Initialising ...
Initialising ...
Initialising ...
Initialising ...
Initialising ...
Initialising ...
Initialising ...
Ash, J.*; 岩崎 弘典*; Mijatovi, T.*; Budner, T.*; Elder, R.*; Elman, B.*; Friedman, M.*; Gade, A.*; Grinder, M.*; Henderson, J.*; et al.
Physical Review C, 103(5), p.L051302_1 - L051302_6, 2021/05
被引用回数:0 パーセンタイル:0.02(Physics, Nuclear)カルシウム同位体は陽子魔法数20を持つため基底状態は球形であるが、変形共存と呼ばれる、数MeV上に変形した状態がある現象が予想されている。回転バンドの存在によってそれが実験的に確かめられるが、Caは安定核の融合反応で作るには中性子が多すぎるため、これまで回転バンドの存在が確かめられていなかった。この研究では、ミシガン州立大学の超伝導サイクロトロンにて中性子過剰核
Kビームを作り、そこから
Li(
K,
)
Ca反応によって
Caの高スピン状態を生成した。そこからの脱励起ガンマ線の観測により、
までの回転バンドの存在を確立した。そのエネルギー準位は、大規模殻模型計算の予言とよく合うことがわかり、
Caでも変形共存が起こることが明らかになった。
Wang, Y.*; Jia, G.*; Cui, X.*; Zhao, X.*; Zhang, Q.*; Gu, L.*; Zheng, L.*; Li, L. H.*; Wu, Q.*; Singh, D. J.*; et al.
Chem, 7(2), p.436 - 449, 2021/02
被引用回数:58 パーセンタイル:99.74(Chemistry, Multidisciplinary)Nanozymes are promising alternatives to natural enzymes, but their use remains limited owing to poor specificity. Overcoming this is extremely challenging due to the intrinsic structural complexity of these systems. We report theoretical design and experimental realization of a series of heterogeneous molybdenum single-atom nanozymes (named Mo-N
-C), wherein we find that the peroxidase-like specificity is well regulated by the coordination numbers of single Mo sites. The resulting Mo
-N
-C catalyst shows exclusive peroxidase-like behavior. It achieves this behavior via a homolytic pathway, whereas Mo
-N
-C and Mo
-N
-C catalysts have a different heterolytic pathway. The mechanism of this coordination-number-dependent enzymatic specificity is attributed to geometrical structure differences and orientation relationships of the frontier molecular orbitals.
Dupont, E.*; Bossant, M.*; Capote, R.*; Carlson, A. D.*; Danon, Y.*; Fleming, M.*; Ge, Z.*; 原田 秀郎; 岩本 修; 岩本 信之; et al.
EPJ Web of Conferences, 239, p.15005_1 - 15005_4, 2020/09
被引用回数:3 パーセンタイル:97.17The OECD-NEA High Priority Request List (HPRL) is a point of reference to guide and stimulate the improvement of nuclear data for nuclear energy and other nuclear applications. The HPRL is application-driven and the requests are submitted by nuclear data users or representatives of the user's communities. A panel of international experts reviews and monitors the requests in the framework of an Expert Group mandated by the NEA Nuclear Science Committee Working Party on International Nuclear Data Evaluation Cooperation (WPEC). After approval, individual requests are divided in two priority categories only, whereas a third category now includes groups of generic requests in a well-defined area (e.g., dosimetry, standard). The HPRL is hosted by the NEA in the form of a relational database publicly available on the web. This contribution provides an overview of HPRL entries, status and outlook. Examples of requests successfully completed will be given and new requests will be described with emphasis on updated nuclear data needs in the fields of nuclear energy, neutron standards, dosimetry, and medical applications.
Lokotko, T.*; Leblond, S.*; Lee, J.*; Doornenbal, P.*; Obertelli, A.*; Poves, A.*; Nowacki, F.*; 緒方 一介*; 吉田 数貴; Authelet, G.*; et al.
