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Hg region; Derivative analysis approachKattikat Melcom, D. T.*; Tsekhanovich, I.*; Guezet, F.*; Andreyev, A.*; Nishio, Katsuhisa
Physical Review C, 114(1), p.014627_1 - 014627_8, 2026/07
Times Cited Count：0 Percentile：0.00(Physics, Nuclear)Batsaikhan, M.; Oba, Hironori*; Karino, Takahiro; Akaoka, Katsuaki; Wakaida, Ikuo*; Iwata, Yoshihiro; Sakamoto, Kan*
Journal of Analytical Atomic Spectrometry, 41(4), p.1324 - 1335, 2026/04
Times Cited Count：0 Percentile：0.00(Chemistry, Analytical)Kam, D. H.*; Grabaskas, D.*; Okano, Yasushi; Uchibori, Akihiro; Starkus, T.*
Nuclear Technology, 212(2), p.347 - 364, 2026/02
Times Cited Count：0 Percentile：0.00(Nuclear Science & Technology)Nakamura, Yuki*; Kojima, Yoshihiro*; Yamashita, Takuya; Shimomura, Kenta; Mizokami, Shinya
Journal of Nuclear Science and Technology, 62(12), p.1226 - 1230, 2025/12
Times Cited Count：0 Percentile：0.00(Nuclear Science & Technology)Collaborative Laboratories for Advanced Decommissioning Science; Institute of Science Tokyo*
JAEA-Review 2025-012, 96 Pages, 2025/10
JAEA-Review-2025-012.pdf:3.99MB
JAEA/CLADS had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). Among the adopted proposals in FY2021, this report summarizes the research results of the "Uncertainty reduction of the FPs transport mechanism and debris degradation behavior and evaluation of the reactor contamination of debris state on the basis of the accident progression scenario of Fukushima Daiichi Nuclear Power Station unit 2 and 3" conducted from FY2021 to FY2023. The present study aims to elucidate the cause of the high dosage under shield plug by clarification of to the cesium behavior of migration, adhesion to structure and deposition as well as evaluate the properties of metal-rich debris predeceasing melted through the materials science approach based on the most probable scenario of accident progression of Unit 2 and 3. Through three years investigation, chemi-absorption configuration of Cs has been elucidated to change with acidity of steel surface during oxidation in humid atmosphere and Cs
O trapping compound as well as penetration depth have found to be importantly considered. For metallic debris, solid oxidation was found to be controlled by Fe
O
formation and molten state was found to tend to preferentially yield ZrO resulting in formation of slate structure during solidification. Present findings obtained are contributing to better improve the accuracy of accident progression scenario in FDNPP in viewpoint of backward analysis.
Takagi, Shinya*; Harada, Sota*; Aritomo, Yoshihiro*; Hirose, Kentaro; Nishio, Katsuhisa
Physical Review C, 112(4), p.044607_1 - 044607_9, 2025/10
Times Cited Count：0 Percentile：0.00(Physics, Nuclear)Taniguchi, Yoshinori; Urano, Kenta; Mihara, Takeshi; Udagawa, Yutaka; Kakiuchi, Kazuo; Katsuyama, Jinya
Proceedings of TopFuel 2025; Nuclear Reactor Fuel Performance Conference (Internet), p.1292 - 1301, 2025/10
Pshenichnikov, A.; Ogi, Hiroshi; Zubekhina, B.; Pham, V. H.
Abstracts of the Technical Poster Session; 9th International Forum on the Decommissioning of the Fukushima Daiichi Nuclear Power Station (Internet), 1 Pages, 2025/08
Takagi, Shinya*; Aritomo, Yoshihiro*; Nakajima, Kota*; Okada, Kazuki; Hirose, Kentaro; Nishio, Katsuhisa
Physical Review C, 112(1), p.014608_1 - 014608_7, 2025/07
Times Cited Count：0 Percentile：0.00(Physics, Nuclear)Katsumura, Kosuke*; Takagi, Junichi*; Miyahara, Naoya*; Uchida, Shunsuke*; Koma, Yoshikazu; Karasawa, Hidetoshi; Miwa, Shuhei; Satou, Yukihiko; Nagai, Haruyasu; Kurata, Masaki; et al.
Nihon Genshiryoku Gakkai-Shi ATOMO
, 67(2), p.128 - 132, 2025/02
no abstracts in English
Matsumura, Taichi; Okumura, Keisuke; Sakamoto, Masahiro; Terashima, Kenichi; Riyana, E. S.; Kondo, Kazuhiro*
Nuclear Engineering and Design, 432, p.113791_1 - 113791_9, 2025/02
Times Cited Count：3 Percentile：49.06(Nuclear Science & Technology)Collaborative Laboratories for Advanced Decommissioning Science; Tokyo Institute of Technology*
JAEA-Review 2024-010, 112 Pages, 2024/08
JAEA-Review-2024-010.pdf:6.49MB
The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2022. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2021, this report summarizes the research results of the "Uncertainty reduction of the FPs transport mechanism and debris degradation behavior and evaluation of the reactor contamination of debris state on the basis of the accident progression scenario of Fukushima Daiichi Nuclear Power Station Unit 2 and 3" conducted in FY2022. The present study aims to elucidate the cause of the high dosage under shield plug by clarification of to the cesium behavior of migration, adhesion to structure and deposition as well as evaluate the properties of metal-rich debris predeceasing melted through the materials science approach based on the most probable scenario of accident progression of Unit 2 and 3. In this fiscal year, the followings were achieved.
