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Journal Articles

Purification of uranium products in crystallization system for nuclear fuel reprocessing

Takeuchi, Masayuki; Yano, Kimihiko; Shibata, Atsuhiro; Sambommatsu, Yuji*; Nakamura, Kazuhito*; Chikazawa, Takahiro*; Hirasawa, Izumi*

Journal of Nuclear Science and Technology, 53(4), p.521 - 528, 2016/04

 Times Cited Count:2 Percentile:23.67(Nuclear Science & Technology)

JAEA Reports

Development of active control technology for impurities in coolant helium using High Temperature Engineering Test Reactor (HTTR)

Hamamoto, Shimpei; Nemoto, Takahiro; Sekita, Kenji; Saito, Kenji

JAEA-Technology 2015-048, 62 Pages, 2016/03

JAEA-Technology-2015-048.pdf:2.58MB

The decarburization may take place depending on the chemical impurity composition in helium gas used as the primary coolant in High-Temperature Gas-cooled Reactors, and will significantly reduce the strength of the alloy. The ability to remove impurities by a helium purification system was designed according to the predicted generation rate of impurities so as to make the coolant become the carburizing atmosphere. It has been confirmed that the coolant becomes the carburizing atmosphere during the operation period of the High Temperature engineering Test Reactor (HTTR). However, it is necessary to consider changes of generation rates of impurities since lifetime of commercial reactor is longer than the life of the HTTR. To avoid the influence of the change of generation rate, the control of removal efficiency of impurity in the helium purification system was considered in this study. To reform the decarburizing into the carburizing atmosphere, it is effective to increase the H$$_{2}$$ and CO concentration in the coolant helium. By controlling the efficiency of the Cooper Oxide Trap (CuOT), it is possible to increase the H$$_{2}$$ and CO concentrations. Therefore, an experiment was carried out by injecting the gas mixture of H$$_{2}$$ and CO into the existing purification system of HTTR to investigate the dependencies of temperature and impurity concentration on the removal efficiency of CuOT. The experimental results are described as the following, (1) By adjusting the temperature of helium at the CuOT within a range from 110$$^{circ}$$C to 50$$^{circ}$$C, it is possible to reduce the removal efficiency of H$$_{2}$$ sufficiently. (2) Temperature change of helium gas in the CuOT is sufficiently reduced by the cooler located at the downstream of the CuOT, which does not affect the primary cooling system of HTTR. As the results, the applicability of removal efficiency control of CuOT was verified to improve the decarburizing atmosphere for the actual HTGR system.

Journal Articles

Production of highly purified no-carrier-added $$^{177}$$Lu for radioimmunotherapy

Watanabe, Satoshi; Hashimoto, Kazuyuki; Watanabe, Shigeki; Iida, Yasuhiko*; Hanaoka, Hirofumi*; Endo, Keigo*; Ishioka, Noriko

Journal of Radioanalytical and Nuclear Chemistry, 303(1), p.935 - 940, 2015/01

 Times Cited Count:9 Percentile:62.76(Chemistry, Analytical)

Journal Articles

Coolant chemistry of the High Temperature Gas-Cooled Reactor 'HTTR'

Sakaba, Nariaki; Nakagawa, Shigeaki; Furusawa, Takayuki*; Emori, Koichi; Tachibana, Yukio

Nihon Genshiryoku Gakkai Wabun Rombunshi, 3(4), p.388 - 395, 2004/12

Chemistry control is important for the helium coolant of High Temperature Gas-cooled Reactors (HTGRs) because impurities cause oxidation of the graphite used in the core and corrosion of high temperature materials used in the heat exchanger. In the High Temperature Engineering Test Reactor (HTTR) which is the first HTGR in Japan, the chemical impurity concentration is restricted and its behaviour is monitored during reactor operations. The impurity is reduced by the helium purification system and the concentration is measured by the helium sampling system installed to the primary and secondary helium system, continuously. This paper describes the impurity behaviour during the rise-to-power test which is the initial power-up of the HTTR. Also, the amount of the emitted impurity to the primary circuit from the graphite component and insulator used at the concentric hot gas duct are evaluated. During the power up, any abnormal impurity increases were not obtained and the chemical composition of the primary circuit is sufficiently in the stability area to avoid carbon deposition.

Journal Articles

Gas purification technology using electron beams

Kojima, Takuji

Shinku, 47(11), p.789 - 795, 2004/11

When flue gas/off gas is irradiated by EB, many free radicals such as OH and active oxygen atom are formed from major components of air: namely nitrogen, oxygen, water and carbon dioxide ecules. The similer reaction can be achieved using UV light and plasma-discharging, but ionizing radiations produce such free radicals at higher density. Such radiation-induced radicals react efficiently with air pollutants, SOx and NOx in coal/oil combustion flue gas at thermal power plants, dioxins in waste incineration flue gas and volatile organic compounds (VOC) even in very low concentration and decompose them into non-toxic substances or change them to removable substances. R & D on EB treatment of flue gas/off gas done in JAERI on the basis of this principle process, as an example, is described in the present paper.

