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An Approach toward evaluation of long-term fission product distributions in the Fukushima Daiichi Nuclear Power Plant after the severe accident

内田 俊介; 唐澤 英年; 木野 千晶*; Pellegrini, M.*; 内藤 正則*; 逢坂 正彦

Nuclear Engineering and Design, 380, p.111256_1 - 111256_19, 2021/08

 被引用回数:0 パーセンタイル:0.01(Nuclear Science & Technology)



Conversion factors bridging radioactive fission product distributions in the primary containment vessel of Fukushima Daiichi NPP and dose rates measured by the containment atmosphere monitoring system

内田 俊介; Pellegrini, M.*; 内藤 正則*

Nuclear Engineering and Design, 380, p.111303_1 - 111303_11, 2021/08

 被引用回数:1 パーセンタイル:81.22(Nuclear Science & Technology)

福島第一原子力発電所(1F)の事故進展解析と同時に廃炉計画立案のためには、プラント全体にわたるFP分布の定量化が必須で、このために多期間FP挙動解析手法を開発している。この解析手法の妥当性は、プラントで測定されたデータに基づいて立証する必要がある。この妥当性立証の有効な手法のひとつがCAMSでの線量率測定データの適用である。しかし、FPの分布(kg, Bq)と線量率(Sv/h)という特性、単位次元の異なるデータを比較するためには、両者を適切につなぐ手段が必要となる。線量率解析が可能な、迅速で、取り扱いが容易で、かつトレーサブルな手法として、多くの線源位置、多核種に関しての線量率換算係数を求めた。この線量率換算係数を用いると、多期間FP挙動解析手法で求めたFP分布から容易に線量率が算出可能である。


3.5.3 汚染水処理技術

内田 俊介

原子力のいまと明日, p.63 - 68, 2019/03



Improvement of plant reliability based on combining of prediction and inspection of crack growth due to intergranular stress corrosion cracking

内田 俊介; 知見 康弘; 笠原 茂樹; 塙 悟史; 岡田 英俊*; 内藤 正則*; 小嶋 正義*; 木倉 宏成*; Lister, D. H.*

Nuclear Engineering and Design, 341, p.112 - 123, 2019/01

 被引用回数:2 パーセンタイル:42.44(Nuclear Science & Technology)



Observation of anisotropic magneto-Peltier effect in nickel

内田 健一*; 大門 俊介*; 井口 亮*; 齊藤 英治

Nature, 558(7708), p.95 - 99, 2018/06

 被引用回数:40 パーセンタイル:92.78(Multidisciplinary Sciences)

The Peltier effect, discovered in 1834, converts a charge current into a heat current in a conductor, and its performance is described by the Peltier coefficient, which is defined as the ratio of the generated heat current to the applied charge current. To exploit the Peltier effect for thermoelectric cooling or heating, junctions of two conductors with different Peltier coefficients have been believed to be indispensable. Here we challenge this conventional wisdom by demonstrating Peltier cooling and heating in a single material without junctions. This is realized through an anisotropic magneto-Peltier effect in which the Peltier coefficient depends on the angle between the directions of a charge current and magnetization in a ferromagnet. By using active thermography techniques, we observe the temperature change induced by this effect in a plain nickel slab. We find that the thermoelectric properties of the ferromagnet can be redesigned simply by changing the configurations of the charge current and magnetization, for instance, by shaping the ferromagnet so that the current must flow around a curve. Our experimental results demonstrate the suitability of nickel for the anisotropic magneto-Peltier effect and the importance of spin-orbit interaction in its mechanism. The anisotropic magneto-Peltier effect observed here is the missing thermoelectric phenomenon in ferromagnetic materials-the Onsager reciprocal of the anisotropic magneto-Seebeck effect previously observed in ferromagnets and its simplicity might prove useful in developing thermal management technologies for electronic and spintronic devices.


