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Saga, Kaname
JAEA-Review 2025-003, 23 Pages, 2025/05
JAEA-Review-2025-003.pdf:1.08MB
Diagnosis and treatment using radioisotopes (RI) in the medical field contribute to improving people's welfare. However, almost all medical RI distributed in Japan are imported from overseas. As a result, geopolitical influences and natural disasters lead to difficulties for importing them. Based on these backgrounds, in Japan, a specialized subcommittee on the production and utilization of medical radioisotopes was established within the Atomic Energy Commission, and in May 2022, it formulated the "Action Plan for Promotion of Production and Utilization of Medical Radioisotopes." Japan Atomic Energy Agency (JAEA) launched the NXR Development Center in FY2024 to separate and recycle valuable elements contained in high-level liquid waste (HLLW). The advantages of using HLLW are that it contains a wide variety of nuclides and in large quantities. Therefore, this report focused on the RI contained in HLLW and evaluated whether it can be supplied for medical use. Specifically, the target supply amount of Sr-90, the parent nuclide of Y-90 approved as a RI for medical use, and the amount of Sr-90 in HLLW were estimated. Based on the estimation, the feasibility of separating medical RI from HLLW in a reprocessing research facility was evaluated. As a result, the HLLW possibly contains an amount of RI equivalent to the domestic medical demand. Although it depends on the RI concentration in the HLLW, a small volume of HLLW, ranging from a few hundred milliliters to a few liters, could potentially produce an amount of medical RI equivalent to domestic demand. In addition, the equipment already installed in research facilities, such as NUCEF at JAEA, may be sufficient to produce the medical RI. It may be possible to meet domestic medical demand for Sr-90, as a source of Y-90, by processing a few hundred milliliters to a few liters of HLLW using an existing research facility.
Futemma, Akira; Sanada, Yukihisa; Nakama, Shigeo; Sasaki, Miyuki; Ochi, Kotaro; Sawahata, Yoshiro*; Kawasaki, Yoshiharu*; Iwai, Takeyuki*; Hiraga, Shogo*; Haginoya, Masashi*; et al.
JAEA-Technology 2024-022, 170 Pages, 2025/03
JAEA-Technology-2024-022.pdf:15.09MB
On March 11, 2011, the 2011 off the Pacific coast of Tohoku Earthquake caused a tsunami that led to the Fukushima Daiichi Nuclear Power Station accident, releasing radioactive material into the environment. Since then, Aerial Radiation Monitoring (ARM) using manned helicopters has been employed to measure radiation distribution. As a commissioned project from the Nuclear Regulation Authority, the Japan Atomic Energy Agency (JAEA) utilizes this technology for emergency monitoring during nuclear facility accidents, aiming to provide prompt results by pre-arranging information on background radiation, topography, and control airspaces around nuclear power plants nationwide. In fiscal year 2023, the commissioned project included conducting ARM around the Sendai Nuclear Power Station and preparing related information. To enhance effectiveness during emergencies, ARM and the first domestic training flight of Unmanned Aerial Vehicles (UAVs) were conducted during the FY2023 Nuclear Energy Disaster Prevention Drill. Furthermore, UAVs radiation monitoring technology was advanced by selecting UAVs and investigating their performance. This report summarizes the results and technical issues identified providing insights to improve emergency preparedness.
Takahashi, Yoshio*; Yamaguchi, Akiko; Yomogida, Takumi
Treatise on Geochemistry, 3rd edition, Vol.6, p.105 - 150, 2025/00
With the recent development of measurement techniques, new approaches to the environmental geochemistry of radionuclides have been applied for various research targets. In this review article, several topics within the last 10-15 years in the field of environmental geochemistry of radionuclides have been discussed. In particular, this article mainly focused on two topics, (i) studies on the migration of radionuclides emitted by the Fukushima Daiichi Nuclear Power Plant (FDNPP) accident in 2011 and (ii) the development of X-ray absorption fine structure (XAFS) spectroscopy and its application to the geochemical processes of radionuclides.