Journal Articles

Leak-tightness characteristics concerning the containment structures of the HTTR

Sakaba, Nariaki; Iigaki, Kazuhiko; Kondo, Masaaki; Emori, Koichi

Nuclear Engineering and Design, 233(1-3), p.135 - 145, 2004/10

 Times Cited Count:5 Percentile:36.48(Nuclear Science & Technology)

The containment structures of the HTTR consist of the reactor containment vessel, the service area, and the emergency air purification system, which minimise the release of fission products in postulated accidents which lead to fission product release from the reactor facilities. The reactor containment vessel is designed to withstand the temperature and pressure transients and to be leak-tight in the case of a rupture of the primary concentric hot gas duct, etc. The pressure inside the service area is maintained at a negative pressure by the emergency air purification system. The emergency air purification system will also remove airborne radio-activity and will maintain a correct pressure in the service area. The leak-tightness characteristics of the containment structures are described in this paper. The measured leakage rates of the reactor containment vessel were enough less than the specified leakage limit of 0.1%/d confirmed during the commissioning tests and annual inspections. The service area was kept the design pressure well below its allowable limitation by the emergency air purification system which filter efficiency of particle removal and iodine removal were well over the limited values. The obtained data demonstrates that the reactor containment structures were fabricated to minimise the release of fission products in the postulated accidents with fission product release from the reactor facilities.

Journal Articles

Short design descriptions of other systems of the HTTR

Sakaba, Nariaki; Furusawa, Takayuki; Kawamoto, Taiki; Ishii, Yoshiki; Ota, Yukimaru

Nuclear Engineering and Design, 233(1-3), p.147 - 154, 2004/10

 Times Cited Count:10 Percentile:57.38(Nuclear Science & Technology)

The HTTR mainly consists of the core components, reactor pressure vessel, cooling systems, instrumentation and control systems, and containment structures. The design of remaining utility systems is described in this paper. They are: auxiliary helium systems which include the helium purification system, the helium sampling system, and the helium storage and supply system; fuel handling and storage system. The helium purification systems are installed in the primary and secondary helium cooling systems in order to reduce the quantity of chemical impurities. The helium sampling systems monitor the concentration of impurities. The helium storage and supply systems keep the steady pressure of the helium system during the normal operation. The fuel handling and storage system is utilised to handle the new and spent fuels safely and reliably.

Journal Articles

Purification technology for flue/off gases using electron beams

Kojima, Takuji

Shokubai, 46(3), p.248 - 253, 2004/04

The present paper describes research and development on purification technology using electron beams for flue/odd gases containing pollutants: removal of sulfate oxide and nitrogen oxide from flue gases of coal/oil combustion power plants, decomposition of dioxins in waste incineration flue gas, and decomposition/removal of toxic volatile organic compounds from off gas.

Journal Articles

Electron beam technologies for control of flue gases/wastewaters and their applications

Kojima, Takuji

Oyo Butsuri, 72(4), p.405 - 414, 2003/04

The advanced technologies are required to control pollutants e.g. dioxins in gas or water at extremely low concentration. The present paper introduces typical basic studies, developments of control technologies, and example of their industrial applications of electron beam technology having the features of oxidation, decomposition and detoxifying of such pollutants even at low concentration. It covers removal of SOx and NOx from coal-combustion flue gas, decomposition of gaseous volatile organic compound in off gas and dioxins in incineration flue-gas, purification of tap and wastewaters, and treatment of sewage/sludge.

JAEA Reports

Establishment of a clean chemistry laboratory at JAERI; Clean Laboratory for Environmental Analysis and Research (CLEAR)

Hanzawa, Yukiko; Magara, Masaaki; Watanabe, Kazuo; Esaka, Fumitaka; Miyamoto, Yutaka; Yasuda, Kenichiro; Gunji, Katsubumi*; Yamamoto, Yoichi; Takahashi, Tsukasa; Sakurai, Satoshi; et al.

JAERI-Tech 2002-103, 141 Pages, 2003/02

JAERI-Tech-2002-103.pdf:10.38MB

The JAERI has established a facility with a cleanroom: the Clean Laboratory for Environmental Analysis and Research (CLEAR). This report is an overview of the design, construction and performance evaluation of the CLEAR in the initial stage of the laboratory operation in June 2001. The CLEAR is a facility to be used for ultra trace analyses of nuclear materials in environmental samples for the safeguards, for the CTBT verification and for researches on environmental sciences. The CLEAR meets double requirements of a cleanroom and for handling of nuclear materials. Much attention was paid to the construction materials of the cleanroom for trace analysis of metal elements using corrosive acids. The air conditioning and purification system, experimental equipment, utilities and safety systems are also demonstrated. The potential contamination from the completed cleanroom atmosphere during the analytical procedure was evaluated. It can be concluded that the CLEAR has provided a suitable condition for reliable analysis of ultra trace amounts of nuclear materials in environmental samples.

