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Journal Articles

Journal Articles

The Kinetics and mechanism of H$$_{2}$$O$$_{2}$$ decomposition at the U$$_{3}$$O$$_{8}$$ surface in bicarbonate solution

McGrady, J.; Kumagai, Yuta; Watanabe, Masayuki; Kirishima, Akira*; Akiyama, Daisuke*; Kitamura, Akira; Kimuro, Shingo

RSC Advances (Internet), 11(46), p.28940 - 28948, 2021/08

 Times Cited Count:0

JAEA Reports

Technical basis of ECCS acceptance criteria for light-water reactors and applicability to high burnup fuel

Nagase, Fumihisa; Narukawa, Takafumi; Amaya, Masaki

JAEA-Review 2020-076, 129 Pages, 2021/03


Each light-water reactor (LWR) is equipped with the Emergency Core Cooling System (ECCS) to maintain the coolability of the reactor core and to suppress the release of radioactive fission products to the environment even in a loss-of-coolant accident (LOCA) caused by breaks in the reactor coolant pressure boundary. The acceptance criteria for ECCS have been established in order to evaluate the ECCS performance and confirm the sufficient safety margin in the evaluation. The limits defined in the criteria were determined in 1975 and reviewed based on state-of-the-art knowledge in 1981. Though the fuel burnup extension and necessary improvements of cladding materials and fuel design have been conducted, the criteria have not been reviewed since then. Meanwhile, much technical knowledge has been accumulated regarding the behavior of high-burnup fuel during LOCAs and the applicability of the criteria to the high-burnup fuel. This report provides a comprehensive review of the history and technical bases of the current criteria and summarizes state-of-the-art technical findings regarding the fuel behavior during LOCAs. The applicability of the current criteria to the high-burnup fuel is also discussed.

Journal Articles

Corrosion property of container using hybrid material for thermal decomposition process of sulfuric acid

Ioka, Ikuo; Kuriki, Yoshiro*; Iwatsuki, Jin; Kawai, Daisuke*; Yokota, Hiroki*; Inagaki, Yoshiyuki; Kubo, Shinji

Proceedings of 2020 International Conference on Nuclear Engineering (ICONE 2020) (Internet), 5 Pages, 2020/08

A thermochemical water-splitting iodine-sulfur processes (IS process) is one of candidates for the large-scale production of hydrogen using heat from solar power. Severe corrosive environment which is thermal decomposition of sulfuric acid exists in the IS process. A hybrid material with the corrosion-resistance and the ductility was made by a plasma spraying and laser treatment. The specimen had excellent corrosion resistance in the condition of 95 mass% boiling sulfuric acid. This was attributed to the formation of SiO$$_{2}$$ on the surface. The container using the hybrid material was experimentally made. The pre-oxidized container using hybrid technique was prepared for the corrosion test in boiling sulfuric acid to evaluate the corrosion characteristics of the container. There was no detaching of the surface with the weld part and the R processing. We proposed the calculation method of corrosion rate from the ions dissolved in the sulfuric acid solution after the corrosion test.

Journal Articles

Oxidation kinetics of silicon carbide in steam at temperature range of 1400 to 1800$$^{circ}$$C studied by laser heating

Pham, V. H.; Nagae, Yuji; Kurata, Masaki; Bottomley, D.; Furumoto, Kenichiro*

Journal of Nuclear Materials, 529, p.151939_1 - 151939_8, 2020/02


 Times Cited Count:2 Percentile:62.87(Materials Science, Multidisciplinary)

Journal Articles

Fracture limit of high-burnup advanced fuel cladding tubes under loss-of-coolant accident conditions

Narukawa, Takafumi; Amaya, Masaki

Journal of Nuclear Science and Technology, 57(1), p.68 - 78, 2020/01

 Times Cited Count:1 Percentile:23.13(Nuclear Science & Technology)

Journal Articles

Behavior of high-burnup advanced LWR fuel cladding tubes under LOCA conditions

Narukawa, Takafumi; Amaya, Masaki

Proceedings of International Nuclear Fuel Cycle Conference / Light Water Reactor Fuel Performance Conference (Global/Top Fuel 2019) (USB Flash Drive), p.912 - 921, 2019/09

Journal Articles

Oxidation of silicon carbide in steam studied by laser heating

Pham, V. H.; Nagae, Yuji; Kurata, Masaki; Furumoto, Kenichiro*; Sato, Hisaki*; Ishibashi, Ryo*; Yamashita, Shinichiro

Proceedings of International Nuclear Fuel Cycle Conference / Light Water Reactor Fuel Performance Conference (Global/Top Fuel 2019) (USB Flash Drive), p.670 - 674, 2019/09

Journal Articles

Oxidation behavior of high-burnup advanced fuel cladding tubes in high-temperature steam

Narukawa, Takafumi; Amaya, Masaki

Journal of Nuclear Science and Technology, 56(7), p.650 - 660, 2019/07

 Times Cited Count:6 Percentile:81.33(Nuclear Science & Technology)

