 健太郎; 西中 一朗; Orlandi, R.; Smallcombe, J.; 大槻 勤*; 関本 俊*; 高宮 幸一*
no journal, ,
福島第一原子力発電所の廃止措置において燃料デブリを取り出す際、臨界監視を行って安全を確保する必要がある。これは、体系内での核分裂事象の頻度を検出することで決定するが、環境からの強いバックグランド線下で事象を検出する必要がある。ここでは、核分裂に伴って放出される高エネルギーの即発線(6MeV以上)を測定する方法を提案する。本研究は、このための基礎データとなるU(n
,f)の線スペクトルを高エネルギー領域まで測定することを目的とする。発表では、開発した線検出器のテスト実験について報告する。
洲嵜 ふみ; 西尾 勝久; 牧井 宏之; 廣瀬 健太郎; Orlandi, R.; Smallcombe, J.
no journal, ,
Multinucleon transfer (MNT) reaction has attracted attention in the fields of nucleosynthesis and the production of superheavy elements because they can produce nuclei with a large neutron number. To produce desired nuclei efficiently and investigate their nuclear properties, it is necessary to determine the optimal beam and target combination and reaction energy, as well as detection angle. The objective of this study is to measure ER cross sections by changing various experimental conditions in order to establish a reliable theoretical model. We have started a program to study MNT reaction using the JAEA Recoil Mass Separator (JAEA-RMS). In contrast to kinematic separators dedicated for fusion reaction, the RMS is advantageous as it can rotate around the target chamber, essential for the study of MNT reactions. As a first attempt, we performed the experiment in the reaction of Si + Bi. The production rate as a function of recoil angle, recoil energy (thus excitation energy), and incident beam-energy dependence were studied. The alpha-decay of the implanted ERs in the focal plane Si detector was observed online. The result is the first to realize the decay measurement in correlated with ERs, produce in the MNT reaction at a finite angle.
Se nuclear shapes with SPICE and TIGRESSSmallcombe, J.; Garnsworthy, A. B.*; Korten, W.*; Singh, P.*; Ali, F. A.*; Andreoiu, C.*; Ansari, S.*; Ball, G. C.*; Barton, C. J.*; Bhattacharjee, S. S.*; et al.
no journal, ,
The phenomenon of shape coexistence is prevalent in the Z34 region, with isotopes of neutron-deficient even Ge, Se and Kr each exhibiting the characteristic low-lying coexisting 0+ bands which display quadrupole deformation different to that of the ground states. In the selenium isotopes, 
Se seem to show a prolate ground structure with shape coexisting oblate excitation, while in 
Se the oblate structure appears to have become the ground state. The exact nature of the low-lying structure Se and any shape coexistence remains uncertain. Combining the Spectrometer for Internal Conversion Electrons (SPICE) with the TIGRESS HPGe Array, a full electron and gamma-ray experimental study of Se, Se was undertaken at the TRIUMF ISAC-II facility to unveil the low-lying structure of these nuclei. Details of the device and experiment will be presented, alongside the experimental results and possible structural interpretations for both isotopes.
西尾 勝久; 岩本 修; 牧井 宏之; 廣瀬 健太郎; Orlandi, R.; 洲嵜 ふみ; 塚田 和明; 浅井 雅人; Smallcombe, J.
no journal, ,
長寿命マイナーアクチノイド(MA)原子核を核変換する加速器駆動炉など次世代の原子炉システムを設計するためには高エネルギーまでの中性子入射断面積が必要である。本発表では、実験データがほとんどない非弾性散乱断面積に加え、核分裂断面積、捕獲断面積、(n,2n)断面積を同時に測定する技術開発の計画を示す。
洲嵜 ふみ; 西尾 勝久; 牧井 宏之; 廣瀬 健太郎; Orlandi, R.; Smallcombe, J.; 浅井 雅人
no journal, ,
重イオン反応における多核子移行反応は中性子数の多い原子核をつくる反応として注目されているが、目的とする原子核を生成する最適な反応と実験条件を決めるには、詳細な実験データの取得と理論の構築が必要である。原子力機構では多核子移行反応で生成される蒸発残留核の詳細な測定をすすめており、最初の結果を示す。
SeSmallcombe, J.
no journal, ,
In the Z=34 region of the atomic chart a pattern of shape coexistence has been observed, with oblate and prolate bands apparently coexisting and switching order as neutron number changes. With recent spectroscopic developments the question of where such an inversion occurs has been drawn into question. Following a detailed electron and gamma ray spectroscopic study of Se previous theoretical descriptions of the nucleus have been invalidated and a new picture of the region has emerged.
