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Kitagaki, Toru; Krasnov, V.*; Ikeda, Atsushi
Journal of Nuclear Materials, 576, p.154224_1 - 154224_14, 2023/04
Times Cited Count:0Dong, F.*; Chen, S.*; Demachi, Kazuyuki*; Yoshikawa, Masanori; Seki, Akiyuki; Takaya, Shigeru
Nuclear Engineering and Design, 404, p.112161_1 - 112161_15, 2023/04
Times Cited Count:0Collaborative Laboratories for Advanced Decommissioning Science; Tokyo Institute of Technology*
JAEA-Review 2022-072, 116 Pages, 2023/03
The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2021. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station (1F), Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2021, this report summarizes the research results of the "Challenge of novel hybrid-waste-solidification of mobile nuclei generated in Fukushima Nuclear Power Station and establishment of rational disposal concept and its safety assessment" conducted in FY2021. The present study aims to establish the rational waste disposal concept of a variety of wastes generated in 1F by the novel hybrid-waste-solidification. The phosphate form of ALPS sediment wastes containing Eu, Ce
, Sr
and Cs
were synthesized as well as radioactive
Sr,
Cs and
I which are both
emitters, AREVA sludge and Iodine Calcium apatite were synthesized, and they were processed to the stabilization treatment such as sintering and Spark Plasma
Collaborative Laboratories for Advanced Decommissioning Science; Tohoku University*
JAEA-Review 2022-071, 123 Pages, 2023/03
The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2021. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2021, this report summarizes the research results of the "Development of a hybrid method for evaluating the long-term structural soundness of nuclear reactor buildings using response monitoring and damage imaging technologies" conducted in FY2021. The present study aims to develop an evaluation method necessary to obtain a perspective on the long-term structural soundness of accident-damaged reactor buildings, where accessibility to work sites is extremely limited due to high radiation dose rate and high contamination. In FY2021, the first year of the three-year plan, the following research items were undertaken by clarifying specific research methods, setting research directions, making necessary preparations, and conducting some tests and other activities.
Collaborative Laboratories for Advanced Decommissioning Science; National Institute of Maritime, Port and Aviation Technology*
JAEA-Review 2022-070, 70 Pages, 2023/03
The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2021. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2020, this report summarizes the research results of the "Research and development of the sample-return technique for fuel debris using the unmanned underwater vehicle" conducted in FY2021. The present study aims to develop a fuel debris sampling device that comprises a neutron detector with radiation resistance and enhanced neutron detection efficiency, an end-effector with powerful cutting and collection capabilities, and a manipulator under the Japan-UK joint research team. We will also develop a fuel debris sampling system that can be mounted on an unmanned vehicle. In addition, we will develop a positioning system to identify the system position, and a technique to project the counting information of optical cameras, sonar, and neutron detectors to be developed
Collaborative Laboratories for Advanced Decommissioning Science; Tohoku University*
JAEA-Review 2022-069, 114 Pages, 2023/03
The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2021. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station (1F), Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2020, this report summarizes the research results of the "Development of a new corrosion mitigation technology using nanobubbles toward corrosion mitigation in PCV system under the influence of /
/
-rays radiolysis" conducted in FY2021. In this work, in order to ensure the long-term reliability of steel structures that ensure important confinement functions in the debris removal process, such as existing PCVs and newly constructed negative pressure maintenance systems and piping, corrosion phenomena in wet environments where
- and
-ray emitting nuclides come into contact with steel are clarified for the first time. At the same time, we will develop a new corrosion prevention technology that has excellent basic applicability to PCVs
Opletal, P.; Sakai, Hironori; Haga, Yoshinori; Tokiwa, Yoshifumi; Yamamoto, Etsuji; Kambe, Shinsaku; Tokunaga, Yo
Journal of the Physical Society of Japan, 92(3), p.034704_1 - 034704_5, 2023/03
We investigate the physical properties of a single crystal of uranium telluride UTe
. We have confirmed that U
Te
crystallizes in the hexagonal structure with three nonequivalent crystallographic uranium sites. The paramagnetic moments are estimated to be approximately 1
per the uranium site, assuming a uniform moment on all the sites. A ferromagnetic phase transition occurs at
= 48 K, where the in-plane magnetization increases sharply, whereas the out of-plane component does not increase significantly. With decreasing temperature further below
under field-cooling conditions, the out-of-plane component increases rapidly around T
= 26 K. In contrast, the in-plane component hardly changes at T
. Specific heat measurement indicates no
-type anomaly around T
, so this is a cross-over suggesting a reorientation of the ordering moments or successive magnetic ordering on the part of the multiple uranium sites.