An Empirical model for the corrosion of stainless steel in BWR primary coolant

内田 俊介*; 塙 悟史; 内藤 正則*; 岡田 英俊*; Lister, D. H.*

Corrosion Engineering, Science and Technology, 52(8), p.587 - 595, 2017/10

 被引用回数:2 パーセンタイル:17.39(Materials Science, Multidisciplinary)



Thermographic measurements of the spin Peltier effect in metal/yttrium-iron-garnet junction systems

大門 俊介*; 内田 健一*; 井口 亮*; 日置 友智*; 齊藤 英治

Physical Review B, 96(2), p.024424_1 - 024424_12, 2017/07

 被引用回数:22 パーセンタイル:80.96(Materials Science, Multidisciplinary)

The spin Peltier effect (SPE), heat-current generation due to spin-current injection, in various metal (Pt, W, and Au single layers and Pt/Cu bilayer)/ferrimagnetic insulator [yttrium-iron-garnet (YIG)] junction systems has been investigated by means of a lock-in thermography (LIT) method. The SPE is excited by a spin current across the metal/YIG interface, which is generated by applying a charge current to the metallic layer via the spin Hall effect. The LIT method enables the thermal imaging of the SPE free from the Joule-heating contribution. Importantly, we observed spin-current-induced temperature modulation not only in the Pt/YIG and W/YIG systems, but also in the Au/YIG and Pt/Cu/YIG systems, excluding the possible contamination by anomalous Ettingshausen effects due to proximity-induced ferromagnetism near the metal/YIG interface. As demonstrated in our previous study, the SPE signals are confined only in the vicinity of the metal/YIG interface; we buttress this conclusion by reducing a spatial blur due to thermal diffusion in an infrared-emission layer on the sample surface used for the LIT measurements. We also found that the YIG-thickness dependence of the SPE is similar to that of the spin Seebeck effect measured in the same Pt/YIG sample, implying the reciprocal relation between them.


Concomitant enhancement of the longitudinal spin Seebeck effect and the thermal conductivity in a Pt/YIG/Pt system at low temperatures

井口 亮*; 内田 健一*; 大門 俊介*; 齊藤 英治

Physical Review B, 95(17), p.174401_1 - 174401_7, 2017/05

 被引用回数:30 パーセンタイル:86.49(Materials Science, Multidisciplinary)

We report a simultaneous measurement of a longitudinal spin Seebeck effect (LSSE) and thermal conductivity in a Pt/Y$$_{3}$$Fe$$_{5}$$O$$_{12}$$ (YIG)/Pt system in a temperature range from 10 to 300 K. By directly monitoring the temperature difference in the system, we excluded thermal artifacts in the LSSE measurements. It is found that both the LSSE signal and the thermal conductivity of YIG exhibit sharp peaks at the same temperature, different from previous reports. The maximum LSSE coefficient is found to be $$S_mathrm{LSSE} > 10 mu$$V/K, one-order-of magnitude greater than the previously reported values. The concomitant enhancement of the LSSE and thermal conductivity of YIG suggests the strong correlation between magnon and phonon transport in the LSSE.


Thermal imaging of spin Peltier effect

大門 俊介*; 井口 亮*; 日置 友智*; 齊藤 英治; 内田 健一*

Nature Communications (Internet), 7, p.13754_1 - 13754_7, 2016/12

 被引用回数:65 パーセンタイル:94.39(Multidisciplinary Sciences)

The Peltier effect modulates the temperature of a junction comprising two different conductors in response to charge currents across the junction, which is used in solid-state heat pumps and temperature controllers in electronics. Recently, in spintronics, a spin counterpart of the Peltier effect was observed. The "spin Peltier effect" modulates the temperature of a magnetic junction in response to spin currents. Here we report thermal imaging of the spin Peltier effect; using active thermography technique, we visualize the temperature modulation induced by spin currents injected into a magnetic insulator from an adjacent metal. The thermal images reveal characteristic distribution of spin-current-induced heat sources, resulting in the temperature change confined only in the vicinity of themetal/insulator interface. This finding allows us to estimate the actual magnitude of the temperature modulation induced by the spin Peltier effect, which is more than one order of magnitude greater than previously believed.


