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Nakahara, Masaumi; Watanabe, So; Ishii, Yasuyuki*; Yamagata, Ryohei*; Yuri, Yosuke*; Yuyama, Takahiro*; Ishizaka, Tomohisa*; Koka, Masashi*; Yamada, Naoto*; Hagura, Naoto*
Nuclear Instruments and Methods in Physics Research B, 554, p.165449_1 - 165449_5, 2024/09
Ion beam induced luminescence analysis of lanthanide complexes in the organic solvents for minor actinides recovery process was carried out to investigate the structures of complexes. In this study, hydrogen ion beam obtained from the single-ended accelerator and argon ion beam obtained from the azimuthally varying field cyclotron were used in Takasaki Ion Accelerators for Advanced Radiation Application in National Institutes for Quantum Science and Technology. In the experiments, ion beam induced luminescence spectra of lanthanide complexes in the organic solvents were measured, and the relationship between the obtained spectra and the structures of complexes was studied.
Kokubun, Yuji; Nakada, Akira; Seya, Natsumi; Koike, Yuko; Nemoto, Masashi; Tobita, Keiji; Yamada, Ryohei*; Uchiyama, Rei; Yamashita, Daichi; Nagai, Shinji; et al.
JAEA-Review 2023-046, 164 Pages, 2024/03
JAEA-Review-2023-046.pdf:4.2MB
The Nuclear Fuel Cycle Engineering Laboratories conducts environmental radiation monitoring around the reprocessing plant in accordance with the "Safety Regulations for Reprocessing Plant of JAEA, Part IV: Environmental Monitoring". This report summarizes the results of environmental radiation monitoring conducted during the period from April 2022 to March 2023 and the results of dose calculations for the surrounding public due to the release of radioactive materials into the atmosphere and ocean. In the results of the above environmental radiation monitoring, many items were affected by radioactive materials emitted from the accident at the Fukushima Daiichi Nuclear Power Plant of Tokyo Electric Power Company, Incorporated (changed to Tokyo Electric Power Company Holdings, Inc. on April 1, 2016), which occurred in March 2011. Also included as appendices are an overview of the environmental monitoring plan, an overview of measurement methods, measurement results and their changes over time, meteorological statistics results, radioactive waste release status, and an evaluation of the data which deviated of the normal range.
Nakahara, Masaumi; Watanabe, So; Yuyama, Takahiro*; Ishizaka, Tomohisa*; Yuri, Yosuke*; Ishii, Yasuyuki*; Yamagata, Ryohei*; Yamada, Naoto*; Koka, Masashi*; Kada, Wataru*; et al.
QST-M-47; QST Takasaki Annual Report 2022, P. 64, 2024/03
An extraction chromatography method has been studied to recover minor actinides from high-level liquid waste. For effective elution of minor actinides in an adsorbent, the structures of complexes are attempted to be evaluated with ion beam induced luminescence. In this study, Eu complexes in the adsorbent were irradiated by Ar
ion beam, and the ion beam induced luminescence spectra of Eu complexes were measured to evaluate the structures of Eu complexes.
Yamada, Ryohei*; Tamakuma, Yuki*; Kuwata, Haruka*; Saigusa, Yumi*; Watanabe, Yuki; Hirota, Seiko*; Jin, Q.*; Cai, Y.*
Hoken Butsuri (Internet), 58(3), p.169 - 177, 2023/11
no abstracts in English
Nakahara, Masaumi; Watanabe, So; Takeuchi, Masayuki; Yuyama, Takahiro*; Ishizaka, Tomohisa*; Ishii, Yasuyuki*; Yamagata, Ryohei*; Yamada, Naoto*; Koka, Masashi*; Kada, Wataru*; et al.
Nuclear Instruments and Methods in Physics Research B, 542, p.144 - 150, 2023/09
Times Cited Count：1 Percentile：63.33(Instruments & Instrumentation)The structures of Eu complexes in the adsorbents prepared with various extractants were evaluated by ion beam induced luminescence analysis in an extraction chromatography for minor actinides recovery. The luminescence of Eu was measured with a proton beam obtained from the single-ended accelerator and an argon ion beam obtained from the azimuthally varying field cyclotron in Takasaki Ion Accelerators for Advanced Radiation Application in National Institutes for Quantum Science and Technology. In this study, it was confirmed that the spectral shape of Eu complexes in the adsorbents varied depending on the kinds of extractants, and the correlation between the change in the spectra and the structures of Eu complexes was investigated.