Saga, Kaname
JAEA-Review 2024-038, 9 Pages, 2024/09
JAEA-Review-2024-038.pdf:0.88MB
The purpose of this report is understanding the elements and radio isotopes with highly useful based on the current trends in the industrial field. The survey was conducted from the viewpoint of the abundance of elements and radio isotopes contained and the demand in the industrial field, and the following survey results were obtained. The economic scale of radio isotopes in the industrial field (including radiation use) has been increasing in recent years in the manufacturing, medical, and agricultural sectors. On the other hand, the domestic production of the utilized radio isotope is still small, and some radio isotopes are entirely imported. Radio isotopes such as Sr-90, Mo-100, Cs-137, and Am-241 from spent fuel are suitable for industrial use because of their abundance in spent fuel and half-lives. As for the utilization of elements, the industrial use of platinum group elements and rare earth elements were explored because these elements are high industrial value and low domestic self-sufficiency. The platinum group elements were evaluated to have the potential to be supplied in a certain amount as a new domestic production source based on their abundance in spent fuel. On the other hand, for rare earth elements, which have also low self-sufficiency rate, the ratio of the amount that could be supplied from spent fuel compared to the current annual supply was evaluated to be less than 1%, and therefore, no effect could be expected. The domestic recycling rate of rare earth elements is low, and the provision of numerical simulation technology, which improves the recycling rate, could highly contribute to the industries. This technology makes it possible to calculate the optimal operating conditions for the separation process, such as the number of processing stages and processing speed, in accordance with the elements to be separated and used.
Be and 
Al under direct muon-induced spallation in granite quartz and its implications for past high-energy cosmic ray fluxesSakurai, Hirohisa*; Kurebayashi, Yutaka*; Suzuki, Soichiro*; Horiuchi, Kazuho*; Takahashi, Yui*; Doshita, Norihiro*; Kikuchi, Satoshi*; Tokanai, Fuyuki*; Iwata, Naoyoshi*; Tajima, Yasushi*; et al.
Physical Review D, 109(10), p.102005_1 - 102005_18, 2024/05
Times Cited Count：0 Percentile：0.00(Astronomy & Astrophysics)Secular variations of galactic cosmic rays (GCRs) are inseparably associated with the galactic activities and should reflect the environments of the local galactic magnetic field, interstellar clouds, and nearby supernova remnants. The high-energy muons produced in the atmosphere by high-energy GCRs can penetrate deep underground and generate radioisotopes in the rock. As long lived radionuclides such as Be and Al have been accumulating in these rocks, concentrations of Be and Al can be used to estimate the long-term variations in high-energy muon yields, corresponding to those in the high-energy GCRs over a few million years. This study measured the production cross sections for muon induced Be and Al by irradiating positive muons with the momentum of 160 GeV/c on the synthetic silica plates and the granite core at the COMPASS experiment line in CERN SPS. In addition, it the contributions of the direct muon spallation reaction and the nuclear reactions by muon-induced particles on the production of long lived radionuclides in the rocks were clarified.
Futemma, Akira; Sanada, Yukihisa; Sasaki, Miyuki; Kawasaki, Yoshiharu*; Iwai, Takeyuki*; Hiraga, Shogo*; Haginoya, Masashi*; Matsunaga, Yuki*; Akutsu, Yuichiro*; Arai, Yoshinori*; et al.
JAEA-Technology 2023-026, 161 Pages, 2024/03
JAEA-Technology-2023-026.pdf:14.66MB
By the accident at Tokyo Electric Power Company's (TEPCO's) Fukushima Daiichi Nuclear Power Station (FDNPS), caused by tsunami triggered by the 2011 off the Pacific coast of Tohoku Earthquake, a large amount of radioactive material was released into the surrounding environment. After the accident, Airborne Radiation Monitoring (ARM) via manned helicopter has been utilized as a method to quickly and extensively measure radiation distribution surrounding FDNPS. In order to utilize ARM and to promptly provide the results during a nuclear emergency, information on background radiation levels, topographical features, and controlled airspace surrounding nationwide nuclear facilities have been prepared in advance. In the fiscal year 2022, we conducted ARM around the Mihama Nuclear Power Station of Kansai Electric Power Company (KEPCO), the Tsuruga Power Station of Japan Atomic Power Company (JAPC), and the Ikata Power Station of Shikoku Electric Power Company (YONDEN), and prepared information on background radiation doses and controlled airspace. In addition, we have developed an aerial radiation detection system via unmanned airplane, which is expected to be an alternative to ARM, during a nuclear emergency. This report summarizes the results and technical issues identified.
