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Futemma, Akira; Sanada, Yukihisa; Nakama, Shigeo; Sasaki, Miyuki; Ochi, Kotaro; Nagakubo, Azusa; Sawahata, Yoshiro*; Kawasaki, Yoshiharu*; Iwai, Takeyuki*; Hiraga, Shogo*; et al.
JAEA-Technology 2024-021, 232 Pages, 2025/03
JAEA-Technology-2024-021.pdf:25.79MB
The 2011 off the Pacific coast of Tohoku Earthquake on March 11, 2011, caused a tsunami that led to the TEPCO's Fukushima Daiichi Nuclear Power Station (FDNPS) accident, releasing a large amount of radioactive material into the surrounding environment. Since the accident, Aerial Radiation Monitoring (ARM) has been used to quickly and widely measure radiation distribution. As a commissioned project from the Nuclear Regulation Authority, the Japan Atomic Energy Agency (JAEA) has continuously conducted ARM around FDNPS using manned and unmanned helicopters. This report summarizes the monitoring results for fiscal year 2023, evaluates changes in dose rate from past results, and discusses the factors contributing to these changes. Additionally, an analysis considering terrain undulation was conducted to improve accuracy for converting ARM data into dose rate. Furthermore, a method to discriminate airborne radon progeny was applied for ARM results to evaluate its impact. Moreover, to perform wide-area monitoring more efficiently, we advanced the development of unmanned airplane monitoring technology.
Group for Fukushima Mapping Project
JAEA-Technology 2024-017, 208 Pages, 2025/03
JAEA-Technology-2024-017.pdf:27.32MB
This report presents results of the investigations on the distribution-mapping project of radioactive substances owing to TEPCO Fukushima Daiichi Nuclear Power Station (FDNPS) conducted in FY2023. Car-borne surveys, a measurement using survey meters, a walk survey and an unmanned helicopter survey were carried out to obtain air dose rate data to create their distribution maps, and temporal changes of the air dose rates were analyzed. Surveys on depth profile of radiocesium and in-situ measurements as for radiocesium deposition were performed. Based on these measurement results, effective half-lives of the temporal changes in the air dose rates and the deposition were evaluated. Score maps to classify the importance of the measurement points were created, and the temporal changes in the score were analyzed. A system to report the tritium concentration level in seawater to the Nuclear Regulation Authority was operated, and the variation of tritium concentration before and after the discharge of ALPS treated water to the ocean was analyzed. Monitoring data in coastal area performed owing to the comprehensive radiation monitoring plan until FY2023 was analyzed. Using the Bayesian hierarchical modeling approach, we obtained maps that integrated air dose rate distribution data acquired through surveys such as car-borne and walk surveys. Representative life patterns that can be expected after the return to the evacuation-designated restricted area were set, and the cumulative exposure doses were evaluated for the local governments and residents in the area. The measurement results for FY2023 were published on the Web site and measurement data were stored as CSV format. Radiation monitoring and analysis of environmental samples owing to the comprehensive radiation monitoring plan were carried out.
Battulga, B.; Nakanishi, Takahiro; Atarashi-Andoh, Mariko; Otosaka, Shigeyoshi*; Koarashi, Jun
Environmental Science and Pollution Research, 31, p.60080 - 60092, 2024/10
A ubiquitous distribution of plastic debris has been reported in aquatic and terrestrial environments; however, the interactions between plastics and radionuclides and the radioactivity of environmental plastics remain largely unknown. Here, we characterize biofilms developing on the surface of plastic debris to explore the role of plastic-associated biofilms as an interaction medium between plastics and radiocesium (
Cs) in the environment. Biofilm samples were extracted from plastics (1-50 mm in size) collected from two contrasting coastal areas in Japan. The radioactivity of plastics was estimated based on the Cs activity concentration of the biofilms and compared seasonally with surrounding environmental samples (i.e., sediment and sand). Cs traces were detected in biofilms with activity concentrations of 21-1300 Bq kg
biofilm (dry weight), corresponding to 0.04-4.5 Bq kg plastic (dry weight). Our results reveal the interaction between Cs and plastics and provide evidence that organic and mineral components in biofilms are essential in Cs retention in environmental plastics.
Futemma, Akira; Sanada, Yukihisa; Nagakubo, Azusa; Kawasaki, Yoshiharu*; Iwai, Takeyuki*; Hiraga, Shogo*; Haginoya, Masashi*; Matsunaga, Yuki*; Akutsu, Yuichiro*; Arai, Yoshinori*; et al.