Nakada, Akira; Kanai, Katsuta; Kokubun, Yuji; Nagaoka, Mika; Koike, Yuko; Yamada, Ryohei*; Kubota, Tomohiro; Hirao, Moe; Yoshii, Hideki*; Otani, Kazunori*; et al.
JAEA-Review 2022-079, 116 Pages, 2023/03
JAEA-Review-2022-079.pdf:2.77MB
Based on the regulations (the safety regulation of Tokai Reprocessing Plant, the safety regulation of nuclear fuel material usage facilities, the radiation safety rule, the regulation about prevention from radiation hazards due to radioisotopes, which are related with the nuclear regulatory acts, the local agreement concerning with safety and environment conservation around nuclear facilities, the water pollution control law, and by law of Ibaraki Prefecture), the effluent control of liquid waste discharged from the Nuclear Fuel Cycle Engineering Laboratories of Japan Atomic Energy Agency has been performed. This report describes the effluent control results of the liquid waste in the fiscal year 2021. In this period, the concentrations and the quantities of the radioactivity in liquid waste discharged from the reprocessing plant, the plutonium fuel fabrication facilities, and the other nuclear fuel material usage facilities were much lower than the limits authorized by the above regulations.
Nakada, Akira; Kanai, Katsuta; Seya, Natsumi; Nishimura, Shusaku; Futagawa, Kazuo; Nemoto, Masashi; Tobita, Keiji; Yamada, Ryohei*; Uchiyama, Rei; Yamashita, Daichi; et al.
JAEA-Review 2022-078, 164 Pages, 2023/03
JAEA-Review-2022-078.pdf:2.64MB
Environmental radiation monitoring around the Tokai Reprocessing Plant has been performed by the Nuclear Fuel Cycle Engineering Laboratories, based on "Safety Regulations for the Reprocessing Plant of Japan Atomic Energy Agency, Chapter IV - Environmental Monitoring". This annual report presents the results of the environmental monitoring and the dose estimation to the hypothetical inhabitant due to the radioactivity discharged from the plant to the atmosphere and the sea during April 2021 to March 2022. In this report, some data include the influence of the accidental release from the Fukushima Daiichi Nuclear Power Station of Tokyo Electric Power Co., Inc. (the trade name was changed to Tokyo Electric Power Company Holdings, Inc. on April 1, 2016) in March 2011. Appendices present comprehensive information, such as monitoring programs, monitoring methods, monitoring results and their trends, meteorological data and discharged radioactive wastes. In addition, the data which were influenced by the accidental release and exceeded the normal range of fluctuation in the monitoring, were evaluated.
Daido, Hiroyuki*; Yamada, Tomonori; Saruta, Koichi; Miyabe, Masabumi; Ito, Chikara; Shibata, Takuya; Inoue, Kaoru*; Terabayashi, Ryohei*; Hasegawa, Shuichi*
Physica Scripta, 98(3), p.035112_1 - 035112_22, 2023/02
Characterization of kW class quasi-continuous wave (a pulse duration of 10 ms) laser interaction with metal targets and those with metal oxide targets are presented in respect to the laser induced breakdown and the successive laser induced melting and evaporation coupled with a mechanical response followed by ejection of various kinds of particles and fragments. An experiment was performed using fiber lasers coupled with a high-speed camera to observe dynamics of the interaction. Ejected fine particles were collected using a cascade impactor and a home-made collector and were observed with electron microscopes. Shapes of irradiation marks were observed with a digital optical microscope. We also measured total ejected mass from a target. The experimental results reveal that firstly the laser threshold intensity of the interaction with the metal target was lower and more stable than those with the metal oxide targets. Secondly, in the stainless steel targets, the dynamics of molten layer created by thermal conduction from the laser heated thin layer and successive particle ejection with less mechanical response by the adjacent solid layer are dominant processes, while in the metal oxide targets, the fracturing in the relatively deeper interaction region coupled with brittle material response having relatively large laser shot to shot fluctuation appears to play a significant role in addition to the laser induced melting.
