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Journal Articles

Research on vitrification technology to immobilize radioactive sludge generated from Fukushima Daiichi Power Plant; Enhanced glass medium

Amamoto, Ippei; Kobayashi, Hidekazu; Kitamura, Naoto*; Takebe, Hiromichi*; Mitamura, Naoki*; Tsuzuki, Tatsuya*; Fukayama, Daigen*; Nagano, Yuichi*; Jantzen, T.*; Hack, K.*

Journal of Nuclear Science and Technology, 53(10), p.1467 - 1475, 2016/10

 Times Cited Count:1 Percentile:14.27(Nuclear Science & Technology)

The iron phosphate glass (IPG) medium is known to be a high-efficiency glass medium, therefore we try to evaluate its applicability to immobilize sludge bearing radioactive nuclides arising from treatment of contaminated water at the stricken Fukushima Daiichi Nuclear Power Plant. For this study, many physical and chemical properties of target materials are necessary to evaluate the behaviours of IPG medium and its waste forms. Inevitably, it will entail the need for many and varied types of experiments to be carried out under high temperature. It is therefore rational to apply appropriate theoretical analysis first so as to reduce the number of experimental run. For this reason, some necessary thermodynamic values for theoretical analysis were estimated by CALPHAD approach followed by making up the calculated phase diagrams. By comparison with experimental results, they were found to be reliable for evaluating the behaviours of IPG medium and its waste forms.

Journal Articles

Applicability of iron phosphate glass medium for loading NaCl originated from seawater used for cooling the stricken power reactors

Kobayashi, Hidekazu; Amamoto, Ippei; Yokozawa, Takuma; Yamashita, Teruo; Nagai, Takayuki; Kitamura, Naoto*; Takebe, Hiromichi*; Mitamura, Naoki*; Tsuzuki, Tatsuya*

Proceedings of 15th International Conference on Environmental Remediation and Radioactive Waste Management (ICEM 2013) (CD-ROM), 6 Pages, 2013/09

no abstracts in English

Journal Articles

Behaviour of IPG waste forms bearing BaSO$$_{4}$$ as the dominant sludge constituent generated from the treatment of water used for cooling the stricken power reactors

Amamoto, Ippei; Kobayashi, Hidekazu; Yokozawa, Takuma; Yamashita, Teruo; Nagai, Takayuki; Kitamura, Naoto*; Takebe, Hiromichi*; Mitamura, Naoki*; Tsuzuki, Tatsuya*

Proceedings of 15th International Conference on Environmental Remediation and Radioactive Waste Management (ICEM 2013) (CD-ROM), 8 Pages, 2013/09

The great amount of water used for cooling the stricken power reactors at Fukushima Dai-ichi has resulted in accumulation of "remaining water". As the remaining water is subsequently contaminated by FPs, etc., it is necessary to decontaminate it in order to reduce the volume of liquid radioactive waste and to reuse it again for cooling the reactors. Various techniques are being applied to remove FP, etc. and to make stable waste forms. One of the methods using the iron phosphate glass as a medium is being developed to stabilize the strontium-bearing sludge whose main component is BaSO$$_{4}$$. From the results hitherto, the iron phosphate glass is regarded as a potential medium for the target sludge.

JAEA Reports

Survey of the geological characteristics on the Japanese Islands for disposal of RI and research institute waste

Hagiwara, Shigeru*; Sakamoto, Yoshiaki; Takebe, Shinichi; Ogawa, Hiromichi; Nakayama, Shinichi

JAERI-Review 2002-038, 107 Pages, 2002/12

JAERI-Review-2002-038.pdf:6.72MB

For the disposal of radioactive waste arising from radioactive utilization facilities and nuclear facilities, it is necessary to establish the disposal system in proportion to half-lives of radionuclides and radioactivity concentration in the waste. It is important to grasp the features of the earth scientific phenomena and geological structure of our country for the disposal system of radioactive waste. Then, for the porpose of the survey of the geological characteristics around the Japanese Islands whole neiborhood, the earth scientific phenomena at present, geological structure and geotectonic history were summarized on the basis of the existing literatures.