Evaluation of ECP measured in in-pile environment

塙 悟史; 内田 俊介; 端 邦樹; 知見 康弘; 笠原 茂樹*; 西山 裕孝

Proceedings of 20th Nuclear Plant Chemistry International Conference (NPC 2016) (USB Flash Drive), 11 Pages, 2016/10



Study of irradiation effect on ECP using in-pile loops in the JMTR

塙 悟史; 内田 俊介; 端 邦樹; 知見 康弘; 笠原 茂樹*; 西山 裕孝

Proceedings of 20th Nuclear Plant Chemistry International Conference (NPC 2016) (USB Flash Drive), 10 Pages, 2016/10



Complete suppression of longitudinal spin Seebeck effect by frozen magnetization dynamics in Y$$_{3}$$Fe$$_{5}$$O$$_{12}$$

吉川 貴史*; 内田 健一*; 大門 俊介*; 齊藤 英治

Journal of the Physical Society of Japan, 85(6), p.065003_1 - 065003_2, 2016/06

 被引用回数:8 パーセンタイル:59.54(Physics, Multidisciplinary)

The spin Seebeck effect (SSE) in a Pt-film/Y$$_{3}$$Fe$$_{5}$$O$$_{12}$$ (YIG)-slab junction system has been investigated at low temperatures and under various magnetic fields in the longitudinal configuration. We found that, by increasing applied magnetic fields, the SSE signal gradually decreases and converges to zero without showing sign reversal. The complete field-induced suppression of the SSE is interpreted in terms of the effect of the Zeeman gap in magnon excitation.


Corrosion of structural materials and electrochemistry in high-temperature water; Relationships among water chemistry, corrosion, oxide film and electrochemical corrosion potential

内田 俊介; 塙 悟史; Kysela, J.*; Lister, D. H.*

Power Plant Chemistry, 18(1), p.6 - 17, 2016/01

原子力発電所の信頼性維持のため、各プラントにはそのシステム,材料,運転履歴に基づくプラント固有の最適水化学制御が必要とされる。電気化学は腐食に係る問題の重要課題の一つである。FAC, IGSCC, PWSCCなど、腐食に係る問題は、ECP,導電率, pHなど電気化学指標に基づいて理解される。ECP,金属表面状態,浸漬時間,その他の環境条件の相関に基づき、電気化学と酸化被膜成長モデルを連成したECPと鋼の腐食速度を評価するためのモデルを開発した。連成モデルに関して得られた結論は以下の通りである。(1)FACによる減肉速度に及ぼす水化学の改善と編流による質量移行係数の影響は本モデルにより適切に評価することができた。(2)ECPに及ぼすH$$_{2}$$O$$_{2}$$, O$$_{2}$$の影響は本モデルで評価でき、浸漬時間の影響は酸化被膜の成長による結果として適切に説明できた。(3)中性子照射によるECPの低下は酸化膜の照射誘起拡散により説明できた。


Advanced water chemistry control based on parameters determined with plant simulation models

内田 俊介; 塙 悟史; Lister, D. H.*

Power Plant Chemistry, 17(6), p.328 - 339, 2015/12



Critical suppression of spin Seebeck effect by magnetic fields

吉川 貴史*; 内田 健一*; 大門 俊介*; Qiu, Z.*; 塩見 雄毅*; 齊藤 英治

Physical Review B, 92(6), p.064413_1 - 064413_9, 2015/08

 被引用回数:127 パーセンタイル:97.6(Materials Science, Multidisciplinary)

The longitudinal spin Seebeck effect (LSSE) in Pt/Y$$_3$$Fe$$_5$$O$$_{12}$$ (YIG) junction systems has been investigated at various magnetic fields and temperatures. We found that the LSSE voltage in a Pt/YIG-slab system is suppressed by applying high magnetic fields and this suppression is critically enhanced at low temperatures. The field-induced suppression of the LSSE in the Pt/YIG-slab system is too large at around room temperature to be explained simply by considering the effect of the Zeeman gap in magnon excitation. This result requires us to introduce a magnon-frequency-dependent mechanism into the scenario of LSSE; low-frequency magnons dominantly contribute to the LSSE. The magnetic field dependence of the LSSE voltage was observed to change by changing the thickness of YIG, suggesting that the thermospin conversion by the low-frequency magnons is suppressed in thin YIG films due to the long characteristic lengths of such magnons.