Physical Review C, 101(3), p.034314_1 - 034314_7, 2020/03
被引用回数:5 パーセンタイル:72.36(Physics, Nuclear)中性子過剰核であるCoに対する(
)ノックアウト反応が理化学研究所RIBFで測定された。
coincidenceの方法で準位構造が決定され、測定された包括的断面積および排他的断面積から暫定的ではあるがスピン・パリティが決定された。殻模型計算との比較により、
Coの低励起状態には球形核と変形核が共存することが示唆された。
Wu, H.*; Wang, Y.*; 池田 篤史; Miller, C. J.*; Waite, T. D.*
Environmental Science; Water Research & Technology, 5(8), p.1400 - 1411, 2019/08
被引用回数:6 パーセンタイル:49.35(Engineering, Environmental)排水プロセスにおける燐成分回収等の目的のため、パイロットスケールの膜分離活性汚泥排水装置に二価鉄(Fe(II))を添加した際の排水装置各部位の鉄・燐の溶存化学種をX線吸収分光(XANES/EXAFS)と因子分析法を組み合わせて検討した。
Zhang, Y.*; Guo, H.*; Kim, S. B.*; Wu, Y.*; Ostojich, D.*; Park, S. H.*; Wang, X.*; Weng, Z.*; Li, R.*; Bandodkar, A. J.*; et al.
Lab on a Chip, 19(9), p.1545 - 1555, 2019/05
被引用回数:73 パーセンタイル:99.26(Biochemical Research Methods)汗中のバイオマーカーおよび非侵襲的な方法で汗を集める方法は、健康および生理学的状態の評価のための汗利用の関心を生み出し、スポーツから臨床医学までの範囲の潜在的用途がある。本論文は、皮膚密着型のマイクロ流体システムを用いた2つの結果について述べる。(1)簡易な身体的および心理的刺激による汗の採取、(2)酵素化学および比色アプローチによる汗中のクレアチニンおよび尿素の濃度の検出。結果、乳児や高齢者などを対象に日常的で非薬理学的な汗の捕捉が可能になり、腎臓疾患のスクリーニング/モニタリングに汗を使用する可能性が示された。
Elekes, Z.*; Kripk,
*; Sohler, D.*; Sieja, K.*; 緒方 一介*; 吉田 数貴; Doornenbal, P.*; Obertelli, A.*; Authelet, G.*; 馬場 秀忠*; et al.
Physical Review C, 99(1), p.014312_1 - 014312_7, 2019/01
被引用回数:7 パーセンタイル:72.63(Physics, Nuclear)(,
)反応による
Niの核構造の探索実験を行った。Lenzi, Nowacki, Poves, Sieja相互作用を用いた殻模型計算では実験結果を説明しうる陽子空孔状態が得られており、理論的な断面積計算は実験値とよい一致を与えた。実験で得られたすべての状態を理論的に一意に決定することはできなかったが、過去の実験結果と同様にNi同位体でのZ = 28の大きなshell gapを示す結果が得られた。
Li, B.; Wang, H.*; 川北 至信; Zhang, Q.*; Feygenson, M.*; Yu, H. L.*; Wu, D.*; 尾原 幸治*; 菊地 龍弥*; 柴田 薫; et al.
Nature Materials, 17(3), p.226 - 230, 2018/03
被引用回数:86 パーセンタイル:96.84(Chemistry, Physical)As a generic property, all substances transfer heat through microscopic collisions of constituent particles. A solid conducts heat through both transverse and longitudinal acoustic phonons, but a liquid employs only longitudinal vibrations. As a result, a solid is usually thermally more conductive than a liquid. In canonical viewpoints, such a difference also serves as the dynamic signature distinguishing a solid from a liquid. Here, we report liquid-like thermal conduction observed in the crystalline AgCrSe. The transverse acoustic phonons are completely suppressed by the ultrafast dynamic disorder while the longitudinal acoustic phonons are strongly scattered but survive, and are thus responsible for the intrinsically ultralow thermal conductivity. This scenario is applicable to a wide variety of layered compounds with heavy intercalants in the van der Waals gaps, manifesting a broad implication on suppressing thermal conduction. These microscopic insights might reshape the fundamental understanding on thermal transport properties of matter and open up a general opportunity to optimize performances of thermoelectrics.