Journal Articles

Experimental determination of the photooxidation of aqueous I$$^{-}$$ as a source of atmospheric I$$_{2}$$

Watanabe, Kosuke*; Matsuda, Shohei; Cuevas, C. A.*; Saiz-Lopez, A.*; Yabushita, Akihiro*; Nakano, Yukio*

ACS Earth and Space Chemistry (Internet), 3(4), p.669 - 679, 2019/04

 Times Cited Count:2 Percentile:26.9(Chemistry, Multidisciplinary)

The photooxidation of aqueous iodide ions (I$$^{-}$$$$_{(aq)}$$) at sea surface results in the emission of gaseous iodine molecules (I$$_{2}$$$$_{(g)}$$) into the atmosphere. It plays a certain role in the transport of iodine from ocean to the atmosphere in the natural cycle of iodine. In this study, we determined the photooxidation parameters, the molar absorption coefficient ($$varepsilon$$$$_{iodide}$$($$lambda$$)) and the photooxidative quantum yields ($$Phi$$$$_{iodide}$$($$lambda$$)) of I$$^{-}$$$$_{(aq)}$$, in the range of 290-500 nm. Through the investigation of the influence of pH and dissolved oxygen (DO) on $$Phi$$$$_{iodide}$$($$lambda$$), the subsequent emission rates of I$$_{2}$$$$_{(g)}$$ following the photooxidation of I$$^{-}$$$$_{(aq)}$$ in deionized water solution (pH 5.6, DO 7.8 mg L$$^{-1}$$) and artificial seawater solution (pH 8.0, DO 7.0 mg L$$^{-1}$$) were estimated. A global chemistry-climate model employed herein to assess the I$$_{2}$$$$_{(g)}$$ ocean emission on a global scale indicated that the photooxidation of I$$^{-}$$$$_{(aq)}$$ by solar light can enhance the atmospheric iodine budget by up to $$sim$$8% over some oceanic regions.

Journal Articles

Effect of re-oxidation rate of additive cations on corrosion rate of stainless steel in boiling nitric acid solution

Irisawa, Eriko; Yamamoto, Masahiro; Kato, Chiaki; Motooka, Takafumi; Ban, Yasutoshi

Journal of Nuclear Science and Technology, 56(4), p.337 - 344, 2019/04

 Times Cited Count:0 Percentile:0.01(Nuclear Science & Technology)

Journal Articles

Effects of ballooning and rupture on the fracture resistance of Zircaloy-4 fuel cladding tube after LOCA-simulated experiments

Yumura, Takanori; Amaya, Masaki

Annals of Nuclear Energy, 120, p.798 - 804, 2018/10

 Times Cited Count:3 Percentile:45.99(Nuclear Science & Technology)

Journal Articles

Improvements in drill-core headspace gas analysis for samples from microbially active depths

Miyakawa, Kazuya; Okumura, Fumiaki*

Geofluids, 2018, p.2436814_1 - 2436814_11, 2018/10

 Times Cited Count:1 Percentile:15.51(Geochemistry & Geophysics)

no abstracts in English

Journal Articles

Oxidation kinetics of Zry-4 fuel cladding in mixed steam-air atmospheres at temperatures of 1273 - 1473 K

Negyesi, M.; Amaya, Masaki

Journal of Nuclear Science and Technology, 54(10), p.1143 - 1155, 2017/10

 Times Cited Count:5 Percentile:58.67(Nuclear Science & Technology)

Journal Articles

Behavior of high-burnup advanced LWR fuels under design-basis accident conditions

Amaya, Masaki; Udagawa, Yutaka; Narukawa, Takafumi; Mihara, Takeshi; Taniguchi, Yoshinori

Proceedings of 2017 Water Reactor Fuel Performance Meeting (WRFPM 2017) (USB Flash Drive), 10 Pages, 2017/09

Journal Articles

Oxidation and reduction behaviors of a prototypic MgO-PuO$$_{2-x}$$ inert matrix fuel

Miwa, Shuhei; Osaka, Masahiko

Journal of Nuclear Materials, 487, p.1 - 4, 2017/04

 Times Cited Count:4 Percentile:50.55(Materials Science, Multidisciplinary)

Oxidation and reduction behaviors of prototypic MgO-based inert matrix fuels (IMFs) containing PuO$$_{2-x}$$ were experimentally investigated by means of thermogravimetry. The oxidation and reduction kinetics of the MgO-PuO$$_{2-x}$$ specimen were determined. The oxidation and reduction rates of the MgO-PuO$$_{2-x}$$ were found to be low compared with those of PuO$$_{2-x}$$. It is note that the changes in O/Pu ratios of MgO-PuO$$_{2-x}$$ from stoichiometry were smaller than those of PuO$$_{2-x}$$ at high oxygen partial pressure. From these results, it can be said that MgO matrix lower the oxygen supply and release of PuO$$_{2-x}$$, which is preferable as the minor actinides incineration devices, since the high oxygen potentials of minor actinide oxides can cause certain problems in terms of thermochemical aspects such as enlarged cladding inner-surface corrosion.