Nakahara, Masaumi; Watanabe, So; Ishii, Yasuyuki*; Yamagata, Ryohei*; Yamada, Naoto*; Koka, Masashi*; Yuyama, Takahiro*; Ishizaka, Tomohisa*; Kada, Wataru*; Hagura, Naoto*
QST-M-39; QST Takasaki Annual Report 2021, P. 62, 2023/02
In an extraction chromatography method for minor actinides recovery, analysis for the structure of complex in a silica-based adsorbent has been studied to separate minor actinides efficiently. In this study, Eu was used as simulated material of minor actinides, and silica-based adsorbents containing Eu complex were prepared. The ion beam induced luminescence spectra of Eu complexes in silica-based adsorbents were measured, and the basic data for the structures of Eu complexes were obtained.
Nakada, Akira; Nakano, Masanao; Kanai, Katsuta; Seya, Natsumi; Nishimura, Shusaku; Nemoto, Masashi; Tobita, Keiji; Futagawa, Kazuo; Yamada, Ryohei; Uchiyama, Rei; et al.
JAEA-Review 2021-062, 163 Pages, 2022/02
JAEA-Review-2021-062.pdf:2.87MB
Environmental radiation monitoring around the Tokai Reprocessing Plant has been performed by the Nuclear Fuel Cycle Engineering Laboratories, based on "Safety Regulations for the Reprocessing Plant of Japan Atomic Energy Agency, Chapter IV - Environmental Monitoring". This annual report presents the results of the environmental monitoring and the dose estimation to the hypothetical inhabitant due to the radioactivity discharged from the plant to the atmosphere and the sea during April 2020 to March 2021. In this report, some data include the influence of the accidental release from the Fukushima Daiichi Nuclear Power Station of Tokyo Electric Power Co., Inc. (the trade name was changed to Tokyo Electric Power Company Holdings, Inc. on April 1, 2016) in March 2011. Appendices present comprehensive information, such as monitoring programs, monitoring methods, monitoring results and their trends, meteorological data and discharged radioactive wastes. In addition, the data which were influenced by the accidental release and exceeded the normal range of fluctuation in the monitoring, were evaluated.
Nakano, Masanao; Nakada, Akira; Kanai, Katsuta; Nagaoka, Mika; Koike, Yuko; Yamada, Ryohei; Kubota, Tomohiro; Yoshii, Hideki*; Otani, Kazunori*; Hiyama, Yoshinori*; et al.
JAEA-Review 2021-040, 118 Pages, 2021/12
JAEA-Review-2021-040.pdf:2.48MB
Based on the regulations (the safety regulation of Tokai Reprocessing Plant, the safety regulation of nuclear fuel material usage facilities, the radiation safety rule, the regulation about prevention from radiation hazards due to radioisotopes, which are related with the nuclear regulatory acts, the local agreement concerning with safety and environment conservation around nuclear facilities, the water pollution control law, and by law of Ibaraki Prefecture), the effluent control of liquid waste discharged from the Nuclear Fuel Cycle Engineering Laboratories of Japan Atomic Energy Agency has been performed. This report describes the effluent control results of the liquid waste in the fiscal year 2020. In this period, the concentrations and the quantities of the radioactivity in liquid waste discharged from the reprocessing plant, the plutonium fuel fabrication facilities, and the other nuclear fuel material usage facilities were much lower than the limits authorized by the above regulations.
Yoshimoto, Masahiro; Nakanoya, Takamitsu; Yamazaki, Yoshio; Saha, P. K.; Kinsho, Michikazu; Yamamoto, Shunya*; Okazaki, Hiroyuki*; Taguchi, Tomitsugu*; Yamada, Naoto*; Yamagata, Ryohei*
Proceedings of 18th Annual Meeting of Particle Accelerator Society of Japan (Internet), p.850 - 854, 2021/10
no abstracts in English
Koike, Yuko; Yamada, Ryohei; Nagaoka, Mika; Nakano, Masanao; Ono, Yosuke; Suitsu, Yuichi
JAEA-Technology 2021-011, 39 Pages, 2021/08
JAEA-Technology-2021-011.pdf:1.56MB
In the Analyzed Liquid Treatment Facility of Japan Nuclear Fuel Co., Ltd. (JNFL) MOX Fuel Fabrication Plant (J-MOX), the interfere by salts with the analysis of gross alpha activity concentration analysis will be caused during the treatment process. Therefore, JNFL devised the desalting method using a solid-phase extraction chromatography. Japan Atomic Energy Agency carried out the experimental study to confirm the validity of this desalting method for the treatment liquid based on the contract with JNFL. This study consists of three experiments as follows: Step 1 - Selection of an optical solid-phase extraction agent, Step 2 - Evaluation of variation optical solid-phase extraction agent, and Step 3 - Application of the imitation liquid waste. The result of Step 1 determined the solid-phase extraction agent (InertSep ME-2) and the optimum condition (aspiration method by manifold (about 5-10 mL/min), 3M nitric acid as eluent, pH: 5, and no adjustment of ionic valence). Then, the result of Step 2 and 3 made sure the validation of this method by obtaining over 70% recovery for the imitation liquid waste sample of the Analyzed Liquid Treatment Facility of J-MOX.