JAEA-Technology 2023-027, 146 Pages, 2024/03
JAEA-Technology-2023-027.pdf:18.12MB
By the accident at Tokyo Electric Power Company's (TEPCO's) Fukushima Daiichi Nuclear Power Station (FDNPS), caused by tsunami triggered by the 2011 off the Pacific coast of Tohoku Earthquake, a large amount of radioactive material was released into the surrounding environment. After the accident, Airborne Radiation Monitoring (ARM) via manned helicopter has been applied as a method to quickly and extensively measure the distribution of radiation. Japan Atomic Energy Agency (JAEA) has continuously conducted ARM via manned helicopter around FDNPS. In this report, we summarize the results of the ARM around FDNPS in the fiscal year 2022, evaluate the changes of ambient dose rates and other parameters based on the comparison to the past ARM results, and discuss the causes of such changes. In order to contribute to improve the accuracy of ambient dose rate conversion, we analyzed the ARM data taking into account undulating topography, and evaluated the effect of this method. Furthermore, the effect of radon progenies in the air on the ARM was evaluated by applying the discrimination method to the measurement results.
Group for Fukushima Mapping Project
JAEA-Technology 2023-024, 176 Pages, 2024/03
JAEA-Technology-2023-024.pdf:22.16MB
This report presents results of the investigations on the distribution-mapping project of radioactive substances owing to TEPCO Fukushima Daiichi Nuclear Power Station (FDNPS) conducted in FY2022. Car-borne surveys, a measurement using survey meters, a walk survey and an unmanned helicopter survey were carried out to obtain air dose rate data to create their distribution maps, and temporal changes of the air dose rates were analyzed. Surveys on depth profile of radiocesium and in-situ measurements as for radiocesium deposition were performed. Based on these measurement results, effective half-lives of the temporal changes in the air dose rates and the deposition were evaluated. Score maps to classify the importance of the measurement points were created, and the factors causing changes in the score when monitoring data from multiple years were used were discussed. The range of fluctuation of past tritium concentration data in seawater was determined, and the causes of the fluctuation were discussed. Monitoring data in coastal area performed in 2022 owing to the comprehensive radiation monitoring plan was summarized, and temporal changes in cesium-137 were analyzed. Using the Bayesian hierarchical modeling approach, we obtained maps that integrated air dose rate distribution data acquired through surveys such as car-borne and walk surveys with respect to the region within 80 km from the FDNPS and Fukushima Prefecture. The measurement results for FY2022 were published on the "Database for Radioactive Substance Monitoring Data", and measurement data were stored as CSV format. Radiation monitoring and analysis of environmental samples owing to the comprehensive radiation monitoring plan were carried out.
Collaborative Laboratories for Advanced Decommissioning Science; Ibaraki University*
JAEA-Review 2023-021, 112 Pages, 2024/02
JAEA-Review-2023-021.pdf:7.1MB
The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2020. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2018, this report summarizes the research results of the "Contribution to Risk Reduction in Decommissioning Works by the Elucidation of Basic Property of Radioactive Microparticles" conducted from FY2018 to FY2021 (this contract was extended to FY2021). The present study aims to understand the basic properties (size, chemical composition, isotopic composition - including concentration of 
-emitters, electrostatic properties, and optical properties, etc.) of fine particles composed of silicate with insoluble properties which contain regions of highly concentrated radioactive cesium (Cs) released to the environment by the accident at the Fukushima Daiichi Nuclear Power Station of TEPCO in 2011 March.
Cs occurring near the Fukushima Dai-ichi Nuclear Power PlantOta, Masakazu; Takahara, Shogo; Yoshimura, Kazuya; Nagakubo, Azusa; Hirouchi, Jun; Hayashi, Naho; Abe, Tomohisa; Funaki, Hironori; Nagai, Haruyasu
Journal of Environmental Radioactivity, 264, p.107198_1 - 107198_15, 2023/08
Times Cited Count：0 Percentile：0.00(Environmental Sciences)One of the current major radiation exposure pathways from the Fukushima Daiichi Nuclear Power Plant (FDNPP) accident-fallout is inhalation of the re-suspended Cs occurring in air. While wind-induced soil particle resuspension has been recognized as a primary mechanism of Cs resuspension, studies following the FDNPP accident suggested that fungal spores can be a significant source of the atmospheric Cs particularly in the rural areas such as difficult-to-return zone (DRZ). To elucidate the relative importance of the two resuspension phenomena, we propose a model simulating resuspension of Cs as soil particles and fungal spores, and applied it to DRZ. Our model's calculation showed that soil particle resuspension was responsible for the surface-air Cs observed during winter-spring, but could not account for the higher Cs concentrations observed in summer-autumn. The higher concentrations in the summer-autumn were in general reproduced by implementing fungal spore Cs emission, that replenished low soil particle Cs resuspension in that period. According to our model's concept, Cs accumulation in fungal spores and high spore emission rate characterized by the rural environment were likely responsible for the abundance of spore Cs in the air. It was inferred that the influence of the fungal spores on the atmospheric Cs would last longer since un-decontaminated forests still exist in DRZ.