Maamoun, I.; Rushdi, M.*; Falyouna, O.*; Eljamal, R.*; Eljamal, O.*
Separation and Purification Technology, 308, p.122863_1 - 122863_16, 2023/03
Times Cited Count:0 Percentile:0(Engineering, Chemical)Yanagisawa, Hiroshi; Umeda, Miki; Motome, Yuiko; Murao, Hiroyuki
JAEA-Technology 2022-030, 80 Pages, 2023/02
Nuclear criticality benchmark analyses were carried out for TRIGA-type reactor systems in which uranium-zirconium hydride fuel rods are loaded by using the continuous-energy Monte Carlo code MVP with the evaluated nuclear data library JENDL-5. The analyses cover two sorts of benchmark data, the IEU-COMP-THERM-003 and IEU-COMP-THERM-013 in the International Criticality Safety Benchmark Evaluation Project (ICSBEP) Handbook, and effective neutron multiplication factors, reactivity worths for control rods etc. were calculated by JENDL-5 in comparison with those by the previous version of JENDL. As the results, it was confirmed that the effective neutron multiplication factors obtained by JENDL-5 were 0.4 to 0.6% greater than those by JENDL-4.0, and that there were no significant differences in the calculated reactivity worths by between JENDL-5 and JENDL-4.0. Those results are considered to be helpful for the confirmation of calculation accuracy in the analyses on NSRR control rod worths, which are planned in the future.
Nagata, Hiroshi; Otsuka, Kaoru; Omori, Takazumi; Hanakawa, Hiroki; Ide, Hiroshi
JAEA-Technology 2022-029, 55 Pages, 2023/02
Japan Materials Testing Reactor (JMTR) was decided as a one of decommission facilities in April 2017. The activation activity of secondary radioactive contamination remaining in the reactor facility was evaluated in order to submit the decommissioning plan to the Nuclear Regulation Authority. Total activation activity was 2.7310
Bq after 12 years, 1.46
10
Bq after 21 years, respectively. The system with high activation activity was the primary cooling system in JMTR. The relatively large radionuclide was H-3, Fe-55, Co-60, Ni-63, Sr-90 and Cs-137. The radioactivity level was classified based on the values of the obtained radioactivity concentration. As a result, the primary cooling system and the drain system was classified as L2, and others was classified as L3. The nuclide that affected classification result was only Co-60 in irradiation facility of HR-1 and OSF-1. H-3, Co-60, Sr-90, Cs-137 and so on were affected classification in other system. When treating and disposing of radioactive waste, evaluation will be carried out based on appropriate methods.
Futemma, Akira; Sanada, Yukihisa; Sasaki, Miyuki; Kawasaki, Yoshiharu*; Iwai, Takeyuki*; Hiraga, Shogo*; Haginoya, Masashi*; Matsunaga, Yuki*; Akutsu, Yuichiro*; Hokama, Tomonori; et al.
JAEA-Technology 2022-028, 127 Pages, 2023/02
A large amount of radioactive material was released by the nuclear disaster of Fukushima Daiichi Nuclear Power Station (FDNPS), Tokyo Electric Power Company, caused by the Great East Japan Earthquake and the following tsunami on March 11, 2011. After the nuclear disaster, airborne radiation monitoring via manned helicopter has been utilized to grasp rapidly and widely the distribution of the radioactive materials surrounding FDNPS. We prepare the data of background radiation dose, geomorphic characteristics and the controlled airspace surrounding nuclear facilities of the whole country in order to make effective use of the monitoring technique as a way of emergency radiation monitoring and supply the results during an accident of a facility. This report has summarized the knowledge noted above achieved by the aerial radiation monitoring around Ohi and Takahama nuclear power stations. In addition, the examination's progress aimed at introducing airborne radiation monitoring via an unmanned plane during a nuclear disaster and the technical issues are summarized in this report.
Futemma, Akira; Sanada, Yukihisa; Nagakubo, Azusa; Kawasaki, Yoshiharu*; Iwai, Takeyuki*; Hiraga, Shogo*; Haginoya, Masashi*; Matsunaga, Yuki*; Akutsu, Yuichiro*; Urabe, Yoshimi*; et al.
JAEA-Technology 2022-027, 148 Pages, 2023/02
By the nuclear disaster of Fukushima Daiichi Nuclear Power Station (FDNPS), Tokyo Electric Power Company (TEPCO), caused by the Great East Japan Earthquake and the following tsunami on March 11, 2011, a large amount of radioactive material was released from the FDNPS. After the nuclear disaster, airborne radiation monitoring via manned helicopter has been conducted around FDNPS. The results of the airborne radiation monitoring and the evaluation for temporal change of dose rate in the fiscal 2021 were summarized in this report. Analysis considering topographical effects was applied to the result of the airborne monitoring to improve the accuracy of the conventional method. In addition, technique for discriminating gamma rays from the ground and those from the airborne Rn-progenies was also utilized to evaluate their effect on airborne radiation monitoring.
