Effect of Ra purity as a target for Ac production using a fast reactor

Sasaki, Yuto; Maeda, Shigetaka

Journal of Radioanalytical and Nuclear Chemistry, 333, p.5987 - 5996, 2024/02

https://doi.org/10.1007/s10967-024-09397-7

Researchers are seeking alternative Ac production methods because of the scarcity of Ac for targeted alpha therapy. Although Ra from waste sources has been considered, obtaining Ra is challenging. Therefore, the authors focused on the contamination of minerals with Th-derived Ra while investigating methods to recover Ra from uranium ores. The effect of 228Ra contamination on Ac production by Ra transmutation using fast reactors was evaluated. Consequently, toxic Ac contaminates Ac. However, using the different half-lives of Ac and Ac, pure Ac can be obtained from the chemical separation of actinium after cooling for 5-8 days.

Assessment report of research and development activities in FY2014; Activity "Fusion Research and Development" (In-advance evaluation)

Fusion Research and Development Directorate

JAEA-Evaluation 2016-002, 40 Pages, 2016/03

JAEA-Evaluation-2016-002.pdf:2.66MB

Japan Atomic Energy Agency (hereinafter referred to as "JAEA") asked the assessment committee, "Evaluation Committee of Research and Development Activities for Fusion" (hereinafter referred to as "Committee") for in-advance evaluation of "Research and Development of the technical system for extraction of fusion energy," in accordance with "General Guideline for the Evaluation of Government R&D Activities" by Cabinet Office, Government of Japan, "Guideline for Evaluation of R&D in Ministry of Education, Culture, Sports, Science and Technology" and "Regulation on Conduct for Evaluation of R&D Activities" by JAEA. In response to the JAEA's request, the Committee assessed the research program of the Fusion Research and Development Directorate (hereinafter referred to as "FRDD") during the period from April 2015 to March 2022. The Committee evaluated the management and research activities of the FRDD based on the explanatory documents prepared by the FRDD, the oral presentations with questions-and-answers by the Director General and the Deputy Director Generals.

Status and prospect of JT-60 plasma control and diagnostic data processing systems for advanced operation scenarios

Kurihara, Kenichi; Yonekawa, Izuru; Kawamata, Yoichi; Sueoka, Michiharu; Hosoyama, Hiroki*; Sakata, Shinya; Oshima, Takayuki; Sato, Minoru; Kiyono, Kimihiro; Ozeki, Takahisa

Fusion Engineering and Design, 81(15-17), p.1729 - 1734, 2006/07

https://doi.org/10.1016/j.fusengdes.2006.04.058

A large tokamak fusion device JT-60 is expected to explore more advanced tokamak discharge scenario towards the ITER and a future power reactor. We believe the following experimental issues are expected to be solved in JT-60. To clarify how to keep a steady-state plasma with high performance, and how to avoid plasma instabilities almost completely. By stimulus of this motivation, several essential development and modifications of plasma control and data acquisition systems have been performed in JT-60. In this report, we discuss the developments to improve the JT-60 plasma control and data acquisition systems. In addition, a future plasma control and data acquisition systems leading to a standard design for a power reactor is envisaged on the basis of the 20-year plasma operation experiences.

Outline of the ITER project

Mori, Masahiro

Koon Gakkai-Shi, 30(5), p.236 - 242, 2004/09

http://ci.nii.ac.jp/naid/10029252321

no abstracts in English

Fusion reactor technology; Challenge to future energy

Seki, Masahiro; Hishinuma, Akimichi; Kurihara, Kenichi; Akiba, Masato; Abe, Tetsuya; Ishitsuka, Etsuo; Imai, Tsuyoshi; Enoeda, Mikio; Ohira, Shigeru; Okumura, Yoshikazu; et al.

Kaku Yugoro Kogaku Gairon; Mirai Enerugi Eno Chosen, 246 Pages, 2001/09

no abstracts in English

Design and analysis of the vacuum vessel for RTO/RC-ITER

Onozuka, Masanori*; Ioki, Kimihiro*; Johnson, G.*; Kodama, T.*; Sonnazzaro, G.*; Utin, Y.*

Fusion Engineering and Design, 51-52(Part.B), p.249 - 255, 2000/11

https://doi.org/10.1016/S0920-3796(00)00330-6

no abstracts in English

Post irradiation examination of (U,Pu) C and (U,Pu) N fuel for fast reactor; Non-destructive examination result of the fuel pin