Abe, Tomohisa; Funaki, Hironori; Yoshimura, Kazuya; Shiribiki, Natsu*; Sanada, Yukihisa
JAEA-Data/Code 2023-001, 38 Pages, 2023/05
JAEA-Data-Code-2023-001.pdf:3.04MB
JAEA-Data-Code-2023-001-appendix(CD-ROM).zip:32.02MB
In this study, commissioned by the Cabinet Office, we conducted a survey on radioactive materials in atmospheric dust in three municipalities (Futaba Town, Okuma Town, and Tomioka Town) in Fukushima Prefecture to contribute to the assessment of internal exposure in the Specified Reconstruction and Revitalization Base (SRRB). Air dust samplers were installed in the targeted municipalities to investigate the atmospheric Cs concentrations and to evaluate internal exposure doses based on measured value. This report summarizes the results of measurements between 2018 and 2021. A database of information on internal exposure dose assessment results based on atmospheric radioactivity concentrations and actual measurements, and meteorological observation data was compiled.
Futemma, Akira; Sanada, Yukihisa; Nagakubo, Azusa; Kawasaki, Yoshiharu*; Iwai, Takeyuki*; Hiraga, Shogo*; Haginoya, Masashi*; Matsunaga, Yuki*; Akutsu, Yuichiro*; Urabe, Yoshimi*; et al.
JAEA-Technology 2022-027, 148 Pages, 2023/02
JAEA-Technology-2022-027.pdf:19.64MB
By the nuclear disaster of Fukushima Daiichi Nuclear Power Station (FDNPS), Tokyo Electric Power Company (TEPCO), caused by the Great East Japan Earthquake and the following tsunami on March 11, 2011, a large amount of radioactive material was released from the FDNPS. After the nuclear disaster, airborne radiation monitoring via manned helicopter has been conducted around FDNPS. The results of the airborne radiation monitoring and the evaluation for temporal change of dose rate in the fiscal 2021 were summarized in this report. Analysis considering topographical effects was applied to the result of the airborne monitoring to improve the accuracy of the conventional method. In addition, technique for discriminating gamma rays from the ground and those from the airborne Rn-progenies was also utilized to evaluate their effect on airborne radiation monitoring.
Group for Fukushima Mapping Project
JAEA-Technology 2022-026, 152 Pages, 2023/01
JAEA-Technology-2022-026.pdf:20.14MB
This report presents results of the investigations on the distribution-mapping project of radioactive substances owing to TEPCO Fukushima Daiichi Nuclear Power Station (FDNPS) conducted in FY2021. Car-borne surveys, a flat ground measurement using survey meters, a walk survey and an unmanned helicopter survey were carried out to obtain air dose rate data to create air dose rate distribution maps, and temporal changes of the air dose rates were analyzed. Surveys on depth profile of radiocesium and in-situ measurements as for radiocesium deposition were performed. Based on these measurement results, effective half-lives of the temporal changes in the air dose rates and the deposition were evaluated. Score maps to classify the importance of the measurement points were created for Fukushima Prefecture and the 80 km zone from the FDNPS, and the factors causing changes in the score when monitoring data from multiple years were used were discussed. Monitoring data in coastal area performed owing to the comprehensive radiation monitoring plan until 2020 was summarized, and temporal changes in cesium-137 were analyzed. Using the Bayesian hierarchical modeling approach, we obtained maps that integrated the air dose rate distribution data obtained in this project with respect to the region within 80 km from the FDNPS and Fukushima Prefecture. The measurement results for FY2021 were published on the "Expansion Site of Distribution Map of Radiation Dose", and measurement data were stored as CSV format. Radiation monitoring and analysis of environmental samples owing to the comprehensive radiation monitoring plan were carried out.