JAEA Reports

Development of the carbon fiber reinforced carbon-carbon composite for High Temperature Gas-cooled Reactors

Sogabe, Toshiaki; Ishihara, Masahiro; Baba, Shinichi; Kojima, Takao; Tachibana, Yukio; Iyoku, Tatsuo; Hoshiya, Taiji; Hiraoka, Toshiharu*; Yamaji, Masatoshi*

JAERI-Research 2002-026, 22 Pages, 2002/11

JAERI-Research-2002-026.pdf:2.41MB

Carbon Fiber Reinforced Carbon-carbon Composites, C/C composites, have been developed and extensively studied their characteristics. C/C composites are considered to be promising materials for the application of a control rod in the next high performance high temperature gas-cooled reactors. In the present paper, details of the development of the candidate C/C composite are described. In the course of the development of the material, especially, feasibility of the production, stableness of the supply and cost are much taken into consideration. As the physical properties of the material, high mechanical strength such as tensile and bending, high fracture strain and fracture toughness and low dimensional change by neutron irradiation have to be met. The developed 2D-C/C composite consists of plain-weave PAN-based carbon fiber cloth and pitch derived matrix. Also, high purification up to the level of nuclear grade was successfully attained in the composite.

JAEA Reports

Transportation of significant metals recovered in real sea experiment of adsorbents

Takeda, Hayato*; Onuma, Kenji*; Tamada, Masao; Kasai, Noboru; Katakai, Akio; Hasegawa, Shin; Seko, Noriaki; Kawabata, Yukiya*; Sugo, Takanobu

JAERI-Tech 2001-062, 66 Pages, 2001/10

JAERI-Tech-2001-062.pdf:5.5MB

Real sea experiment for the recovery of significant metals such as uranium and vanadium has been carried out at the offing of Mutsu establishment to evaluate the adsorption performance of adsorbent synthesized by radiation-induced graft-polymerization. After elution of uranium and vanadium from the adsorbent, their metals were adsorbed onto the conventional chelate resin. This chelate resin in a plastic column was further put in a cylindrical stainless transport container. The container was transported to the facility for separation and purification by a truck for the exclusive loading. The maximum concentration is 60 Bq/g when the uranium is adsorbed on the chelate resin. Transportation of recovered metals can be treated as general substance since these amount and concentration are out of legal control. However, the recovered metals were transported in conformity to L type transportation as a voluntary regulation. The strength analysis of the container was equal to the safety level of IP-2 type which is higher transportation grade than L type .

Journal Articles

Performance tests of reactor containment structures of the HTTR

Iigaki, Kazuhiko; Sakaba, Nariaki; Kawaji, Satoshi; Iyoku, Tatsuo

Transactions of 16th International Conference on Structural Mechanics in Reactor Technology (SMiRT-16) (CD-ROM), 7 Pages, 2001/08

no abstracts in English

JAEA Reports

Impurity measurement test of HTTR; At the commissioning tests

Sakaba, Nariaki; Emori, Koichi; Saruta, Toru

JAERI-Tech 99-072, p.125 - 0, 1999/10

JAERI-Tech-99-072.pdf:5.85MB

no abstracts in English

JAEA Reports

Performance tests of the reactor containment structures of HTTR

Sakaba, Nariaki; Iigaki, Kazuhiro; Kawaji, Satoshi; Iyoku, Tatsuo

JAERI-Tech 98-013, 152 Pages, 1998/03

JAERI-Tech-98-013.pdf:7.69MB

no abstracts in English

Journal Articles

Preparation of pure tritium for a liquid D$$_{2}$$/T$$_{2}$$ target of muon-catalyzed fusion experiments

Kudo, Hiroshi; Fujie, Makoto; Tanase, Masakazu; Kato, Mineo; Kurosawa, Kiyoyuki; Sugai, Hiroyuki; Umezawa, Hirokazu; Matsuzaki, Teiichiro*; Nagamine, Kanetada*

Applied Radiation and Isotopes, 43(5), p.577 - 583, 1992/00

no abstracts in English

Journal Articles

Desorption behavior of plutonium from anion-exchange resin with HNO$$_{3}$$-HI mixed acid solution

Usuda, Shigekazu; Sakurai, Satoshi; Hirata, Masaru; Umezawa, Hirokazu

Sep. Sci. Technol., 25(11-12), p.1225 - 1237, 1990/00

 Times Cited Count:1 Percentile:27.62(Chemistry, Multidisciplinary)

no abstracts in English

JAEA Reports

Development of an Apparatus for Cyclic Corrosion Test in Simulated VHTR Helium Environment

; Shindo, Masami; Kondo, Tatsuo

JAERI-M 83-093, 16 Pages, 1983/07

JAERI-M-83-093.pdf:1.45MB

no abstracts in English

Journal Articles

Preliminary design of a fusion reactor fuel cleanup system by the palladium alloy membrane method

; Konishi, Satoshi; Naruse, Yuji

Nucl.Technol./Fusion, 3, p.471 - 484, 1983/00

no abstracts in English

Journal Articles

A Preliminary study on the production of tritium from neutron-irradiated litium-aluminum alloy

Tanase, Masakazu; Yamaguchi, Koichi; Tanaka, Kichizo

Radioisotopes, 31, p.571 - 578, 1982/00

no abstracts in English

25 (Records 1-20 displayed on this page)