; ; ; Matsumoto, Shinichiro

JNC TN9410 2000-009, 65 Pages, 2000/09

JNC-TN9410-2000-009.pdf:4.36MB

In order to evaluate irradiation behavior of(U, Pu) C and (U, Pu) N fuel using fast reactor, (U, Pu) C and (U, Pu) N fuel pins were irradiated in JOYO for the fist time in Japan. In this study, one (U, Pu) C fuel pin and two (U, Pu) N fuel pins were irradiated to maximum burn up about 40GWd/t. Post irradiation examination of (U, Pu) C and (U, Pu) N fuel pins started in Fuel Monitoring Facility (FMF) at JNC from October 1999, and it ended in March, 2000. The results of non-destructive post irradiation examination reported in this document. Main results are shown in the following. (1)The soundness of all (U,Pu) C and (U,Pu) N fuel pins were confirmed from the non-destructive examination result. (2)The fuel stack elongation of (U,Pu) C and (U,Pu) N is bigger than it of the MOX fuel for fast reactor. (3)The singular behavior from the gamma ray scanning measurement in the stack area was not confirmed. The migration of Cs137 to lower insulator pellet and outside of the pellet was confirmed in (U,Pu) N B9NO2 pin. In (U,Pu) C fuel, the migration of Cs137 was not confirmed. (4)In (U,Pu) C B9CO1 pin and (U,Pu) N B9NO2 pin in which the gap width was small, diameter of cladding increase around 50 m in the stack area which originates for FCMI was confirmed. In (U,Pu) N B9NO1 pin in which the gap width was wide, the ovality which originates from the relocation of the pellet was confirmed. (5)Fission gas release rate of (U,Pu) N were 3.3% and 5.2%, and the low value compared to the MOX fuel was shown.

Irradiation tests report of the 35th cycle in "JOYO"

JNC TN9440 2000-008, 79 Pages, 2000/08

JNC-TN9440-2000-008.pdf:2.33MB

This report summarizes the operating and irradiatlon data of the experimental reactor "JOYO" 35th cycle. Irradiation tests in the 35th cycle are as follows: (1)C-type irradiation rig (C4F) (a)High burnup performance test of advanced austenitic stainless steel cladding fuel pins (in collaboration with France) (2)C-type irradiation rig (C6D) (a)Large diameter fuel pins irradiation tests (3)Core Materials Irradiation Rig (CMIR-5) (a)Cladding tube materials irradiation tests for "MONJU" (4)Structure Materials Irradiation Rigs (SMIR) (a)Decision of material design base standard of structure materials for prototype reactor and large scale reactor (5)Upper core structure irradiation Plug Rig (UPR-1-5) (a)Upper core neutron spectrum effect and accelerated irradiation effect (6)SurVeillance un-instrument Irradiation Rig (SVIR) (a)Confimation of surveillance irradiation condition for "JOYO" (b)Material irradiation tests (based on a contract with universities) The maximum burnup driver assembly "PFD253" reached 67,600 MWd/t (pin average).

Analysis of Cm contained in irradiated fuel of experimental fast reactor "JOYO"; Development of the analytical technique and measurement of Cm

Osaka, Masahiko; Koyama, Shinichi; Mitsugashira, Toshiaki; Morozumi, Katsufumi; Namekawa, Takashi

JNC TN9400 2000-058, 49 Pages, 2000/04

JNC-TN9400-2000-058.pdf:1.22MB

The analytical technique for Cm contained in a MOX FUEL was developed and analysis of Cm contained in irradiated fuel of experimental fast reactor "JOYO" was carried out, to contribute to evaluation of transmutation characteristics of MA nuclide in the fast reactor. The procedure of ion-exchange separation of Cm with nitric acid-methanol mixed media essential for the isotopic analysis in irradiated MOX fuel was adopted considering for being rapid and easy. The fundamental test to grasp separation characteristics of this procedure, such as Cm elution position and separation capacity between Cm and Am or Eu, was carried out. ln applying this procedure to the analysis of Cm contained in actual specimen, separation condition was evaluated and optimized, and the procedure consist of impurity removal and Am removal process was devised. This procedure resulted in high recovery rate of Cm and high removal rate of Am and impurity which becomes a problem in sample handling and mass-spectrometry such as Eu and Cs. The Cm separation test from irradiated MOX fuel was carried out using this technique, and Cm isotopic ratio analysis was enabled. The analytical technique for Cm contained in irradiated MOX fuel was established using the procedure of ion-exchange separation with nitric acid-methanol mixed media. The analysis of Cm contained in irradiated MOX fuel of experimental fast reactor "Joyo" was carried out. As a result, it was revealed from measured data that Cm content rate was 1.4 4.0lO atom%, small amount of Cm was generated and Cm isotopic ratio was constant above burn-up 60GWd/t.

JOYO coolant sodium and cover gas purity control database (MK-II core)

; Nemoto, Masaaki; Saikawa, Takuya*; Sukegawa, Kazuya*

JNC TN9410 2000-008, 66 Pages, 2000/03

JNC-TN9410-2000-008.pdf:1.39MB

The experimental fast reactor "JOYO" served as the MK-II irradiation bed core for testing fuel and material for FBR development for 15 years from 1982 to 1997. During the MK-II operation, impurities concentrations in the sodium and the argon gas were determined by 67 samples of primary sodium, 81 samples of secondary sodium, 75 samples of primary argon gas, 89 samples of secondary argon gas (the overflow tank) and 89 samples of secondary argon gas (the dump tank). The sodium and the argon gas purity control data were accumulated from in thirty-one duty operations, thirteen special test operations and eight annual inspections. These purity control results and related plant data were compiled into database, which were recorded on CD-ROM for user convenience. Purity control data include concentration of oxygen, carbon, hydrogen, nitrogen, chlorine, iron, nickel and chromium in sodium, concentration of oxygen, hydrogen, nitrogen, carbon monoxide, carbon dioxide, methane and helium in argon gas with the reactor condition.