Journal Articles

Sorption characteristics of actinium and protactinium onto soils

Sakamoto, Yoshiaki; Ishii, Tomoaki*; Inagawa, Satoshi*; Gunji, Yasuyoshi*; Takebe, Shinichi; Ogawa, Hiromichi; Sasaki, Tomozo*

Journal of Nuclear Science and Technology, 39(Suppl.3), p.481 - 484, 2002/11

Sorption behavior of 227Ac and 233Pa onto several kinds of soils has been studied with a sequential extraction technique, for safety assessment of shallow land disposal of uranium bearing waste. After a batch sorption experiment, the sorbed form of 227Ac and 233Pa onto the soils was fractionated into ion exchange form (extraction by KCl+CaCl2), association with Fe+Mn oxides (extraction by NH2OH-HCl and oxalic acid), association with organic materials (extraction by H2O2) and fixation into soil (residual). From the results of the sequential extraction, major part of 227Ac sorbed onto the soils was found in the fraction of the ion exchange form and the fixation into the soils. On the other hand, major part of 233Pa was found in the fraction of the association with Fe+Mn oxides and the fixation into the soils. These results suggest that the sorption behavior of 227Ac and 233Pa is related to the irreversible sorption reaction onto the soils.

Journal Articles

Measurement of distribution coefficients of U series radionuclides on soils under shallow land environment, 2; pH dependence of distribution coefficients

Sakamoto, Yoshiaki; Ishii, Tomoaki*; Inagawa, Satoshi*; Gunji, Yasuyoshi*; Takebe, Shinichi; Ogawa, Hiromichi; Sasaki, Tomozo*

Genshiryoku Bakkuendo Kenkyu, 8(1), p.65 - 76, 2001/09

In order to study adsorption behavior of U series radionuclides(Pb, Ra, Th, Ac, Pa and U) in aerated zone environment (loam-rein water system) and aquifer environment(sand-groundwater system) for safety assessment of U bearing waste), pH dependence of distribution coefficients of each element have been obtained. The pH dependence of distribution coefficients of U, Ac, Th, Ra and Pb was analyzed by model calculation of adsorption behavior based on chemical forms of each elements and soil surface characteristics, which are a cation exchange capacity and surface charge. From model calculation of adsorption behavior, the distribution coefficients' values and adsorption behavior of Pb, Ra, Th, Ac and U could be showed by a combination of cation exchange and surface-complexation adsorption model.

Journal Articles

Measurement of distribution coefficients for uranium series radionuclides under shallow land environment condition, 1

Ishii, Tomoaki*; Inagawa, Satoshi*; Gunji, Yasuyoshi*; Sakamoto, Yoshiaki; Takebe, Shinichi; Ogawa, Hiromichi; Sasaki, Tomozo*

Genshiryoku Bakkuendo Kenkyu, 8(1), p.55 - 64, 2001/09

Distribution coefficients of Uranium series nuclide(Pb,Ra,Ac,Th,Pa and U) were obtained under aerated zone environment and aquifer environment, for the safety evaluation of shallow underground disposal of uranium bearing waste. The distribution coefficients of them on 4 kinds of soil such as the loam in the rain water as for aerated zone environment and on 3 kinds of soil and rock such as the sand in groundwater as for aquifer environment have been measured by batch method. The distribution coefficients in aerated zone environment were one or two orders in magnitude higher than that in aquifer environment, except Ac. And, there was approximately the linear correlation on the relationship between cation exchange capacity and specific surface area, which are representative physical property of the soil, and distribution coefficient of lead, radium and protactinium.

Journal Articles

Effect of flow field on colloid deposition in filtration process of polystyrene latex particles through columns packed glass beads

Chinju, H.*; Nagasaki, Shinya*; Tanaka, Satoru*; Sakamoto, Yoshiaki; Takebe, Shinichi; Ogawa, Hiromichi

Journal of Nuclear Science and Technology, 38(8), p.645 - 654, 2001/08

 Times Cited Count:3 Percentile:28.03(Nuclear Science & Technology)

no abstracts in English

Journal Articles

Sorption behavior of radium and actinium on soils

Sakamoto, Yoshiaki; Takebe, Shinichi; Ogawa, Hiromichi; Muraoka, Susumu; Ishii, Tomoaki*; Inagawa, Satoshi*; Gunji, Yasuyoshi*

Materials Research Society Symposium Proceedings, Vol.663, p.1207 - 1214, 2001/00

no abstracts in English

JAEA Reports

Integrated disposal system concering to waste of RI and research institute

Hagiwara, Shigeru*; Sakamoto, Yoshiaki; Takebe, Shinichi; Okuda, Katsuzo*; Ogawa, Hiromichi

JAERI-Research 2000-039, 119 Pages, 2000/09

JAERI-Research-2000-039.pdf:5.04MB

no abstracts in English

JAEA Reports

Survey of the characteristics on the neogene sedimentary rocks in northern Kanto and northeast Japan along the pacific coast