-rays from slow neutron-induced fission of 
U with STEFFWright, T.*; Harada, Hideo; Kimura, Atsushi; 121 of others*
European Physical Journal A, 60(3), p.70_1 - 70_11, 2024/03
Times Cited Count：0 Percentile：0.00(Physics, Nuclear)Riyana, E. S.; Okumura, Keisuke; Sakamoto, Masahiro; Matsumura, Taichi; Terashima, Kenichi; Kanno, Ikuo
Journal of Nuclear Science and Technology, 61(2), p.269 - 276, 2024/02
Times Cited Count：0 Percentile：0.00(Nuclear Science & Technology)Horii, Yuta; Hirooka, Shun; Uno, Hiroki*; Ogasawara, Masahiro*; Tamura, Tetsuya*; Yamada, Tadahisa*; Furusawa, Naoya*; Murakami, Tatsutoshi; Kato, Masato
Journal of Nuclear Materials, 588, p.154799_1 - 154799_20, 2024/01
Times Cited Count：8 Percentile：74.73(Materials Science, Multidisciplinary)The thermal conductivities of near-stoichiometric (U,Pu,Am)O doped with NdO/SmO, which is major fission product (FP) generated by a uranium-plutonium mixed oxides (MOX) fuel irradiation, as simulated fission products are evaluated at 1073-1673 K. The thermal conductivities are calculated from the thermal diffusivities that are measured using the laser flash method. To evaluate the thermal conductivity from a homogeneity viewpoint of Nd/Sm cations in MOX, the specimens with different homogeneity of Nd/Sm are prepared using two kinds of powder made by ball-mill and fusion methods. A homogeneous Nd/Sm distribution decreases the thermal conductivity of MOX with increasing Nd/Sm content, whereas heterogeneous Nd/Sm has no influence. The effect of Nd/Sm on the thermal conductivity is studied using the classical phonon transport model (A+BT)
. The dependences of the coefficients A and B on the Nd/Sm content (C
and C
, respectively) are evaluated as: A(mK/W)=1.70 
10
+ 0.93C + 1.20C, B(m/W)=2.39 10
.
Konno, Chikara
Journal of Nuclear Science and Technology, 61(1), p.121 - 126, 2024/01
Times Cited Count：2 Percentile：24.52(Nuclear Science & Technology)The JENDL-4.0/HE neutron and proton ACE files were produced in 2017 and those of 22 nuclei for neutron and 25 nuclei for proton were bundled in the PHITS code. Recently it was found that the following five data in the JENDL-4.0/HE neutron and proton ACE files had any problems; ACE files for 
N and 
O, heating numbers, damage energy production cross sections, secondary neutron multiplicities and fission cross sections. Thus new JENDL-4.0/HE neutron and proton ACE files were produced with the problems fixed. This paper describes the problems and how to produce the new neutron and proton ACE files in detail.
Tuya, D.; Nagaya, Yasunobu
Journal of Nuclear Engineering (Internet), 4(4), p.691 - 710, 2023/11
The Monte Carlo method is used to accurately estimate various quantities such as k-eigenvalue and integral neutron flux. However, when a distribution of a quantity is desired, the Monte Carlo method does not typically provide continuous distribution. Recently, the functional expansion tally and kernel density estimation methods have been developed to provide continuous distribution. In this paper, we propose a method to estimate a continuous distribution of a quantity using artificial neural network (ANN) model with Monte Carlo-based training data. As a proof of concept, a continuous distribution of iterated fission probability (IFP) is estimated by ANN models in two systems. The IFP distributions by the ANN models were compared with the Monte Carlo-based data and the adjoint angular neutron fluxes by the PARTISN code. The comparisons showed varying degrees of agreement or discrepancy; however, it was observed that the ANN models learned the general trend of the IFP distributions.
Hirooka, Shun; Horii, Yuta; Sunaoshi, Takeo*; Uno, Hiroki*; Yamada, Tadahisa*; Vauchy, R.; Hayashizaki, Kohei; Nakamichi, Shinya; Murakami, Tatsutoshi; Kato, Masato
Journal of Nuclear Science and Technology, 60(11), p.1313 - 1323, 2023/11
Times Cited Count：5 Percentile：56.11(Nuclear Science & Technology)Additive MOX pellets are fabricated by a conventional dry powder metallurgy method. NdO and SmO are chosen as the additive materials to simulate the corresponding soluble fission products dispersed in MOX. Shrinkage curves of the MOX pellets are obtained by dilatometry, which reveal that the sintering temperature is shifted toward a value higher than that of the respective regular MOX. The additives, however, promote grain growth and densification, which can be explained by the effect of oxidized uranium cations covering to a pentavalent state. Ceramography reveals large agglomerates after sintering, and Electron Probe Micro-Analysis confirms that inhomogeneous elemental distribution, whereas XRD reveals a single face-centered cubic phase. Finally, by grinding and re-sintering the specimens, the cation distribution homogeneity is significantly improved, which can simulate spent nuclear fuels with soluble fission products.
Katsumura, Kosuke*; Takagi, Junichi*; Hosomi, Kenji*; Miyahara, Naoya*; Koma, Yoshikazu; Imoto, Jumpei; Karasawa, Hidetoshi; Miwa, Shuhei; Shiotsu, Hiroyuki; Hidaka, Akihide*; et al.
Nihon Genshiryoku Gakkai-Shi ATOMO, 65(11), p.674 - 679, 2023/11
no abstracts in English
Fukahori, Tokio
INDC(JPN)-210 (Internet), 5 Pages, 2023/10
The U(n,f) cross section values were not correctly compiled in the ENDF format, and wrong values are disseminated in the JENDL/HE-2007 file. The high energy part of the U(n,f) cross section for the JENDL/HE-2007 library was evaluated by using the results of the FISCAL code. The correct U(n,f) cross section values of the JENDL/HE-2007 library above 200 MeV is given in this report.