Shand, C. M.*; Podolyk, Zs.*; G
rska, M.*; Doornenbal, P.*; Obertelli, A.*; Nowacki, F.*; Otsuka, T.*; Sieja, K.*; Tostevin, J. A.*; Tsunoda, T.*; et al.
Physics Letters B, 773, p.492 - 497, 2017/10
被引用回数:20 パーセンタイル:88.12(Astronomy & Astrophysics)Low-lying states in neutron-rich Zn nuclei were measured for the first time via in-beam
-ray spectroscopy at RIKEN. These include the 4
to 2
in
Zn and the 2
to 0
and 4
to 2
in
Zn. The reduced E(
) energies and increased E(4
)/E(2
) ratios at
=52,54 compared to
Zn attest that the magicity is confined just on the neutron number
=50 only. The levels observed in
Zn suggest the onset of deformation towards heavier Zn isotopes. The data were compared to state-of-the-art shell model calculations.
Jungclaus, A.*; Grawe, H.*; 西村 俊二*; Doornenbal, P.*; Lorusso, G.*; Simpson, G. S.*; Sderstr
m, P.-A.*; 炭竃 聡之*; Taprogge, J.*; Xu, Z. Y.*; et al.
Physics Letters B, 772, p.483 - 488, 2017/09
被引用回数:8 パーセンタイル:62.28(Astronomy & Astrophysics)A new high-spin isomer in the neutron-rich nucleus Cd was populated in the projectile fission of a
U beam at the Radioactive Isotope Beam Factory at RIKEN. A half-life of T
= 6.3(8) ms was measured for the new state which was tentatively assigned a spin/parity of (15
). The isomeric state decays via the emission of a 309-keV
ray with
multipolarity. The experimental results are compared to shell model calculations performed using state-of-the-art realistic effective interactions and to the neighbouring nucleus
Cd. The comparison with calculations shows that adjustments of the pairing and multipole parts of the effective interaction derived from the CD-Bonn nucleon-nucleon potential are required in order to describe the properties of nuclei in the region around
Sn.
Morales, A. I.*; Benzoni, G.*; Watanabe, H.*; 角田 佑介*; Otsuka, T.*; 西村 俊二*; Browne, F.*; Daido, R.*; Doornenbal, P.*; Fang, Y.*; et al.
Physics Letters B, 765, p.328 - 333, 2017/02
被引用回数:30 パーセンタイル:93.9(Astronomy & Astrophysics)The level schemes of neutron-rich isotopes Co and
Ni were populated in the
decay of
Fe and studied using
-delayed
-ray spectroscopy of the
decay, at the RIBF in RIKEN, Japan. The experimental results were compared to state-of-the-art shell-model calculations, and indicate a dominance of prolate deformation in the low-lying states, coexisting with spherical states. The
decay of the
isobars is shown to progress in accordance to a new type of shell evolution, the so-called Type II, which involves many particle-hole excitations across energy gaps.
Jungclaus, A.*; Grawe, H.*; 西村 俊二*; Doornenbal, P.*; Lorusso, G.*; Simpson, G. S.*; Sderstr
m, P. A.*; 炭竃 聡之*; Taprogge, J.*; Xu, Z. Y.*; et al.
Physical Review C, 94(2), p.024303_1 - 024303_8, 2016/08
被引用回数:15 パーセンタイル:77.19(Physics, Nuclear)The decay of the semi-magic nucleus
Cd has been studied at the RIBF facility at the RIKEN Nishina Center. The high statistics of the present experiment allowed for a revision of the established level scheme of
In and the observation of additional
feeding to high lying core-excited states in
In. The experimental results are compared to shell-model calculations employing a model space consisting of the full major
neutron and
proton shells, and good agreement is found.
Li, B.; Luo, X. H.*; Wang, H.*; Ren, W. J.*; Yano, S.*; Wang, C.-W.*; Gardner, J. S.*; Liss, K.-D.*; Miao, P.*; Lee, S.-H.*; et al.