Collaborative Laboratories for Advanced Decommissioning Science; The University of Tokyo*
JAEA-Review 2022-061, 59 Pages, 2023/02
The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2021. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2021, this report summarizes the research results of the "Research on radioactive aerosol control and decontamination at Fukushima Daiichi Nuclear Power Station decommissioning" conducted in FY2021. The present study aims to develop a safe laser decontamination system that simultaneously incorporates an advanced particle detection and characterization system together with aerosol dispersion control in collaboration with the UK researchers. By using the UK partner's fundamental studies related to aerosol and water interface interactions, various methods such as electro-chemical processing of water-mist particles and spray droplets will be applied for effective control of ultra-fine aerosol particle dispersions in a large containment volume. With the help of advanced aerosol
Collaborative Laboratories for Advanced Decommissioning Science; Waseda University*
JAEA-Review 2022-054, 150 Pages, 2023/02
The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2021. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (hereafter referred to "1F"). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2019, this report summarizes the research results of the "Estimation of the in-depth debris status of Fukushima Unit-2 and Unit-3 with multi-physics modeling" conducted from FY2019 to FY2021. Since the final year of this proposal was FY2021, the results for three fiscal years were summarized. Continuous update on understanding of the damaged 1F reactors is important for safe and efficient decommissioning of the reactors. This study aimed to estimate the in-depth debris status of the damaged 1F Unit-2 and Unit-3 through multi-physics modeling, which comprises of MPS method, simulated molten debris relocation experiment and high-temperature melt property data acquisition in the three-year project from FY2019. As the results, a new insight has been gained
Collaborative Laboratories for Advanced Decommissioning Science; Tokyo Institute of Technology*
JAEA-Review 2022-053, 89 Pages, 2023/02
The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2021. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2021, this report summarizes the research results of the "Uncertainty reduction of the FPs transport mechanism and debris degradation behavior and evaluation of the reactor contamination of debris state on the basis of the accident progression scenario of Fukushima Daiichi Nuclear Power Station Unit 2 and 3" conducted in FY2021. The present study aims to elucidate the cause of the high dosage under shield plug by clarification of to the cesium behavior of migration, adhesion to structure and deposition as well as evaluate the properties of metal-rich debris predeceasing melted through the materials science approach based on the most probable scenario of accident progression of Unit 2 and 3. In this fiscal year, the followings were achieved. Chemical configuration and
Sakai, Akihiro
Dai-33-Kai Genshiryoku Shisetsu Dekomisshoningu Gijutsu Koza Tekisuto, p.31 - 63, 2023/02
The Japan Atomic Energy Agency (JAEA) is promoting the project for concrete-vault disposal and landfill-type disposal of radioactive waste generated from research facilities, etc. This report introduces current status of technical development for JAEA's disposal project as following items; (1) kinds of research facilities and characteristics of radioactivity inventory of the waste, (2) the structures of the disposal facilities which JAEA conceptually designed, (3) development of waste acceptance criteria for major radioactive waste for the JAEA disposal facilities, (4) the concept of the criteria for disposal of uranium bearing waste, that has been established in 2021.
Kido, Kentaro; Kaneko, Masashi
Journal of Computational Chemistry, 44(4), p.546 - 558, 2023/02
Times Cited Count:0 Percentile:0(Chemistry, Multidisciplinary)Okubo, Takahiro*; Takei, Akihiro*; Tachi, Yukio; Fukatsu, Yuta; Deguchi, Kenzo*; Oki, Shinobu*; Shimizu, Tadashi*
Journal of Physical Chemistry A, 127(4), p.973 - 986, 2023/02
Times Cited Count:0The identification of adsorption sites of Cs on clay minerals has been studied in the fields of environmental chemistry. The nuclear magnetic resonance (NMR) experiments allow direct observations of the local structures of adsorbed Cs. The NMR parameters of Cs, derived from solid-state NMR experiments, are sensitive to the local neighboring structures of adsorbed Cs. However, determining the Cs positions from NMR data alone is difficult. This paper describes an approach for identifying the expected atomic positions of Cs adsorbed on clay minerals by combining machine learning (ML) with experimentally observed chemical shifts. A linear ridge regression model for ML is constructed from the smooth overlap of atomic positions descriptor and gauge-including projector augmented wave (GIPAW) ab initio data. The
Cs chemical shifts can be instantaneously calculated from the Cs positions on any clay layers using ML. The inverse analysis from the ML model can derive the atomic positions from experimentally observed chemical shifts.
Fukahori, Tokio
Kaku Deta Nyusu (Internet), (134), p.34 - 45, 2023/02
On the occasion of the 60th anniversary of the founding of the Sigma Committee in the Atomic Energy Society of Japan, we will attempt to record and preserve its history as a reference for future activities.
Vauchy, R.; Hirooka, Shun; Watanabe, Masashi; Kato, Masato
Scientific Reports (Internet), 13, p.2217_1 - 2217_8, 2023/02