Futemma, Akira; Sanada, Yukihisa; Sasaki, Miyuki; Kawasaki, Yoshiharu*; Iwai, Takeyuki*; Hiraga, Shogo*; Haginoya, Masashi*; Matsunaga, Yuki*; Akutsu, Yuichiro*; Hokama, Tomonori; et al.
JAEA-Technology 2022-028, 127 Pages, 2023/02
JAEA-Technology-2022-028.pdf:15.21MB
A large amount of radioactive material was released by the nuclear disaster of Fukushima Daiichi Nuclear Power Station (FDNPS), Tokyo Electric Power Company, caused by the Great East Japan Earthquake and the following tsunami on March 11, 2011. After the nuclear disaster, airborne radiation monitoring via manned helicopter has been utilized to grasp rapidly and widely the distribution of the radioactive materials surrounding FDNPS. We prepare the data of background radiation dose, geomorphic characteristics and the controlled airspace surrounding nuclear facilities of the whole country in order to make effective use of the monitoring technique as a way of emergency radiation monitoring and supply the results during an accident of a facility. This report has summarized the knowledge noted above achieved by the aerial radiation monitoring around Ohi and Takahama nuclear power stations. In addition, the examination's progress aimed at introducing airborne radiation monitoring via an unmanned plane during a nuclear disaster and the technical issues are summarized in this report.
Sr and 
Cs by AMSHonda, Maki; Martschini, M.*; Wieser, A.*; Marchhart, O.*; Lachner, J.*; Priller, A.*; Steier, P.*; Golser, R.*; Sakaguchi, Aya*
JAEA-Conf 2022-001, p.85 - 90, 2022/11
Accelerator mass spectrometry (AMS) is an analytical method that combines mass spectrometry with a tandem accelerator, which has been used mainly in nuclear physics experiments. AMS is used to measure radionuclides with half-lives of 10
-10
years. For radionuclides with half-lives of this order, the method of measuring their mass is 10-10
times more sensitive than measuring their activity. Because of this advantage, AMS has been widely applied in Earth and planetary sciences, atomic energy research, and other fields. Among the various studies, Wallner et al. (2021, 2016) have achieved excellent work in Earth and planetary sciences. For example, they have attained the ultra-sensitive analysis of 
Fe and 
Pu in environmental samples. These are radionuclides produced by rapid-neutron-capture (
-process) nucleosynthesis. Our recent work shows that a new AMS system (VERA, University of Vienna), which combines laser isobaric separation and a typical AMS system, has been successfully applied to the ultra-sensitive determination of Sr and Cs in environment. For Sr in environmental samples, the 
-ray measurement by the milking of the daughter nuclide Y is still the principal method, which takes 3-6 weeks. The new AMS method has a detection limit of 
0.1 mBq, which is comparable to that of -ray measurement, with a more straightforward chemical treatment than -measurement. Our achievement demonstrates that AMS can be a practical new method for determining Sr in the environment.
Shimada, Asako; Taniguchi, Yoshinori; Kakiuchi, Kazuo; Ohira, Saki; Iida, Yoshihisa; Sugiyama, Tomoyuki; Amaya, Masaki; Maruyama, Yu
Scientific Reports (Internet), 12(1), p.2086_1 - 2086_11, 2022/02
Times Cited Count：3 Percentile：28.39(Multidisciplinary Sciences)no abstracts in English
Futemma, Akira; Sanada, Yukihisa; Sasaki, Miyuki; Kawasaki, Yoshiharu*; Iwai, Takeyuki*; Hiraga, Shogo*; Sato, Kazuhiko*; Haginoya, Masashi*; Matsunaga, Yuki*; Kikuchi, Hikaru*; et al.