Hagiwara, Hiroki; Kondo, Keietsu; Hidaka, Akihide
Journal of Radioanalytical and Nuclear Chemistry, 331(12), p.5905 - 5914, 2022/12
Times Cited Count：3 Percentile：44.16(Chemistry, Analytical)Battulga, B.; Atarashi-Andoh, Mariko; Nakanishi, Takahiro; Koarashi, Jun
Science of the Total Environment, 849, p.157758_1 - 157758_11, 2022/11
Times Cited Count：7 Percentile：48.42(Environmental Sciences)Characterizing plastic-associated biofilms is key to the better understanding of organic material and mineral cycling in the "Plastisphere"-the thin layer of microbial life on plastics. In this study, we propose a new method to extract biofilms from environmental plastics, in order to evaluate the properties of biofilm-derived organic matter through stable carbon (
C) and nitrogen (
N) isotope signatures and their interactions with radionuclides especially radiocesium (Cs). After ultrasound-assisted separation from the plastics, biofilm samples were successfully collected via a sequence of syringe treatments. Biofilm-derived organic matter samples (14.5-65.4 mg) from four river mouths in Japan showed Cs activity concentrations of 
75 to 820 Bq kg biofilm (dw), providing evidence that environmental plastics, mediated by developed biofilms, serve as a carrier for Cs in the coastal environment. Significant differences in the (C and N signatures were also obtained for the biofilms, indicating the different sources, pathways, and development processes of biofilms on plastics.
Cs falloutOta, Masakazu; Koarashi, Jun
Science of the Total Environment, 816, p.151587_1 - 151587_21, 2022/04
Times Cited Count：8 Percentile：53.64(Environmental Sciences)In forests affected by the Fukushima Daiichi Nuclear Power Plant accident, trees became contaminated with Cs. However, Cs transfer processes determining tree contamination (particularly for stem wood, which is a prominent commercial resource in Fukushima) remain insufficiently understood. This study proposes a model for simulating the dynamic behavior of Cs in a forest tree-litter-soil system and applied it to two contaminated forests (cedar plantation and natural oak stand) in Fukushima. The model-calculated results and inter-comparison of the results with measurements elucidated the relative impact of distinct Cs transfer processes determining tree contamination. The transfer of Cs to trees occurred mostly (
99%) through surface uptake of Cs directly trapped by leaves or needles and bark during the fallout. By contrast, root uptake of Cs from the soil was unsubstantial and several orders of magnitude lower than the surface uptake over a 50-year period following the accident. As a result, the internal contamination of the trees proceeded through an enduring recycling (translocation) of Cs absorbed on the tree surface at the time of the accident. A significant surface uptake of Cs at the bark was identified, contributing 100% (leafless oak tree) and 30% (foliated cedar tree; the remaining surface uptake occurred at the needles) of the total Cs uptake by trees. It was suggested that the trees growing at the study sites are currently (as of 2021) in a decontamination phase; the activity concentration of Cs in the stem wood decreases by 3% per year, mainly through radioactive decay of Cs and partly through a dilution effect from tree growth.
Ando, Masaki; Saito, Kimiaki
JAEA-Technology 2021-032, 66 Pages, 2022/03
JAEA-Technology-2021-032.pdf:3.84MB
Since the occurrence of the accident at the TEPCO Fukushima Daiichi Nuclear Power Station, the Japan Atomic Energy Agency (JAEA) has been conducting a series of car-borne survey over a wide area in the eastern part of Japan using the monitoring system KURAMAII. In this report, outline of the car-borne surveys are summarized and the following characteristics of the temporal changes in each prefecture and region were investigated using the measured data obtained from 2012 to 2019; 1) Average and maximum values for each prefecture for the six years from 2014 to 2019, 2) Average values for each prefecture from 2012 to 2019, 3) Average values for each evacuation order area category, regional category, and northern Soso-area municipality in Fukushima Prefecture from 2012 to 2019, and 4) Average and maximum values for each municipality in each prefecture for four times (at almost two-year intervals) of the measurement results from 2012 to 2018.
Futemma, Akira; Sanada, Yukihisa; Ishizaki, Azusa; Kawasaki, Yoshiharu*; Iwai, Takeyuki*; Hiraga, Shogo*; Sato, Kazuhiko*; Haginoya, Masashi*; Matsunaga, Yuki*; Kikuchi, Hikaru*; et al.