Nugraha, E. D.*; Hosoda, Masahiro*; Kusdiana*; Untara*; Mellawati, J.*; Nurokhim*; Tamakuma, Yuki*; Ikram, A.*; Syaifudin, M.*; Yamada, Ryohei; et al.
Scientific Reports (Internet), 11(1), p.14578_1 - 14578_16, 2021/07
Times Cited Count：19 Percentile：82.87(Multidisciplinary Sciences)Mamuju is one of the regions in Indonesia which retains natural conditions but has relatively high exposure to natural radiation. The goals of the present study were to characterize exposure of the entire Mamuju region as a high natural background radiation area (HNBRA) and to assess the existing exposure as a means for radiation protection of the public and the environment. A cross-sectional study method was used with cluster sampling areas by measuring all parameters that contribute to external and internal radiation exposures. It was determined that Mamuju was a unique HNBRA with the annual effective dose between 17 and 115 mSv, with an average of 32 mSv. The lifetime cumulative dose calculation suggested that Mamuju residents could receive as much as 2.2 Sv on average which is much higher than the average dose of atomic bomb survivors for which risks of cancer and non-cancer diseases are demonstrated. The study results are new scientific data allowing better understanding of health effects related to chronic low-dose-rate radiation exposure and they can be used as the main input in a future epidemiology study.
Yamada, Ryohei; Kono, Takahiko; Nakajima, Junya; Hirouchi, Jun; Tsuji, Tomoya; Umeda, Masayuki; Igarashi, Yu*; Koike, Hiromi*
Hoken Butsuri (Internet), 56(1), p.32 - 38, 2021/03
no abstracts in English
Yoshimoto, Masahiro; Nakanoya, Takamitsu; Yamazaki, Yoshio; Saha, P. K.; Kinsho, Michikazu; Yamamoto, Shunya*; Okazaki, Hiroyuki*; Taguchi, Tomitsugu*; Yamada, Naoto*; Yamagata, Ryohei*
JPS Conference Proceedings (Internet), 33, p.011019_1 - 011019_7, 2021/03
The multi-turn charge-exchange H
beam injection scheme with stripper foils is one of the key techniques to achieve a MW-class high power proton beam. The J-PARC RCS adopts Hybrid type Boron-doped Carbon (HBC) stripper foil, which was developed in KEK to improve the lifetime. Indeed, the RCS user operation confirmed that HBC foil has the great advantage of a longer lifetime against high beam irradiation. To examine characteristics of the HBC foils, various beam studies were performed, such as the stripping efficiency measurement and long-term observation with an H beam in the J-PARC RCS, foil analysis using RBS, EDR and PIXE methods, and SEM and TEM observation after the ion beam irradiation in Takasaki Ion Accelerators for Advanced Radiation Application (TIARA) on National Institutes for Quantum and Radiological Science and Technology (QST). Recently, the deposition apparatus for the HBC foils from the KEK Tsukuba-site was relocated to the JAEA Tokai-site, and we started fabrication of new HBC foil in 2017. (The new one fabricated in JAEA we call J-HBC foil.) And, we continue investigations in TIARA with the J-HBC foils. Furthermore, in-depth researches by changing the process parameters of the foil deposition are carried on. Recent results suggest that the amount of the boron doped in the foil is more important parameter than the ratio of the discharge amount of carbon from cathode and anode electrodes. In this presentation, we will report the details of recent analysis of the J-HBC foil.
Nakano, Masanao; Fujii, Tomoko; Nagaoka, Mika; Koike, Yuko; Yamada, Ryohei; Kubota, Tomohiro; Yoshii, Hideki*; Otani, Kazunori*; Hiyama, Yoshinori*; Kikuchi, Masaaki*; et al.