Okuda, Katsuzo*; Takebe, Shinichi; Sakamoto, Yoshiaki; Hagiwara, Shigeru*; Ogawa, Hiromichi

JAERI-Review 99-023, p.100 - 0, 1999/10

JAERI-Review-99-023.pdf:4.63MB

no abstracts in English

JAEA Reports

Distribution coefficients of $$^{237}$$Np and $$^{241}$$Am in sedimentary geological formation

Tanaka, Tadao; Takebe, Shinichi; Ogawa, Hiromichi; Muraoka, Susumu

JAERI-Research 98-018, 20 Pages, 1998/03

JAERI-Research-98-018.pdf:0.94MB

no abstracts in English

JAEA Reports

Field test of radionuclide migration; Cooperative research between JAERI and CIRP

*; Yamamoto, Tadatoshi; ; Takebe, Shinichi; Ogawa, Hiromichi; Tanaka, Tadao; Mukai, Masayuki; Komiya, Tomokazu; S.Li*; Z.Wang*; et al.

JAERI-Research 94-009, 44 Pages, 1994/07

JAERI-Research-94-009.pdf:1.69MB

no abstracts in English

Journal Articles

Evaluation of migration of cesium-137 adsorbed on fine soil particles through natural aerated soil layer

Ogawa, Hiromichi; Takebe, Shinichi; Yamamoto, Tadatoshi

Journal of Nuclear Science and Technology, 28(3), p.248 - 254, 1991/03

no abstracts in English

JAEA Reports

Migration behavior of radionuclide in soil layer of final storage; Radionuclide migration test in aerated soil layer by precipitation

Yamamoto, Tadatoshi; Takebe, Shinichi; Ogawa, Hiromichi; Tanaka, Tadao; Mukai, Masayuki; Komiya, Tomokazu; *;

JAERI-M 89-189, 18 Pages, 1989/11

JAERI-M-89-189.pdf:0.65MB

no abstracts in English

JAEA Reports

Migration behavior of radionuclide in soil layer of final storage site; Radionuclide migration test in aerated soil layer by radioactive contaminated water

Yamamoto, Tadatoshi; Takebe, Shinichi; Ogawa, Hiromichi; Tanaka, Tadao; Mukai, Masayuki; Komiya, Tomokazu; *;

JAERI-M 89-144, 23 Pages, 1989/10

JAERI-M-89-144.pdf:0.87MB

no abstracts in English

Oral presentation

Fundamental study on immobilization of sludge generated from treatment of remaining water used for cooling of the stricken power reactors

Amamoto, Ippei; Kobayashi, Hidekazu; Yokozawa, Takuma; Yamashita, Teruo; Nagai, Takayuki; Suzuki, Yoshikazu*; Takebe, Hiromichi*; Mitamura, Naoki*; Tsuzuki, Tatsuya*

no journal, , 

The great amount of water used for cooling the stricken reactors at Fukushima Dai-ichi Nuclear Power Plant following the earthquake and tsunami of 11 March 2011 had resulted in accumulation of "remaining water" in some buildings. From public announcements, it seems likely the decontamination process of La Hague reprocessing plant would be employed as one of the treatment processes for the remaining water contaminated by FPs such as Cs, Sr, etc.. Based on literature study, Cs would precipitate with ferrocyanide compound as well as Sr with BaSO$$_{4}$$ by applying the above-mentioned process. In this study, BaSO$$_{4}$$ as the simulated sludge was loaded into the iron phosphate glass (IPG) medium under different melting temperature. Based on the results, the performance of IPG containing BaO (decomposed from BaSO$$_{4}$$) improved with increase loading of BaO up to 48 mol% at lower melting temperature.

Oral presentation

Applicability of vitrification method for waste generated from treatment of contaminated water, 3; Preliminary experiment on vitrification of the sludge

Amamoto, Ippei; Yokozawa, Takuma; Yamashita, Teruo; Nagai, Takayuki; Nakamura, Hirotaka*; Takebe, Hiromichi*; Mitamura, Naoki*; Tsuzuki, Tatsuya*; Kobayashi, Hidekazu

no journal, , 

no abstracts in English

Oral presentation

Applicability of vitrification method for waste generated from treatment of contaminated water, 2; Outline of sludge vitrification and selection of glass medium

Amamoto, Ippei; Kobayashi, Hidekazu; Yokozawa, Takuma; Yamashita, Teruo; Nagai, Takayuki; Suzuki, Yoshikazu*; Takebe, Hiromichi*; Mitamura, Naoki*; Tsuzuki, Tatsuya*

no journal, , 

no abstracts in English

34 (Records 1-20 displayed on this page)