JAEA-Technology 2021-020, 138 Pages, 2021/11
JAEA-Technology-2021-020.pdf:17.11MB
A large amount of radioactive material was released by the nuclear disaster of Fukushima Daiichi Nuclear Power Station (FDNPS), Tokyo Electric Power Company, caused by the Great East Japan Earthquake and the following tsunami on March 11, 2011. After the nuclear disaster, airborne radiation monitoring via manned helicopter has been utilized to grasp rapidly and widely the distribution of the radioactive materials surrounding FDNPS. We prepare the data of background radiation dose, geomorphic characteristics and the controlled airspace surrounding nuclear facilities of the whole country in order to make effective use of the monitoring technique as a way of emergency radiation monitoring and supply the results during an accident of a facility. This report is summarized that the knowledge as noted above achieved by the aerial radiation monitoring around Tsuruga and Mihama nuclear power station, research reactors in Kindai University Atomic Energy Research Institute and Institute for Integrated Radiation and Nuclear Science, Kyoto University. In addition, examination's progress aimed at introduction of airborne radiation monitoring via unmanned plane during nuclear disaster and the technical issues are summarized in this report.
Okumura, Keisuke
Fission Product Behavior under Severe Accident, p.70 - 72, 2021/05
no abstracts in English
Futemma, Akira; Sanada, Yukihisa; Kawasaki, Yoshiharu*; Iwai, Takeyuki*; Hiraga, Shogo*; Sato, Kazuhiko*; Haginoya, Masashi*; Matsunaga, Yuki*; Kikuchi, Hikaru*; Ishizaki, Azusa; et al.
JAEA-Technology 2020-019, 128 Pages, 2021/02
JAEA-Technology-2020-019.pdf:15.75MB
A large amount of radioactive material was released by the nuclear disaster of Fukushima Daiichi Nuclear Power Station (FDNPS), Tokyo Electric Power Company, caused by the Great East Japan Earthquake and the following tsunami on March 11, 2011. After the nuclear disaster, airborne radiation monitoring using manned helicopter has been utilized to grasp rapidly and widely the distribution of the radioactive materials around FDNPS. We prepare the data of background radiation dose, geomorphic characteristics and the controlled airspace around nuclear facilities of the whole country in order to make effective use of the monitoring technique as a way of emergency radiation monitoring and supply the results during accidents of the facilities. Furthermore, the airborne radiation monitoring has been conducted in Integrated Nuclear Emergency Response Drill to increase effectiveness of the monitoring. This report is summarized that the knowledge as noted above achieved by the aerial radiation monitoring around Higashidori nuclear power station, the nuclear fuel reprocessing plant in Rokkasho village and Shika nuclear power station, the full details of the aerial radiation monitoring in Integrated Nuclear Emergency Response Drill in the fiscal 2019. In addition, examination's progress aimed at introduction of airborne radiation monitoring using unmanned helicopter during nuclear disaster and the technical issues are summarized in this report.
Onuki, Toshihiko*; Ozaki, Takuo*; Kozai, Naofumi; Utsunomiya, Satoshi*
Behavior of Radionuclides in the Environment I; Function of Particles in Aquatic System, p.67 - 92, 2020/00
It has been experimentally revealed that microorganisms transform radionuclides. For example, cells of microorganisms such as bacteria and yeast accumulate actinides on the surface. Phosphate ions released from microorganism cells precipitate actinides as phosphates. This chapter discusses the role of environmental microorganisms on migration of actinides in the groundwater around Lake Karachai where a lot of radioactive wastes from nuclear facilities of the Soviet Union.
Tanaka, Kazuya; Kaplan, D. I.*; Onuki, Toshihiko
Applied Geochemistry, 85(Part B), p.119 - 120, 2017/10
Times Cited Count：0 Percentile：0.00(Geochemistry & Geophysics)We have prepared a special issue for Applied Geochemistry entitled "Transformation and Fate of Natural and Anthropogenic Radionuclides in the Environments". Here, we present 13 peer-reviewed articles on the general theme of natural and anthropogenic radionuclides in different environments. At the same time, these articles cover various topics of field research on the distribution of radionuclides, as well as laboratory experiments on adsorption and redox chemistry of these. The articles have been written by the attendees of the session at the Goldschmidt 2016 held in Yokohama, Japan, and by other authors who submitted their manuscripts to Applied Geochemistry focusing on the theme of the special issue.