JAEA-Review 2020-070, 120 Pages, 2021/02
JAEA-Review-2020-070.pdf:2.47MB
Based on the regulations (the safety regulation of Tokai Reprocessing Plant, the safety regulation of nuclear fuel material usage facilities, the radiation safety rule, the regulation about prevention from radiation hazards due to radioisotopes, which are related with the nuclear regulatory acts, the local agreement concerning with safety and environment conservation around nuclear facilities, the water pollution control law, and by law of Ibaraki Prefecture), the effluent control of liquid waste discharged from the Nuclear Fuel Cycle Engineering Laboratories of Japan Atomic Energy Agency has been performed. This report describes the effluent control results of the liquid waste in the fiscal year 2019. In this period, the concentrations and the quantities of the radioactivity in liquid waste discharged from the reprocessing plant, the plutonium fuel fabrication facilities, and the other nuclear fuel material usage facilities were much lower than the limits authorized by the above regulations.
Ogura, Koya*; Hosoda, Masahiro*; Tamakuma, Yuki*; Suzuki, Takahito*; Yamada, Ryohei; Negemi, Ryoju*; Tsujiguchi, Takakiyo*; Yamaguchi, Masaru*; Shiroma, Yoshitaka*; Iwaoka, Kazuki*; et al.
International Journal of Environmental Research and Public Health, 18(3), p.978_1 - 978_16, 2021/02
Times Cited Count：7 Percentile：66.08(Environmental Sciences)Hosoda, Masahiro*; Nugraha, E. D.*; Akata, Naofumi*; Yamada, Ryohei; Tamakuma, Yuki*; Sasaki, Michiya*; Kelleher, K.*; Yoshinaga, Shinji*; Suzuki, Takahito*; Rattanapongs, C. P.*; et al.
Science of the Total Environment, 750, p.142346_1 - 142346_11, 2021/01
Times Cited Count：23 Percentile：84.59(Environmental Sciences)The biological effects of low dose-rate radiation exposures on humans remains unknown. In fact, the Japanese nation still struggles with this issue after the Fukushima Dai-ichi Nuclear Power Plant accident. Recently, we have found a unique area in Indonesia where naturally high radiation levels are present, resulting in chronic low dose-rate radiation exposures. We aimed to estimate the comprehensive dose due to internal and external exposures at the particularly high natural radiation area, and to discuss the enhancement mechanism of radon. A car-borne survey was conducted to estimate the external doses from terrestrial radiation. Indoor radon measurements were made in 47 dwellings over three to five months, covering the two typical seasons, to estimate the internal doses. Atmospheric radon gases were simultaneously collected at several heights to evaluate the vertical distribution. The absorbed dose rates in air in the study area vary widely between 50 nGy h
and 1109 nGy h. Indoor radon concentrations ranged from 124 Bq m
to 1015 Bq m. That is, the indoor radon concentrations measured exceed the reference levels of 100 Bq m recommended by the World Health Organization. Furthermore, the outdoor radon concentrations measured were comparable to the high indoor radon concentrations. The annual effective dose due to external and internal exposures in the study area was estimated to be 27 mSv using the median values. It was found that many residents are receiving radiation exposure from natural radionuclides over the dose limit for occupational exposure to radiation workers. This enhanced outdoor radon concentration might be as a result of the stable atmospheric conditions generated at an exceptionally low altitude. Our findings suggest that this area provides a unique opportunity to conduct an epidemiological study related to health effects due to chronic low dose-rate radiation exposure.
Nakano, Masanao; Fujii, Tomoko; Nagaoka, Mika; Inoue, Kazumi; Koike, Yuko; Yamada, Ryohei; Yoshii, Hideki*; Otani, Kazunori*; Hiyama, Yoshinori*; Kikuchi, Masaaki*; et al.
JAEA-Review 2019-045, 120 Pages, 2020/03
JAEA-Review-2019-045.pdf:2.54MB
Based on the regulations (the safety regulation of Tokai Reprocessing Plant, the safety regulation of nuclear fuel material usage facilities, the radiation safety rule, the regulation about prevention from radiation hazards due to radioisotopes, which are related with the nuclear regulatory acts, the local agreement concerning with safety and environment conservation around nuclear facilities, the water pollution control law, and by law of Ibaraki Prefecture), the effluent control of liquid waste discharged from the Nuclear Fuel Cycle Engineering Laboratories of Japan Atomic Energy Agency has been performed. This report describes the effluent control results of the liquid waste in the fiscal year 2018. In this period, the concentrations and the quantities of the radioactivity in liquid waste discharged from the reprocessing plant, the plutonium fuel fabrication facilities, and the other nuclear fuel material usage facilities were much lower than the limits authorized by the above regulations.