Journal Articles

Corrosion test of HTGR graphite with SiC coating

Chikhray, Y.*; Kulsartov, T.*; Shestakov, V.*; Kenzhina, I.*; Askerbekov, S.*; Sumita, Junya; Ueta, Shohei; Shibata, Taiju; Sakaba, Nariaki; Abdullin, Kh.*; et al.

Proceedings of 8th International Topical Meeting on High Temperature Reactor Technology (HTR 2016) (CD-ROM), p.572 - 577, 2016/11

Application of SiC as corrosion-resistive coating over graphite remains important task for HTGR. This study presents the results of chemical interaction of the SiC gradient coating over the high-density IG-110 graphite with water vapor in the temperature up to 1673 K. The experiments at 100 Pa of water vapor showed that the passive reaction caused to form SiO$$_{2}$$ film on the surface of SiC coating. Active corrosion of SiC in 1Pa of water vapor leads to deposits of various carbon composites on its surface.

Journal Articles

In situ X-ray diffraction study of the oxide formed on alloy 600 in borated and lithiated high-temperature water

Watanabe, Masashi*; Yonezawa, Toshio*; Shobu, Takahisa; Shiro, Ayumi; Shoji, Tetsuo*

Corrosion, 72(9), p.1155 - 1169, 2016/09

 Times Cited Count:0 Percentile:0.01(Materials Science, Multidisciplinary)

Journal Articles

The Effect of crystal textures on the anodic oxidization of zirconium in a boiling nitric acid solution

Kato, Chiaki; Ishijima, Yasuhiro; Ueno, Fumiyoshi; Yamamoto, Masahiro

Journal of Nuclear Science and Technology, 53(9), p.1371 - 1379, 2016/09


 Times Cited Count:2 Percentile:25.63(Nuclear Science & Technology)

The effects of crystal textures and the potentials in the anodic oxidation of zirconium in a boiling nitric acid solution were investigated to study the stress corrosion cracking of zirconium in nitric acid solutions. The growth of the zirconium oxide film dramatically changed depending on the applied potential at a closed depassivation potential (1.47 V vs. SSE). At 1.5 V, the zirconium oxide film rapidly grows, and its growth exhibits cyclic oxidation kinetics in accordance with a nearly cubic rate law. The zirconium oxide film grows according to the quantity of electric charge, and the growth rate does not depend on the crystal texture in the pretransition region before the cyclic oxidation kinetics. However, the growth and cracking under the thick oxide film depend on the crystal texture in the transition region. On the normal direction side, the oxide film thickness decreases on average since some areas of the thick oxide film are separated from the specimen surface owing to the cracks in the thick oxide. On the rolling direction side, cracks are found under the thick oxide film, which deeply propagate along the RD without an external stress. The cracks under the thick oxide film propagate to the center of the oxide layer. The cracks in the oxide layer propagate in the (0002)Zr plane in the zirconium matrix. The oxide layer consists of string-like zirconium oxide and zirconium hydride. The string-like zirconium oxide contains orthorhombic ZrO$$_{2}$$ in addition to monoclinic ZrO$$_{2}$$. As one assumption for the mechanism of crack initiation and propagation without an external stress, it is considered that the oxidizing zirconium hydrides precipitate in the (0002)Zr and then the phase transformation from orthorhombic ZrO$$_{2}$$ to monoclinic ZrO$$_{2}$$ in the oxide layer causes the crack propagation in the (0002) plane.

JAEA Reports

Effect of solid boric acid on the high temperature oxidation behavior of Zircaloy-4

Komiyama, Daisuke; Amaya, Masaki

JAEA-Research 2016-013, 20 Pages, 2016/08


The boric acid in the coolant may precipitate on the fuel cladding surface in the case that the blockage of coolant flow path etc. occurs and/or the cooling of fuel becomes insufficient during a LOCA (Loss-Of-Coolant Accident) in PWRs. While there is much knowledge about the compatibility between Zircaloy-4 and boric acid under normal operation conditions, such knowledge under high temperature condition, e.g. LOCA, has not been sufficient. In this study, isothermal heating tests were carried out by using Zircaloy-4 plates with solid boric acid in various atmospheres at up to 900$$^{circ}$$C; and the stability of boric acid, the reaction between Zircaloy-4 and boric acid and the effect of solid boric acid on the high temperature oxidation behavior of Zircaloy-4 were investigated. From the results obtained, it was suggested that, if boric acid anhydride remained on the surface of Zircaloy-4, the boric acid anhydride prevented the surface of Zircaloy-4 from contacting oxidizing atmosphere and mitigated the high-temperature oxidation of Zircaloy-4. In the case that solid boric acid adhered to the surface of pre-oxidized Zircaloy-4 and they have been heated up to high temperature, it was indicated that the solid boric acid penetrated into the gaps in the pre-oxide layer and the penetrated solid boric acid mitigated the oxidation of Zircaloy-4 thereafter.

236 (Records 1-20 displayed on this page)