Physical Review B, 93(22), p.224405_1 - 224405_6, 2016/06
被引用回数:35 パーセンタイル:84.98(Materials Science, Multidisciplinary)Competition between ferromagnetic and antiferromagnetic phases on frustrated lattices in hexagonal Laves phase compound HfTa
Fe
is investigated by using neutron diffraction as a function of temperature and magnetic fields and density-functional-theory calculations. At 325 K, the compound orders into the 120
frustrated antiferromagnetic state with well-reduced magnetic moment and an in-plane lattice contraction simultaneously sets in. With further cooling down, however, the accumulated distortion in turn destabilizes this susceptible frustrated structure. The frustration is completely relieved at 255 K when the first-order transition to the ferromagnetic state takes place, where a colossal negative volumetric thermal expansion,
/K, is obtained. Meanwhile, the antiferromagnetic state can be suppressed by few Tesla magnetic fields, which results in a colossal positive magnetostriction. Such delicate competition is attributed to the giant magnetic fluctuation inherent in the frustrated antiferromagnetic state. Therefore, the magnetoelastic instability is approached even under a small perturbation.
Jungclaus, A.*; Gargano, A.*; Grawe, H.*; Taprogge, J.*; 西村 俊二*; Doornenbal, P.*; Lorusso, G.*; Shimizu, Y.*; Simpson, G. S.*; Sderstr
m, P.-A.*; et al.
Physical Review C, 93(4), p.041301_1 - 041301_6, 2016/04
被引用回数:17 パーセンタイル:80.54(Physics, Nuclear)For the first time, the decay of excited states in a nucleus situated "south-east" of Sn have been observed, in a region where experimental information is limited to ground-state properties. Six
rays from
Cd, produced in the fragmentation of a
U beam at RIBF at RIKEN. The
rays were studied using the EURICA array of Ge detectors. The new experimental information is compared to results from realistic shell-model calculations, which are the first in this region far from stability. Comparison with calculations suggests that at least four out of six new transitions can be attributed to the particle-hole configuration of one neutron in the
and one proton hole in the
orbits, respectively. This work constitutes an important first step towards the exploration of nuclear structure in this unknown region of the nuclear chart.
Morales, A. I.*; Benzoni, G.*; Watanabe, H.*; 西村 俊二*; Browne, F.*; Daido, R.*; Doornenbal, P.*; Fang, Y.*; Lorusso, G.*; Patel, Z.*; et al.
Physical Review C, 93(3), p.034328_1 - 034328_14, 2016/03
被引用回数:21 パーセンタイル:84.2(Physics, Nuclear)Low-lying excited states in Ni have been investigated at RIKEN by studying the
decay of
Co to
Ni.
Co was separated with BigRIPS, implanted into the WaS3ABi Silicon array, and the
ray measured using the EURICA
spectrometer. From the analysis, 60 new
-ray transitions and 21 new levels in
Ni were observed. The new experimental information is compared to shell-model calculations which include neutron excitation across the
shell. The calculations reproduce rather well the observed states, implying that a clear understanding of these low-lying excitations has been achieved.
櫻井 大督; 佐伯 修*; Carr, H.*; Wu, H.-Y.*; 山本 卓宏*; Duke, D.*; 高橋 成雄*
IEEE Transactions on Visualization and Computer Graphics, 22(1), p.945 - 954, 2016/01
被引用回数:3 パーセンタイル:32.7(Computer Science, Software Engineering)単変量のトポロジーは、Morse理論の形をとって、科学技術現場でデータを解析及び可視化するための計算ツールを提供してきた。等値線間の接続性が変化する様子は、等値線を1点に縮約することで、Reebグラフとして表現できる。多変量データについては、等値線はファイバー(値域の点の逆像)に一般化され、そのためこの分野はファイバートポロジーとして知られている。しかしながら、ファイバートポロジーはMorse理論に比べれば未開拓の状態にあり、また現在の研究は人の手による可視化に頼っている。そのため本稿では、多変量関数:
に含まれるファイバーの特異性を可視化するインターフェイスを紹介する。本インターフェイスはファイバートポロジーでの伝統的可視化作業に則っているが、Reebグラフを拡張したReeb空間に基づく3次元ビューをも新規に導入している。本インターフェイスの妥当性を評価するために、我々はいくつかのケースで検討し、支援可能かどうか検証を進めている。本発表では数学分野での利用を想定し、そのワークフローを支援できるかどうか、当該分野の専門の数学者と、経験の浅い数学者とを対象に検証したのでその結果について発表する。
Benzoni, G.*; Morales, A. I.*; Watanabe, H.*; 西村 俊二*; Coraggio, L.*; Itaco, N.*; Gargano, A.*; Browne, F.*; Daido, R.*; Doornenbal, P.*; et al.