Asai, Shiho; Saito, Kyoichi*
Biomedical Research on Trace Elements, 28(1), p.1 - 10, 2017/04
Radionuclides are commonly determined with radiometry and mass spectrometry. For 
-emitting nuclides, the activities can be measured without chemical separation due to the strong penetration ability. In contrast, the measurements of alpha and beta-emitting nuclides are generally associated with tedious and time-consuming chemical separation procedures to remove concomitants. Thus, an adsorbent that achieves rapid separation is desirable to reduce separation time and workload. Our research team has developed compact cartridge-type solid phase extraction materials which enable to facilitate separation procedures. In this review, basic separation performances of the developed cartridges were overviewed along with two application examples to radionuclide-containing samples.
Yamamoto, Yoichi
Isotope News, (736), p.31 - 33, 2015/08
The Takasaki radionuclide (RN) station for the Comprehensive Nuclear-Test-Ban Treaty (CTBT) has been in operation for monitoring of radioactive noble gases (radioxenon) by the Japan Atomic Energy Agency (JAEA) since 2007, first as a test run prior to receiving the certification. The noble gas system in the station was certified by the CTBT Organization (CTBTO) on December 19, 2014. Monitoring of radioxenon is expected to have a particularly valuable role in detection of an underground nuclear test. The Takasaki RN station detected radioxenon isotopes simultaneously with radioactive concentration exceeding normal background range in April, 2013. This abnormal event was identified as being associated with the nuclear test declared by North Korea in February, 2013. Since the Takasaki RN station is located at the east end of Asia, it is receiving widespread international attention as the station for radionuclides dispersed by the westerlies.
Saito, Kimiaki; Onda, Yuichi*
Journal of Environmental Radioactivity, 139, p.240 - 249, 2015/01
Times Cited Count：56 Percentile：92.23(Environmental Sciences)no abstracts in English
Nagai, Haruyasu; Kurihara, Osamu*
Nihon Genshiryoku Gakkai-Shi ATOMO
, 56(12), p.791 - 795, 2014/12
no abstracts in English
Nagaishi, Ryuji; Morita, Keisuke; Yamagishi, Isao; Hino, Ryutaro; Ogawa, Toru
Proceedings of 2014 Nuclear Plant Chemistry Conference (NPC 2014) (USB Flash Drive), 9 Pages, 2014/10
Two years after Three Mile Island Unit 2 (TMI-2) loss-of-coolant accident, radioactive contaminated water has been processed by Submerged Demineralizer System (SDS) with two types of zeolite adsorbents to remove radioactive nuclides. During and after the process, adsorption amount and distribution of nuclides on the zeolites, residual water content and thermal conductivity in the SDS vessels have been measured or estimated for verification of safety in the process, subsequent transportation and disposal. Hydrogen generation has been also evaluated mainly by direct monitoring in the large-scale of vessel after the process. In this work, the revaluation of hydrogen generation was demonstrated on the basis of the open information of vessel, and the latest experimental data obtained in adsorption and radiolysis occurring in small-scale of zeolite-water mixtures. As a result, the evaluated data was found to be comparable with the reported data obtained in the large-scale of real vessel.
Otosaka, Shigeyoshi; Amano, Hikaru; Ito, Toshimichi; Kawamura, Hideyuki; Kobayashi, Takuya; Suzuki, Takashi; Togawa, Orihiko; Chaykovskaya, E. L.*; Lishavskaya, T. S.*; Novichkov, V. P.*; et al.
Journal of Environmental Radioactivity, 91(3), p.128 - 145, 2006/00
Times Cited Count：21 Percentile：42.42(Environmental Sciences)Distributions of radionuclides (Sr, 
Cs and 
Pu) in seabed sediment in the Japan Sea were observed during 1998-2002. Observed inventories of anthropogenic radionuclides in sediment ranged 0.1-86 Bq m
for Sr, 23-379 Bq m for Cs and 0.1-86 Bq m for Pu. In the deep part (
2 km depth) of the western Japan Basin, Pu/Cs inventory ratios were larger than those in the central Yamato Basin although inventories of radionuclides were not different between basins. The higher Pu/Cs ratios in the western Japan Basin were derived by the production of Pu-enriched particle in the surface layer and effective sinking of particulate materials in this region. In the marginal Yamato Basin and the Ulleung Basin, both inventories and Pu/Cs ratios in sediment were larger than those in the central Yamato Basin. In the eastern/southern Japan Sea, it was suggested that the supply of particulate radionuclides by the TWC enhanced accumulation of radionuclides in this region.