Intrinsic surface magnetic anisotropy in Y$$_{3}$$Fe$$_{5}$$O$$_{12}$$ as the origin of low-magnetic-field behavior of the spin Seebeck effect

内田 健一*; 大江 純一郎*; 吉川 貴史*; 大門 俊介*; Hou, D.*; Qiu, Z.*; 齊藤 英治

Physical Review B, 92(1), p.014415_1 - 014415_8, 2015/07

 被引用回数:26 パーセンタイル:77.37(Materials Science, Multidisciplinary)

The magnetic-field dependence of the longitudinal spin Seebeck effect (LSSE) in a Pt/Y$$_{3}$$Fe$$_{5}$$O$$_{12}$$ (YIG)-slab junction system was found to deviate from a bulk magnetization curve of the YIG slab in a low field range. In this paper, we show that the deviation originates from the difference between surface and bulk magnetization processes in the YIG slab and that it appears even when removing possible extrinsic magnetic anisotropy due to surface roughness and replacing the Pt layer with different materials. This result indicates that the anomalous field dependence of the LSSE is due to an intrinsic magnetic property of the YIG surface. Our numerical calculation based on the Landau-Lifshitz-Gilbert equation shows that the deviation between the LSSE and bulk magnetization curves is qualitatively explained by introducing easy-axis perpendicular magnetic anisotropy near the surface of YIG.


Determining water chemistry conditions in nuclear reactor coolants

Lister, D. H.*; 内田 俊介

Journal of Nuclear Science and Technology, 52(4), p.451 - 466, 2015/04

 被引用回数:13 パーセンタイル:43.75(Nuclear Science & Technology)



Laser micro-processing as a tool for constructing insulator-based magnonic crystal

大門 俊介*; 井口 亮*; 内田 健一*; 齊藤 英治

Journal of Physics D; Applied Physics, 48(16), p.164014_1 - 164014_4, 2015/04

 被引用回数:6 パーセンタイル:27.89(Physics, Applied)

Y$$_{3}$$Fe$$_{5}$$O$$_{12}$$ (YIG) films with a periodic-antidot-array structure fabricated by laser microprocessing is shown to exhibit clear characteristics of two-dimensional (2D) magnonic crystals. The experimental results demonstrate that the spin-wave-resonance spectra in the YIG films are modulated by the periodic antidot structure. The frequency and lattice constant dependences of the spectra are well reproduced by a numerical calculation based on magnonic band structures of the 2D magnonic crystals. Since the laser micro-processing is compatible with various thin-film fabrication methods, it can be a powerful tool for constructing magnonic crystals.


Sign of inverse spin Hall voltages generated by ferromagnetic resonance and temperature gradients in yttrium iron garnet platinum bilayers

Schreier, M.*; Bauer, G. E. W.*; Vasyuchka, V.*; Flipse, J.*; 内田 健一*; Lotze, J.*; Lauer, V.*; Chumak, A.*; Serga, A.*; 大門 俊介*; et al.

Journal of Physics D; Applied Physics, 48(2), p.025001_1 - 025001_5, 2015/01

 被引用回数:47 パーセンタイル:89.51(Physics, Applied)

We carried out a concerted effort to determine the absolute sign of the inverse spin Hall effect voltage generated by spin currents injected into a normal metal. We focus on yttrium iron garnet (YIG)|platinum bilayers at room temperature, generating spin currents by microwaves and temperature gradients. We find consistent results for different samples and measurement setups that agree with theory. We suggest a right-hand-rule to define a positive spin Hall angle corresponding to the voltage expected for the simple case of scattering of free electrons from repulsive Coulomb charges.


Verification and validation procedures of calculation codes for determining corrosive conditions in the BWR primary cooling system based on water radiolysis and mixed potential models

内田 俊介*; 和田 陽一*; 山本 誠二*; 高木 純一*; 久宗 健志*

Journal of Nuclear Science and Technology, 51(1), p.24 - 36, 2014/01

 被引用回数:5 パーセンタイル:36.81(Nuclear Science & Technology)


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