Physics Letters B, 751, p.107 - 112, 2015/12
被引用回数:19 パーセンタイル:80.73(Astronomy & Astrophysics)The decays of
Mn have been measured at the RIBF facility at RIKEN using the EURICA
spectrometer combined with an active stopper consisting of a stack of Si detectors. Half-lives and
-delayed neutron emission probabilities have been extracted for these decays, together with first experimental information on excited states populated in
Fe. The data indicate a continuously increasing deformation for Fe isotopes up to A=70, and interpreted to be due to the interplay between quadrupole correlation of specific neutron orbitals and the monopole component of the proton-neutron interaction.
Taprogge, J.*; Jungclaus, A.*; Grawe, H.*; 西村 俊二*; Doornenbal, P.*; Lorusso, G.*; Simpson, G. S.*; Sderstr
m, P.-A.*; 炭竃 聡之*; Xu, Z. Y.*; et al.
Physical Review C, 91(5), p.054324_1 - 054324_11, 2015/05
被引用回数:24 パーセンタイル:86.13(Physics, Nuclear)The decay of
Cd, produced in relativistic fission of a
U beam, was studied at the RIKEN Nishina Center. From the
-ray analysis, 31 excited states and 69
ray transitions were established in the level scheme of
In, and compared with state-of-the-art shell-model calculations. It was found that the
decay of
Cd is dominated by Gamow teller transitions, but a non-negligible contribution to the
decay is also made by first-forbidden transitions. To estimate the contribution of first-forbidden transitions is important for calculations of the
-decay half-lives of nuclei in this region.
Lorusso, G.*; 西村 俊二*; Xu, Z. Y.*; Jungclaus, A.*; Shimizu, Y.*; Simpson, G. S.*; Sderstr
m, P.-A.*; Watanabe, H.*; Browne, F.*; Doornenbal, P.*; et al.
Physical Review Letters, 114(19), p.192501_1 - 192501_7, 2015/05
被引用回数:130 パーセンタイル:97.86(Physics, Multidisciplinary)The -decay half-lives of 110 neutron-rich isotopes of the elements from Rb to Sn were measured at the RIBF Facility at RIKEN, Japan. The new data demonstrate the persistence of shell structure far from stability and have direct implications for the
-process calculations. In particular, the new half-lives have a global impact on the calculated
-process elemental abundances, and alleviate the underproduction of isotopes just above and below the A=130 peak, which in the past required the introduction of shell structure modifications. Reaction-network calculations based on the new data reinforce the notion that the r-process abundance pattern may result from the freeze-out of a (n,
)
(
,n) equilibrium.
菊池 満; Fasoli, A.*; 滝塚 知典*; Diamond, P. H.*; Medvedev, S.*; Wu, Y.*; Duan, X.*; 岸本 泰明*; 花田 和明*; Pueschel, M. J.*; et al.
Proceedings of 8th IAEA Technical Meeting on Steady State Operation of Magnetic Fusion Devices (CD-ROM), 20 Pages, 2015/05
D型形状でHモード運転の標準的なトカマクは優れた閉じ込め性能を示すものの、過渡的、定常的な熱負荷の問題で大きな課題を持っている。これらを解決する方法として将来を見据えた幅ひろい考え方として形状制御を用いて熱制御を緩和する方式について講演する。