JAEA-Technology 2021-029, 132 Pages, 2022/02
JAEA-Technology-2021-029.pdf:24.58MB
By the nuclear disaster of Fukushima Daiichi Nuclear Power Station (FDNPS), Tokyo Electric Power Company (TEPCO), caused by the Great East Japan Earthquake and the following tsunami on March 11, 2011, a large amount of radioactive material was released from the FDNPS. After the nuclear disaster, airborne radiation monitoring using manned helicopter has been conducted around FDNPS. The results of the airborne radiation monitoring and the evaluation for temporal change of dose rate in the fiscal 2020 were summarized in this report. Analysis considering topographical effects was applied to the result of the airborne monitoring to improve the accuracy of conventional method. In addition, technique for discriminating gamma rays from the ground and those from the airborne Rn-progenies was also utilized to evaluate their effect on airborne radiation monitoring.
Group for Fukushima Mapping Project
JAEA-Technology 2021-025, 159 Pages, 2022/01
JAEA-Technology-2021-025.pdf:46.66MB
This report presents results of the investigations on the distribution-mapping project of radioactive substances owing to TEPCO Fukushima Daiichi Nuclear Power Station (FDNPS) conducted in FY2020. Car-borne surveys, a flat ground measurement using survey meters, a walk survey and an unmanned helicopter survey were carried out to obtain air dose rate data. Air dose rate distribution maps were created and temporal changes of the air dose rates were analyzed. Regarding radiocesium deposition into the ground, surveys on depth profile of radiocesium and in-situ measurements were performed. Based on these measurement results, effective half-lives of the temporal changes in the air dose rates and the deposition were evaluated. In the examination of scoring for classifying the importance of measurement points, a score map was created for Fukushima Prefecture and the 80 km zone from the FDNPS, and the factors causing changes in the score when monitoring data from multiple years were used were discussed. Using the Bayesian hierarchical modeling approach, we obtained maps that integrated the air dose rate distribution data obtained from aircraft monitoring, car-borne surveys, and walk surveys with respect to the region within 80 km from the FDNPS and Fukushima Prefecture. The measurement results for FY2020 were published on the "Expansion Site of Distribution Map of Radiation Dose", and measurement data were stored as CSV format. Radiation monitoring and analysis of environmental samples owing to the comprehensive radiation monitoring plan were carried out.
Hagiwara, Hiroki; Funaki, Hironori; Shiribiki, Natsu*; Kanno, Marina*; Sanada, Yukihisa
Journal of Radioanalytical and Nuclear Chemistry, 331(1), p.415 - 426, 2022/01
Times Cited Count：7 Percentile：63.20(Chemistry, Analytical)Abe, Tomohisa; Yoshimura, Kazuya; Sanada, Yukihisa
Aerosol and Air Quality Research, 21(7), p.200636_1 - 200636_11, 2021/07
Times Cited Count：4 Percentile：17.74(Environmental Sciences)Futemma, Akira; Sanada, Yukihisa; Ishizaki, Azusa; Kawasaki, Yoshiharu*; Iwai, Takeyuki*; Hiraga, Shogo*; Sato, Kazuhiko*; Haginoya, Masashi*; Matsunaga, Yuki*; Kikuchi, Hikaru*; et al.
JAEA-Technology 2020-018, 121 Pages, 2021/02
JAEA-Technology-2020-018.pdf:15.15MB
By the nuclear disaster of Fukushima Daiichi Nuclear Power Station (FDNPS), Tokyo Electric Power Company (TEPCO), caused by the Great East Japan Earthquake and the following tsunami on March 11, 2011, a large amount of radioactive material was released from the FDNPS. After the nuclear disaster, airborne radiation monitoring using manned helicopter has been conducted around FDNPS. The results in the fiscal 2019 were summarized in this report. Analysis taken topographical effects into consideration was applied to the result of airborne monitoring to improve the precision of conventional method. In addition, discrimination method of gamma rays from Rn-progenies was also utilized to evaluate their effect on aerial radiation monitoring.
Collaborative Laboratories for Advanced Decommissioning Science; Ibaraki University*
JAEA-Review 2020-033, 84 Pages, 2021/01
JAEA-Review-2020-033.pdf:4.9MB
JAEA/CLADS had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project in FY2019. Among the adopted proposals in FY2018, this report summarizes the research results of the "Contribution to Risk Reduction in Decommissioning Works by the Elucidation of Basic Property of Radioactive Microparticles" conducted in FY2019.
